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Tian-Xiang Zhu

Publications and source records attributed to Tian-Xiang Zhu.

16 recordsLinked to original sources

Random access and high dimensional integrated quantum memory

Random-access quantum memory (RAQM) is a fundamental building block for scalable quantum networks and photonic quantum computing. While existing realizations rely on gaseous physical systems, solid-state platforms--particularly integrated architectures--offer distinct practical advantages for scalable deployment. However, current integrated quantum memories are limited to single-channel operation, which precludes both RAQM and the manipulation of high-dimensional photonic states. Here, we demonstrate an 11-channel integrated quantum memory based on laser-written waveguide arrays in an $^{151}$Eu$^{3+}$:Y$_2$SiO$_5$ crystals. On-chip electrode arrays allow independent control of the read-out time in each channel via Stark-shift-induced atomic interference. The device achieves random-access quantum storage of three time-bin qubits with a fidelity exceeding 99%, and stores five-dimensional path-encoded quantum states with a fidelity above 96%. This multichannel integrated quantum memory supports flexible functionality through its random-access operation and establishes a practical hardware platform for high-dimensional quantum networks implemented in integrated architectures.

quant-ph↗

A Metropolitan-scale Multiplexed Quantum Repeater with Bell Nonlocality

Quantum repeaters can overcome exponential photon loss in optical fibers, enabling heralded entanglement between distant quantum memories. The definitive benchmark for this entanglement is Bell nonlocality; however, recent metropolitan-scale demonstrations based on single-photon interference (SPI) schemes have been limited to generating low-quality entanglement, falling short of Bell nonlocality certification. Here, we introduce a multiplexed quantum repeater protocol based on time measurements (MQR-TM), successfully combining the high heralding rate of SPI schemes with the phase robustness of two-photon interference (TPI) schemes. This approach achieves heralded entanglement distribution between two solid-state quantum memories over a record 14.5~km separation, generating a Bell state with a fidelity of $78.6 \pm 2.0\%$. We observe a CHSH-Bell inequality violation by 3.7 standard deviations, marking the first certification of Bell nonlocality in metropolitan-scale quantum repeaters. Our architecture supports autonomous quantum node operation without fiber channel phase stabilization, offering a practical framework for scalable quantum-repeater networks.

quant-ph↗

Heterogeneous entanglement between a trapped ion and a solid-state quantum memory

Hybrid quantum networks offer a promising architecture for scalable quantum information processing and a future quantum internet, as they can combine the complementary strengths of disparate physical platforms. While single-atom systems provide deterministic quantum logic gates, atomic ensembles enable large-capacity quantum storage. However, generating entanglement between such heterogeneous systems has remained an open challenge, primarily due to fundamental spectral mismatches and system complexity. Here, we demonstrate a hybrid quantum network that entangles a single trapped $\mathrm{^{171}Yb^{+}}$ ion and a quantum memory based on $\rm ^{153}Eu^{3+}\colon\!Y_2SiO_5$ crystal over a 75-m separation. Using polarization-maintaining quantum frequency conversion, we map spin-photon entanglement onto a hybrid entanglement between a single spin qubit and a collective excitation of the quantum memory. The resulting entangled state achieves a fidelity of $(89.21 \pm 2.23)\%$ and violates the CHSH-Bell inequality by 6 standard deviations ($S = 2.328 \pm 0.055$), confirming nonlocality between two heterogeneous nodes. This work establishes entanglement between a quantum processing module with a multiplexed quantum memory node, representing a key step toward a scalable, multifunctional quantum internet.

quant-ph↗

Efficient integrated quantum memory for light

Scalable implementation of quantum networks and photonic processors require integrated photonic memories with high efficiency, yet current integrated systems have been limited to storage efficiencies below 27.8%. Here, we demonstrate highly efficient integrated quantum memories based on rare-earth-iondoped crystals coupled with impedance-matched microcavities, realized in two novel architectures: 200-micrometer-thin membranes of Eu3+:Y2SiO5 integrated with fiber-based microcavities, and waveguide-based cavities fabricated using femtosecond lasers. Our approach achieves reliable integrated quantum storage with record efficiencies of 80.3(7)% for weak coherent pulses and 69.8(1.6)% for telecom-heralded single photons, alongside the storage of 20 temporal modes with an average efficiency of 51.3(2)%. Moreover, the thin-membrane Eu3+:Y2SiO5 architecture enables spectrally tunable efficient quantum storage via variable strain, providing a flexible interface for quantum networks. By combining high efficiency, large multimode capacity, and tunability, our devices establish a versatile hardware foundation for scalable quantum repeaters and chip-scale photonic processors.

