arXiv subjects

Tian Shang

Publications and source records attributed to Tian Shang.

At least 19 recordsLinked to original sources

arXiv2026

Unconventional superconductivity in ScIr$_2$ chiral crystal with a kagome lattice

Materials with a kagome lattice host exotic quantum phenomena driven by the interplay between band topology, spin-orbit coupling, magnetism, and electronic correlations. While magnetism of kagome materials has been widely investigated, their unconventional superconductivity (SC) remains largely unexplored due to the limited availability of suitable materials. Here, we report evidence of unconventional SC in the ScIr$_{2-x}$Si$_{x}$ family by combining muon-spin spectroscopy measurements with band-structure calculations. The parent ScIr$_2$ undergoes a structural phase transition from a high-$T$ cubic- to a low-$T$ rhombohedral phase, while the Ir kagome layer remains, albeit slightly distorted. Although the structural transition is suppressed by Si substitution, the superconducting pairing of ScIr$_{2-x}$Si$_{x}$ remains well described by a two-gap model. Since at least one of the gaps has nodes, this indicates an unconventional SC. Its unconventional nature can be explained by the distinct flat bands occurring near the Fermi level, leading to strong electronic correlations in the ScIr$_{2-x}$Si$_{x}$ family. Moreover, the low-$T$ phase of ScIr$_2$ exhibits an Ir chiral chain; therefore, it can be classified as a topological chiral crystal. Overall, the unusual properties of the ScIr$_{2-x}$Si$_{x}$ family make it an interesting, albeit rare, system for studying the interplay between unconventional SC, flat bands, and chirality.

cond-mat.supr-con↗

arXiv2026

Strain-tunable charge localization coupled to complex magnetic orders in EuAl$_4$

Charge localization is particularly interesting when coupled to antiferromagnetic spin structures. Coupled spin-charge orders are well established in elemental chromium and correlated oxide superconductors, yet the interplay between charge order and more complex magnetic textures -- such as skyrmion lattices and chiral spin structures -- remains largely unexplored. Here we report a comprehensive study of how charge localization couples to the unusually rich sequence of magnetic phases in EuAl$_4$. Using x-ray diffraction under applied magnetic field and uniaxial pressure, we demonstrate a direct coupling between the charge and spin order parameters. In the absence of external stimuli, charge localization is markedly enhanced upon entering the magnetically ordered phases. Strikingly, this effect is highly susceptible to strain: uniaxial pressure applied along the charge-order propagation direction further enhances localization, whereas pressure applied perpendicular to it weakens it. Application of magnetic field reveals both competitive and possible collaborative interactions between spin and charge ordering.This flexible coupling between spin and charge ordering opens a new route to designing symmetry-breaking states. Chiral charge order may for example be patterned from spin structures with that symmetry.

cond-mat.str-el↗

arXiv2026

Strongly frustrated 2D magnetism in a 3D hexagonal perovskite

Exotic quantum phenomena are often found to occur in spin systems that exhibit low-dimensional magnetism. By combining nuclear magnetic resonance, neutron scattering, and muon-spin spectroscopy ($\mu$SR) techniques, we report a rare instance of strongly frustrated two-dimensional (2D) magnetism in a three-dimensional (3D) hexagonal perovskite. Here, Ba$_2$La$_2$MnTe$_2$O$_{12}$, a triangular-lattice magnet, is shown to undergo a magnetic transition at $T_\mathrm{N} \approx$ 4.4 K, below which the manganese moments form a 120$^{\circ}$ AFM order within the $ab$-plane, while staying disordered along the $c$-axis. This exotic ground state, which exhibits ideal 2D magnetism, is highly consistent with the persistently strong spin fluctuations and the large internal field distributions revealed by zero-field $\mu$SR. Further, the 2D magnetism also leads to a significant frustration, much larger than that of most known magnetically-ordered frustrated systems. Our work on Ba$_2$La$_2$MnTe$_2$O$_{12}$ not only challenges the interpretations of magnetic order in other 3D hexagonal perovskites, but it also provides insight into how the dimensionality affects the exotic magnetic states.

