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Titus Franz

Publications and source records attributed to Titus Franz.

At least 19 recordsLinked to original sources

Emergence of spin entanglement with the pseudogap onset in the Fermi-Hubbard model

Despite decades of intense theoretical and experimental investigation, the two-dimensional Fermi-Hubbard model still resists a complete microscopic understanding. Conventional approaches typically probe global observables and locally resolved correlation functions. Here, we develop a complementary perspective based on the measurement of entanglement. Using both an ultracold-atom quantum simulator and numerical simulations based on the dynamical vertex approximation, we find that entanglement is closely tied to the onset of the enigmatic pseudogap regime: spin-singlet entanglement emerges only as the pseudogap sets in and, in contrast to classical correlations, remains confined to nearest-neighbour sites in this regime. Our results, therefore, disfavour purely classical-fluctuation theories of the pseudogap and constrain microscopic models to those that develop nearest-neighbour spin-singlet entanglement at the pseudogap onset.

cond-mat.str-el

Observation of Strong-to-Weak Spontaneous Symmetry Breaking in a Dephased Fermi Gas

Symmetry-based classification of quantum phases of matter is one of the most foundational organizing principles in physics; however, an analogous framework for mixed, decohered quantum states has only begun to emerge. A central new concept is strong-to-weak spontaneous symmetry breaking (SW-SSB), a sharp transition in mixed quantum states that is invisible to any observable linear in the density matrix and that has since been predicted across a broad class of open and monitored quantum systems. It also provides a unifying language for phenomena as disparate as the decodability of topological quantum memories and the emergence of classical hydrodynamics from decohered quantum dynamics. Here we report the first experimental observation of SW-SSB, in dephased single-component fermionic matter imaged by a quantum gas microscope. A quantum-classical estimator built on a machine-learned Gaussian reference state gives direct access to the nonlinear R\'enyi-1 and R\'enyi-2 correlators that diagnose SW-SSB, and reveals long-range R\'enyi order in the dephased Fermi liquid. Adding a commensurate superlattice drives the underlying fermions through a metal-to-insulator transition that, after full dephasing, manifests as a sharp SW-SSB phase transition. Our results uncover the symmetry principle behind information-theoretic transitions in open quantum systems, and extend Landau's symmetry paradigm into the regime of real, decohering quantum devices.

cond-mat.quant-gas

Realizing the Emery Model in Optical Lattices for Quantum Simulation of Cuprates and Nickelates

The microscopic origin of high-temperature superconductivity in cuprates remains one of the central open questions in condensed matter physics. Growing experimental and theoretical evidence suggests that the bare single-band Fermi-Hubbard model may not fully capture properties of cuprates such as superconductivity, motivating us to revisit the canonical three-band model of the copper-oxide planes - the Emery model - from which the single-band counterpart was originally derived. Here, we propose and analyze a quantum simulation scheme for realizing the Emery model in regimes relevant to cuprates and infinite-layer nickelates with today's ultracold atom quantum simulation platforms, enabling the exploration of the three-band physics on system sizes that are challenging for current numerical methods. Specifically, we show that a two-dimensional optical lattice with a superimposed pattern of repulsive potentials can be designed to study low-temperature properties for variable parameter regimes of the Emery model relevant to cuprates as well as infinite-layer nickelates. Our results pave the way for real material simulations with ultracold atom quantum simulators and a better understanding of the physics of unconventional superconductors.

cond-mat.quant-gas

Constructing Arbitrary Coherent Rearrangements in Optical Lattices

Coherent control of motional degrees of freedom of ultracold atoms in optical lattices offers a promising route towards programmable quantum dynamics with massive particles. We propose and analyze a scheme for implementing coherent rearrangement of ultracold atoms, corresponding to arbitrary unitary transformations on single-particle motional states. Exploiting an analogy between dynamics in optical superlattices and discrete linear optics, we employ the Clements scheme to systematically construct any global $N$-dimensional single-particle unitary from tunneling and phase shifts in arrays of double wells. Tunneling is controlled globally, while local operations are achieved through site-resolved potential shifts. We numerically investigate the susceptibility of the scheme to intensity noise and addressing crosstalk. We identify key subroutines enabled by this unitary construction, including the Discrete Fourier Transform and the implementation of non-native Hamiltonians. Extending the scheme to two dimensions enables all-to-all atomic rearrangement with a circuit depth that scales sublinearly with the atom number, providing a high-density and highly scalable approach to atom rearrangement.