quant-ph↗

Remote Quantum Networks based on Quantum Memories

Quantum networks, capable of transmitting arbitrary quantum states, provide a foundation for a wide range of quantum applications, including distributed quantum computing, distributed quantum sensing, and quantum communication. Photons are the natural carrier of information in quantum networks, but the exponential loss of optical fiber channels prevents the construction of large-scale quantum networks. A potential solution is implementing quantum repeaters based on quantum memories, which can efficiently establish long-distance entanglement from short-distance entanglement. In the past decades, intense efforts have been devoted to constructing large-scale quantum networks based on various atomic quantum memories. In this Perspective, we present a concise overview of current advancements in remote quantum networks, elucidate the imminent challenges that must be addressed, and discuss the future directions.

quant-ph↗

A millisecond integrated quantum memory for photonic qubits

Quantum memories for light are essential building blocks for quantum repeaters and quantum networks. Integrated operations of quantum memories could enable scalable application with low-power consumption. However, the photonic quantum storage lifetime in integrated optical waveguide has so far been limited to tens of microseconds, falling short of the requirements for practical applications. Here, we demonstrate quantum storage of photonic qubits for 1.021 ms based on a laser-written optical waveguide fabricated in a 151Eu3+:Y2SiO5 crystal. Spin dephasing of 151Eu3+ is mitigated through dynamical decoupling applied via on-chip electric waveguides and we obtain a storage efficiency of 12.0(0.5)% at 1.021 ms, which is a demonstration of integrated quantum memories that outperforms the efficiency of a simple fiber delay line. Such long-lived waveguide-based quantum memory could support applications in quantum repeaters, and further combination with critical magnetic fields could enable potential application as transportable quantum memories.

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Nonlocal photonic quantum gates over 7.0 km

Quantum networks provide a prospective paradigm to connect separated quantum nodes, which relies on the distribution of long-distance entanglement and active feedforward control of qubits between remote nodes. Such approaches can be utilized to construct nonlocal quantum gates, forming building blocks for distributed quantum computing and other novel quantum applications. However, these gates have only been realized within single nodes or between nodes separated by a few tens of meters, limiting the ability to harness computing resources in large-scale quantum networks. Here, we demonstrate nonlocal photonic quantum gates between two nodes spatially separated by 7.0 km using stationary qubits based on multiplexed quantum memories, flying qubits at telecom wavelengths, and active feedforward control based on field-deployed fibers. Furthermore, we illustrate quantum parallelism by implementing the Deutsch-Jozsa algorithm and the quantum phase estimation algorithm between the two remote nodes. These results represent a proof-of-principle demonstration of quantum gates over metropolitan-scale distances and lay the foundation for the construction of large-scale distributed quantum networks relying on existing fiber channels.

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Realization of edge states along a synthetic orbital angular momentum dimension

The synthetic dimension is a rising method to study topological physics, which enables us to implement high-dimensional physics in low-dimensional geometries. Photonic orbital angular momentum (OAM), a degree of freedom characterized by discrete yet unbounded, serves as a suitable synthetic dimension. However, a sharp boundary along a synthetic OAM dimension has not been demonstrated, dramatically limiting the investigation of topological edge effects in an open boundary lattice system. In this work, we make a sharp boundary along a Floquet Su-Schrieffer-Heeger OAM lattice and form approximate semi-infinite lattices by drilling a pinhole on the optical elements in a cavity. The band structures with zero ($\pmπ$) energy boundary states are measured directly, benefiting from the spectra detection of the cavity. Moreover, we obtain the edge modes moving from the gap to the bulk by dynamically changing the boundary phase, and we reveal that interference near the surface leads to spectrum discretization. Our work provides a new perspective to observe edge effects and explore practical photonics tools.

physics.optics↗

Laser Direct Writing of Visible Spin Defects in Hexagonal Boron Nitride for Applications in Spin-Based Technologies

