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Tommaso Calarco

Publications and source records attributed to Tommaso Calarco.

At least 37 records · Page 2Linked to original sources

Coherent Control of a Long-Lived Nuclear Memory Spin in a Germanium-Vacancy Multi-Qubit Node

The ability to process and store information on surrounding nuclear spins is a major requirement for group-IV color center-based repeater nodes. We demonstrate coherent control of a ${}^{13}$C nuclear spin strongly coupled to a negatively charged germanium-vacancy center in diamond with coherence times beyond 2.5s at mK temperatures, which is the longest reported for group-IV defects. Detailed analysis allows us to model the system's dynamics, extract the coupling parameters, and characterize noise. We estimate an achievable memory time of 18.1s with heating limitations considered, paving the way to successful applications as a quantum repeater node.

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Experimental error suppression in Cross-Resonance gates via multi-derivative pulse shaping

While quantum circuits are reaching impressive widths in the hundreds of qubits, their depths have not been able to keep pace. In particular, cloud computing gates on multi-qubit, fixed-frequency superconducting chips continue to hover around the 1% error range, contrasting with the progress seen on carefully designed two-qubit chips, where error rates have been pushed towards 0.1%. Despite the strong impetus and a plethora of research, experimental demonstration of error suppression on these multi-qubit devices remains challenging, primarily due to the wide distribution of qubit parameters and the demanding calibration process required for advanced control methods. Here, we achieve this goal, using a simple control method based on multi-derivative, multi-constraint pulse shaping, which acts simultaneously against multiple error sources. Our approach establishes a two to fourfold improvement on the default calibration scheme, demonstrated on four qubits on the IBM Quantum Platform with limited and intermittent access, enabling these large-scale fixed-frequency systems to fully take advantage of their superior coherence times. The achieved CNOT fidelities of 99.7(1)% on those publically available qubits come from both coherent control error suppression and accelerated gate time.

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Long distance spin shuttling enabled by few-parameter velocity optimization

Spin qubit shuttling via moving conveyor-mode quantum dots in Si/SiGe offers a promising route to scalable miniaturized quantum computing. Recent modeling of dephasing via valley degrees of freedom and well disorder dictate a slow shutting speed which seems to limit errors to above correction thresholds if not mitigated. We increase the precision of this prediction, showing that typical errors for 10 $μ$m shuttling at constant speed results in O(1) error, using fast, automatically differentiable numerics and including improved disorder modeling and potential noise ranges. However, remarkably, we show that these errors can be brought to well below fault-tolerant thresholds using trajectory shaping with very simple parametrization with as few as 4 Fourier components, well within the means for experimental in-situ realization, and without the need for targeting or knowing the location of valley near degeneracies.

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The Role of Bases in Quantum Optimal Control

Quantum Optimal Control (QOC) supports the advance of quantum technologies by tackling its problems at the pulse level: Numerical approaches iteratively work towards a given target by parametrising the applied time-dependent fields with a finite set of variables. The effectiveness of the resulting optimisation depends on the complexity of the problem and the number of variables. We consider different parametrisations in terms of basis functions, asking whether the choice of the applied basis affects the quality of the optimisation. Furthermore, we consider strategies to choose the most suitable basis. For the comparison, we test three different randomisable bases - introducing the sinc and sigmoid bases as alternatives to the Fourier basis - on QOC problems of varying complexity. For each problem, the basis-specific convergence rates result in a unique ranking. Especially for expensive evaluations, e.g., in closed-loop, a potential speed-up by a factor of up to 10 may be crucial for the optimisation's feasibility. We conclude that a problem-dependent basis choice is an influential factor for QOC efficiency and provide advice for its approach.

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Optimal two-qubit gates in recurrence protocols of entanglement purification

We propose and investigate a method to optimize recurrence entanglement purification protocols. The approach is based on a numerical search in the whole set of SU(4) matrices with the aid of a quasi-Newton algorithm. Our method evaluates average concurrences where the probabilistic occurrence of mixed entangled states is also taken into account. We show for certain families of states that optimal protocols are not necessarily achieved by bilaterally applied controlled-NOT gates. As we discover several optimal solutions, the proposed method offers some flexibility in experimental implementations of entanglement purification protocols and interesting perspectives in quantum information processing.

