arXiv subjects

Tongshuai Zhu

Publications and source records attributed to Tongshuai Zhu.

13 recordsLinked to original sources

arXiv2026

Floquet spin-group framework and its application to light-tailored spin splitting in collinear magnets

Altermagnets combine momentum-dependent spin splitting with vanishing net magnetization, opening new opportunities for spintronics. Recent studies have shown that periodic driving by linearly or circularly polarized light, as well as by multicolor light fields, can control spin splitting in altermagnets and conventional antiferromagnets, and can even generate spin splitting patterns absent in equilibrium. Despite this progress, a unified principle connecting the dynamical symmetry of light to the symmetry of spin-split bands remains lacking, limiting the systematic design of light-induced spin structures. Here, by combining the spin group of crystals with the dynamical group of light, we establish a unified Floquet spin group framework for the study of periodically driven collinear magnets with negligible spin-orbit coupling. This framework systematically determines the allowed parity, momentum dependence, and nodal structure of spin splitting under different driving protocols. Guided by this symmetry classification, we show that odd-parity, even-parity, and mixed-parity spin splittings can be switched within the same material by tailoring the driving field. We further uncover higher-order $h$-wave and $k$-wave spin splittings in three-dimensional systems. Our work establishes a unified symmetry framework for light-controlled spin splitting and provides general principles for engineering nonequilibrium spin-band structures in altermagnets and related magnetic materials.

cond-mat.mes-hall↗

arXiv2026

Linearly Polarized Light-Induced Anomalous Hall Effect and Topological Phase Transitions in an Altermagnetic Topological Insulator

A recently identified class of collinear magnetic order, characterized by vanishing net magnetization yet unconventional spin splitting, known as altermagnets (AMs), has attracted significant research interest. Controlling the unconventional spin splitting and the associated band topology in AMs offers opportunities for realizing novel spin and topological transport phenomena. In this work, using Floquet engineering with periodically driven linearly polarized light (LPL), we explore light-induced control of an AM topological insulator. Remarkably, we find that AMs and conventional antiferromagnets (AFMs) exhibit distinct responses under LPL irradiation. Specifically, since LPL breaks neither time-reversal ($\mathcal{T}$) symmetry nor parity-time-reversal ($\mathcal{PT}$) symmetry, it is incapable of generating spin splitting or inducing an anomalous Hall effect (AHE) in conventional AFMs. In contrast, AMs intrinsically lack both $\mathcal{T}$ and $\mathcal{PT}$ symmetries. Their spin-up and spin-down bands are related by the combined symmetry of time reversal $\mathcal{T}$ and a crystal rotation. We show that LPL readily breaks these symmetries, thereby triggering a finite AHE exclusively in AMs. Furthermore, LPL can drive the AM topological insulator into a fully spin-polarized Chern insulating phase. Our findings not only provide a robust experimental scheme to distinguish AMs from conventional AFMs, but also establish a promising pathway toward dissipationless spintronic applications.

cond-mat.mes-hall↗

arXiv2026

Floquet odd-parity collinear magnets

Altermagnets (AMs), recently discovered unconventional magnets distinct from both ferro- and antiferromagnets, have rapidly emerged as a prominent research topic in condensed matter physics. AMs are characterized by alternating collinear magnetic moments with zero net magnetization in real space, and spin splittings with even-parity symmetry in momentum space. However, their counterparts exhibiting odd-parity spin splittings are generally thought to be absent in collinear magnets. Here, we show that such unconventional odd-parity magnets can be induced from collinear antiferromagnets by symmetry engineering. Remarkably, using effective model analysis within Floquet-theory framework, we demonstrate that circularly polarized light irradiation of conventional antiferromagnetic lattices breaks a spin-preserving pseudo-time-reversal symmetry and induces both $p$- and $f$-wave magnets, realizing novel magnetic states dubbed Floquet odd-parity collinear magnets. Moreover, we also uncover light-induced antiferromagnetic Chern insulating states in the $f$-wave magnets. The proposed Floquet odd-parity magnet is confirmed by first-principles calculations of MnPSe$_{3}$ under circularly polarized light. Our work not only proposes a new class of unconventional magnets, but also opens an avenue for light-induced magnetic phenomena in spintronic applications.

cond-mat.mes-hall↗

arXiv2025

Switchable axionic magnetoelectric effect via spin-flop transition in topological antiferromagnets

The MnBi$_2$Te$_4$ material family has emerged as a key platform for exploring magnetic topological phases, most notably exemplified by the experimental realization of the axion insulator state. While spin dynamics are known to significantly influence the axion state, a profound understanding of their interplay remains elusive. In this work, we employ an antiferromagnetic spin-chain model to demonstrate that an external magnetic field induces extrinsic perpendicular magnetic anisotropy. We find that an in-plane field stabilizes the antiferromagnetic order, whereas an out-of-plane field destabilizes it and triggers spin-flop transitions. Remarkably, near the surface spin-flop transition in even-layer MnBi$_2$Te$_4$ films, the axion insulator state undergoes a sharp switching behavior accompanied by distinct magnetoelectric responses. Furthermore, we propose that this switchable axionic magnetoelectric effect can be utilized to convert alternating magnetic field signals into measurable square-wave magneto-optical outputs, thereby realizing an axionic analog of a zero-crossing detector. Our findings could open a pathway toward potential applications of axion insulators in next-generation spintronic devices.

