arXiv subjects

Timothy J. Davis

Publications and source records attributed to Timothy J. Davis.

14 recordsLinked to original sources

arXiv2026

Analysis of the Topology of a Plasmonic Target-Skyrmion Texture

Topological concepts are frequently used to describe structured optical fields, including plasmonic near fields. Topological descriptions in terms of skyrmion numbers implicitly assume the compactness of the underlying manifold. Even when skyrmion-like textures appear locally, the compactness is usually not fulfilled in extended optical fields. Here, we use photoemission electron microscopy to investigate a plasmonic nano-focus that exhibits a sequence of radially extending alternating skyrmion and antiskyrmion textures. The full spatio-temporal reconstruction of the electric field vectors and their topology is accessible by vector polarimetry. The experiments confirm the expected oscillatory behavior of the skyrmion number and demonstrate that a global skyrmion number cannot be assigned in such non-compact fields.

physics.optics↗

arXiv2024

Plasmonic Twistronics: Discovery of Plasmonic Skyrmion Bags

The study of van der Waals heterostructures with an interlayer twist, known as "twistronics", has been instrumental in advancing contemporary condensed matter research. Most importantly, it has underpinned the emergence of a multitude of strongly-correlated phases, many of which derive from the topology of the physical system. Here, we explore the application of the twistronics paradigm in plasmonic systems with nontrivial topology, by creating a moir\'e skyrmion superlattice using two superimposed plasmonic skyrmion lattices, twisted at a "magic" angle. The complex electric field distribution of the moir\'e skyrmion superlattice is measured using time-resolved vector microscopy, revealing that each super-cell possesses very large topological invariants and harbors a "skyrmion bag", the size of which is controllable by the twist angle and center of rotation. Our work shows how twistronics leads to a diversity of topological features in optical fields, providing a new route to locally manipulate electromagnetic field distributions, which is crucial for future structured light-matter interaction.

physics.optics↗

arXiv2024

Spatio-temporal topology of plasmonic spin meron pairs revealed by polarimetric photo-emission microscopy

Topology is the study of geometrical properties and spatial relations unaffected by continuous changes, and has become an important tool for understanding complex physical systems. Although recent optical experiments have inferred the existence of vector fields with the topologies of merons, the inability to extract the full three dimensional vectors misses a richer set of topologies that have not yet been fully explored. In our work, we extend the study of the topology of electromagnetic fields on surfaces to a spin quasi-particle with the topology of a meron pair, formed by interfering surface plasmon polaritons, and show that the in-plane vectors are constrained by the embedding topology of the space as dictated by the Poincare-Hopf theorem. In addition we explore the time evolution of the three dimensional topology of the spin field formed by femtosecond laser pulses. These experiments are possible using our here developed method called polarimetric photoemission electron microscopy (polarimetric PEEM) that combines an optical pump-probe technique and polarimetry with photo-emission electron microscopy. This method allows for the accurate generation of surface plasmon polariton fields and their subsequent measurement, revealing both the spatial distribution of the full three-dimensional electromagnetic fields at deep sub-wavelength resolution and their time evolution.

physics.optics↗

arXiv2024

Skyrmion Bag Robustness in Plasmonic Bilayer and Trilayer Moir\'e Superlattices

Twistronics is studied intensively in twisted 2D heterostructures and its extension to trilayer moir\'e structures has proven beneficial for the tunability of unconventional correlated states and superconductivity in twisted trilayer graphene. Just recently, the concept of twistronics has been applied to plasmonic lattices with nontrivial topology, demonstrating that bilayer moir\'e skyrmion lattices harbor multi-skyrmion textures called skyrmion bags. Here, we explore the properties of plasmonic trilayer moir\'e superlattices that are created by the interference of three twisted skyrmion lattices. More specifically, we explore the properties of periodic superlattices and their topological invariants. We also demonstrate that twisted trilayer skyrmion lattices harbor the same skyrmion bags as twisted bilayer skyrmion lattices. We quantify the robustness of these skyrmion bags by the stability of their topological numbers against certain disturbance fields that leads to experimental designs for topological textures with maximum robustness.