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Quantum state preparation via engineered ancilla resetting

In this theoretical investigation, we study the effectiveness of a protocol that incorporates periodic quantum resetting to prepare ground states of frustration-free parent Hamiltonians. This protocol uses a steering Hamiltonian that enables local coupling between the system and ancillary degrees of freedom. At periodic intervals, the ancillary system is reset to its initial state. For infinitesimally short reset times, the dynamics can be approximated by a Lindbladian whose steady state is the target state. For finite reset times, however, the spin chain and the ancilla become entangled between reset operations. To evaluate the performance of the protocol, we employ Matrix Product State simulations and quantum trajectory techniques, focusing on the preparation of the spin-1 Affleck-Kennedy-Lieb-Tasaki state. Our analysis considers convergence time, fidelity, and energy evolution under different reset intervals. Our numerical results show that ancilla system entanglement is essential for faster convergence. In particular, there exists an optimal reset time at which the protocol performs best. Using a simple approximation, we provide insights into how to optimally choose the mapping operators applied to the system during the reset procedure. Furthermore, the protocol shows remarkable resilience to small deviations in reset time and dephasing noise. Our study suggests that stroboscopic maps using quantum resetting may offer advantages over alternative methods, such as quantum reservoir engineering and quantum state steering protocols, which rely on Markovian dynamics.

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Gate-set evaluation metrics for closed-loop optimal control on nitrogen-vacancy center ensembles in diamond

A recurring challenge in quantum science and technology is the precise control of their underlying dynamics that lead to the desired quantum operations, often described by a set of quantum gates. These gates can be subject to application-specific errors, leading to a dependence of their controls on the chosen circuit, the quality measure and the gate-set itself. A natural solution would be to apply quantum optimal control in an application-oriented fashion. In turn, this requires the definition of a meaningful measure of the contextual gate-set performance. Therefore, we explore and compare the applicability of quantum process tomography, linear inversion gate-set tomography, randomized linear gate-set tomography, and randomized benchmarking as measures for closed-loop quantum optimal control experiments, using a macroscopic ensemble of nitrogen-vacancy centers in diamond as a test-bed. Our work demonstrates the relative trade-offs between those measures and how to significantly enhance the gate-set performance, leading to an improvement across all investigated methods.

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Large spin shuttling oscillations enabling high-fidelity single qubit gates

Semiconductor quantum dots have shown impressive breakthroughs in the last years, with single and two qubit gate fidelities matching other leading platforms and scalability still remaining a relative strength. However, due to qubit wiring considerations, mobile electron architectures have been proposed to facilitate upward scaling. In this work, we examine and demonstrate the possibility of significantly outperforming static EDSR-type single-qubit pulsing by taking advantage of the larger spatial mobility to achieve larger Rabi frequencies and reduce the effect of charge noise. Our theoretical results indicate that fidelities are ultimately bottlenecked by spin-valley physics, which can be suppressed through the use of quantum optimal control, and we demonstrate that, across different potential regimes and competing physical models, shuttling based single-qubit gates retain significant advantage over existing alternatives.

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Exponentiation of Parametric Hamiltonians via Unitary interpolation

The effort to generate matrix exponentials and associated differentials, required to determine the time evolution of quantum systems, frequently constrains the evaluation of problems in quantum control theory, variational circuit compilation, or Monte-Carlo sampling. We introduce two ideas for the time-efficient approximation of matrix exponentials of linear multi-parametric Hamiltonians. We modify the Suzuki-Trotter product formula from an approximation to an interpolation schemes to improve both accuracy and computational time. This allows us to achieve high fidelities within a single interpolation step, which can be computed directly from cached matrices. We furthermore define the interpolation on a grid of system parameters, and show that the infidelity of the interpolation converges with $4^\mathrm{th}$ order in the number of interpolation bins.