cond-mat.str-el↗

arXiv2026

Investigating the intrinsic anomalous Hall effect in MnPt3 topological semimetal

The cubic Cu$_3$Au-type $X$Pt$_3$ family ($X$ = V, Cr, and Mn) is a topological semimetal characterized by anti-crossing gapped nodal lines near the Fermi level, which give rise to significant Berry curvatures and thus to the anomalous Hall effect (AHE). Among the three members, CrPt$_3$ has been experimentally verified to exhibit a large anomalous Hall conductivity (AHC), while its counterparts MnPt$_3$ and VPt$_3$ remain largely unexplored. Here, a series of MnPt$_3$ thin films with varying thicknesses (20--70 nm) was epitaxially grown on the MgO substrates using magnetron sputtering and was systematically investigated by magnetization, electrical resistivity, and Hall resistivity measurements. MnPt$_3$ films undergo a ferromagnetic transition at a Curie temperature $T_\mathrm{C}$, which increases as the film thickness increases, reaching $\sim$ 344 K for the 70-nm-thick film. All the anomalous Hall transport properties of MnPt$_3$ films, including the resistivity, conductivity, and angle, exhibit a strong correlation with their magnetic properties. The scaling analysis suggests that the intrinsic Berry-curvature mechanism dominates the observed AHE, while the extrinsic contributions are much smaller. The intrinsic AHC increases as the film thickness increases, while the extrinsic AHC is thickness-independent. Such an enhanced intrinsic AHC in the MnPt$_3$ films is most likely attributed to the strain effect, implying that it serves as an effective method to tune the electronic band topology in the $X$Pt$_3$ topological semimetal.

cond-mat.str-el↗

arXiv2026

Engineering of Orbital Hybridization: An Exotic Strategy to Manipulate Orbital Current

Current-induced spin-orbit torque (SOT) plays a crucial role in the next-generation spin-orbitronics. Enhancing its efficiency is both fundamentally and practically interesting and remains a challenge to date. Recently, orbital counterparts of spin effects that do not rely on the spin-orbit coupling (SOC) have been found as an alternative mechanism to realize it. This work highlights the engineering of copper oxidation states for manipulating the orbital current and its torque in the CuO$_x$-based heterostructures. The orbital hybridization and thus the orbital-Rashba-Edelstein effect at the CuO$_x$/Cu interfaces are significantly enhanced by increasing the copper oxidation state, yielding a torque efficiency that is almost ten times larger than the conventional heavy metals. The Cu$_4$O$_3$/Cu interface, rather than the widely accepted CuO/Cu interface, is revealed to account for the enhanced SOT performance in the CuO$_x$-based heterostructures. In addition, the torque efficiency can be alternatively switched between high and low thresholds through the redox reaction. The current results establish an exotic and robust strategy for engineering the orbital current and SOT for spin-orbitronics, which applies to other weak-SOC materials.

cond-mat.mtrl-sci↗

arXiv2025

Investigating the origin of topological-Hall-like resistivity in Zn-doped Mn2Sb ferrimagnet

Skyrmions and other chiral spin textures have been extensively studied as potential building blocks for novel spintronic devices. Hall-resistivity anomalies that deviate from magnetization scaling, known as the topological Hall effect, have been widely employed as evidence for the presence of chiral spin textures in magnetic materials. However, recent studies on magnetic thin films have revealed a drawback of this approach, as the presumed topological Hall contribution may in fact originate from trivial mechanisms. Here, we investigate the magnetic and transport properties of a Zn-doped Mn2Sb ferrimagnet, whose related compounds have previously been suggested to exhibit a topological Hall effect arising from chiral spin textures. Hall-resistivity anomalies are also observed in our sample, yet they show little correlation with the magnetic or metamagnetic transitions and are therefore clearly distinct from those in magnetic compounds hosting chiral spin textures. Most importantly, additional Lorentz transmission electron microscopy measurements rule out the existence of chiral spin textures in this ferrimagnet. Therefore, instead of a nontrivial origin, we attribute the Hall-resistivity anomalies to the combined effect of multiple anomalous Hall channels resulting from sample inhomogeneity. Our work shows that the difficulties of identifying chiral spin textures through transport measurements also apply to bulk systems, prompting some existing results to be revisited.

