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Tingjun Zhang

Publications and source records attributed to Tingjun Zhang.

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Crystal electric field excitations and an effective-spin-$1/2$ ground doublet in the hyperkagome magnet Yb$_3$Sc$_2$Ga$_3$O$_{12}$

We use inelastic neutron scattering (INS) to determine the crystal electric field (CEF) excitations of Yb$^{3+}$ in the rare-earth hyperkagome magnet Yb$_3$Sc$_2$Ga$_3$O$_{12}$. Three nearly dispersionless magnetic excitations are observed near 58, 68, and 74~meV, corresponding to transitions from the ground-state Kramers doublet to the three excited doublets of the $J=7/2$ multiplet. A Stevens-operator analysis constrained by the local $222$ ($D_2$) symmetry reproduces the excitation energies and spectral weights and yields an Ising-type ground-state $g$ tensor. The first excited doublet lies approximately 58~meV above the ground state, establishing a well-isolated effective $J_{\mathrm{eff}}=1/2$ degree of freedom over the low-temperature regime relevant to collective magnetism. Notably, the directly measured CEF spectrum substantially revises the level scheme previously inferred from bulk measurements, while preserving the essential low-energy pseudospin description. Two independent fitting protocols give consistent excitation energies, ground-doublet wave functions, and $g$ tensors, despite the nonuniqueness of the individual CEF parameters. The resulting single-ion model also reproduces the characteristic susceptibility, magnetization, and field evolution of the Schottky anomaly in specific heat. These results establish the microscopic single-ion basis needed to construct an effective exchange Hamiltonian and to interpret future measurements of low-energy collective excitations in Yb$_3$Sc$_2$Ga$_3$O$_{12}$.

cond-mat.str-el

Spin nematic liquid crystal and scalar spin chirality in tetragonal lattice YbMnBi$_2$

A spin nematic order, analogous to the nematic liquid crystal, characterizes the spontaneous breaking of spin-space rotational symmetry while preserving time-reversal ($T$) symmetry. In contrast, scalar spin chirality (SSC), a composite three-spin order, breaks $T$ symmetry and is known to induce an anomalous Hall effect (AHE). Although a spin nematic phase has been suggested in frustrated magnets and the square-lattice iridate, how it might affect magnetotransport properties is unknown. Here we use polarized neutron scattering to show that tetragonal $A$MnBi$_2$ ($A$ = Ca, Yb) is a strictly $c$-axis-aligned collinear antiferromagnet (C-type), with $T_N \approx 270$ K and 290 K, respectively. On cooling from 450 K to $T_N$, low-energy spin excitations in YbMnBi$_2$ spontaneously change from isotropic to anisotropic in spin space within the tetragonal plane, forming a dynamic spin nematic phase around 400 K due to heavy Yb-induced spin-orbit coupling, before gapping out below $T_N$. Similar measurements on CaMnBi$_2$ reveal isotropic paramagnetic scattering without a spin nematic phase above $T_N$. Under an in-plane magnetic field, the Yb$^{3+}$ moments may interact with the dynamic spin nematic phase to induce nonzero SSC, giving rise to AHE and an anomalous Nernst effect (ANE) in YbMnBi$_2$ that are absent in CaMnBi$_2$ above $T_N$. A symmetry-based Ginzburg-Landau analysis shows that coupling terms between the nematic order and SSC are allowed under an external magnetic field, which could explain the rapid increase of AHE with field in YbMnBi$_2$. Our results provide compelling evidence for dynamic SSC-induced AHE and ANE in the paramagnetic phase of a compensated collinear antiferromagnet, opening a new avenue for the physics of composite spin orders and room-temperature spintronics without magnetic order.

cond-mat.str-el

$d$-spacing distributions as a probe of nematoelastic response in iron-based superconductors

