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Tobias Ritschel

Publications and source records attributed to Tobias Ritschel.

At least 19 recordsLinked to original sources

Extraordinary Lifetime Enhancement of Coherent Phonon-Amplitude Modes in the Excitonic Insulator Phase of Ta2Pd3Te5

The excitonic insulator (EI) is an electronic phase of condensed excitons. However, in many prototypical materials the presence of a concurrent structural transition complicates the identification of a purely electronic origin of the ordered state. Here, we investigate Ta2Pd3Te5, in which an EI phase develops below TC ~ 100 K in the absence of a detectable structural transition. We characterize the excitonic condensate via its coherent phonon-amplitude response. Most strikingly, an extraordinarily strong lifetime enhancement of these modes sets in below TC which we establish as a new and robust fingerprint linked to exciton condensation. We discuss possibilities to capture the enhancement when taking into account a coupling of excitonic and lattice effects in line with the coupled phonon-amplitude response. Within an order-parameter polaron picture coupling to the excitonic state may dress the phonon mode and thereby suppress its relaxation and a phenomenological model combines the anharmonic phonon response and a reduced electronic scattering due to the gap opening in the EI phase.

cond-mat.str-el↗

Volumetric Inverse Rendering via Neural Radiative Transfer

Volumetric inverse rendering seeks to recover the optical properties of participating media from images. Existing approaches either rely on differentiable stochastic light transport simulation, which require substantial algorithmic effort, or use simplified models that fail to capture global illumination. We propose a formulation that reconciles physically complete light transport with general-purpose neural optimization. The optical properties of the medium and the full light field are represented as neural fields and estimated through a joint optimization process. Global illumination is enforced via a residual objective derived from the Radiative Transfer Equation in local differential form, complemented by a volume rendering term along primary viewing rays to mitigate \rev{low-frequency} bias. We demonstrate reconstruction of spatially varying, color-resolved scattering, absorption, and phase function parameters from multi-view images. Beyond reconstruction, the same framework supports learning generative models of participating media with physical optical properties under global illumination.

cs.GR↗

Uniaxial-Stress-Induced Magnetic Transitions in the Triangular-Lattice Antiferromagnet PdCrO2

Uniaxial stress is a promising method to tune magnetic frustration, allowing its effects to be studied in a precise way. In this work, uniaxial stress is applied to the triangular-lattice antiferromagnet PdCrO2. The Cr-Cr magnetic interaction is very sensitive to interatomic separation, so laboratory-achievable stress can induce substantial changes in magnetic structure. Results from three types of measurement are presented: X-ray diffraction, the stress-strain relationship, and neutron diffraction. The combined data show that the elastic moduli of PdCrO2 are strongly affected by stress-induced changes in magnetic structure. A new, first-order stress-induced magnetic transition is observed, at which the lattice constant shrinks by 0.21%. The lattice stiffens dramatically across this transition: the Young's modulus increases by about 80 GPa, and the Poisson ratio falls from about 1 to about 0.4. This stiffening indicates that the magnetic order "locks," that is, becomes insensitive to lattice strain. This locking might occur because the new stress-induced magnetic order nests the Fermi surface of the Pd sheets. Other frustrated magnets, including candidate spin liquids, may show similarly strong coupling between magnetic and elastic degrees of freedom.

cond-mat.str-el↗

An evaluation framework for sparse 4D (3D + time) imaging reconstruction via bootstrapped cross-validation