quant-ph

Quantum information scrambling in strongly disordered Rydberg spin systems

Despite the fact that power-law interactions occur in a plethora of physical systems, their many-body dynamics is far less understood than that of nearest-neighbor interacting systems. Here, we study information scrambling in strongly disordered spin systems with power-law interactions via out-of-time-order correlators (OTOCs). Numerically, we find pronounced differences in the dynamical spreading of OTOCs between nearest-neighbor and power-law interacting systems. This deviation persists even for short-range interactions, opposing the common view that these interactions produce dynamics equivalent to the nearest-neighbor case. In a detailed experimental proposal, tailored but not limited to Rydberg tweezer setups, we present a protocol to extract OTOCs in XXZ Heisenberg spin systems with tunable anisotropy and programmable disorder based on currently available techniques.

quant-ph

Phase-Sensitive Measurements on a Fermi-Hubbard Quantum Processor

Fermionic quantum processors are a promising platform for quantum simulation of correlated fermionic matter. In this work, we study a hardware-efficient protocol for measuring complex expectation values of the time-evolution operator, commonly referred to as Loschmidt echoes, with fermions in an optical superlattice. We analyze the algorithm for the Fermi-Hubbard model at half-filling as well as at finite doping. The method relies on global quench dynamics and short imaginary time evolution, the latter being realized by architecture-tailored pulse sequences starting from a product state of plaquettes. Our numerical results show that complex Loschmidt echoes can be efficiently obtained for large many-body states over a broad spectral range. This allows one to measure spectral properties of the Fermi-Hubbard model, such as the local density of states, and paves the way for the study of finite-temperature properties in current fermionic quantum simulators.

quant-ph

Observation of hysteresis in an isolated quantum system of disordered Heisenberg spins

We find energy-dependent hysteresis in an isolated Heisenberg quantum spin system, similar to thermomagnetic hysteresis in canonical spin glasses in contact with a thermal reservoir. Analogous to zero-field cooling and field cooling in conventional magnetic materials, an annealing protocol is devised to control the energy in an isolated system. Depending on the strength of disorder, the susceptibilities at zero field bifurcate at a specific energy, which signals the presence of different magnetic regimes. This behavior is apparent both in a numerical simulation by exact diagonalization of the Heisenberg Hamiltonian with twelve particles, as well as in an experiment with thousands of Rydberg atoms representing dipolar interacting quantum spins. The annealing protocols open a new path to explore the energy-dependent phase structure of spin systems at low energies. Our observation of a nonthermal metastable regime might indicate the existence of a phase transition to a novel state of isolated quantum spin systems.

quant-ph

High-fidelity collisional quantum gates with fermionic atoms

Quantum simulations of electronic structure and strongly correlated quantum phases are widely regarded as among the most promising applications of quantum computing. These computations naturally benefit from native fermionic encodings, which intrinsically restrict the Hilbert space to physical states consistent with fermionic statistics and conservation laws like particle number and magnetization independent of gate errors. While ultracold atoms in optical lattices are established as powerful analog simulators of strongly correlated fermionic matter, neutral-atom platforms have concurrently emerged as versatile, scalable architectures for spin-based digital quantum computation. Unifying these capabilities requires high-fidelity gates that preserve motional degrees of freedom of fermionic atoms, paving the way for a new generation of programmable fermionic quantum processors. Here we demonstrate collisional entangling gates with fidelities up to 99.75(6)% and Bell state lifetimes exceeding $10\,s$, realized via controlled interactions of fermionic atoms in an optical superlattice. Using quantum gas microscopy, we microscopically characterize spin-exchange and pair-tunneling gates, and realize a robust, composite pair-exchange gate, a fundamental primitive for quantum chemistry simulations. Our results establish controlled collisions in optical lattices as a competitive and complementary approach to high entangling gate fidelities in neutral-atom quantum computers. When embedded within a fermionic architecture, this capability enables the preparation of complex quantum states and advanced readout protocols for a new class of scalable analog-digital hybrid quantum simulators. Combined with local addressing, these gates mark a crucial step towards a fully digital fermionic quantum computer based on the controlled motion and entanglement of fermionic neutral atoms.

cond-mat.quant-gas

Observation of emergent scaling of spin-charge correlations at the onset of the pseudogap

In strongly correlated materials, interacting electrons are entangled and form collective quantum states, resulting in rich low-temperature phase diagrams. Notable examples include cuprate superconductors, in which superconductivity emerges at low doping out of an unusual "pseudogap" metallic state above the critical temperature. The Fermi-Hubbard model, describing a wide range of phenomena associated with strong electron correlations, still offers major computational challenges despite its simple formulation. In this context, ultracold atoms quantum simulators have provided invaluable insights into the microscopic nature of correlated quantum states. Here, we use a quantum gas microscope Fermi-Hubbard simulator to explore a wide range of dopings and temperatures in a regime where a pseudogap is known to develop. By measuring multi-point correlation functions up to fifth order, we uncover a novel universal scaling behaviour in magnetic and higher-order spin-charge correlations characterised by a doping-dependent temperature scale. Accurate comparisons with determinant Quantum Monte Carlo and Minimally Entangled Typical Thermal States simulations confirm that this temperature scale is comparable to the pseudogap temperature T*. Our quantitative findings reveal a novel qualitative behaviour of magnetic properties and spin-charge correlations in an emergent pseudogap and pave the way towards the exploration of charge pairing and collective phenomena expected at lower temperatures.