cond-mat.mes-hall↗

arXiv2025

Giant Splitting of Folded Dirac Bands in Kekulé-ordered Graphene with Eu Intercalation

Kekulé-ordered graphene on SiC realized by intercalating two-dimensional metal layers offers a versatile platform for exploring intriguing quantum states and phenomena. Here, we achieve the intercalation of $(\mathrm{\sqrt{3}\times\sqrt{3}})\mathit{R}30^\circ$-ordered Eu layer between epitaxial graphene and SiC substrate, realizing a Kekulé graphene with large local magnetic moments of intercalated Eu atoms. Combining angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) calculations, we revealed that the Kekul{é} order folds the Dirac cones of graphene from the corners to the Brillouin zone center via intervalley scattering, forming the replica Dirac bands with gap opening. More intriguingly, the Dirac fermions in the replica Dirac bands show a strong exchange coupling with the localized magnetic moments of Eu $4f$ orbitals, resulting in a giant splitting of the folded Dirac bands. The observation of strong coupling between Dirac fermions and local magnetic moments of Eu $4f$ electrons via Kekulé order pave a new way for generating Dirac band splitting in graphene, advancing the potential applications of Kekulé-ordered graphene in spintronics, as well as exploring intriguing physical properties and correlation states for quantum technology.

cond-mat.str-el↗

arXiv2024

Light-induced giant enhancement of nonreciprocal transport at KTaO3-based interfaces

Nonlinear transport is a unique functionality of noncentrosymmetric systems, which reflects profound physics, such as spin-orbit interaction, superconductivity and band geometry. However, it remains highly challenging to enhance the nonreciprocal transport for promising rectification devices. Here, we observe a light-induced giant enhancement of nonreciprocal transport at the superconducting and epitaxial CaZrO3/KTaO3 (111) interfaces. The nonreciprocal transport coefficient undergoes a giant increase with three orders of magnitude up to 105 A-1T-1. Furthermore, a strong Rashba spin-orbit coupling effective field of 14.7 T is achieved with abundant high-mobility photocarriers under ultraviolet illumination, which accounts for the giant enhancement of nonreciprocal transport coefficient. Our first-principles calculations further disclose the stronger Rashba spin-orbit coupling strength and the longer relaxation time in the photocarrier excitation process, bridging the light-property quantitative relationship. Our work provides an alternative pathway to boost nonreciprocal transport in noncentrosymmetric systems and facilitates the promising applications in opto-rectification devices and spin-orbitronic devices.

cond-mat.mes-hall↗

arXiv2022

Floquet engineering of magnetic topological insulator MnBi$_2$Te$_4$ films

Floquet engineering is an important way to manipulate the electronic states of condensed matter physics. Recently, the discovery of the magnetic topological insulator MnBi$_2$Te$_4$ and its family provided a valuable platform to study magnetic topological phenomena, such as, the quantum anomalous Hall effect, the axion insulator state and the topological magnetoelectric effect. In this work, based on the effective model and first-principles calculations in combination with the Floquet theory, we reveal that the circularly polarized light (CPL) induces the sign reversal of the Chern number of odd-septuple-layer (SL) MnBi$_2$Te$_4$ thin films. In contrast, the CPL drives the axion insulator state into the quantum anomalous Hall state in even-SL MnBi$_2$Te$_4$ thin films. More interestingly, if the topmost van der Waals gap between the surface layer and the below bulk in MnBi$_2$Te$_4$ films is slightly expanded, a high Chern number $|C|=2$ can be realized under the CPL. Our work demonstrates that the light can induce rich magnetic topological phases in MnBi$_2$Te$_4$ films, which might have potential applications in optoelectronic devices.

cond-mat.mes-hall↗

arXiv2022

Axionic surface wave in dynamical axion insulators

The electromagnetic response of three-dimensional topological insulators can be described by an effective axion action with a quantized axion field. Once both time-reversal and inversion symmetries are broken, for example, in antiferromagnetic topological insulators, the axion field becomes dynamical along with magnetic fluctuations. The dynamical axion field, when coupled to electromagnetic fields, can lead to rich physical phenomena. Here, based on the modified Maxwell's equations, we reveal the existence of an exotic type of polariton excitation, termed a surface axion polariton, which propagates in the interface between a dynamical axion insulator and a dielectric. When doping the dynamical axion insulator to be metallic, the coexistence of axion-photon coupling and plasmon-photon coupling will further generate a mixed surface axion plasmon polariton. We also propose a Kretschmann-Raether configuration to experimentally detect the surface axion polariton. Our result provides an alternative way to study the axion electrodynamics in condensed matter physics.