cond-mat.str-el↗

arXiv2025

Anomalous Hall effect and rich magnetic phase diagram of Mn$_{100-x}$Rh$_{x}$ epitaxial films

A series of Mn$_{100-x}$Rh$_x$ ($20 \le x \le 50$) thin films were epitaxially grown on the MgO substrate using magnetron sputtering technique, and were systematically investigated by magnetization, longitudinal electrical resistivity, and transverse Hall resistivity. After optimizing the growth conditions, phase-pure Mn$_{100-x}$Rh$_x$ films with a cubic CsCl-type structure were obtained, and their magnetic phase diagram was built. The manipulation of Rh content leads to a rich magnetic phase diagram, where three different regimes can be identified: for $x < 40$, Mn$_{100-x}$Rh$_x$ films undergo a ferromagnetic (FM) transition below $T_\mathrm{C} \approx$ 330-350 K; for $40 \le x \le 45$, in addition to the FM transition at $T_\mathrm{C} \approx$ 200 K, Mn$_{100-x}$Rh$_x$ films undergo a FM-to-antiferromagnetic (AFM) transition at $T_\mathrm{N} \approx$ 120 K; finally for $x > 45$, only one AFM transition at $T_\mathrm{N} \approx$ 150 K can be tracked. All the Mn$_{100-x}$Rh$_x$ films exhibit distinct anomalous Hall effect in their magnetically ordered state, which is most likely due to the intrinsic Berry-curvature mechanism. In addition, all the anomalous Hall transport properties, including the resistivity, conductivity, and angle exhibit a strong correlation with the magnetic properties of Mn$_{100-x}$Rh$_x$ films, which become most evident for $x$ = 35. Our systematic investigations suggest a strong correlation between magnetic properties and electronic band topology in Mn$_{100-x}$Rh$_x$ films, highlighting their great potential for AFM spintronics.

cond-mat.str-el↗

arXiv2025

A chemical avenue to manipulate field-reentrant superconducting rivalries in infinite layer nickelates

Recently, preliminary magnetic field-reentrant superconductivity manifested in high-temperature (Tc) Eu-doped infinite-layer (IL) nickelates, beyond analogous discoveries exclusively in low-Tc systems. This evokes intriguing fundamental issues about potential quantum-phase boundary and criticality between unconventional superconductivity and field-reentrant-one, which are inexplicable owing to formidable challenges in growing IL-nickelates towards later-series rare-earths. Herein, we open up chemical avenues to enable effective growth of (RE1-yRE'y)1-xEuxNiO2 (RE/RE': Pr, Nd, Sm, Gd, Dy), giving rise to discoveries of RE-4f-related quantum competition between high-Tc and reentrant superconductivity. Robust magnetic-field-reentrant superconductivity with uniaxial anisotropy is observed at superconducting-dome boundaries, stemming from Eu2+-4f7 associated competition between magnetic-fluctuation promoted pairing and exchange-field interactions. Their quantum-criticality is further modulable via RE(RE')-magnetism, which either reinforces reentrancy or elevates Tc (40.1 K) with more robust critical-current-density (~266 kA/cm2 at 2 K) beyond Sr-/Ca-doped counterparts. Our synthetic route enables the establishment of an ideal platform via IL-nickelates for studying 4f-related unconventional superconductivity and quantum-criticality.