Four-dimensional (4D; 3D + time) microscopic imaging has emerged as a powerful technique for investigating dynamic phenomena in complex systems, enabling direct visualization of structural evolution in space and time. However, when pushing the limits of spatiotemporal resolution, most time-resolved imaging techniques yield inherently sparse 4D datasets. While deep learning-based reconstruction methods have shown promise in reconstructing 4D from sparse spatiotemporal measurements, a practical approach for evaluating their performance in the absence of a 4D reference has, to the best of our knowledge, been lacking. Here, we present a bootstrapped cross-validation framework that estimates reconstruction performance by quantifying correlations between reconstructions generated from independently sampled subsets of the acquired data, as inspired by the 3D validation strategy in cryo-electron microscopy, where reconstructions from split datasets are compared to assess resolutions. This enables both qualitative and quantitative assessment in the absence of ground truth. We investigate two representative scenarios with sparse and ultra-sparse X-ray datasets and validate this approach using 4D-ONIX, a 4D deep-learning reconstruction method, on simulated water droplet collision experiments. The proposed approach provides a reference-free framework for performance estimation and support for better-informed experimental strategies across a wide range of ultrafast imaging applications.

eess.IV↗

Photons x Force: Differentiable Radiation Pressure Modeling

We propose a system to optimize parametric designs subject to radiation pressure, \ie the effect of light on the motion of objects. This is most relevant in the design of spacecraft, where radiation pressure presents the dominant non-conservative forcing mechanism, which is the case beyond approximately 800 km altitude. Despite its importance, the high computational cost of high-fidelity radiation pressure modeling has limited its use in large-scale spacecraft design, optimization, and space situational awareness applications. We enable this by offering three innovations in the simulation, in representation and in optimization: First, a practical computer graphics-inspired Monte-Carlo (MC) simulation of radiation pressure. The simulation is highly parallel, uses importance sampling and next-event estimation to reduce variance and allows simulating an entire family of designs instead of a single spacecraft as in previous work. Second, we introduce neural networks as a representation of forces from design parameters. This neural proxy model, learned from simulations, is inherently differentiable and can query forces orders of magnitude faster than a full MC simulation. Third, and finally, we demonstrate optimizing inverse radiation pressure designs, such as finding geometry, material or operation parameters that minimizes travel time, maximizes proximity given a desired end-point, minimize thruster fuel, trains mission control policies or allocated compute budget in extraterrestrial compute.

cs.GR↗

Uniaxial strain-driven ferroelastic domain control in LaAlO3

Multiferroic domain walls in functional oxides exhibit properties distinct from the bulk and are increasingly exploited as active elements in nanoelectronic and photonic devices. Deterministic control of domain populations has typically remained limited to local control, or removal with temperature. Here we demonstrate continuous, reversible manipulation of the ferroelastic domain structure in single-crystal LaAlO$_3$ using in-situ uniaxial strain. Combining atomic force microscopy, X-ray diffraction, and Raman spectroscopy with first-principles calculations we map the complete microscopic evolution of the twin domain population through the strain-driven transition from the rhombohedral $R\bar{3}c$ ground state toward the predicted orthorhombic $Fmmm$ phase. Applied strains below $0.5\%$ produce pronounced surface flattening and large-scale domain reorganisation, establishing uniaxial strain as a technically accessible control parameter for ferroelastic domain engineering. These results open a route to active, real-time programming of domain architectures in LaAlO$_3$-based heterostructures, with implications for strain-tunable superconducting interfaces, nanoscale phonon-polariton optics, and ultrafast lattice control.

cond-mat.mtrl-sci↗

Cross-Atlantic Research Agenda for Scalable Grid Architectures and Distributed Flexibility

Electric power systems are rapidly evolving into deeply digital, cyber-physical infrastructures in which large fleets of distributed energy resources must be coordinated as system-level flexibility across multiple spatial and temporal scales. Despite growing distributed energy resource deployment, existing grid and market architectures lack scalable, interoperable mechanisms to reliably translate device-level flexibility into grid-aware services, creating risks to reliability, affordability, and resilience at high penetration. We propose that scalable and reliable coordination of distributed energy resource-based flexibility in future power systems is fundamentally an architectural problem that can be addressed through laminar cyber-physical design using minimal, standardized interoperability interfaces that link device autonomy with system-level objectives. To assess this claim, we present and discuss a layered cyber-physical systems architecture and explicate its implementation through standards-based interfaces, Flexibility Functions, hierarchical control, and case studies spanning U.S. and Danish regulatory, market, and operational contexts. Empirical evidence from New York's Grid of the Future proceedings, Danish Smart Energy Operating System pilots, and operational aggregator deployments demonstrates that such architecture enables predictable, grid-aware flexibility while preserving device autonomy, interoperability, reliability, and quality of service. These results support a cross-Atlantic research agenda centered on joint testbeds, harmonized interoperability mechanisms, and coordinated policy experiments to accelerate the deployment of resilient, scalable, and flexible clean energy systems.

