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Tong Gao

Publications and source records attributed to Tong Gao.

23 records · Page 2Linked to original sources

Anomalous Nernst Effect in Dirac Semimetal Cd3As2

Dirac and Weyl semimetals display a host of novel properties. In Cd$_3$As$_2$, the Dirac nodes lead to a protection mechanism that strongly suppresses backscattering in zero magnetic field, resulting in ultrahigh mobility ($\sim$ 10$^7$ cm$^2$ V$^{-1}$ s$^{-1}$). In applied magnetic field, an anomalous Nernst effect is predicted to arise from the Berry curvature associated with the Weyl nodes. We report observation of a large anomalous Nernst effect in Cd$_3$As$_2$. Both the anomalous Nernst signal and transport relaxation time $τ_{tr}$ begin to increase rapidly at $\sim$ 50 K. This suggests a close relation between the protection mechanism and the anomalous Nernst effect. In a field, the quantum oscillations of bulk states display a beating effect, suggesting that the Dirac nodes split into Weyl states, allowing the Berry curvature to be observed as an anomalous Nernst effect.

cond-mat.mes-hall↗

Analytical structure, dynamics, and coarse-graining of a kinetic model of an active fluid

We analyze one of the simplest active suspensions with complex dynamics: a suspension of immotile "Extensor" particles that exert active extensile dipolar stresses on the fluid in which they are immersed. This is relevant to several experimental systems, such as recently studied tripartite rods that create extensile flows by consuming a chemical fuel. We first describe the system through a Doi-Onsager kinetic theory based on microscopic modeling. This theory captures the active stresses produced by the particles that can drive hydrodynamic instabilities, as well as the steric interactions of rod-like particles that lead to nematic alignment. This active nematic system yields complex flows and disclination defect dynamics very similar to phenomenological Landau-deGennes Q-tensor theories for active nematic fluids, as well as by more complex Doi-Onsager theories for polar microtubule/motor-protein systems. We apply the quasi-equilibrium Bingham closure, used to study suspensions of passive microscopic rods, to develop a non-standard Q-tensor theory. We demonstrate through simulation that this "BQ-tensor" theory gives an excellent analytical and statistical accounting of the suspension's complex dynamics, at a far reduced computational cost. Finally, we apply the BQ-tensor model to study the dynamics of Extensor suspensions in circular and bi-concave domains. In circular domains, we reproduce previous results for systems with weak nematic alignment, but for strong alignment find novel dynamics with activity-controlled defect production and absorption at the boundaries of the domain. In bi-concave domains, a Fredericks-like transition occurs as the width of the neck connecting the two disks is varied.

cond-mat.soft↗

High-Pressure Synthesis and Characterization of $β$-GeSe - A Semiconductor with Six-Rings in an Uncommon Boat Conformation

Two-dimensional materials have significant potential for the development of new devices. Here we report the electronic and structural properties of $β$-GeSe, a previously unreported polymorph of GeSe, with a unique crystal structure that displays strong two-dimensional structural features. $β$-GeSe is made at high pressure and temperature and is stable under ambient conditions. We compare it to its structural and electronic relatives $α$-GeSe and black phosphorus. The $β$ form of GeSe displays a boat conformation for its Ge-Se six-ring, while the previously known $α$ form, and black phosphorus, display the more common chair conformation for their six-rings. Electronic structure calculations indicate that $β$-GeSe is a semiconductor, with an approximate bulk band gap of $Δ~\approx$ 0.5 eV, and, in its monolayer form, $Δ~\approx$ 0.9 eV. These values fall between those of $α$-GeSe and black phosphorus, making $β$-GeSe a promising candidate for future applications. The resistivity of our $β$-GeSe crystals measured in-plane is on the order of $ρ\approx$ 1 $Ω$cm, while being essentially temperature independent.

cond-mat.mtrl-sci↗

Multiscale modeling and simulation of microtubule/motor protein assemblies

Microtubules and motor proteins self organize into biologically important assemblies including the mitotic spindle and the centrosomal microtubule array. Outside of cells, microtubule-motor mixtures can form novel active liquid-crystalline materials driven out of equilibrium by ATP-consuming motor proteins. Microscopic motor activity causes polarity-dependent interactions between motor proteins and microtubules, but how these interactions yield such larger-scale dynamical behavior such as complex flows and defect dynamics is not well understood. We develop a multiscale theory for microtubule-motor systems in which Brownian dynamics simulations of polar microtubules driven by motors are used to study microscopic organization and stresses created by motor-mediated microtubule interactions. We identify polarity-sorting and crosslink tether relaxation as two polar-specific sources of active destabilizing stress. We then develop a continuum Doi-Onsager model that captures polarity sorting and the hydrodynamic flows generated by these polar-specific active stresses. In simulations of active nematic flows on immersed surfaces, the active stresses drive turbulent flow dynamics and continuous generation and annihilation of disclination defects. The dynamics follow from two instabilities, and accounting for the immersed nature of the experiment yields unambiguous characteristic length and time scales. When turning off the hydrodynamics in the Doi-Onsager model, we capture formation of polar lanes as observed in the Brownian dynamics simulation.

cond-mat.soft↗

Multiscale polar theory of microtubule and motor-protein assemblies

Microtubules and motor proteins are building blocks of self-organized subcellular biological structures such as the mitotic spindle and the centrosomal microtubule array. These same ingredients can form new "bioactive" liquid-crystalline fluids that are intrinsically out of equilibrium and which display complex flows and defect dynamics. It is not yet well understood how microscopic activity, which involves polarity-dependent interactions between motor proteins and microtubules, yields such larger scale dynamical structures. In our multiscale theory, Brownian dynamics simulations of polar microtubule ensembles driven by crosslinking motors allow us to study microscopic organization and stresses. Polarity sorting and crosslink relaxation emerge as two polar-specific sources of active destabilizing stress. On larger length scales, our continuum Doi-Onsager theory captures the hydrodynamic flows generated by polarity-dependent active stresses. The results connect local polar structure to flow structures and defect dynamics.

cond-mat.soft↗