cond-mat.supr-con↗

arXiv2025

Discovery of nodal-line superconductivity in chiral crystals

Chiral crystals, whose key feature is the structural handedness, host exotic quantum phenomena driven by the interplay of band topology, spin-orbit coupling (SOC), and electronic correlations. Due to the limited availability of suitable chiral-crystal materials, their unconventional superconductivity (SC) remains largely unexplored. Here, we report the discovery of unconventional SC in the La(Rh,Ir)Si family of materials by combining muon-spin spectroscopy, band-structure calculations, and perturbation theory. This family, characterized by a double-helix chiral structure, hosts exotic multifold fermions that are absent in other topological chiral crystals. While LaRhSi behaves as a fully-gapped superconductor, the substitution of 4$d$-Rh by 5$d$-Ir significantly enhances the SOC and leads to the emergence of topological nodal-line SC in LaIrSi. The developed model shows that the nodal-line SC arises from an isotropic SOC with a specific strength. Such an exotic mechanism expands our conventional understanding of material candidates for unconventional SC, which typically rely on a significantly anisotropic SOC to promote the triplet pairing. Our work establishes a new type of phase diagram, which provides a comprehensive roadmap for identifying and engineering unconventional SC in chiral crystals. Furthermore, it calls for renewed investigations of unconventional SC in other widely studied superconductors with a chiral structure.

cond-mat.supr-con↗

arXiv2025

Strongly correlated electronic superconductivity in the noncentrosymmetric Re-Os-based high/medium-entropy alloys

The class of unconventional superconductors, particularly noncentrosymmetric superconductors, has been highly considered as potential materials for understanding the complex properties of quantum materials. Here, five previously unreported Re3.5Os3.5Ta0.5Hf0.5Nb3, Re3Os3Ta0.5Hf0.5Nb3, Re3.5Os3.5Mo0.5Hf0.5Nb3, Re3.5Os3.5Mo0.5W0.5Nb3, and Re3Os3Mo0.5Hf0.5Nb3 Re-Os-based high/medium-entropy alloys (MEAs-HEAs) with valence electron count ranging from 6.45 to 6.81 were synthesized and investigated using x-ray diffraction, transport, magnetization, and specific heat measurements. Our analyses confirm that all five compounds crystallize in a noncentrosymmetric {\alpha}-Mn-type structure and exhibit type-II superconductivity with Tc values from 4.20 K to 5.11 K, respectively. Unexpectedly, despite being immersed in an acidic environment for one month, the structures and superconducting properties of HEAs remain stable. Our findings indicate that the Tc increases with an increasing valence electron count in MEAs-HEAs. Furthermore, these noncentrosymmetric {\alpha}-Mn-type HEA superconductors have large Kadowaki-Woods ratios (KWR), implying the presence of strong electronic correlations.

cond-mat.supr-con↗

arXiv2025

Large unconventional anomalous Hall effect far above room temperature in epitaxial Fe$_3$Ga$_4$ films

Noncoplanar spin textures usually exhibit a finite scalar spin chirality (SSC) that can generate effective magnetic fields and lead to additional contributions to the Hall effect, namely topological or unconventional anomalous Hall effect (UAHE). Unlike topological spin textures (e.g., magnetic skyrmions), materials that exhibit fluctuation-driven SSC and UAHE are rare. So far, their realization has been limited to either low temperatures or high magnetic fields, both of which are unfavorable for practical applications. Identifying new materials that exhibit UAHE in a low magnetic field at room temperature is therefore essential. Here, we report the discovery of a large UAHE far above room temperature in epitaxial Fe$_3$Ga$_4$ films, where the fluctuation-driven SSC stems from the field-induced transverse-conical-spiral phase. Considering their epitaxial nature and the large UAHE stabilized at room temperature in a low magnetic field, Fe$_3$Ga$_4$ films represent an exciting, albeit rare, case of a promising candidate material for spintronic devices.

cond-mat.mtrl-sci↗

arXiv2025

Multiband superconductivity in the topological Kramers nodal-line semimetals

Recent band-structure calculations predict that the ruthenium-based ternary silicides are three-dimensional Kramers nodal line semimetals. Among them, NbRuSi and TaRuSi show bulk superconductivity (SC) below $T_c \sim 3$ K and 4 K, as well as spontaneous magnetic fields. The latter indicates the breaking of time-reversal symmetry and, thus, unconventional SC in both compounds. Previous temperature-dependent muon-spin spectroscopy studies failed to distinguish whether such compounds exhibit single-gap or multi-gap SC. Here, we report on systematic measurements of the field-dependent muon-spin relaxation rates in the superconducting state and on temperature-dependent electrical resistivity and specific heat under applied magnetic fields. Both the upper critical field and the field-dependent superconducting relaxation are well described by a two-band model. By combining our experimental results with numerical band-structure calculations, we provide solid evidence for multiband SC in NbRuSi and TaRuSi, and thus offer further insight into the unconventional- and topological nature of their superconductivity.

