arXiv subjects

Tianyou Wang

Publications and source records attributed to Tianyou Wang.

52 records · Page 3Linked to original sources

arXiv2023

Coalescence of immiscible droplets in liquid environments

Hypothesis: Droplet coalescence process is important in many applications and has been studied extensively when two droplets are surrounded by gas. However, the coalescence dynamics would be different when the two droplets are surrounded by an external viscous liquid. The coalescence of immiscible droplets in liquids has not been explored. Experiments: In the present research, the coalescence of two immiscible droplets in low- and high-viscosity liquids is investigated and compared with their miscible counterparts experimentally. The coalescence dynamics is investigated via high-speed imaging, and theoretical models are proposed to analyze the growth of the liquid bridge. Findings: We find that, the liquid bridge $r$ evolves differently due to the constraint from the triple line in the bridge region, which follows $r\propto {{t}^{{2}/{3}}}$ for low-viscosity surroundings. While for high-viscosity surroundings, the liquid bridge grows at a constant velocity ${{u}_{r}}$ which varies with the surrounding viscosity ${{μ}_{s}}$ as ${{u}_{r}}\propto {{μ}_{s}}^{{1}/{2}}$. In the later stage of the bridge growth, the bridge evolution again merges with the well-established power-law regime $r\propto {{t}^{{1}/{2}}}$, being either in low or high-viscosity liquids. Moreover, a new inertia-viscous-capillary timescale is proposed, which unifies the combined influence of inertia, viscous, and capillary forces on the evolution of the liquid bridge in liquid environments, highlighting the joint role of inertia and viscous resistance in the coalescence process.

physics.flu-dyn↗

arXiv2023

Breakup of particle-laden droplets in airflow

The atomisation of suspension containing liquid and dispersed particles is prevalent in many applications. Previous studies of droplet breakup mainly focused on homogeneous fluids, and the heterogeneous effect of particles on the breakup progress is unclear. In this study, the breakup of particle-laden droplets in airflow is investigated experimentally. Combining synchronised high-speed images from the side view and the 45$^\circ$ view, we compare the morphology of particle-laden droplets with that of homogeneous fluids in different breakup modes. The results show that the higher effective viscosity of particle-laden droplets affects the initial deformation, and the heterogeneous effect of particles appears in the later breakup stage. To evaluate the heterogeneous effect of particles quantitatively, we eliminate the effect of the higher effective viscosity of particle-laden droplets by comparing cases corresponding to the same inviscid Weber number. The quantitative comparison reveals that the heterogeneous effect of particles accelerates the fragmentation of liquid film and promotes localised rapid piercing. A correlation length that depends on the particle diameter and the volume fraction is proposed to characterise the length scale of the concentration fluctuation under the combined effect of the initial flattening and later stretching during the droplet breakup process. Based on this correlation length, the fragment size distributions are analysed, and the scaling results agree well with the experimental data.

physics.flu-dyn↗

arXiv2023

Melting process of frozen sessile droplets on superhydrophobic surfaces

Superhydrophobic surfaces can exhibit icephobicity in many ways due to their large contact angles and small rolling angles. The melting process of frozen droplets on superhydrophobic surfaces is still unclear, hindering the understanding of surface icephobicity. In this experimental study of the melting process of frozen sessile droplets on superhydrophobic surfaces, we find two types of melting morphologies with opposite vortex directions on a single-scale nano-structured (SN) superhydrophobic substrate and a hierarchical-scale micro-nano-structured (HMN) superhydrophobic substrate. Melting pattern visualizations and flow field measurements showwed Marangoni convection and natural convection occuring in the melting sessile droplets. For the HMN superhydrophobic substrate, the internal flow was found to be dominated by Marangoni convection due to the temperature gradient along the surface of the droplet. For the SN superhydrophobic substrate, Marangoni convection was inhibited by the superhydrophobic particles at the surface of the droplet, which were shed from the fragile superhydrophobic substrate during the freezing--melting process, as confirmed by surface characterizations of the substrate and flow measurements of a water pool. These results will help researchers better understand the melting process of frozen droplets and in designing novel icephobic surfaces for numerous applications.