Optically addressable spins in two-dimensional hexagonal boron nitride (hBN) attract widespread attention for their potential advantage in on-chip quantum devices, such as quantum sensors and quantum network. A variety of spin defects have been found in hBN, but no convenient and deterministic generation methods have been reported for other defects except negatively charged boron vacancy ($V_B^-$). Here we report that by using femtosecond laser direct writing technology, we can deterministically create spin defect ensembles with spectra range from 550 nm to 800 nm on nanoscale hBN flakes. Positive single-peak optically detected magnetic resonance (ODMR) signals are detected in the presence of magnetic field perpendicular to the substrate, and the contrast can reach 0.8%. With the appropriate thickness of hBN flakes, substrate and femtosecond laser pulse energy, we can deterministically and efficiently generate bright spin defect array. Our results provide a convenient deterministic method to create spin defects in hBN, which will motivate more endeavors for future researches and applications of spin-based technologies such as quantum magnetometer array.

physics.optics↗

On-demand storage of photonic qubits at telecom wavelengths

Quantum memories at telecom wavelengths are crucial for the construction of large-scale quantum networks based on existing fiber networks. On-demand storage of telecom photonic qubits is a fundamental request for such networking applications but yet to be demonstrated. Here we demonstrate the storage and on-demand retrieval of telecom photonic qubits using a laser-written waveguide fabricated in an $^{167}$Er$^{3+}$:Y$_2$SiO$_5$ crystal. Both ends of the waveguide memory are directly connected with fiber arrays with a fiber-to-fiber efficiency of 51%. Storage fidelity of 98.3(1)% can be obtained for time-bin qubits encoded with single-photon-level coherent pulses, which is far beyond the maximal fidelity that can be achieved with a classical measure and prepare strategy. This device features high reliability, easy scalability and can be directly integrated into fiber networks, which could play an essential role in fiber-based quantum networks.

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On-demand multimode optical storage in a laser-written on-chip waveguide

Quantum memory is a fundamental building block for large-scale quantum networks. On-demand optical storage with a large bandwidth, a high multimode capacity and an integrated structure simultaneously is crucial for practical application. However, this has not been demonstrated yet. Here, we fabricate an on-chip waveguide in a $\mathrm {^{151}Eu^{3+}:Y_2SiO_5}$ crystal with insertion losses of 0.2 dB, and propose a novel pumping scheme to enable spin-wave atomic frequency comb (AFC) storage with a bandwidth of 11 MHz inside the waveguide. Based on this, we demonstrate the storage of 200 temporal modes using the AFC scheme and conditional on-demand storage of 100 temporal modes using the spin-wave AFC scheme. The interference visibility between the readout light field and the reference light field is $99.0\% \pm 0.6\%$ and $97\% \pm 3\%$ for AFC and spin-wave AFC storage, respectively, indicating the coherent nature of this low-loss, multimode and integrated storage device.

physics.optics↗

On-demand Integrated Quantum Memory for Polarization Qubits

Photonic polarization qubits are widely used in quantum computation and quantum communication due to the robustness in transmission and the easy qubit manipulation. An integrated quantum memory for polarization qubits is a fundamental building block for large-scale integrated quantum networks. However, on-demand storing polarization qubits in an integrated quantum memory is a long-standing challenge due to the anisotropic absorption of solids and the polarization-dependent features of microstructures. Here we demonstrate a reliable on-demand quantum memory for polarization qubits, using a depressed-cladding waveguide fabricated in a 151Eu3+: Y2SiO5 crystal. The site-2 151Eu3+ ions in Y2SiO5 crystal provides a near-uniform absorption for arbitrary polarization states and a new pump sequence is developed to prepare a wideband and enhanced absorption profile. A fidelity of 99.4\pm0.6% is obtained for the qubit storage process with an input of 0.32 photons per pulse, together with a storage bandwidth of 10 MHz. This reliable integrated quantum memory for polarization qubits reveals the potential for use in the construction of integrated quantum networks.