physics.optics↗

arXiv2023

Momentum space separation of quantum path interferences between photons and surface plasmon polaritons in nonlinear photoemission microscopy

Quantum path interferences occur whenever multiple equivalent and coherent transitions result in a common final state. Such interferences strongly modify the probability of a particle to be found in that final state, a key concept of quantum coherent control. When multiple nonlinear and energy-degenerate transitions occur in a system, the multitude of possible quantum path interferences is hard to disentangle experimentally. Here, we analyze quantum path interferences during the nonlinear emission of electrons from hybrid plasmonic and photonic fields using time-resolved photoemission electron microscopy. We experimentally distinguish quantum path interferences by exploiting the momentum difference between photons and plasmons and through balancing the relative contributions of their respective fields. Our work provides a fundamental understanding of the nonlinear photon-plasmon-electron interaction. Distinguishing emission processes in momentum space, as introduced here, will ultimately allow nano-optical quantum-correlations to be studied without destroying the quantum path interferences.

cond-mat.mes-hall↗

arXiv2022

Thin film notch filters as platforms for biological image processing

Many image processing operations involve the modification of the spatial frequency content of images. Here we demonstrate object-plane spatial frequency filtering utilizing the angular sensitivity of a commercial spectral bandstop filter. This approach to all-optical image processing is shown to generate real-time pseudo-3D images of transparent biological and other samples, such as human cervical cancer cells. This work demonstrates the potential of non-local, non-interferometric approaches to image processing for uses in label-free biological cell imaging and dynamical monitoring.

physics.optics↗

arXiv2021

Real time phase imaging with an asymmetric transfer function metasurface

The conversion of phase variations in an optical wavefield into intensity information is of fundamental importance for optical imaging technology including microscopy of biological cells. While conventional approaches to phase-imaging commonly rely on bulky optical components or computational post processing, meta-optical devices have recently demonstrated all-optical, ultracompact image processing methods. Here we describe a metasurface that exploits photonic spin-orbit coupling to create an asymmetric optical transfer function for real time phase-imaging. The effect of the asymmetry on transmission through the device is demonstrated experimentally with the generation of high contrast pseudo-3D intensity images of phase variations in an optical wavefield without the need for post-processing. This non-interferometric method has potential applications in biological live cell imaging and real-time wavefront sensing.

physics.optics↗

arXiv2019

Near-perfect absorber as a subwavelength thickness spatial frequency filter for optical image processing

Spatial frequency filtering is a fundamental enabler of information processing methods in biological and technical imaging. Most filtering methods, however, require either bulky and expensive optical equipment or some degree of computational processing. Here we experimentally demonstrate on-chip, all-optical spatial frequency filtering using a thin-film perfect absorber structure. We give examples of edge enhancement in an amplitude image as well as conversion of a phase gradient in a wave field into an intensity modulation.

physics.optics↗

arXiv2018

Near-Perfect Absorption of Light by Plasmene Sheets

Near-perfect absorbers (NPAs) efficiently absorb visible light with a layered nanostructure that is thinner than the diffusion lengths of photogenerated charge carriers. We overcame existing limitations in fabricating their nanoparticulate surface by depositing \textit{plasmene}, a tightly-packed two-dimensional lattice of metal nanoparticles formed through self-assembly. The plasmene NPAs absorb up to 98\% of incident visible light, with modelling showing the improvement on existing NPAs arises from the structural ordering of the plasmene. We also demonstrate control of NPAs' absorption profile through the use of anisotropic building blocks in plasmene. These property enhancements may broaden the application of NPAs to structural colour, sensing and photocatalysis.