physics.flu-dyn↗

arXiv2023

Coalescence of immiscible sessile droplets on a partial wetting surface

Droplet coalescence is a common phenomenon and plays an important role in multi-disciplinary applications. Previous studies mainly consider the coalescence of miscible liquid, even though the coalescence of immiscible droplets on a solid surface is a common process. In this study, we explore the coalescence of two immiscible droplets on a partial wetting surface experimentally and theoretically. We find that the coalescence process can be divided into three stages based on the timescales and force interactions involved, namely (I) the growth of the liquid bridge, (II) the oscillation of the coalescing sessile droplet, and (III) the formation of a partially-engulfed compound sessile droplet and the subsequent retraction. In stage I, the immiscible interface is found not to affect the scaling of the temporal evolution of the liquid bridge, which follows the same 2/3 power law as that of miscible droplets. In Stage II, by developing a new capillary timescale considering both surface and interfacial tensions, we show that the interfacial tension between the two immiscible liquids functions as a nonnegligible resistance to the oscillation which decreases the oscillation periods. In Stage III, a modified Ohnesorge number is developed to characterize the visco-capillary and inertia-capillary timescales involved during the displacement of water by oil; a new model based on energy balance is proposed to analyze the maximum retraction velocity, highlighting that the viscous resistance is concentrated in a region close to the contact line.

physics.flu-dyn↗

arXiv2023

Variation of Critical Crystallization Pressure for the Formation of Square Ice in Graphene Nanocapillaries

Two-dimensional square ice in graphene nanocapillaries at room temperature is a fascinating phenomenon and has been confirmed experimentally. Instead of temperature for bulk ice, the high van der Waals pressure becomes an all-important factor to induce the formation of square ice and needs to be studied further. By all-atom molecular dynamics simulations of water confined between two parallel graphene sheets, which are changed in size (the length and the width of the graphene sheets) over a wide range, we find that the critical crystallization pressure for the formation of square ice in nanocapillary strongly depends on the size of the graphene sheet. The critical crystallization pressure slowly decreases as the graphene size increases, converging to approximately macroscopic crystallization pressure. The unfreezable threshold for graphene size is obtained by estimating the actual pressure and it is difficult to form the square ice spontaneously in practice when the graphene sheet is smaller than the threshold. Moreover, the critical crystallization pressure fluctuates when the graphene size is minuscule, and the range of oscillation narrows as the sheet size increases, converging to the macroscopic behavior of a single critical icing pressure for large sheets. The graphene size also affects the stability and crystallization time of square ice.

physics.flu-dyn↗

arXiv2023

Droplet breakup in airflow with strong shear effect

The deformation and breakup of droplets in airflows is important in spray and atomisation processes, but the shear effect in non-uniform airflow is rarely reported. In this study, the deformation and breakup of droplets in a shear flow of air is investigated experimentally using high-speed imaging, digital image processing, and particle image velocimetry. The results show that in airflow with a strong shear effect, the droplet breakup exhibits unique features due to the uplift and stretching produced by the interaction between the deformed droplet and the shear layer. The breakup process can be divided into three stages according to the droplet morphology and the breakup mechanism, namely the sheet breakup, the swing breakup, and the rim breakup stages. Theoretical analysis reveals that the swing breakup is governed by the transverse Rayleigh-Taylor instability. A regime map of the droplet breakup is produced, and the transitions between different regimes are obtained theoretically. The stretching liquid film during the droplet deformation and the fragment size distribution after droplet breakup are analysed quantitatively, and the results show that they are determined by the competition of breakup at different stages affected by the shear. Finally, the effect of the droplet viscosity is investigated, and the viscosity inhibits the droplet breakup in a strong shear airflow.

physics.flu-dyn↗

arXiv2022

Numerical simulation of secondary breakup of shear-thinning droplets

The breakup of non-Newtonian droplets is ubiquitous in numerous applications. Although the non-Newtonian property can significantly change the droplet breakup process, most previous studies consider Newtonian droplets, and the effects of the non-Newtonian properties on the breakup process are still unclear. This study focuses on the secondary breakup of shear-thinning droplets by numerical simulation. The volume of fluid method is used to capture interface dynamics on adaptive grids. To compare shear-thinning droplets and Newtonian droplets, a new definition of the Ohnesorge number is proposed by considering the characteristic shear rate in the droplet induced by the airflow. The results show that compared with the Newtonian fluid, the shear-thinning properties can change the effective viscosity distribution inside the droplet, alter the local deformation, change the droplet morphology, and affect the transition in the droplet breakup regime.

physics.flu-dyn↗

arXiv2022

Cavity deformation and bubble entrapment during the impact of droplets on a liquid pool