cond-mat.str-el

Local control and mixed dimensions: Exploring high-temperature superconductivity in optical lattices

The simulation of high-temperature superconducting materials by implementing strongly correlated fermionic models in optical lattices is one of the major objectives in the field of analog quantum simulation. Here we show that local control and optical bilayer capabilities combined with spatially resolved measurements create a versatile toolbox to study fundamental properties of both nickelate and cuprate high-temperature superconductors. On the one hand, we present a scheme to implement a mixed-dimensional (mixD) bilayer model that has been proposed to capture the essential pairing physics of pressurized bilayer nickelates. This allows for the long-sought realization of a state with long-range superconducting order in current lattice quantum simulation machines. In particular, we show how coherent pairing correlations can be accessed in a partially particle-hole transformed and rotated basis. On the other hand, we demonstrate that control of local gates enables the observation of $d$-wave pairing order in the two-dimensional (single-layer) repulsive Fermi-Hubbard model through the simulation of a system with attractive interactions. Lastly, we introduce a scheme to measure momentum-resolved dopant densities, providing access to observables complementary to solid-state experiments -- which is of particular interest for future studies of the enigmatic pseudogap phase appearing in cuprates.

cond-mat.quant-gas

Optical superlattice for engineering Hubbard couplings in quantum simulation

Quantum simulations of Hubbard models with ultracold atoms rely on the exceptional control of coherent motion provided by optical lattices. Here we demonstrate enhanced tunability using an optical superlattice in a fermionic quantum gas microscope. With our phase-stable bichromatic design, we achieve a precise control of tunneling and tilt throughout the lattice, as evidenced by long-lived coherent double-well oscillations and next-nearest-neighbor quantum walks in a staggered configuration. We furthermore present correlated quantum walks of two particles initiated through a resonant pair-breaking mechanism. Finally, we engineer tunable spin couplings through local offsets and create a spin ladder with ferromagnetic and antiferromagnetic couplings along the rungs and legs, respectively. Our work underscores the high potential of optical superlattices for engineering, simulating, and detecting strongly correlated many-body quantum states.

cond-mat.quant-gas

Time-reversal in a dipolar quantum many-body spin system

Time reversal in a macroscopic system is contradicting daily experience. It is practically impossible to restore a shattered cup to its original state by just time reversing the microscopic dynamics that led to its breakage. Yet, with the precise control capabilities provided by modern quantum technology, the unitary evolution of a quantum system can be reversed in time. Here, we implement a time-reversal protocol in a dipolar interacting, isolated many-body spin system represented by Rydberg states in an atomic gas. By changing the states encoding the spin, we flip the sign of the interaction Hamiltonian, and demonstrate the reversal of the relaxation dynamics of the magnetization by letting a demagnetized many-body state evolve back-in-time into a magnetized state. We elucidate the role of atomic motion using the concept of a Loschmidt echo. Finally, by combining the approach with Floquet engineering, we demonstrate time reversal for a large family of spin models with different symmetries. Our method of state transfer is applicable across a wide range of quantum simulation platforms and has applications far beyond quantum many-body physics, reaching from quantum-enhanced sensing to quantum information scrambling.

quant-ph

Formation of stripes in a mixed-dimensional cold-atom Fermi-Hubbard system

The relation between d-wave superconductivity and stripes is fundamental to the understanding of ordered phases in cuprates. While experimentally both phases are found in close proximity, numerical studies on the related Fermi-Hubbard model have long been investigating whether stripes precede, compete or coexist with superconductivity. Such stripes are characterised by interleaved charge and spin density wave ordering where fluctuating lines of dopants separate domains of opposite antiferromagnetic order. Here we show first signatures of stripes in a cold-atom Fermi-Hubbard quantum simulator. By engineering a mixed-dimensional system, we increase their typical energy scales to the spin exchange energy, enabling us to access the interesting crossover temperature regime where stripes begin to form. We observe extended, attractive correlations between hole dopants and find an increased probability to form larger structures akin to stripes. In the spin sector, we study correlation functions up to third order and find results consistent with stripe formation. These higher-order correlation measurements pave the way towards an improved microscopic understanding of the emergent properties of stripes and their relation to other competing phases. More generally, our approach has direct relevance for newly discovered high-temperature superconducting materials in which mixed dimensions play an essential role.

