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Tomislav Ivek

Publications and source records attributed to Tomislav Ivek.

12 recordsLinked to original sources

Dreaming up scale invariance via inverse renormalization group

We explore how minimal neural networks can invert the renormalization group (RG) coarse-graining procedure in the two-dimensional Ising model, effectively ``dreaming up'' microscopic configurations from coarse-grained states. This task - formally impossible at the level of configurations - can be approached probabilistically, allowing machine learning models to reconstruct scale-invariant distributions without relying on microscopic input. We demonstrate that even neural networks with as few as three trainable parameters can learn to generate critical configurations, reproducing the scaling behavior of observables such as magnetic susceptibility, heat capacity, and Binder ratios. A real-space renormalization group analysis of the generated configurations confirms that the models capture not only scale invariance but also reproduce nontrivial eigenvalues of the RG transformation. While the inversion is necessarily imperfect, these minimal models robustly reproduce the RG-relevant structure of the critical distribution. Surprisingly, we find that increasing network complexity by introducing multiple layers offers no significant benefit. These findings suggest that simple local rules, akin to those generating fractal structures, are sufficient to encode the universality of critical phenomena, creating an opportunity for efficient generative models of statistical ensembles in physics.

cond-mat.stat-mech

Spin-Reorientation-Driven Linear Magnetoelectric Effect in Topological Antiferromagnet Cu$_3$TeO$_6$

The search for new materials for energy-efficient electronic devices has gained unprecedented importance. Among the various classes of magnetic materials driving this search are antiferromagnets, magnetoelectrics, and systems with topological spin excitations. Cu$_3$TeO$_6$ is a material that belongs to all three of these classes. Combining static electric polarization and magnetic torque measurements with phenomenological simulations we demonstrate that magnetic-field-induced spin reorientation needs to be taken into account to understand the linear magnetoelectric (ME) effect in Cu$_3$TeO$_6$. Our calculations reveal that the magnetic field pushes the system from the nonpolar ground state to the polar magnetic structures. However, nonpolar structures only weakly differing from the obtained polar ones exist due to the weak effect that the field-induced breaking of some symmetries has on the calculated structures. Among those symmetries is the $PT$ ($\overline{1}'$) symmetry, preserved for Dirac points found in Cu$_3$TeO$_6$. Our findings establish Cu$_3$TeO$_6$ as a promising playground to study the interplay of spintronics-related phenomena.

cond-mat.str-el

Reconstruction of Incomplete Wildfire Data using Deep Generative Models

We present our submission to the Extreme Value Analysis 2021 Data Challenge in which teams were asked to accurately predict distributions of wildfire frequency and size within spatio-temporal regions of missing data. For the purpose of this competition we developed a variant of the powerful variational autoencoder models dubbed the Conditional Missing data Importance-Weighted Autoencoder (CMIWAE). Our deep latent variable generative model requires little to no feature engineering and does not necessarily rely on the specifics of scoring in the Data Challenge. It is fully trained on incomplete data, with the single objective to maximize log-likelihood of the observed wildfire information. We mitigate the effects of the relatively low number of training samples by stochastic sampling from a variational latent variable distribution, as well as by ensembling a set of CMIWAE models trained and validated on different splits of the provided data. The presented approach is not domain-specific and is amenable to application in other missing data recovery tasks with tabular or image-like information conditioned on auxiliary information.

stat.ML

Control of a polar order via magnetic field in a vector-chiral magnet

Vector-chiral (VC) antiferromagnetism is a spiral-like ordering of spins which may allow ferroelectricity to occur due to loss of space inversion symmetry. In this paper we report direct experimental observation of ferroelectricity in the VC phase of $β$-TeVO$_4$, a frustrated spin chain system with pronounced magnetic anisotropy and a rich phase diagram. Saturation polarization is proportional to neutron scattering intensities that correspond to the VC magnetic reflection. This implies that inverse Dzyaloshinskii-Moriya mechanism is responsible for driving electric polarization. Linear magnetoelectric coupling is absent, however an unprecedented dependence of electric coercive field on applied magnetic field reveals a novel way of manipulating multiferroic information.