The impact of droplets on a liquid pool is ubiquitous in nature and important in many industrial applications. A droplet impacting on a liquid pool can result in the pinch-off of a regular bubble or entrap a large bubble under certain impact conditions. In this study, the cavity deformation and the bubble entrapment during the impact of droplets on a liquid pool are studied by combined experimental measurements and numerical simulations. The time evolution of the free surface profile obtained in the numerical simulation is in good agreement with the experimental results. The cavity created by the droplet impact affects the pinch-off of regular bubbles and the entrapment of large bubbles. The regular bubble pinch-off is the direct consequence of the capillary wave propagating downward along the interface of the cavity and merging at the bottom of the cavity. In contrast, the large bubble entrapment is due to the merging of the liquid crowns at the mouth of the cavity. Gravity and environmental pressure play important roles in cavity deformation and bubble entrapment after droplet impact on liquid pools. The maximum depth of the cavity decreases as the gravitational effect becomes stronger. The phenomenon of regular bubble pinch-off may disappear as the gravity decreases. We find that the regular bubble pinch-off can transform into large bubble entrapment when increasing environmental pressure. The size of the large bubble entrapped decreases with increasing the environmental pressure due to the larger difference in the pressure and the vorticity around the liquid crown at increased environmental pressure. Finally, the regime map of bubble entrapment after the droplet impact is obtained.

physics.flu-dyn↗

arXiv2022

Two-dimensional partitioned square ice confined in graphene/graphite nanocapillaries

As one of the most fascinating confined water/ice phenomena, two-dimensional square ice has been extensively studied and experimentally confirmed in recent years. Apart from the unidirectional homogeneous square icing patterns considered in previous studies, the multidirectional partitioned square icing patterns are discovered in this study and characterized by molecular dynamics (MD) simulations. Square icing parameters are proposed to quantitatively distinguish the partitioned patterns from the homogeneous patterns and the liquid water. The number of graphene monolayers n is varied in this study, and the results show that it is more energetically favorable to form partitioned square icing patterns when the water molecules are confined between graphite sheets (n >= 2) compared to graphene (n = 1). This phenomenon is insensitive to n as long as n >= 2, because of the short-range nature of the interaction between water molecules and the carbon substrate. Moreover, it is energetically unfavorable to form partitioned square icing patterns for a single layer of water molecules even for n >= 2, verifying that the interaction between layers of water molecules is another dominant factor in the formation of partitioned structures. The conversion from partitioned structure to homogenous square patterns is investigated by changing the pressure and the temperature. Based on the comprehensive MD simulations, this study unveils the formation mechanism of the partitioned square icing patterns.

physics.flu-dyn↗

arXiv2021

Crown rupture during droplet impact on a dry smooth surface at increased pressure

The impact of droplets at increased environmental pressure is important in many industrial applications. Previous studies mainly considered the impact process at standard or reduced environmental pressure, and the effect of high environmental pressure is unclear. In this study, we experimentally investigate the impact of ethanol droplets on dry smooth surfaces at increased environmental pressure. The effects of the environmental pressure on the splashing and rupture of the crown during the impact process are analyzed. The results show that surrounding gas with high environmental pressure can lead to the splashing of the crown in a 'thread rupture' mode and the sizes of the secondary droplets from the rim of the liquid crown increase with the environmental pressure. The threshold for the transition from spreading to splashing during the impact process is obtained based on the theory of aerodynamics analysis of the lamella. At increased environmental pressure, the threshold speed of the impact decreases with increasing the environmental pressure because the wedge of the lamella is prevented from moving forward and is driven to detach from the substrate by the air ahead, which has a higher density due to the higher environmental pressure.

physics.flu-dyn↗

arXiv2021

Droplet splashing during the impact on liquid pools of shear-thinning fluids with yield stress

The impact of droplets on liquid pools is ubiquitous in nature and many industrial applications. Most previous studies of droplet impact focus on Newtonian fluids, while less attention has been paid to the impact dynamics of non-Newtonian droplets, even though non-Newtonian fluids are widely used in many applications. In this study, the splashing dynamics of shear-thinning droplets with yield stress are studied by combined experiments and simulations. The formation and the propagation of the ejecta sheet produced during the splashing process are considered, and the velocity, the radius, and the time of the ejecta sheet emergence are analyzed. The results show that the non-Newtonian fluid properties significantly affect the splashing process. The ejecta sheet of the splashing becomes easier to form as the flow index reduces, the large yield stress can affect the thickness of the ejecta sheet, and the spreading radius collapses into a geometrical radius due to that the inertia force is the dominant factor in the ejecta sheet propagation.