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Analyzing the collective emission of a Rydberg-blockaded single-photon source based on an ensemble of thermal atoms

An ensemble of Rubidum atoms can be excited with lasers such that it evolves into an entangled state with just one collective excitation within the Rydberg blockade radius. The decay of this state leads to the emission of a single, antibunched photon. For a hot vapor of Rubidium atoms in a micro cell we numerically study the feasibility of such a single-photon source under different experimental conditions like the atomic density distribution and the choice of electronic states addressed by the lasers. For the excitation process with three rectangular lasers pulses, we simulate the coherent dynamics of the system in a truncated Hilbert space. We investigate the radiative behavior of the moving Rubidum atoms and optimize the laser pulse sequence accordingly. We find that the collective decay of the single-excitation leads to a fast and directed photon emission and further, that a pulse sequence similar to a spin echo increases the directionality of the photon. Finally, we analyze the residual double-excitations and find that they do not exhibit these collective decay properties and play only a minor deleterious role.

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Compensating for non-linear distortions in controlled quantum systems

Predictive design and optimization methods for controlled quantum systems depend on the accuracy of the system model. Any distortion of the input fields in an experimental platform alters the model accuracy and eventually disturbs the predicted dynamics. These distortions can be non-linear with a strong frequency dependence so that the field interacting with the microscopic quantum system has limited resemblance to the input signal. We present an effective method for estimating these distortions which is suitable for non-linear transfer functions of arbitrary lengths and magnitudes provided the available training data has enough spectral components. Using a quadratic estimation, we have successfully tested our approach for a numerical example of a single Rydberg atom system. The transfer function estimated from the presented method is incorporated into an open-loop control optimization algorithm allowing for high-fidelity operations in quantum experiments.

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Optimizing optical potentials with physics-inspired learning algorithms

We present our new experimental and theoretical framework which combines a broadband superluminescent diode (SLED/SLD) with fast learning algorithms to provide speed and accuracy improvements for the optimization of 1D optical dipole potentials, here generated with a Digital Micromirror Device (DMD). To characterize the setup and potential speckle patterns arising from coherence, we compare the superluminescent diode to a single-mode laser by investigating interference properties. We employ Machine Learning (ML) tools to train a physics-inspired model acting as a digital twin of the optical system predicting the behavior of the optical apparatus including all its imperfections. Implementing an iterative algorithm based on Iterative Learning Control (ILC) we optimize optical potentials an order of magnitude faster than heuristic optimization methods. We compare iterative model-based offline optimization and experimental feedback-based online optimization. Our methods provide a new route to fast optimization of optical potentials which is relevant for the dynamical manipulation of ultracold gases.

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Information Theoretical Limits for Quantum Optimal Control Solutions: Error Scaling of Noisy Channels

Accurate manipulations of an open quantum system require a deep knowledge of its controllability properties and the information content of the implemented control fields. By using tools of information and quantum optimal control theory, we provide analytical bounds (information-time bounds) to characterize our capability to control the system when subject to arbitrary sources of noise. Moreover, since the presence of an external noise field induces open quantum system dynamics, we also show that the results provided by the information-time bounds are in very good agreement with the Kofman-Kurizki universal formula describing decoherence processes. Finally, we numerically test the scaling of the control accuracy as a function of the noise parameters, by means of the dressed chopped random basis (dCRAB) algorithm for quantum optimal control.

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QuOCS: The Quantum Optimal Control Suite

Quantum optimal control includes the family of pulse-shaping algorithms that aim to unlock the full potential of a variety of quantum technologies. Our Quantum Optimal Control Suite (QuOCS) unites experimental focus and model-based approaches in a unified framework. The easy usage and installation of QuOCS and the availability of various combinable optimization strategies is designed to improve the performance of many quantum technology platforms, such as color defects in diamond, superconducting qubits, atom- or ion-based quantum computers. It can also be applied to the study of more general phenomena in physics. In this paper, we describe the software and the main toolbox of gradient-free and gradient-based algorithms. We then show how the user can connect it to their experiment. In addition, we provide illustrative examples where our optimization suite solves typical quantum optimal control problems, in both open- and closed-loop settings. Integration into existing experimental control software is already provided for the experiment control software Qudi [J. M. Binder et al., SoftwareX, 6, 85-90, (2017)], and further extensions are investigated and highly encouraged. QuOCS is available from GitHub, under Apache License 2.0, and can be found on the PyPI repository.

