Searcharxiv⌕ Search

arXiv subjects

Tianheng Wei

Publications and source records attributed to Tianheng Wei.

7 recordsLinked to original sources

Observation of flat-bottom U-shaped energy gap in high-Tc nickelate (La,Pr)3Ni2O7 thin films

The discovery of high transition temperature (high-Tc) superconductivity in Ruddlesden-Popper (R-P) bilayer nickelates under high pressure has stimulated extensive work to understand the underlying mechanism and search for superconductors with higher Tc. The recent realization of superconductivity in R-P bilayer nickelate thin films with onset Tc above 40 K at ambient-pressure enables the use of a wide array of powerful experimental tools to investigate the unconventional high-Tc superconductivity in bilayer nickelates. Here, using ultra-low temperature scanning tunneling microscopy/spectroscopy (STM/S) and electrical transport study, we report the first successful observation of an energy-symmetric, flat-bottom U-shaped gap with zero residual density of states around the Fermi level in the high-Tc nickelate (La,Pr)3Ni2O7 thin film grown on SrLaAlO4 substrate. Before and after STM/S studies, transport measurements on the same sample reveal consistent superconducting behaviors showing zero resistance, with an onset Tc above 40 K and zero resistance Tc above 20 K. The tunneling spectra exhibit highly unconventional temperature evolution, characterized by a rapid filling of the U-shaped energy gap to a V-shaped gap as the temperature increases. Furthermore, the U-shaped energy gap is reduced under a c-axis magnetic field of 14 T. The energy-symmetric U-shaped gap, taken together with its dependence on magnetic field and temperature, is consistent with the behavior of a superconducting gap, suggesting a nodeless gap function at ultra-low temperatures. Our findings shed new lights on the nature of high-Tc superconductivity and provide an encouraging and thought-provoking hint for a local superconductivity with Tc above liquid nitrogen boiling temperature in nickelate superconductors at ambient or zero pressure.

cond-mat.supr-con↗

A possible superconducting gap signature with filling temperature around 40 K in hexagonal iron telluride islands

Superconductivity in the iron-chalcogenide series FeSe-Fe(Te, Se)-FeTe has been restricted to the near neighbor of iron selenide (FeSe), with a general consensus that iron telluride (FeTe) is not superconducting. In this study, we report the method to grow FeTe islands with atomically flat surface and hexagonal lattice on SrTiO3 (001) substrates, in which a gap structure with a gap-filling temperature close to 40 K is detected by scanning tunneling spectroscopy. Such signature is examined under various conditions and reminiscent of a superconducting gap structure. This work might offer a potential platform to explore new superconductors at ambient pressure.

cond-mat.supr-con↗

Observation of superconducting pair density modulation within lattice unit cell

In unconventional high-temperature (high-Tc) superconductors, the pair density wave state, an exotic superconducting order showing spatially periodic order parameter modulations with the period of several unit cells and translational symmetry breaking, has attracted broad attention. However, the superconducting pair density modulation within a single unit cell (PDM) has never been carefully investigated before. Here, using scanning tunneling microscopy/spectroscopy, we report the observation of PDM in monolayer high-Tc iron chalcogenide films epitaxially grown on SrTiO3(001). The superconductivity modulations are characterized by the superconducting gap size and the coherence peak sharpness. Further analysis shows that the local maxima and minima in the superconducting gap modulation are centered at the crystallographic locations of the chalcogen atoms, revealing the breaking of the glide-mirror symmetry of the chalcogen atoms in monolayer high-Tc iron chalcogenide films grown on SrTiO3(001). Our findings provide precise microscopic information on superconductivity within the lattice unit cell and may promote the understanding of unconventional high-Tc superconductivity.

cond-mat.supr-con↗

Dynamical Coulomb Blockade as a Signature of the Sign-Reversing Cooper Pairing Potential

