arXiv subjects

Tomas Novotny

Publications and source records attributed to Tomas Novotny.

At least 19 recordsLinked to original sources

arXiv2012

Noise calculations within the second-order von Neumann approach

We extend the second-order von Neumann approach within the generalized master equation formalism for quantum electronic transport to include the counting field. The resulting non-Markovian evolution equation for the reduced density matrix of the system resolved with respect to the number of transported charges enables the evaluation of the noise and higher-order cumulants of the full counting statistics. We apply this formalism to an analytically solvable model of a single-level quantum dot coupled to highly biased leads with Lorentzian energy-dependent tunnel coupling and demonstrate that, although reproducing exactly the mean current, the resonant tunneling approximation is not exact for the noise and higher order cumulants. Even if it may fail in the regime of strongly non-Markovian dynamics, this approach generically improves results of lower-order and/or Markovian approaches.

cond-mat.mes-hall↗

arXiv2011

Nonequilibrium phonon backaction on the current noise in atomic-sized junctions

We study backaction effects of phonon heating due to tunneling electrons on the current noise in atomic-sized junctions. Deriving a generalized kinetic approximation within the extended Keldysh Green's functions technique, we demonstrate the existence of a characteristic backaction contribution to the noise in case of low external phonon damping. We provide a physically intuitive interpretation of this contribution at large voltage in terms of slow fluctuations of the phonon occupation, and show that it generally gives a significant correction to the noise above the phonon emission threshold.

cond-mat.mes-hall↗

arXiv2010

Current noise in molecular junctions: effects of the electron-phonon interaction

We study inelastic effects on the electronic current noise in molecular junctions, due to the coupling between transport electrons and vibrational degrees of freedom. Using a full counting statistics approach based on the generalized Keldysh Green's function technique, we calculate in an unified manner both the mean current and the zero-frequency current noise. For multilevel junctions with weak electron-phonon coupling, we give analytical formulas for the lowest order inelastic corrections to the noise in terms of universal temperature- and voltage-dependent functions and junction-dependent prefactors, which can be evaluated microscopically, e.g. with ab-initio methodologies. We identify distinct terms corresponding to the mean-field contribution to noise and to the vertex corrections, and we show that the latter contribute substantially to the inelastic noise. Finally, we illustrate our results by a simple model of two electronic levels which are mutually coupled by the electron-phonon interaction and show that the inelastic noise spectroscopy is a sensitive diagnostic tool.

cond-mat.mes-hall↗

arXiv2010

Counting statistics of transport through Coulomb blockade nanostructures: High-order cumulants and non-Markovian effects

Recent experimental progress has made it possible to detect in real-time single electrons tunneling through Coulomb blockade nanostructures, thereby allowing for precise measurements of the statistical distribution of the number of transferred charges, the so-called full counting statistics. These experimental advances call for a solid theoretical platform for equally accurate calculations of distribution functions and their cumulants. Here we develop a general framework for calculating zero-frequency current cumulants of arbitrary orders for transport through nanostructures with strong Coulomb interactions. Our recursive method can treat systems with many states as well as non-Markovian dynamics. We illustrate our approach with three examples of current experimental relevance: bunching transport through a two-level quantum dot, transport through a nano-electromechanical system with dynamical Franck-Condon blockade, and transport through coherently coupled quantum dots embedded in a dissipative environment. We discuss properties of high-order cumulants as well as possible subtleties associated with non-Markovian dynamics.

cond-mat.mes-hall↗

arXiv2009

Phonon-assisted current noise in molecular junctions

We investigate the effects of phonon scattering on the electronic current noise through nanojunctions using the non-equilibrium Green's functions formalism extended to include the counting field. In the case of weak electron-phonon coupling and a single broad electronic level we derive an analytic expression for the current noise at arbitrary temperature and identify physically distinct contributions based on their voltage dependence. We apply our theory to the experimentally relevant case of a deuterium molecule placed in a break-junction and predict a significant inelastic contribution to the current noise.

cond-mat.mes-hall↗

arXiv2009

Universal oscillations in counting statistics

Noise is a result of stochastic processes that originate from quantum or classical sources. Higher-order cumulants of the probability distribution underlying the stochastic events are believed to contain details that characterize the correlations within a given noise source and its interaction with the environment, but they are often difficult to measure. Here we report measurements of the transient cumulants < > of the number n of passed charges to very high orders (up to m=15) for electron transport through a quantum dot. For large m, the cumulants display striking oscillations as functions of measurement time with magnitudes that grow factorially with m. Using mathematical properties of high-order derivatives in the complex plane we show that the oscillations of the cumulants in fact constitute a universal phenomenon, appearing as functions of almost any parameter, including time in the transient regime. These ubiquitous oscillations and the factorial growth are system-independent and our theory provides a unified interpretation of previous theoretical studies of high-order cumulants as well as our new experimental data.

