arXiv subjects

Tilman Pfau

Publications and source records attributed to Tilman Pfau.

At least 73 records · Page 4Linked to original sources

arXiv2016

Rydberg polaritons in a thermal vapor

We present a pulsed four-wave mixing (FWM) scheme via a Rydberg state to create, store and retrieve collective Rydberg polaritons. The storage medium consists of a gas of thermal Rb atoms confined in a 220 μm thick cell, which are heated above room temperature. The experimental sequence consists of a pulsed excitation of Rydberg polaritons via the D1 line, a variable delay or storage time, and a final retrieval pulse via the D2 line. The lifetime of the Rydberg polaritons is around 1.2 ns, almost entirely limited by the excitation bandwidth and the corresponding motional dephasing of the atoms. The presented scheme combined with a tightly confined atomic ensemble is a good candidate for a deterministic single-photon source, as soon as strong interactions in terms of a Rydberg blockade are added.

physics.atom-ph↗

arXiv2016

Observation of quantum droplets in a strongly dipolar Bose gas

Quantum fluctuations are the origin of genuine quantum many-body effects, and can be neglected in classical mean-field phenomena. Here we report on the observation of stable quantum droplets containing $\sim$ 800 atoms which are expected to collapse at the mean-field level due to the essentially attractive interaction. By systematic measurements on individual droplets we demonstrate quantitatively that quantum fluctuations stabilize them against the mean-field collapse. We observe in addition interference of several droplets indicating that this stable many-body state is phase coherent.

cond-mat.quant-gas↗

arXiv2016

Observation of mixed singlet-triplet Rb$_2$ Rydberg molecules

We present high-resolution spectroscopy of Rb$_\text{2}$ ultralong-range Rydberg molecules bound by mixed singlet-triplet electron-neutral atom scattering. The mixing of the scattering channels is a consequence of the hyperfine interaction in the ground-state atom, as predicted recently by Anderson et al. \cite{Anderson2014b}. Our experimental data enables the determination of the effective zero-energy singlet $s$-wave scattering length for Rb. We show that an external magnetic field can tune the contributions of the singlet and the triplet scattering channels and therefore the binding energies of the observed molecules. This mixing of molecular states via the magnetic field results in observed shifts of the molecular line which differ from the Zeeman shift of the asymptotic atomic states. Finally, we calculate molecular potentials using a full diagonalization approach including the $p$-wave contribution and all orders in the relative momentum $k$, and compare the obtained molecular binding energies to the experimental data.

physics.atom-ph↗

arXiv2015

Pulsed Rydberg four-wave mixing with motion-induced dephasing in a thermal vapor

We report on time-resolved pulsed four-wave mixing (FWM) signals in a thermal Rubidium vapor involving a Rydberg state. We observe FWM signals with dephasing times up to 7 ns, strongly dependent on the excitation bandwidth to the Rydberg state. The excitation to the Rydberg state is driven by a pulsed two-photon transition on ns time scales. Combined with a third cw de-excitation laser, a strongly directional and collective emission is generated according to a combination of the phase matching effect and averaging over Doppler classes. In contrast to a previous report [1] using off-resonant FWM, at a resonant FWM scheme we observe additional revivals of the signal shortly after the incident pulse has ended. We infer that this is a revival of motion-induced constructive interference between the coherent emissions of the thermal atoms. The resonant FWM scheme reveals a richer temporal structure of the signals, compared to similar, but off-resonant excitation schemes. A simple explanation lies in the selectivity of Doppler classes. Our numerical simulations based on a four-level model including a whole Doppler ensemble can qualitatively describe the data.