Electronic nematicity in iron-based superconductors (FeSCs) couples bilinearly to orthorhombic strain, allowing nematic correlations to appear in the lattice response. Here we use neutron Larmor diffraction to measure the temperature-dependent distribution of relative $d$ spacings in electron-doped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, hole-doped Ba$_{0.83}$K$_{0.17}$Fe$_2$As$_2$, FeSe, and Fe$_{1.07}$Te. In Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ crystals without intentionally applied uniaxial stress, the in-plane distribution width, $\varepsilon_{\rm FWHM}$, increases on cooling in the tetragonal phase and can be described phenomenologically by a Curie--Weiss-like form. The fitted scale $T^*$ decreases with Co doping and evolves similarly to the nematic phase diagram inferred from elastoresistance, although the two experiments probe different response functions. Related broadening in Ba$_{0.83}$K$_{0.17}$Fe$_2$As$_2$ and FeSe supports extending this interpretation beyond electron-doped BaFe$_2$As$_2$. By contrast, Fe$_{1.07}$Te shows no extended Curie--Weiss-like regime without applied stress, whereas uniaxial pressure produces a strongly anisotropic broadening that can contain contributions from both the field-biased lattice response and inhomogeneous loading. A mean-field model with bilinear nematoelastic coupling and spatially varying symmetry-breaking stress explains the Curie--Weiss-like broadening in terms of the renormalized orthorhombic compliance. Neutron Larmor diffraction therefore provides a bulk-sensitive probe of nematic-related lattice broadening that complements electronic and elastic measurements.

cond-mat.supr-con

Spectroscopic Demarcation of Emergent Photons and Spinons in a Dipolar-Octupolar Quantum Spin Liquid

The identification of fractionalized excitations in quantum spin liquids (QSLs) remains a central challenge in condensed matter physics. In dipolar-octupolar (DO) pyrochlores, such as $\text{Ce}_2\text{Zr}_2\text{O}_7$, the candidate $\pi$-flux quantum spin ice (QSI) state is predicted to host both gapless emergent photons and a continuum of spinons. However, resolving these modes at zero field is complicated by their spectral overlap and the presence of nonmagnetic scattering near zero energy. Here, we report neutron scattering experiments on $\text{Ce}_2\text{Zr}_2\text{O}_7$ under a magnetic field along the $[1,1,1]$ direction. In contrast to previous unpolarized studies at zero-field that relied on high-temperature subtraction, we use a same-temperature high-field subtraction protocol to isolate the photon mode. Leveraging the selective coupling of the magnetic field to the dipolar degrees of freedom, we demonstrate the spectroscopic demarcation of these excitations. We observe that weak fields ($\approx 0.15$ T) suppress the low-energy photon weight while leaving the high-energy spinon continuum robust, albeit hardened. Our results, supported by gauge mean-field theory and exact diagonalization calculations, provide strong evidence for the $\pi$-flux QSI state and introduce a powerful field-tuning protocol for investigating DO-QSLs.

cond-mat.str-el

Evidence for itinerant electron-local moment interaction in Li-doped $\alpha$-MnTe

We use inelastic neutron scattering (INS) and angle-resolved photoemission spectroscopy (ARPES) to study the impact of Li doping on the semiconducting altermagnet $\alpha$-MnTe. Introducing Li results in a spin reorientation from in-plane to out-of-plane direction and increases the density of itinerant carriers. While our ARPES measurements do not indicate any notable doping-induced changes in the electronic band structure or the magnitude of the altermagnetic band splitting, our INS measurements reveal an abrupt carrier-induced decrease in the spin wave lifetime near the zone boundary at high energies. This finding is consistent with a new magnon decay channel driven by doping-induced subtle changes in the band structure and enhanced interactions between Mn$^{2+}$ local moments and itinerant electrons. By extracting the local dynamic susceptibility from INS spectra and applying the total moment sum rule, we find that both undoped and Li-doped $\alpha$-MnTe exhibit the full expected Mn$^{2+}$ local moment of $\approx5.9~\mu_\mathrm{B}$ with $S=5/2$. These findings suggest that $\alpha$-MnTe hosts robust local-moment altermagnetism which shows a breakdown at high energies upon addition of itinerant carriers, highlighting the importance of carrier-spin coupling in magneto-transport and spin dynamic properties of altermagnets even in the dilute-carrier limit.