quant-ph↗

On-demand quantum storage of photonic qubits in an on-chip waveguide

Photonic quantum memory is the core element in quantum information processing (QIP). For the scalable and convenient practical applications, great efforts have been devoted to the integrated quantum memory based on various waveguides fabricated in solids. However, on-demand storage of qubits, which is an essential requirement for QIP, is still challenging to be implemented using such integrated quantum memory. Here we report the on-demand storage of time-bin qubits in an on-chip waveguide memory on the surface of a $^{151}$Eu$^{3+}$:Y$_2$SiO$_5$ crystal, utilizing the Stark modulated atomic frequency comb protocol. A qubit storage fidelity of $99.3\%\pm0.2\%$ is obtained with a input of 0.5 photons per pulse, far beyond the highest fidelity achievable using the classical measure-and-prepare strategy. The developed integrated quantum memory with the on-demand retrieval capability, represents an important step towards practical applications of integrated quantum nodes in quantum networks.

quant-ph↗

Coherent Optical Memory Baesd on A Laser-written On-chip Waveguide

Quantum memory is the core device for the construction of large-scale quantum networks. For scalable and convenient practical applications, integrated optical memories, especially on-chip optical memories, are crucial requirements because they can be easily integrated with other on-chip devices. Here, we report the coherent optical memory based on a type-IV waveguide fabricated on the surface of a rare-earth ion-doped crystal (i.e. $\mathrm{Eu^{3+}}$:$\mathrm{Y_2SiO_5}$). The properties of the optical transition ($\mathrm{{^7}F{_0}\rightarrow{^5}D{_0}}$) of the $\mathrm{Eu^{3+}}$ ions inside the surface waveguide are well preserved compared to those of the bulk crystal. Spin-wave atomic frequency comb storage is demonstrated inside the type-IV waveguide. The reliability of this device is confirmed by the high interference visibility of ${97\pm 1\%}$ between the retrieval pulse and the reference pulse. The developed on-chip optical memory paves the way towards integrated quantum nodes.

quant-ph↗

Hyperfine Structure and Coherent Dynamics of Rare Earth Spins Explored with Electron-Nuclear Double Resonance at Sub-Kelvin Temperatures

An experimental platform of ultralow-temperature pulsed ENDOR (electron-nuclear double resonance) spectroscopy is constructed for the bulk materials. Coherent property of the coupled electron and nuclear spins of the rare-earth (RE) dopants in a crystal (143Nd3+:Y2SiO5) is investigated from 100 mK to 6 K. At the lowest working temperatures, two-pulse-echo coherence time exceeding 2 ms and 40 ms are achieved for the electron and nuclear spins, while the electronic Zeeman and hyperfine population lifetimes are more than 15 s and 10 min. With the aid of the near-unity electron spin polarization at 100 mK, the complete hyperfine level structure with 16 energy levels is measured using ENDOR technique without the assistance of the reconstructed spin Hamiltonian. These results demonstrate the suitability of the deeply cooled paramagnetic RE-doped solids for memory components aimed for quantum communication and quantum computation. The developed experimental platform is expected to be a powerful tool for paramagnetic materials from various research fields.

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Reliable coherent optical memory based on a laser-written waveguide

$\mathrm {^{151}Eu^{3+}}$-doped yttrium silicate ($\mathrm {^{151}Eu^{3+}:Y_2SiO_5}$ ) crystal is a unique material that possesses hyperfine states with coherence time up to 6 h. Many efforts have been devoted to the development of this material as optical quantum memories based on the bulk crystals, but integrable structures (such as optical waveguides) that can promote $\mathrm {^{151}Eu^{3+}:Y_2SiO_5}$-based quantum memories to practical applications, have not been demonstrated so far. Here we report the fabrication of type 2 waveguides in a $\mathrm {^{151}Eu^{3+}:Y_2SiO_5}$ crystal using femtosecond-laser micromachining. The resulting waveguides are compatible with single-mode fibers and have the smallest insertion loss of $4.95\ dB$. On-demand light storage is demonstrated in a waveguide by employing the spin-wave atomic frequency comb (AFC) scheme and the revival of silenced echo (ROSE) scheme. We implement a series of interference experiments based on these two schemes to characterize the storage fidelity. Interference visibility of the readout pulse is $0.99\pm 0.03$ for the spin-wave AFC scheme and $0.97\pm 0.02$ for the ROSE scheme, demonstrating the reliability of the integrated optical memory.

quant-ph↗