cond-mat.supr-con↗

arXiv2025

Superconductivity in the Medium-Entropy/High-Entropy Re-based Alloys with a Non-Centrosymmetric $\alpha$-Mn Lattice

Medium or high-entropy alloys (MEAs-HEAs) and rhenium-based compounds with a non-centrosymmetric (NC) structure have received a lot of attention for offering a fertile soil in search for unconventional superconductivity. Here, five previously unreported NC Re-based MEA-HEA superconductors with an $\alpha$-Mn lattice are successfully synthesized, with their superconducting transition temperatures (Tcs) ranging from 4 to 5 K. An increase in the superconducting transition temperature (Tc) can be achieved by modulating the valence electron count (VEC) through compositional adjustments. Magnetization measurements confirm that all the synthesized Re-based MEA-HEAs are bulk type-II superconductors. Specific heat analysis reveals that the superconducting state of these HEAs can be well described by a single-gap s-wave model. Our results show that the Kadowaki-Woods ratio of these $\alpha$-Mn MEA/HEA superconductors are close to the typical value of heavy fermion compounds, suggesting the existence of strong electronic correlation. These findings provide promising material platforms to study the role of high disorder in the origin of superconductivity in the NC MEAs-HEAs.

cond-mat.supr-con↗

arXiv2025

Anatomy of anomalous Hall effect due to magnetic fluctuations

The anomalous Hall {\color{black} e}ffect (AHE) has emerged as a key indicator of time-reversal symmetry breaking (TRSB) and topological features in electronic band structures. Absent of a magnetic field, the AHE requires spontaneous TRSB but has proven hard to probe due to averaging over domains. The anomalous component of the Hall effect is thus frequently derived from extrapolating the magnetic field dependence of the Hall response. We show that discerning whether the AHE is an intrinsic property of the field free system becomes intricate in the presence of strong magnetic fluctuations. {\color{black}As a study case,} we use the Weyl semimetal PrAlGe, where TRSB can be toggled via a ferromagnetic transition, providing a transparent view of the AHE's topological origin. Through a combination of thermodynamic, transport and muon spin relaxation measurements, we contrast the behaviour below the ferromagnetic transition temperature to that of strong magnetic fluctuations above. Our results {\color{black}on PrAlGe provide general insights into the} interpretation of anomalous Hall signals in systems where TRSB is debated, such as families of Kagome metals or certain transition metal dichalcogenides.

cond-mat.str-el↗

arXiv2024

Observation of Orbital-Selective Dual Modulations in an Anisotropic Antiferromagnetic Kagome Metal TbTi3Bi4

Orbital selectivity is pivotal in dictating the phase diagrams of multiorbital systems, with prominent examples including the orbital-selective Mott phase and superconductivity, etc. The intercalation of anisotropic layers represents an effective method for enhancing orbital selectivity and, thereby shaping the low-energy physics of multiorbital systems. Despite its potential, related experimental studies remain limited. In this work, we systematically examine the interplay between orbital selectivity and magnetism in the newly discovered anisotropic kagome TbTi3Bi4 single crystal, and report a unidirectional, orbital-selective band reconstruction within the antiferromagnetic (AFM) state. By combining soft X-ray and vacuum ultraviolet angle-resolved photoemission spectroscopy (ARPES) measurements with orbital-resolved density functional theory (DFT) calculations, we identify that the band reconstruction is a manifestation of the AFM order, driven by a 1/3 nesting instability of the intercalated Tb 5dxz orbitals. Such an orbital-selective modulation leads the unusual momentum-dependent band folding and the emergence of symmetry-protected Dirac cones only at the M1 point. More importantly, the discovery of orbital-selective 3 x 1 AFM order offers crucial insights into the underlying mechanism of the fractional magnetization plateau in this Kagome AFM metal. Our findings not only underscore the essential role of both conducting and localized electrons in determining the magnetic orders of LnTi3Bi4 (Ln = Lanthanide) kagome metals but also offer a pathway for manipulating magnetism through selective control of anisotropic electronic structures.