physics.atom-ph↗

arXiv2015

Photoassociation of spin polarized Chromium

We report the homonuclear photoassociation (PA) of ultracold ${}^{52}\mathrm{Cr}$ atoms in an optical dipole trap. This constitutes the first measurement of PA in an element with total electron spin $\tilde{S}>1$. Although Cr, with its ${}^{7}\mathrm{S}_{3}$ ground and ${}^{7}\mathrm{P}_{4,3,2}$ excited states, is expected to have a complicated PA spectrum we show that a spin polarized cloud exhibits a remarkably simple PA spectrum when circularly polarized light is applied. Over a scan range of 20 GHz below the ${}^{7}\mathrm{P}_{3}$ asymptote we observe two distinct vibrational series each following a LeRoy-Bernstein law for a $C_3 / R^{3}$ potential with excellent agreement. We determine the $C_3$ coefficients of the Hund's case c) relativistic adiabatic potentials to be -1.83$\pm$0.02 a.u. and -1.46$\pm$0.01a.u.. Theoretical non-rotating Movre-Pichler calculations enable a first assignment of the series to $Ω=6_u$ and $5_g$ potential energy curves. In a different set of experiments we disturb the selection rules by a transverse magnetic field which leads to additional PA series.

physics.atom-ph↗

arXiv2015

Probing a scattering resonance in Rydberg molecules with a Bose-Einstein condensate

We present spectroscopy of a single Rydberg atom excited within a Bose-Einstein condensate. We not only observe the density shift as discovered by Amaldi and Segre in 1934, but a line shape which changes with the principal quantum number n. The line broadening depends precisely on the interaction potential energy curves of the Rydberg electron with the neutral atom perturbers. In particular, we show the relevance of the triplet p-wave shape resonance in the Rydberg electron-Rb(5S) scattering, which significantly modifies the interaction potential. With a peak density of 5.5x10^14 cm^-3, and therefore an inter-particle spacing of 1300 a0 within a Bose-Einstein condensate, the potential energy curves can be probed at these Rydberg ion - neutral atom separations. We present a simple microscopic model for the spectroscopic line shape by treating the atoms overlapped with the Rydberg orbit as zero-velocity, uncorrelated, point-like particles, with binding energies associated with their ion-neutral separation, and good agreement is found.

physics.atom-ph↗

arXiv2015

Broad universal Feshbach resonances in the chaotic spectrum of Dysprosium atoms

We report on the observation of weakly-bound dimers of bosonic Dysprosium with a strong universal s-wave halo character, associated with broad magnetic Feshbach resonances. These states surprisingly decouple from the chaotic backgound of narrow resonances, persisting across many such narrow resonances. In addition they show the highest reported magnetic moment $μ\simeq20\,μ_{\rm B}$ of any ultracold molecule. We analyze our findings using a coupled-channel theory taking into account the short range van der Waals interaction and a correction due to the strong dipole moment of Dysprosium. We are able to extract the scattering length as a function of magnetic field associated with these resonances and obtain a background scattering length $a_{\rm bg}=91(16)\,a_0$. These results offer prospects of a tunability of the interactions in Dysprosium, which we illustrate by observing the saturation of three-body losses.

cond-mat.quant-gas↗

arXiv2015

Observing the Rosensweig instability of a quantum ferrofluid

Ferrofluids show unusual hydrodynamic effects due to the magnetic nature of their constituents. For increasing magnetization a classical ferrofluid undergoes a Rosensweig instability and creates self-organized ordered surface structures or droplet crystals. A Bose-Einstein condensate with strong dipolar interactions is a quantum ferrofluid that also shows superfluidity. The field of dipolar quantum gases is motivated by the search for new phases that break continuous symmetries. The simultaneous breaking of continuous symmetries like the phase invariance for the superfluid state and the translational symmetry for a crystal provides the basis of novel states of matter. However, interaction-induced crystallization in a superfluid has not been observed. Here we use in situ imaging to directly observe the spontaneous transition from an unstructured superfluid to an ordered arrangement of droplets in an atomic dysprosium Bose-Einstein condensate. By utilizing a Feshbach resonance to control the interparticle interactions, we induce a finite-wavelength instability and observe discrete droplets in a triangular structure, growing with increasing atom number. We find that these states are surprisingly long-lived and measure a hysteretic behaviour, which is typical for a crystallization process and in close analogy to the Rosensweig instability. Our system can show both superfluidity and, as shown here, spontaneous translational symmetry breaking. The presented observations do not probe superfluidity in the structured states, but if the droplets establish a common phase via weak links, this system is a very good candidate for a supersolid ground state.