cond-mat.mes-hall↗

arXiv2009

Bubble merging in breathing DNA as a vicious walker problem in opposite potentials

We investigate the coalescence of two DNA-bubbles initially located at weak domains and separated by a more stable barrier region in a designed construct of double-stranded DNA. In a continuum Fokker-Planck approach, the characteristic time for bubble coalescence and the corresponding distribution are derived, as well as the distribution of coalescence positions along the barrier. Below the melting temperature, we find a Kramers-type barrier crossing behavior, while at high temperatures, the bubble corners perform drift-diffusion towards coalescence. In the calculations, we map the bubble dynamics on the problem of two vicious walkers in opposite potentials. We also present a discrete master equation approach to the bubble coalescence problem. Numerical evaluation and stochastic simulation of the master equation show excellent agreement with the results from the continuum approach. Given that the coalesced state is thermodynamically stabilized against a state where only one or a few base pairs of the barrier region are re-established, it appears likely that this type of setup could be useful for the quantitative investigation of thermodynamic DNA stability data as well as the rate constants involved in the unzipping and zipping dynamics of DNA, in single molecule fluorescence experiments.

cond-mat.stat-mech↗

arXiv2009

Josephson Junctions as Threshold Detectors of the Full Counting Statistics: Open issues

I study the dynamics of a Josephson junction serving as a threshold detector of fluctuations which is subjected to a general non-equilibrium electronic noise source whose characteristics is to be determined by the junction. This experimental setup has been proposed several years ago as a prospective scheme for determining the Full Counting Statistics of the electronic noise source. Despite of intensive theoretical as well as experimental research in this direction the promise has not been quite fulfilled yet and I will discuss what are the unsolved issues. First, I review a general theory for the calculation of the exponential part of the non-equilibrium switching rates of the junction and compare its predictions with previous results found in different limiting cases by several authors. I identify several possible weak points in the previous studies and I report a new analytical result for the linear correction to the rate due to the third cumulant of a non-Gaussian noise source in the limit of a very weak junction damping. The various analytical predictions are then compared with the results of the developed numerical method. Finally, I analyze the status of the so-far publicly available experimental data with respect to the theoretical predictions and discuss briefly the suitability of the present experimental schemes in view of their potential to measure the whole FCS of non-Gaussian noise sources as well as their relation to the available theories.

cond-mat.stat-mech↗

arXiv2009

Analytical calculation of the excess current in the OTBK theory

We present an analytical derivation of the excess current in Josephson junctions within the Octavio-Tinkham-Blonder-Klapwijk theory for both symmetric and asymmetric barrier strengths. We confirm the result found numerically by Flensberg et al. for equal barriers [Phys. Rev. B 38, 8707 (1988)], including the prediction of negative excess current for low transparencies, and we generalize it for differing barriers. Our analytical formulae provide for convenient fitting of experimental data, also in the less studied, but practically relevant case of the barrier asymmetry.

cond-mat.supr-con↗

arXiv2009

Charge conservation breaking within generalized master equation description of electronic transport through dissipative double quantum dots

We report an observation of charge conservation breaking in a model study of electronic current noise of transport through a dissipative double quantum dot within generalized master equation formalism. We study the current noise through a double quantum dot coupled to two electronic leads in the high bias limit and a dissipative heat bath in the weak coupling limit. Our calculations are based on the solution of a Markovian generalized master equation. Zero-frequency component of the current noise calculated within the system, i.e., between the two dots, via the quantum regression theorem exhibits unphysical negative values. On the other hand, current noise calculated for currents between the dots and the leads by the counting variable approach shows no anomalies and seems physically plausible. We inquire into the origin of this discrepancy between two nominally equivalent approaches and show that it stems from the simultaneous presence of the two types of baths, i.e., the electronic leads and the dissipative bosonic bath. This finding raises interesting questions concerning conceptual foundations of the theory describing multiple-baths open quantum systems widely encountered in nanoscience.

cond-mat.mes-hall↗

arXiv2008

Interplay between interference and Coulomb interaction in the ferromagnetic Anderson model with applied magnetic field