physics.app-ph↗

arXiv2017

Plasmonic Hot-Carrier Extraction: Mechanisms of Electron Emission

When plasmonic nanoparticles are coupled with semiconductors, highly energetic hot carriers can be extracted from the metal-semiconductor interface for various applications in light energy conversion. Hot charge-carrier extraction upon plasmon decay using such an interface has been argued to occur after the formation of an intermediate electron population with a uniform momentum distribution. The efficiency of the charge separation process is thus discussed to be limited by this spatial homogeneity in certain plasmon-induced applications. Here we demonstrate using visible pump, near-infrared probe transient absorption spectroscopy that increases in the contact area between metal and semiconductor leads to an increase in the quantum yield for hot electron injection that is inconsistent with the homogeneous energy-momentum distribution of hot-electrons. Instead, further analysis of the experimental data suggests that the highly energetic electrons are emitted across the interface via a surface charge emission mechanism that occurs via a plasmon excitation

physics.chem-ph↗

arXiv2017

Optical chirality from dark-field illumination of planar plasmonic nanostructures

Dark-field illumination is shown to make planar chiral nanoparticle arrangements exhibit circular dichroism in extinction analogous to true chiral scatterers. Circular dichrosim is experimentally observed at the maximum scattering of single oligomers consisting rotationally symmetric arrangements of gold nanorods, with strong agreement to numerical simulation. A dipole model is developed to show that this effect is caused by a difference in the geometric projection of a nanorod onto the handed orientation of electric fields created by a circularly polarized dark-field that is normally incident on a glass substrate. Owing to this geometric origin, the wavelength of the peak chiral response is also experimentally shown to shift depending on the separation between nanoparticles. All presented oligomers have physical dimensions less than the operating wavelength, and the applicable extension to closely packed planar arrays of oligomers is demonstrated to amplify the magnitude of circular dichroism. The realization of strong chirality in these oligomers demonstrates a new path to engineer optical chirality from planar devices using dark-field illumination.

physics.optics↗

arXiv2017

Plasmonic edge states: an electrostatic eigenmode description

We consider periodic arrangements of metal nanostructures and study the effect of periodicity on the localised surface plasmon resonance of the structures within an electrostatic eigenmode approximation. We show that within this limit, the collective surface plasmon resonances of the periodic structures can be expressed in terms of superpositions of the eigenmodes of uncoupled nanostructures that exhibit a standing--wave character delocalised across the entire periodic structure. The formalism derived successfully enables the design and accounts for the observation of plasmonic edge-states in periodic structures.

physics.optics↗

arXiv2016

Hot Carrier extraction with plasmonic broadband absorbers

Hot charge carrier extraction from metallic nanostructures is a very promising approach for applications in photo-catalysis, photovoltaics and photodetection. One limitation is that many metallic nanostructures support a single plasmon resonance thus restricting the light-to-charge-carrier activity to a spectral band. Here we demonstrate that a monolayer of plasmonic nanoparticles can be assembled on a multi-stack layered configuration to achieve broad-band, near-unit light absorption, which is spatially localised on the nanoparticle layer. We show that this enhanced light absorbance leads to $\sim$ 40-fold increases in the photon-to-electron conversion efficiency by the plasmonic nanostructures. We developed a model that successfully captures the essential physics of the plasmonic hot-electron charge generation and separation in these structures. This model also allowed us to establish that efficient hot carrier extraction is limited to spectral regions where the photons possessing energies higher than the Schottky junctions and the localised light absorption of the metal nanoparticles overlap.

physics.chem-ph↗

arXiv2015

Photo-induced electron transfer in the strong coupling regime: Waveguide-plasmon polaritons

Reversible exchange of photons between a material and an optical cavity can lead to the formation of hybrid light--matter states where material properties such as the work function\cite{Hutchison_AM2013a}, chemical reactivity\cite{Hutchison_ACIE2012a}, ultra--fast energy relaxation \cite{Salomon_ACIE2009a,Gomez_TJOPCB2012a} and electrical conductivity\cite{Orgiu_NM2015a} of matter differ significantly to those of the same material in the absence of strong interactions with the electromagnetic fields. Here we show that strong light--matter coupling between confined photons on a semiconductor waveguide and localised plasmon resonances on metal nanowires modifies the efficiency of the photo--induced charge--transfer rate of plasmonic derived (hot) electrons into accepting states in the semiconductor material. Ultra--fast spectroscopy measurements reveal a strong correlation between the amplitude of the transient signals, attributed to electrons residing in the semiconductor, and the hybridization of waveguide and plasmon excitations.

physics.optics↗