cond-mat.quant-gas↗

arXiv2015

Imaging single Rydberg electrons in a Bose-Einstein condensate

The quantum mechanical states of electrons in atoms and molecules are distinct orbitals, which are fundamental for our understanding of atoms, molecules and solids. Electronic orbitals determine a wide range of basic atomic properties, allowing also for the explanation of many chemical processes. Here, we propose a novel technique to optically image the shape of electron orbitals of neutral atoms using electron-phonon coupling in a Bose-Einstein condensate. To validate our model we carefully analyze the impact of a single Rydberg electron onto a condensate and compare the results to experimental data. Our scheme requires only well-established experimental techniques that are readily available and allows for the direct capture of textbook-like spatial images of single electronic orbitals in a single shot experiment.

physics.atom-ph↗

arXiv2015

Atomic vapor spectroscopy in integrated photonic structures

We investigate an integrated optical chip immersed in atomic vapor providing several waveguide geometries for spectroscopy applications. The narrow-band transmission through a silicon nitride waveguide and interferometer is altered when the guided light is coupled to a vapor of rubidium atoms via the evanescent tail of the waveguide mode. We use grating couplers to couple between the waveguide mode and the radiating wave, which allow for addressing arbitrary coupling positions on the chip surface. The evanescent atom-light interaction can be numerically simulated and shows excellent agreement with our experimental data. This work demonstrates a next step towards miniaturization and integration of alkali atom spectroscopy and provides a platform for further fundamental studies of complex waveguide structures.

physics.atom-ph↗

arXiv2014

Quantum correlations and entanglement in far-from-equilibrium spin systems

By applying complementary analytic and numerical methods, we investigate the dynamics of spin-$1/2$ XXZ models with variable-range interactions in arbitrary dimensions. The dynamics we consider is initiated from uncorrelated states that are easily prepared in experiments, and can be equivalently viewed as either Ramsey spectroscopy or a quantum quench. Our primary focus is the dynamical emergence of correlations and entanglement in these far-from-equilibrium interacting quantum systems: we characterize these correlations by the entanglement entropy, concurrence, and squeezing, which are inequivalent measures of entanglement corresponding to different quantum resources. In one spatial dimension, we show that the time evolution of correlation functions manifests a non-perturbative dynamic singularity. This singularity is characterized by a universal power-law exponent that is insensitive to small perturbations. Explicit realizations of these models in current experiments using polar molecules, trapped ions, Rydberg atoms, magnetic atoms, and alkaline-earth and alkali atoms in optical lattices, along with the relative merits and limitations of these different systems, are discussed.

cond-mat.quant-gas↗

arXiv2014

Efficient demagnetization cooling of atoms and its limits

Demagnetization cooling relies on spin-orbit coupling that brings motional and spin degrees of freedom into thermal equilibrium. In the case of a gas, one has the advantage that the spin degree of freedom can be cooled very efficiently using optical pumping. We investigate demagnetization cooling of a chromium gas in a deep optical dipole trap over a large temperature range and reach high densities up to $5\times 10^{19} m^{-3}$. We study the loss mechanism under such extreme conditions and identify excited-state collisions as the main limiting process. We discuss that in some systems demagnetization cooling has a realistic potential of reaching degeneracy by optical cooling only.

cond-mat.quant-gas↗

arXiv2014

Ultracold atom-electron interaction: from two to many-body physics

The transition from a few-body system to a many-body system can result in new length scales, novel collective phenomena or even in a phase transition. Such a threshold behavior was shown for example in 4He droplets, where 4He turns into a superfluid for a specific number of particles [1]. A particularly interesting question in this context is at which point a few-body theory can be substituted by a mean field model, i. e. where the discrete number of particles can be treated as a continuous quantity. Such a transition from two non-interacting fermionic particles to a Fermi sea was demonstrated recently [2]. In this letter, we study a similar crossover to a many-body regime based on ultralong-range Rydberg molecules [3] forming a model system with binary interactions.

physics.atom-ph↗

arXiv2014

Triple stack glass-to-glass anodic bonding for optogalvanic spectroscopy cells with electrical feedthroughs