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Continuous quantum gate sets and pulse class meta-optimization

Reducing the circuit depth of quantum circuits is a crucial bottleneck to enabling quantum technology. This depth is inversely proportional to the number of available quantum gates that have been synthesised. Moreover, quantum gate synthesis and control problems exhibit a vast range of external parameter dependencies, both physical and application-specific. In this article we address the possibility of learning families of optimal control pulses which depend adaptively on various parameters, in order to obtain a global optimal mapping from the space of potential parameter values to the control space, and hence continuous classes of gates. Our proposed method is tested on different experimentally relevant quantum gates and proves capable of producing high-fidelity pulses even in presence of multiple variable or uncertain parameters with wide ranges.

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Iterative shaping of optical potentials for one-dimensional Bose-Einstein condensates

The ability to manipulate clouds of ultra-cold atoms is crucial for modern experiments on quantum manybody systems and quantum thermodynamics as well as future metrological applications of Bose-Einstein condensate. While optical manipulation offers almost arbitrary flexibility, the precise control of the resulting dipole potentials and the mitigation of unwanted disturbances is quite involved and only heuristic algorithms with rather slow convergence rates are available up to now. This paper thus suggests the application of iterative learning control (ILC) methods to generate fine-tuned effective potentials in the presence of uncertainties and external disturbances. Therefore, the given problem is reformulated to obtain a one-dimensional tracking problem by using a quasicontinuous input mapping which can be treated by established ILC methods. Finally, the performance of the proposed concept is illustrated in a simulation scenario.

eess.SY↗

Robust Magnetometry with Single NV Centers via Two-step Optimization

Shallow Nitrogen-Vacancy (NV) centers are promising candidates for high-precision sensing applications; these defects, when positioned a few nanometers below the surface, provide an atomic-scale resolution along with substantial sensitivity. However, the dangling bonds and impurities on the diamond surface result in a complex environment which reduces the sensitivity and is unique to each shallow NV center. To avoid the environment's detrimental effect, we apply feedback-based quantum optimal control. We first show how a direct search can improve the initialization/readout process. In a second step, we optimize microwave pulses for pulsed Optically Detected Magnetic Resonance (ODMR) and Ramsey measurements. Throughout the sensitivity optimizations, we focus on robustness against errors in the control field amplitude. This feature not only protects the protocols' sensitivity from drifts but also enlarges the sensing volume. The resulting ODMR measurements produce sensitivities below 1$μ$T\,Hz$^{-\frac{1}{2}}$ for an 83\% decrease in control power, increasing the robustness by approximately one third. The optimized Ramsey measurements produce sensitivities below 100\,nT\,Hz$^{-\frac{1}{2}}$ giving a two-fold sensitivity improvement. Being on par with typical sensitivities obtained via single NV magnetometry, the complementing robustness of the presented optimization strategy may provide an advantage for other NV-based applications.

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Experimental realization of optimal time-reversal on an atom chip for quantum undo operations

We report on the use of the dCRAB optimal control algorithm to realize time-reversal procedures for the implementation of quantum undo operations, to be applied in quantum technology contexts ranging from quantum computing to quantum communications. By means of the undo command, indeed, the last performed operation can be time-reversed so as to perfectly restore a condition in which an arbitrary new operation, chosen by the external user, can be applied. Moreover, by further generalizing this concept, the undo command can also allow for the reversing of a quantum operation in a generic instant of the past. Here, thanks to optimal time-reversal routines, all these functionalities are experimentally implemented on the five-fold F=2 Hilbert space of a Bose-Einstein condensate (BEC) of non-interacting $^{87}$Rb atoms in the ground state, realized with an atom chip. Specifically, each time-reversal transformation is attained by designing an optimal modulated radio frequency field, achieving on average an accuracy of around 92% in any performed test. The experimental results are accompanied by a thermodynamic interpretation based on the Loschmidt echo. Our findings are expected to promote the implementation of time-reversal operations in a real scenario of gate-based quantum computing with a more complex structure than the five-level system here considered.

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