cond-mat.str-el↗

arXiv2024

Coexistence of insulator-like paramagnon and metallic spin-orbit exciton modes in SrIrO$_3$

We probe the spectrum of elementary excitations in SrIrO$_3$ by using heterostructured [(SrIrO$_3$)$_m$/(SrTiO$_3$)$_l$] samples to approach the bulk limit. Our resonant inelastic x-ray scattering (RIXS) measurements at the Ir $L_3$-edge reveal a robust low-lying collective magnetic mode with an antiferromagnetic (AF) dispersion similar to the insulators Sr$_2$IrO$_4$ and Sr$_3$Ir$_2$O$_7$, albeit with a large gap and much larger linewidth. At higher energies we find the spin-orbit exciton, also strongly broadened, but with an inverted dispersion and doubled periodicity that are controlled by the charge hopping. These results demonstrate that the AF paramagnon persists, somewhat counterintuitively, far into the metallic regime of the insulator-metal transition driven by the degree of confinement in the heterostructure. We conclude that these two excitations, which are contrasting but coexisting hallmarks of strong AF pseudospin and charge fluctuations in a spin-orbit-coupled Mott-Slater material, are properties intrinsic to the ground state of semimetallic perovskite SrIrO$_3$.

cond-mat.str-el↗

arXiv2024

Experimental progress in Eu(Al,Ga)$_4$ topological antiferromagnets

The non-trivial magnetic and electronic phases occurring in topological magnets are often entangled, thus leading to a variety of exotic physical properties. Recently, the BaAl$_4$-type compounds have been extensively investigated to elucidate the topological features appearing in their real- and momentum spaces. In particular, the topological Hall effect and the spin textures, typical of the centrosymmetric Eu(Al,Ga)$_4$ family, have stimulated extensive experimental and theoretical research. In this topical review, we discuss the latest findings regarding the Eu(Al,Ga)$_4$ topological antiferromagnets and related materials, arising from a vast array of experimental techniques. We show that Eu(Al,Ga)$_4$ represents a suitable platform to explore the interplay between lattice-, charge-, and spin degrees of freedom, and associated emergent phenomena. Finally, we address some key questions open to future investigation.

cond-mat.str-el↗

arXiv2024

Nodeless superconductivity and topological nodal states in molybdenum carbide

The orthorhombic molybdenum carbide superconductor with $T_c$ = 3.2 K was investigated by muon-spin rotation and relaxation ($\mu$SR) measurements and by first-principle calculations. The low-temperature superfluid density, determined by transverse-field $\mu$SR, suggests a fully-gapped superconducting state in Mo$_2$C, with a zero-temperature gap $\Delta_0$ = 0.44 meV and a magnetic penetration depth $\lambda_0$ = 291 nm. The time-reversal symmetry is preserved in the superconducting state, as confirmed by the absence of an additional muon-spin relaxation in the zero-field $\mu$SR spectra. Band-structure calculations indicate that the density of states at the Fermi level is dominated by the Mo $4d$-orbitals, which are marginally hybridized with the C $2p$-orbitals over a wide energy range. The symmetry analysis confirms that, in the absence of spin-orbit coupling (SOC), Mo$_2$C hosts twofold-degenerate nodal surfaces and fourfold-degenerate nodal lines. When considering SOC, the fourfold-degenerate nodal lines cross the Fermi level and contribute to the electronic properties. Our results suggest that, similarly to other phases of carbides, also the orthorhombic transition-metal carbides host topological nodal states and may be potential candidates for future studies of topological superconductivity.

cond-mat.supr-con↗