cond-mat.str-el

Persisting correlation between electrical transport and magnetic dynamics in M-type hexaferrites

In this work we present frequency-dependent magnetic susceptibility and dc electric transport properties of three different compositions of hexaferrite Ba$_{1-x}$Pb$_{x}$Fe$_{12-y}$Al$_{y}$O$_{19}$. We find a correlation between activation energies of dc electric transport and ac magnetic susceptibility which persists in the whole researched range of aluminium substitution $x=0$ to $3.3$. This result is discussed in the context of charged magnetic domain walls, the pinning of which is determined by charge carriers activated over the transport gap. Our work points toward a general relaxational mechanism in ferrimagnetic semiconductors which directly affects dynamic magnetic properties via electric transport.

cond-mat.str-el

BlackBox: Generalizable Reconstruction of Extremal Values from Incomplete Spatio-Temporal Data

We describe our submission to the Extreme Value Analysis 2019 Data Challenge in which teams were asked to predict extremes of sea surface temperature anomaly within spatio-temporal regions of missing data. We present a computational framework which reconstructs missing data using convolutional deep neural networks. Conditioned on incomplete data, we employ autoencoder-like models as multivariate conditional distributions from which possible reconstructions of the complete dataset are sampled using imputed noise. In order to mitigate bias introduced by any one particular model, a prediction ensemble is constructed to create the final distribution of extremal values. Our method does not rely on expert knowledge in order to accurately reproduce dynamic features of a complex oceanographic system with minimal assumptions. The obtained results promise reusability and generalization to other domains.

cs.LG

Metal-Insulator Transition in the Dimerized Organic Conductor $κ$-(BEDT-TTF)$_2$Hg(SCN)$_2$Br

The organic charge-transfer salt $κ$-(BEDT-TTF)$_{2}$Hg(SCN)$_{2}$Br is a quasi two-dimensional metal with a half-filled conduction band at ambient conditions. When cooled below $T=80$ K it undergoes a pronounced transition to an insulating phase where the resistivity increases many orders of magnitude. In order to elucidate the nature of this metal-insulator transition we have performed comprehensive transport, dielectric and optical investigations. The findings are compared with other dimerized $κ$-(BEDT-TTF) salts, in particular the Cl-analogue, where a charge-order transition takes place at $T_{\rm CO}=30$ K.

cond-mat.str-el

Semimetallic and charge-ordered $α$-(BEDT-TTF)$_2$I$_3$: on the role of disorder in dc transport and dielectric properties

$α$-(BEDT-TTF)$_2$I$_3$ is a prominent example of charge ordering among organic conductors. In this work we explore the details of transport within the charge-ordered as well as semimetallic phase at ambient pressure. In the high-temperature semimetallic phase, the mobilities and concentrations of both electrons and holes conspire in such a way to create an almost temperature-independent conductivity as well as a low Hall effect. We explain these phenomena as a consequence of a predominantly inter-pocket scattering which equalizes mobilities of the two types of charge carriers. At low temperatures, within the insulating charge-ordered phase two channels of conduction can be discerned: a temperature-dependent activation which follows the mean-field behavior, and a nearest-neighbor hopping contribution. Together with negative magnetoresistance, the latter relies on the presence of disorder. The charge-ordered phase also features a prominent dielectric peak which bears a similarity to relaxor ferroelectrics. Its dispersion is determined by free-electron screening and pushed by disorder well below the transition temperature. The source of this disorder can be found in the anion layers which randomly perturb BEDT-TTF molecules through hydrogen bonds.

cond-mat.str-el

Electrically-induced phase transition in $α$-(BEDT-TTF)$_2$I$_3$: Indications for high-mobility hot charge carriers