Coulomb blockade occurs for electrons tunneling into nanoislands because of the quantization of charge. Here, using spectroscopy measurements of nonmagnetic islands grown on a high-Tc superconductor [one-unit-cell (1-UC) FeSe], we systematically investigate the dynamical Coulomb blockade (DCB), which is found to reflect the Cooper pairing potential in the superconducting substrate. The tunneling spectra are acquired on single-crystalline Pb nanoislands and show a clear suppression of the tunnel current around zero bias-voltage with a gap-like structure. The observed spectral gaps can be attributed to DCB based on our comprehensive investigations, including experiments with finely varying island sizes and calculations of the spectra using the P(E) theory of DCB. Our detailed analysis suggests that the observed DCB can be related to the sign-reversing pairing potential in the 1-UC FeSe substrate below the islands. The sign reversal is furthermore revealed in a transition of the superconducting gap of FeSe from a U- to a V-like lineshape as the distance between neighboring doublet islands is decreased, indicating the presence of a nodal-like gap as expected for a sign-reversing superconductor. Our configuration of nonmagnetic nanoislands on a high-Tc superconductor for spectroscopy measurements may serve as a local, spatially sensitive, and tunable probe for detecting the sign-reversing order parameter in unconventional superconductors.

cond-mat.supr-con↗

Intertwined charge and pair density orders in a monolayer high-Tc iron-based superconductor

Symmetry-breaking electronic phase in unconventional high-temperature (high-Tc) superconductors is a fascinating issue in condensed-matter physics, among which the most attractive phases are charge density wave (CDW) phase with four unit-cell periodicity in cuprates and nematic phase breaking the C4 rotational symmetry in iron-based superconductors (FeSCs). Recently, pair density wave (PDW), an exotic superconducting phase with non-zero momentum Cooper pairs, has been observed in high-Tc cuprates and the monolayer FeSC. However, the interplay between the CDW, PDW and nematic phase remains to be explored. Here, using scanning tunneling microscopy/spectroscopy, we detected commensurate CDW and CDW-induced PDW orders with the same period of lambda = 4aFe (aFe is the distance between neighboring Fe atoms) in a monolayer high-Tc Fe(Te,Se) film grown on SrTiO3(001) substrate. Further analyses demonstrate the observed CDW is a smectic order, which breaks both translation and C4 rotational symmetry. Moreover, the smecticity of the CDW order is strongest near the superconducting gap but weakens near defects and in an applied magnetic field, indicating the interplay between the smectic CDW and PDW orders. Our works provide a new platform to study the intertwined orders and their interactions in high-Tc superconductors.

cond-mat.supr-con↗

Anisotropic gap structure and sign reversal symmetry in monolayer Fe(Se,Te)

The iron-based superconductors are an ideal platform to reveal the enigma of the unconventional superconductivity and potential topological superconductivity. Among them, the monolayer Fe(Se,Te)/SrTiO3(001), which is proposed to be topological nontrivial, shows interface-enhanced high-temperature superconductivity in the two dimensional limit. However, the experimental studies on the superconducting pairing mechanism of monolayer Fe(Se,Te) films are still limited. Here, by measuring quasiparticle interference in monolayer Fe(Se,Te)/SrTiO3(001), we report the observation of the anisotropic structure of the large superconducting gap and the sign change of the superconducting gap on different electron pockets. The results are well consistent with the 'bonding-antibonding' s+- wave pairing symmetry driven by spin fluctuations in conjunction with spin-orbit coupling. Our work is of basic significance not only for a unified superconducting formalism in the iron-based superconductors, but also for understanding of topological superconductivity in high-temperature superconductors.

cond-mat.supr-con↗

Discovery of a pair density wave state in a monolayer high-Tc iron-based superconductor

The pair density wave (PDW) is an extraordinary superconducting state where Cooper pairs carry nonzero momentum. It can emerge when the full condensation of zero momentum Cooper pairs is frustrated. Evidence for the existence of intrinsic PDW order in high-temperature (high-Tc) cuprate superconductors and kagome superconductors has emerged recently. However, the PDW order in iron-based high-Tc superconductors has not been observed experimentally. Here, using scanning tunneling microscopy/spectroscopy, we report the discovery of the PDW state in monolayer iron-based high-Tc Fe(Te,Se) films grown on SrTiO3(001) substrates. The PDW state with a period of λ~3.6a_Fe (a_Fe is the distance between neighboring Fe atoms) is observed at the domain walls by the spatial electronic modulations of the local density of states, superconducting gap, and the π-phase shift boundaries of the PDW around the dislocations of the intertwined charge density wave order. The discovery of the PDW state in the monolayer Fe(Te,Se) film provides a low-dimensional platform to study the interplay between the correlated electronic states and unconventional Cooper pairing in high-Tc superconductors.

cond-mat.supr-con↗