We study the competition between interference due to multiple single-particle paths and Coulomb interaction in a simple model of an Anderson-like impurity with local-magnetic-field-induced level splitting coupled to ferromagnetic leads. The model along with its potential experimental relevance in the field of spintronics serves as a nontrivial benchmark system where various quantum transport approaches can be tested and compared. We present results for the linear conductance obtained by a spin-dependent implementation of the density matrix renormalization group scheme which are compared with a mean-field solution as well as a seemingly more advanced Hubbard-I approximation. We explain why mean-field yields nearly perfect results, while the more sophisticated Hubbard-I approach fails, even at a purely conceptual level since it breaks hermiticity of the related density matrix. Furthermore, we study finite bias transport through the impurity by the mean-field approach and recently developed higher-order density matrix equations. We find that the mean-field solution fails to describe the plausible results of the higher-order density matrix approach both quantitatively and qualitatively as it does not capture some essential features of the current-voltage characteristics such as negative differential conductance.

cond-mat.mes-hall↗

arXiv2008

The influence of charge detection on counting statistics

We consider the counting statistics of electron transport through a double quantum dot with special emphasis on the dephasing induced by a nearby charge detector. The double dot is embedded in a dissipative enviroment, and the presence of electrons on the double dot is detected with a nearby quantum point contact. Charge transport through the double dot is governed by a non-Markovian generalized master equation. We describe how the cumulants of the current can be obtained for such problems, and investigate the difference between the dephasing mechanisms induced by the quantum point contact and the coupling to the external heat bath. Finally, we consider various open questions of relevance to future research.

cond-mat.mes-hall↗

arXiv2008

Counting Statistics of Non-Markovian Quantum Stochastic Processes

We derive a general expression for the cumulant generating function (CGF) of non-Markovian quantum stochastic transport processes. The long-time limit of the CGF is determined by a single dominating pole of the resolvent of the memory kernel from which we extract the zero-frequency cumulants of the current using a recursive scheme. The finite-frequency noise is expressed not only in terms of the resolvent, but also initial system-environment correlations. As an illustrative example we consider electron transport through a dissipative double quantum dot for which we study the effects of dissipation on the zero-frequency cumulants of high orders and the finite-frequency noise.

cond-mat.mes-hall↗

arXiv2008

Non-Markovian signatures in the current noise of a charge qubit

We investigate the current noise of a charge qubit coupled to a phonon bath in different parameter regimes. We find, using the theory of Full Counting Statistics of non-Markovian systems, that the current fluctuations are strongly influenced by memory effects generated from the interplay between quantum coherence and the dynamics of the phonon bath.

cond-mat.mes-hall↗

arXiv2007

Non-Markovian dynamics in the theory of full counting statistics

We consider the theoretical description of real-time counting of electrons tunneling through a Coulomb-blockade quantum dot using a detector with finite bandwidth. By tracing out the quantum dot we find that the dynamics of the detector effectively is non-Markovian. We calculate the cumulant generating function corresponding to the resulting non-Markovian rate equation and find that the measured current cumulants behave significantly differently compared to those of a Markovian transport process. Our findings provide a novel interpretation of noise suppression found in a number of systems.

cond-mat.mes-hall↗

arXiv2006

Bubble coalescence in breathing DNA: Two vicious walkers in opposite potentials

We investigate the coalescence of two DNA-bubbles initially located at weak segments and separated by a more stable barrier region in a designed construct of double-stranded DNA. The characteristic time for bubble coalescence and the corresponding distribution are derived, as well as the distribution of coalescence positions along the barrier. Below the melting temperature, we find a Kramers-type barrier crossing behaviour, while at high temperatures, the bubble corners perform drift-diffusion towards coalescence. The results are obtained by mapping the bubble dynamics on the problem of two vicious walkers in opposite potentials.

cond-mat.stat-mech↗

arXiv2005

Josephson current through a molecular transistor in a dissipative environment

We study the Josephson coupling between two superconductors through a single correlated molecular level, including Coulomb interaction on the level and coupling to a bosonic environment. All calculations are done to the lowest, i.e., the fourth, order in the tunneling coupling and we find a suppression of the supercurrent due to the combined effect of the Coulomb interaction and the coupling to environmental degrees of freedom. Both analytic and numerical results are presented.

cond-mat.mes-hall↗

arXiv2005

Noise and Bistabilities in Quantum Shuttles

We present a study of current fluctuations in two models proposed as quantum shuttles. Based on a numerical evaluation of the first three cumulants of the full counting statistics we have recently shown that a giant enhancement of the zero-frequency current noise in a single-dot quantum shuttle can be explained in terms of a bistable switching between two current channels. By applying the same method to a quantum shuttle consisting of a vibrating quantum dot array, we show that the same mechanism is responsible for a giant enhancement of the noise in this model, although arising from very different physics. The interpretation is further supported by a numerical evaluation of the finite-frequency noise. For both models we give numerical results for the effective switching rates.

cond-mat.mes-hall↗