We demonstrate the use of an anodic bonding technique for building a vacuum tight vapor cell for the use of Rydberg spectroscopy of alkali atoms with thin film electrodes on the inside of the cell. The cell is fabricated by simultaneous triple stack glass-to-glass anodic bonding at 300°C. This glue-free, low temperature sealing technique provides the opportunity to include thin film electric feedthroughs. The pressure broadening is only limited by the vapor pressure of rubidium and the lifetime is at least four months with operating temperatures up to 230°C.

physics.atom-ph↗

arXiv2014

Alignment of D-state Rydberg molecules

We report on the formation of ultralong-range Rydberg D-state molecules via photoassociation in an ultracold cloud of rubidium atoms. By applying a magnetic offset field on the order of 10 G and high resolution spectroscopy, we are able to resolve individual rovibrational molecular states. A full theory, using the Born-Oppenheimer approximation including s- and p-wave scattering, reproduces the measured binding energies. The calculated molecular wavefunctions show that in the experiment we can selectively excite stationary molecular states with an extraordinary degree of alignment or anti-alignment with respect to the magnetic field axis.

physics.atom-ph↗

arXiv2013

Rydberg dressing: Understanding of collective many-body effects and implications for experiments

The strong interaction between Rydberg atoms can be used to control the strength and character of the interatomic interaction in ultracold gases by weakly dressing the atoms with a Rydberg state. Elaborate theoretical proposals for the realization of various complex phases and applications in quantum simulation exist. Also a simple model has been already developed that describes the basic idea of Rydberg dressing in a two-atom basis. However, an experimental realization has been elusive so far. We present a model describing the ground state of a Bose-Einstein condensate dressed with a Rydberg level based on the Rydberg blockade. This approach provides an intuitive understanding of the transition from pure twobody interaction to a regime of collective interactions. Furthermore it enables us to calculate the deformation of a three-dimensional sample under realistic experimental conditions in mean-field approximation. We compare full three-dimensional numerical calculations of the ground state to an analytic expression obtained within Thomas-Fermi approximation. Finally we discuss limitations and problems arising in an experimental realization of Rydberg dressing based on our experimental results. Our work enables the reader to straight forwardly estimate the experimental feasibility of Rydberg dressing in realistic three-dimensional atomic samples.

cond-mat.quant-gas↗

arXiv2013

Ground state of a two component dipolar Fermi gas in a harmonic potential

Interacting two component Fermi gases are at the heart of our understanding of macroscopic quantum phenomena like superconductivity. Changing nature of the interaction is expected to head to novel quantum phases. Here we study the ground state of a two component fermionic gas in a harmonic potential with dipolar and contact interactions. Using a variational Wigner function we present the phase diagram of the system with equal but opposite values of the magnetic moment. We identify the second order phase transition from paramagnetic to ferronematic phase. Moreover, we show the impact of the experimentally relevant magnetic field on the stability and the magnetization of the system. We also investigate a two component Fermi gas with large but almost equal values of the magnetic moment to study how the interplay between contact and dipolar interactions affects the stability properties of the mixture. To be specific we discuss experimentally relevant parameters for ultracold $^{161}$Dy.

cond-mat.quant-gas↗

arXiv2013

Coupling a single electron to a Bose-Einstein condensate

The coupling of electrons to matter is at the heart of our understanding of material properties such as electrical conductivity. One of the most intriguing effects is that electron-phonon coupling can lead to the formation of a Cooper pair out of two repelling electrons, the basis for BCS superconductivity. Here we study the interaction of a single localized electron with a Bose-Einstein condensate (BEC) and show that it can excite phonons and eventually set the whole condensate into a collective oscillation. We find that the coupling is surprisingly strong as compared to ionic impurities due to the more favorable mass ratio. The electron is held in place by a single charged ionic core forming a Rydberg bound state. This Rydberg electron is described by a wavefunction extending to a size comparable to the dimensions of the BEC, namely up to 8 micrometers. In such a state, corresponding to a principal quantum number of n=202, the Rydberg electron is interacting with several tens of thousands of condensed atoms contained within its orbit. We observe surprisingly long lifetimes and finite size effects due to the electron exploring the wings of the BEC. Based on our results we anticipate future experiments on electron wavefunction imaging, investigation of phonon mediated coupling of single electrons, and applications in quantum optics.

physics.atom-ph↗