cond-mat.quant-gas

Pair localization in dipolar systems with tunable positional disorder

Strongly interacting quantum systems subject to quenched disorder exhibit intriguing phenomena such as glassiness and many-body localization. Theoretical studies have mainly focused on disorder in the form of random potentials, while many experimental realizations naturally feature disorder in the interparticle interactions. Inspired by cold Rydberg gases, where such disorder can be engineered using the dipole blockade effect,we study a Heisenberg XXZ spin model where the disorder is exclusively due to random spin-spin couplings, arising from power-law interactions between randomly positioned spins. Using established spectral and eigenstate properties and entanglement entropy, we show that this system exhibits a localization crossover and identify strongly interacting pairs as emergent local conserved quantities in the system, leading to an intuitive physical picture consistent with our numerical results.

quant-ph

Observation of anisotropy-independent magnetization dynamics in spatially disordered Heisenberg spin systems

An important step towards a comprehensive understanding of far-from-equilibrium dynamics of quantum many-body systems is the identification of unifying features that are independent of microscopic details of the system. We experimentally observe such robust features in the magnetization relaxation dynamics of disordered Heisenberg XX-, XXZ- and Ising Hamiltonians. We realize these Heisenberg spin models with tunable anisotropy parameter and power-law interactions in an ensemble of Rydberg atoms by encoding the spin in suitable Rydberg state combinations. We consistently observe stretched-exponential relaxation of magnetization for all considered spin models, collapsing onto a single curve after appropriate rescaling of time. This robust short-time relaxation behavior is explained by a perturbative treatment that exploits the strong disorder in pairwise couplings, which leads to a description in terms of approximately independent pairs of spins. In numerical simulations of small systems, we show that these pairs of spins constitute approximate local integrals of motion, which remain at least partially conserved on a timescale exceeding the duration of the relaxation dynamics of the magnetization.

quant-ph

Emergent pair localization in a many-body quantum spin system

Understanding how closed quantum systems dynamically approach thermal equilibrium presents a major unresolved problem in statistical physics. Generically, non-integrable quantum systems are expected to thermalize as they comply with the Eigenstate Thermalization Hypothesis. However, in the presence of strong disorder, the dynamics can possibly slow down to a degree that systems fail to thermalize on experimentally accessible timescales, as in spin glasses or many-body localized systems. In general, particularly in long-range interacting quantum systems, the specific nature of the disorder necessary for the emergence of a prethermal, metastable state--distinctly separating the timescales of initial relaxation and subsequent slow thermalization--remains an open question. We study an ensemble of Heisenberg spins with a tunable distribution of random coupling strengths realized by a Rydberg quantum simulator. We observe a drastic change in the late-time magnetization when increasing disorder strength. The data is well described by models based on pairs of strongly interacting spins, which are treated as thermal for weak disorder and isolated for strong disorder. Our results indicate a crossover into a pair-localized prethermal regime in a closed quantum system of thousands of spins in the critical case where the exponent of the power law interaction matches the spatial dimension.

quant-ph

Nonlinear absorption in interacting Rydberg electromagnetically-induced-transparency spectra on two-photon resonance

We experimentally investigate the nonlinear transmission spectrum of coherent light fields propagating through a Rydberg EIT medium with strong atomic interactions. In contrast to previous investigations, which have largely focused on resonant control fields, we explore here the full two-dimensional spectral response of the Rydberg gas. Our measurements confirm previously observed spectral features for a vanishing control-field detuning, but also reveal significant differences on two-photon resonance. In particular, we find qualitative deficiencies of mean-field models and rate-equation simulations as well as a third-order nonlinear susceptibility that accounts for pair-wise interaction effects at low probe-field intensities in describing the nonlinear probe-field response under EIT conditions. Our results suggest that a more complete understanding of Rydberg-EIT and emerging photon interactions requires to go beyond existing simplified models as well as few-photon theories.

physics.atom-ph

A stationary Rydberg polariton

We propose a novel scheme for coupling a Rydberg state to a stationary light polariton, based on a dual-V level scheme. We investigate the properties of the resulting stationary Rydberg polariton, and show that its form and its quadratic dispersion relation closely resemble that of the stationary light polariton of the underlying dual-V scheme. We consider the influence of a Rydberg impurity on the system and find strong interaction-induced absorption of the involved probe field. The proposed scheme for a stationary Rydberg polariton might find applications for realizing interacting polaritons with increased interaction time.

quant-ph