physics.flu-dyn↗

arXiv2020

Droplet deformation and breakup in shear flow of air

The deformation and breakup of droplets in air flows is important in many applications of spray and atomization processes. However, the shear effect of airflow has never been reported. In this study, the deformation and breakup of droplets in the shear flow of air is investigated experimentally using high-speed imaging, digital image processing, and particle image velocimetry. We identify a new breakup mode of droplets, i.e., the butterfly breakup, in which the strong aerodynamic pressure on the lower part of the droplet leads to the deflection of the droplet and then the formation of a butterfly-shaped bag. A regime map of the droplet breakup is produced, and the transitions between different modes are obtained based on scaling analysis. The elongation and the fragmentation of the droplet rim are analyzed, and the results show that they are significantly affected by the shear via the formation and the growth of nodes on the rim.

physics.flu-dyn↗

arXiv2019

A Method for Arbitrary Instance Style Transfer

The ability to synthesize style and content of different images to form a visually coherent image holds great promise in various applications such as stylistic painting, design prototyping, image editing, and augmented reality. However, the majority of works in image style transfer have focused on transferring the style of an image to the entirety of another image, and only a very small number of works have experimented on methods to transfer style to an instance of another image. Researchers have proposed methods to circumvent the difficulty of transferring style to an instance in an arbitrary shape. In this paper, we propose a topologically inspired algorithm called Forward Stretching to tackle this problem by transforming an instance into a tensor representation, which allows us to transfer style to this instance itself directly. Forward Stretching maps pixels to specific positions and interpolate values between pixels to transform an instance to a tensor. This algorithm allows us to introduce a method to transfer arbitrary style to an instance in an arbitrary shape. We showcase the results of our method in this paper.

cs.CV↗

arXiv2019

Two jets during the impact of viscous droplets onto a less-viscous liquid pool

It is generally accepted that the Worthington jet occurs when a droplet impacts onto a liquid pool. However, in this experimental study of the impact of viscous droplets onto a less-viscous liquid pool, we identify another jet besides the Worthington jet, forming a two-jet phenomenon. The two jets, a surface-climbing jet and the Worthington jet, may appear successively during one impact event. By carefully tuning the impact condition, we find that the two-jet phenomenon is jointly controlled by the droplet-pool viscosity ratio, the droplet Weber number, and the droplet-pool miscibility. The mechanism of the surface-climbing jet is completely different from that of the Worthington jet: the liquid in the pool climbs along the surface of the droplet and forms a liquid layer which converges at the droplet apex and produces the surface-climbing jet. This surface-climbing jet has a very high speed, i.e., an order of magnitude higher than the droplet impact speed. The effects of the impact speed, droplet viscosity, droplet size, and surface tension on the surface-climbing jet are also analysed. This study does not only provide physical insights into the mechanism of droplet and jet dynamics, but also be helpful in the optimisation of the droplet impact process in many relevant applications.

physics.flu-dyn↗

arXiv2019

Reduced residence time of droplet impact on heated surfaces

The impact of droplets is a ubiquitous phenomenon, and reducing the residence time of the impact process is important for many potential applications. In this study of the impact dynamics on heated surfaces, we identify a mode of droplet bouncing (bouncing-with-spray mode) that can reduce the residence time significantly compared with the traditional retraction-bouncing mode. Comparing with other strategies to reduce the residence time, this approach induced by heat is simple and reliable. The reduction in the residence time is due to the burst of vapor bubbles in the liquid film, which results in the formation of holes in the liquid film and consequently the recoiling of the liquid film from the holes. A scaling law is proposed for the transition boundary between the retraction-bouncing mode and the bouncing-with-spray mode in the film boiling regime, and it agrees well with the experimental data. This model can also explain the transition between these two modes in the transition boiling regime.

physics.flu-dyn↗

arXiv2018

Flow structure of compound droplets moving in microchannels

Compound droplets can be used in substance encapsulation and material compartmentalization to achieve a precise control over the relevant processes in many applications, such as bioanalysis, pharmaceutical manufacturing, and material synthesis. The flow fields in compound droplets directly affect the performance of these applications, but it is challenging to measure them experimentally. In this study, the flow in compound droplets in axisymmetric microchannels is simulated using the Finite Volume Method, and the interface is captured using the Level Set Method with surface tension accounted for via the Ghost Fluid Method. The combination of the Level Set Method and the Ghost Fluid Method reduces spurious currents that are produced unphysically near the interface, and achieves a precise simulation of the complex flow field within compound droplets. The shape of compound droplets, the vortical patterns, the velocity fields, and the eccentricity are investigated and the effects of the key dimensionless parameters, including the size of the compound droplet, the size of the core droplet, the capillary number, and the viscosity ratio, are analyzed. The flow structures in multi-layered compound droplets are also studied. This study not only unveils the complex flow structure within compound droplets moving in microchannels, but can also be used to achieve a precise control over the relevant processes in a wide range of applications of compound droplets.

physics.flu-dyn↗