SearcharxivSearch

arXiv subjects

Tianfu Zhang

Publications and source records attributed to Tianfu Zhang.

3 recordsLinked to original sources

Bimodal Synchronization Performance: Why Noise and Sparse Connectivity Can Improve Collective Timing

Pulse-coupled oscillator models inspired by firefly synchronization are widely used to study decentralized time coordination in distributed systems. We analyze a discrete-time, discrete-phase firefly-inspired synchronization model and show that collective synchrony emerges only near a critical balance between the quorum threshold (fraction of pulsing neighbors required to trigger a phase update) and the pulse duration (how long agents remain detectable to others). Within this parameter region, the system exhibits bimodal performance: it either reaches near-perfect synchronization or becomes trapped in stable multi-cluster states, where symmetrically phase-offset subgroups mutually reinforce one another and prevent global synchrony. Our analysis shows that reducing connectivity or introducing noise suppresses these low-performance states by breaking such symmetric interactions, indicating that highly connected or noiseless systems are not necessarily optimal for collective synchronization.

cs.MA

Unlocking Cryogenic Energy Storage by Constructing Dipole Glass with Unit-cell-level Polar Disorder

Cryogenic energy storage is vital for frontier technologies including deep-space exploration and quantum computing, yet conventional electrochemical energy systems fail below ~230 K due to frozen ion migration. While relaxor-based dielectric capacitors provide high efficiency at room temperature, the intrinsic freezing/growth of polar nanodomains at extended cryogenic regime limits their applications with deteriorated hysteresis losses. Here, we realize superior cryogenic energy-storage performance by designing unit-cell-level disordered dipole-glass state in Pb0.6Sr0.4ZrO3 thin films with composition near antiferroelectric-paraelectric phase boundary. The antiferroelectric-derived dipole-glass introduces enhanced unit-cell-level complexity of dipole interaction that suppresses long-range ferroelectric order. This enables ultralow-hysteresis operation (efficiency > 88%) down to 4 K, delivering record-high energy density (211 J/cm^3) at 9 MV/cm, stability over 10^8 charge/discharge cycles and microsecond-scale charge/discharge capability. This work establishes a dipole-glass paradigm for cryogenic dielectric capacitors, opening a new avenue to highly-efficient energy-storage systems with broad applications in frontier nanoelectronics.

cond-mat.mtrl-sci

Antiferroelectric Oxide Thin-Films: Fundamentals, Properties, and Applications

Antiferroelectrics have received blooming interests because of a wide range of potential applications in energy storage, solid-state cooling, thermal switch, transducer, actuation, and memory devices. Many of those applications are the most prospective in thin film form. The antiferroelectric ordering in thin films is highly sensitive to a rich set of factors, such as lattice strain, film thickness, surface and interface effects as well as film stoichiometry. To unlock the full potential of these materials and design high-quality thin films for functional devices, a comprehensive and systematic understanding of their behavior is essential. In conjunction with the necessary fundamental background of antiferroelectrics, we review recent progress on various antiferroelectric oxide thin films, the key parameters that trigger their phase transition and the device applications that rely on the robust responses to electric, thermal, and optical stimuli. Current challenges and future perspectives highlight new and emerging research directions in this field. It is hoped that this review can boost the development of antiferroelectric thin-film materials and device design, stimulating more researchers to explore the unknowns together.

cond-mat.mtrl-sci