The two-dimensional organic conductor $α$-(BEDT-TTF)$_2$I$_3$ undergoes a metal-insulator transition at $T_{\rm CO}=135$ K due to electronic charge ordering. We have conducted time-resolved investigations of its electronic properties in order to explore the field- and temperature-dependent dynamics. At a certain threshold field, the system switches from low-conducting to a high-conducting state, accompanied by a negative differential resistance. Our time-dependent infrared investigations indicate that close to $T_{\rm CO}$ the strong electric field pushes the crystal into a metallic state with optical properties similar to the one for $T>T_{\rm CO}$. Well into the insulating state, however, at $T=80$ K, the spectral response evidences a completely different electronically-induced high-conducting state. Applying a two-state model of hot electrons explains the observations by excitation of charge carriers with a high mobility. They resemble the Dirac-like charge-carriers with a linear dispersion of the electronic bands found in $α$-(BEDT-TTF)$_2$I$_3$ at high-pressure. Extensive numerical simulations quantitatively reproduce our experimental findings in all details.

cond-mat.str-el

Effect of magnesium ions on dielectric relaxation in semidilute DNA aqueous solutions

The effect of magnesium ion Mg2+ on the dielectric relaxation of semidilute DNA aqueous solutions has been studied by means of dielectric spectroscopy in the 100 Hz-100 MHz frequency range. De Gennes-Pfeuty-Dobrynin semidilute solution correlation length is the pertinent fundamental length scale for sufficiently low concentration of added salt, describing the collective properties of Mg-DNA solutions. No relaxation fingerprint of the DNA denaturation bubbles, leading to exposed hydrophobic core scaling, was detected at low DNA concentrations, thus indicating an increased stability of the double-stranded conformation in Mg-DNA solutions as compared to the case of Na-DNA solutions. Some changes are detected in the behavior of the fundamental length scale pertaining to the single molecule DNA properties, reflecting modified electrostatic screening effects of the Odijk-Skolnick-Fixman type. All results consistently demonstrate that Mg2+ ions interact with DNA in a similar way as Na1+ ions do, their effect being mostly describable through an enhanced screening.

physics.bio-ph

Search for quantum electronic dipoles in the dimerized κ-(BEDT-TTF)2Cu[N(CN)2]Cl salt

The Mott insulator κ-(BEDT-TTF)2Cu[N(CN)2]Cl consists of molecular dimers arranged on an anisotropic triangular lattice and develops a canted antiferromagnetic ground state. It has recently been suggested that this system features purely electronic ferroelectricity which requires an electric dipole moment. Optical spectroscopy clearly rules out charge imbalance in this system, which excludes the existence of quantum electric dipoles on the dimers and subsequently a dipolar spin coupling. We suggest that the prominent in-plane dielectric response in κ-(BEDT-TTF)2Cu[N(CN)2]Cl is due to short-range discommensurations of the antiferromagnetic phase in the temperature range 30 < T < 50 K, and domain wall relaxations at lower temperatures.

cond-mat.str-el

Absence of charge order in the dimerized κ-phase BEDT-TTF salts

Utilizing infrared vibrational spectroscopy we have investigated dimerized two-dimensional organic salts in order to search for possible charge redistribution that might cause electronic dipoles and ferroelectricity: the quantum spin liquid κ-(BEDT-TTF)2Cu2(CN)3, the antiferromagnetic Mott insulator κ-(BEDT-TTF)2$Cu[N(CN)2]Cl, and the superconductor κ-(BEDT-TTF)2$Cu[N(CN)2]Br. None of them exhibit any indication of charge disproportionation upon cooling down to low temperatures. No modification in the charge distribution is observed around T = 6 K where a low-temperature anomaly has been reported for the spin-liquid κ-(BEDT-TTF)2$Cu2(CN)3. In this compound the in-plane optical response and vibrational coupling are rather anisotropic, indicating that the tilt of the BEDT-TTF molecules in c-direction and their coupling to the anion layers has to be considered in the explanation of the electromagnetic properties.

cond-mat.str-el