eess.SY↗

SAMa: Material-aware 3D Selection and Segmentation

Decomposing 3D assets into material parts is a common task for artists, yet remains a highly manual process. In this work, we introduce Select Any Material (SAMa), a material selection approach for in-the-wild objects in arbitrary 3D representations. Building on SAM2's video prior, we construct a material-centric video dataset that extends it to the material domain. We propose an efficient way to lift the model's 2D predictions to 3D by projecting each view into an intermediary 3D point cloud using depth. Nearest-neighbor lookups between any 3D representation and this similarity point cloud allow us to efficiently reconstruct accurate selection masks over objects' surfaces that can be inspected from any view. Our method is multiview-consistent by design, alleviating the need for costly per-asset optimization, and performs optimization-free selection in seconds. SAMa outperforms several strong baselines in selection accuracy and multiview consistency and enables various compelling applications, such as replacing the diffuse-textured materials on a text-to-3D output with PBR materials or selecting and editing materials on NeRFs and 3DGS captures.

cs.CV↗

Learning Neural Antiderivatives

Neural fields offer continuous, learnable representations that extend beyond traditional discrete formats in visual computing. We study the problem of learning neural representations of repeated antiderivatives directly from a function, a continuous analogue of summed-area tables. Although widely used in discrete domains, such cumulative schemes rely on grids, which prevents their applicability in continuous neural contexts. We introduce and analyze a range of neural methods for repeated integration, including both adaptations of prior work and novel designs. Our evaluation spans multiple input dimensionalities and integration orders, assessing both reconstruction quality and performance in downstream tasks such as filtering and rendering. These results enable integrating classical cumulative operators into modern neural systems and offer insights into learning tasks involving differential and integral operators.

cs.LG↗

Strain-control of electronic superlattice domains in CsV$_{3}$Sb$_{5}$

The kagome metals AV$_{3}$Sb$_{5}$ (A = K, Rb, Cs) provide a unique platform to investigate the physics of interacting electrons, a central challenge in condensed matter physics. A key obstacle in unraveling their correlated behavior is to determine which structural and electronic degrees of freedom are involved and how they couple. Here we address this important issue with a novel approach, namely by exploring the strain dependence of electronic superlattices in CsV$_{3}$Sb$_{5}$. Using high-resolution x-ray diffraction, we track the detwinning of the $2\times 2\times 4$ electronic crystal and uncover a gigantic strain response of its domains. We further show that the detwinned $2\times 2\times 4$ phase exhibits an intrinsic 2$\textbf{q}$-modulation and strong mode coupling. Density functional theory reveals that the structural $2\times 2\times 4$ modulation couples strongly to the V $3d$-orbitals, naturally explaining its pronounced strain response. In contrast, the $2\times 2\times 2$ phase at lower temperatures remains essentially unaffected by small uniaxial strain. This dichotomy points to fundamental differences in the symmetry breaking and stabilization mechanisms of the two electronic orders. More specifically, our results provide evidence for the active role of orbital degrees of freedom, which can realize distinct, complex ordering patterns driven by competing interactions.