cond-mat.str-el

Interacting spin and charge density waves in kagome metal FeGe

Unveiling the interplay between spin density wave (SDW) and charge density wave (CDW) orders in correlated electron materials is important to obtain a comprehensive understanding of their electronic, structural, and magnetic properties. Kagome lattice materials are interesting because their flat electronic bands, Dirac points, and van Hove singularities can enable a variety of exotic electronic and magnetic phenomena. The kagome metal FeGe, which exhibits a CDW order deep within an A-type antiferromagnetic (AFM) phase, was found to respond dramatically to post-growth annealing - with the ability to tune the CDW repeatedly from long-range order to no (or extremely weak) order. Additionally, neutron scattering studies suggest that incommensurate magnetic peaks that onsets at $T_{Canting}$ = $T_{SDW} \approx$ 60 K in the system arise from a SDW order instead of the AFM double cone structure. Here we use inelastic neutron scattering to show two distinct spin excitations exist below $T_{Canting}$ corresponding to two coexisting magnetic orders in the system in both sets of annealed samples with and without CDW. While CDW order or no order can dramatically affect the onset temperature of $T_{Canting}$ and elastic incommensurate magnetic scattering, its impact on low-energy spin fluctuations is more limited. In both samples, a pair of gapless incommensurate spin excitations arising from the SDW order wavevector coexist with gapped commensurate spin waves from the A-type AFM order across $T_{Canting}$. Low-energy spin excitations for both samples couple dynamically to the lattice through enhanced magnetic scattering intensity on cooling below $T_{CDW}$, regardless the status of the static long-range CDW order. The incommensurate SDW order in the long-range CDW ordered sample also induces a tiny in-plane lattice distortion of the kagome lattice that is absent in the no CDW ordered sample.

cond-mat.str-el

Strain-tunable anomalous Hall effect in hexagonal MnTe

The ability to control and manipulate time-reversal ($T$) symmetry-breaking phases with near-zero net magnetization is a sought-after goal in spintronic devices. The recently discovered hexagonal altermagnet manganese telluride ($\alpha$-MnTe) is a prime example. It has a compensated altermagnetic ground state where the magnetic moments are aligned in each layer and stacked antiparallel along the $c$ axis, yet it exhibits a spontaneous anomalous Hall effect (AHE) that breaks the $T$-symmetry with a vanishingly small $c$-axis ferromagnetic (FM) moment. However, the presence of three 120$^\circ$ separated in-plane magnetic domains presents a challenge in understanding the origin of the AHE and the effective control of the altermagnetic state. Here we use neutron scattering to show that symmetry breaking anisotropic strain, induced by compressive uniaxial pressure along the nearest-neighbor (NN) Mn-Mn bond directions, detwins $\alpha$-MnTe into a single in-plane magnetic domain. This control over in-plane domains allows us to unambiguously establish that the in-plane moments are aligned along the NNN Mn-Mn bond direction, irrespective of the applied strain directions. Mounting the sample on a piezoelectric strain cell along both NN and NNN directions can drive the sample into a single-domain state that significantly sharpens the AHE hysteresis loop and extends the AHE to lower temperatures. Furthermore, tuning the uniaxial strain reverses the sign of the AHE near room temperature. Remarkably, this is achieved without altering the altermagnetic phase-transition temperature or substantially changing the small $c$-axis FM moment. Combined with our phenomenological model, we argue that these effects result from the modification of the electronic Berry curvature by a combination of both spin-orbit coupling and strain. (See the full abstract in the PDF.)

cond-mat.str-el