cond-mat.str-el↗

Generative Video Bi-flow

We propose a novel generative video model to robustly learn temporal change as a neural Ordinary Differential Equation (ODE) flow with a bilinear objective which combines two aspects: The first is to map from the past into future video frames directly. Previous work has mapped the noise to new frames, a more computationally expensive process. Unfortunately, starting from the previous frame, instead of noise, is more prone to drifting errors. Hence, second, we additionally learn how to remove the accumulated errors as the joint objective by adding noise during training. We demonstrate unconditional video generation in a streaming manner for various video datasets, all at competitive quality compared to a conditional diffusion baseline but with higher speed, i.e., fewer ODE solver steps.

cs.CV↗

Stochastic Gradient Estimation for Higher-order Differentiable Rendering

We derive methods to compute higher order differentials (Hessians and Hessian-vector products) of the rendering operator. Our approach is based on importance sampling of a convolution that represents the differentials of rendering parameters and shows to be applicable to both rasterization and path tracing. We further suggest an aggregate sampling strategy to importance-sample multiple dimensions of one convolution kernel simultaneously. We demonstrate that this information improves convergence when used in higher-order optimizers such as Newton or Conjugate Gradient relative to a gradient descent baseline in several inverse rendering tasks.

cs.GR↗

Physics-informed 4D X-ray image reconstruction from ultra-sparse spatiotemporal data

The unprecedented X-ray flux density provided by modern X-ray sources offers new spatiotemporal possibilities for X-ray imaging of fast dynamic processes. Approaches to exploit such possibilities often result in either i) a limited number of projections or spatial information due to limited scanning speed, as in time-resolved tomography, or ii) a limited number of time points, as in stroboscopic imaging, making the reconstruction problem ill-posed and unlikely to be solved by classical reconstruction approaches. 4D reconstruction from such data requires sample priors, which can be included via deep learning (DL). State-of-the-art 4D reconstruction methods for X-ray imaging combine the power of AI and the physics of X-ray propagation to tackle the challenge of sparse views. However, most approaches do not constrain the physics of the studied process, i.e., a full physical model. Here we present 4D physics-informed optimized neural implicit X-ray imaging (4D-PIONIX), a novel physics-informed 4D X-ray image reconstruction method combining the full physical model and a state-of-the-art DL-based reconstruction method for 4D X-ray imaging from sparse views. We demonstrate and evaluate the potential of our approach by retrieving 4D information from ultra-sparse spatiotemporal acquisitions of simulated binary droplet collisions, a relevant fluid dynamic process. We envision that this work will open new spatiotemporal possibilities for various 4D X-ray imaging modalities, such as time-resolved X-ray tomography and more novel sparse acquisition approaches like X-ray multi-projection imaging, which will pave the way for investigations of various rapid 4D dynamics, such as fluid dynamics and composite testing.

eess.IV↗

Bracket Diffusion: HDR Image Generation by Consistent LDR Denoising

We demonstrate generating HDR images using the concerted action of multiple black-box, pre-trained LDR image diffusion models. Relying on a pre-trained LDR generative diffusion models is vital as, first, there is no sufficiently large HDR image dataset available to re-train them, and, second, even if it was, re-training such models is impossible for most compute budgets. Instead, we seek inspiration from the HDR image capture literature that traditionally fuses sets of LDR images, called "exposure brackets'', to produce a single HDR image. We operate multiple denoising processes to generate multiple LDR brackets that together form a valid HDR result. The key to making this work is to introduce a consistency term into the diffusion process to couple the brackets such that they agree across the exposure range they share while accounting for possible differences due to the quantization error. We demonstrate state-of-the-art unconditional and conditional or restoration-type (LDR2HDR) generative modeling results, yet in HDR.

cs.GR↗

Blind Augmentation: Calibration-free Camera Distortion Model Estimation for Real-time Mixed-reality Consistency

Real camera footage is subject to noise, motion blur (MB) and depth of field (DoF). In some applications these might be considered distortions to be removed, but in others it is important to model them because it would be ineffective, or interfere with an aesthetic choice, to simply remove them. In augmented reality applications where virtual content is composed into a live video feed, we can model noise, MB and DoF to make the virtual content visually consistent with the video. Existing methods for this typically suffer two main limitations. First, they require a camera calibration step to relate a known calibration target to the specific cameras response. Second, existing work require methods that can be (differentiably) tuned to the calibration, such as slow and specialized neural networks. We propose a method which estimates parameters for noise, MB and DoF instantly, which allows using off-the-shelf real-time simulation methods from e.g., a game engine in compositing augmented content. Our main idea is to unlock both features by showing how to use modern computer vision methods that can remove noise, MB and DoF from the video stream, essentially providing self-calibration. This allows to auto-tune any black-box real-time noise+MB+DoF method to deliver fast and high-fidelity augmentation consistency.

cs.CV↗

4D-ONIX: A deep learning approach for reconstructing 3D movies from sparse X-ray projections

The X-ray flux provided by X-ray free-electron lasers and storage rings offers new spatiotemporal possibilities to study in-situ and operando dynamics, even using single pulses of such facilities. X-ray Multi-Projection Imaging (XMPI) is a novel technique that enables volumetric information using single pulses of such facilities and avoids centrifugal forces induced by state-of-the-art time-resolved 3D methods such as time-resolved tomography. As a result, XMPI offers the potential to acquire 3D movies (4D) at least three orders of magnitude faster than current methods. However, it is exceptionally challenging to reconstruct 4D from highly sparse projections as acquired by XMPI with current algorithms. Here, we present 4D-ONIX, a Deep Learning (DL)-based approach that learns to reconstruct 3D movies (4D) from an extremely limited number of projections. It combines the computational physical model of X-ray interaction with matter and state-of-the-art DL methods. We demonstrate the potential of 4D-ONIX to generate high-quality 4D by generalizing over multiple experiments with only two to three projections per timestamp for binary droplet collisions and additive manufacturing. We envision that 4D-ONIX will become an enabling tool for 4D analysis, offering new spatiotemporal resolutions to study processes not possible before.

eess.IV↗

Neural Differential Appearance Equations

We propose a method to reproduce dynamic appearance textures with space-stationary but time-varying visual statistics. While most previous work decomposes dynamic textures into static appearance and motion, we focus on dynamic appearance that results not from motion but variations of fundamental properties, such as rusting, decaying, melting, and weathering. To this end, we adopt the neural ordinary differential equation (ODE) to learn the underlying dynamics of appearance from a target exemplar. We simulate the ODE in two phases. At the "warm-up" phase, the ODE diffuses a random noise to an initial state. We then constrain the further evolution of this ODE to replicate the evolution of visual feature statistics in the exemplar during the generation phase. The particular innovation of this work is the neural ODE achieving both denoising and evolution for dynamics synthesis, with a proposed temporal training scheme. We study both relightable (BRDF) and non-relightable (RGB) appearance models. For both we introduce new pilot datasets, allowing, for the first time, to study such phenomena: For RGB we provide 22 dynamic textures acquired from free online sources; For BRDFs, we further acquire a dataset of 21 flash-lit videos of time-varying materials, enabled by a simple-to-construct setup. Our experiments show that our method consistently yields realistic and coherent results, whereas prior works falter under pronounced temporal appearance variations. A user study confirms our approach is preferred to previous work for such exemplars.

cs.CV↗

Learning to Rasterize Differentiably

Differentiable rasterization changes the standard formulation of primitive rasterization -- by enabling gradient flow from a pixel to its underlying triangles -- using distribution functions in different stages of rendering, creating a "soft" version of the original rasterizer. However, choosing the optimal softening function that ensures the best performance and convergence to a desired goal requires trial and error. Previous work has analyzed and compared several combinations of softening. In this work, we take it a step further and, instead of making a combinatorial choice of softening operations, parameterize the continuous space of common softening operations. We study meta-learning tunable softness functions over a set of inverse rendering tasks (2D and 3D shape, pose and occlusion) so it generalizes to new and unseen differentiable rendering tasks with optimal softness.

cs.GR↗