cond-mat.mes-hall↗

arXiv2022

Direct Visualization and Manipulation of Tunable Quantum Well State in Semiconducting Nb2SiTe4

Quantum well states (QWSs) can form at the surface or interfaces of materials with confinement potential. They have broad applications in electronic and optical devices such as high mobility electron transistor, photodetector and quantum well laser. The properties of the QWSs are usually the key factors for the performance of the devices. However, direct visualization and manipulation of such states are in general challenging. In this work, by using angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling microscopy/spectroscopy (STM/STS), we directly probe the QWSs generated on the vacuum interface of a narrow band gap semiconductor Nb2SiTe4. Interestingly, the position and splitting of QWSs could be easily manipulated via potassium (K) dosage onto the sample surface. Our results suggest Nb2SiTe4 to be an intriguing semiconductor system to study and engineer the QWSs, which has great potential in device applications.

cond-mat.mtrl-sci↗

arXiv2020

Tunable dynamical magnetoelectric effect in antiferromagnetic topological insulator MnBi$_2$Te$_4$ films

More than forty years ago, axion was postulated as an elementary particle with a low mass and weak interaction in particle physics to solve the strong $\mathcal{CP}$ (charge conjugation and parity) puzzle. Axions are also considered as a possible component of dark matter of the universe. However, the existence of axions in nature has not been confirmed. Interestingly, axions arise as pseudoscalar fields derived from the Chern-Simons theory in condensed matter physics. In antiferromagnetic insulators, the axion field can become dynamical induced by spin-wave excitations and exhibits rich exotic phenomena, such as, the chiral magnetic effect, axionic polariton and so on. However, the study of the dynamical axion field is rare due to the lack of real materials. Recently, MnBi$_2$Te$_4$ was discovered to be an antiferromagnetic topological insulator with a quantized axion field protected by the inversion symmetry $\mathcal{P}$ and the magnetic-crystalline symmetry $\mathcal{S}$. Here, we studied MnBi$_2$Te$_4$ films in which both the $\mathcal{P}$ and $\mathcal{S}$ symmetries are spontaneously broken and found that the dynamical axion field and largely tunable dynamical magnetoelectric effects can be realized through tuning the thickness of MnBi$_2$Te$_4$ films, the temperature and the element substitution. Our results open a broad avenue to study axion dynamics in antiferromagnetic topological insulator MnBi$_2$Te$_4$ and related materials, and also is hopeful to promote the research of dark matter.

cond-mat.mes-hall↗

arXiv2020

Large Magnetoresistance in Topological Insulator Candidate TaSe3

Large unsaturated magnetoresistance (XMR) with magnitude about 1000% is observed in topological insulator candidate TaSe3 from our high field (up to 38 T) measurements. Two oscillation modes, associated with one hole pocket and two electron pockets in the bulk, respectively, are detected from our Shubnikov-de Hass (SdH) measurements, consistent with our first-principles calculations. With the detailed Hall measurements performed, our two-band model analysis exhibits an imperfect density ratio n_h/n_e closing 0.9 at T< 20 K , which suggests that the carrier compensations account for the XMR in TaSe3.

cond-mat.mtrl-sci↗

arXiv2020

Large dynamical axion field in topological antiferromagnetic insulator Mn$_2$Bi$_2$Te$_5$

The dynamical axion field is a new state of quantum matter where the magnetoelectric response couples strongly to its low-energy magnetic fluctuations. It is fundamentally different from an axion insulator with a static quantized magnetoelectric response. The dynamical axion field exhibits many exotic phenomena such as axionic polariton and axion instability. However, these effects have not been experimentally confirmed due to the lack of proper topological magnetic materials. Here by combining analytic models and first-principles calculations, we predict a series of van der Waal layered Mn$_2$Bi$_2$Te$_5$-related topological antiferromagnetic materials could host the long-sought dynamical axion field with a topological origin. We also show a large dynamical axion field can be achieved in antiferromagnetic insulating states close to the topological phase transition. We further propose the optical and transport experiments to detect such a dynamical axion field. Our results could directly aid and facilitate the search for topological-origin large dynamical axion field in realistic materials.

cond-mat.mes-hall↗

arXiv2019

Topological axion states in magnetic insulator MnBi$_2$Te$_4$ with the quantized magnetoelectric effect

Topological states of quantum matter have attracted great attention in condensed matter physics and materials science. The study of time-reversal-invariant (TRI) topological states in quantum materials has made tremendous progress in both theories and experiments. As a great success, thousands of TRI topological materials are predicted through sweeping search. Richer exotic phenomena are expected to appear in magnetic topological materials because of varied magnetic configurations, but this study falls much behind due to the complex magnetic structures and transitions. Here, we predict the tetradymite-type compound MnBi$_2$Te$_4$ and its related materials host interesting magnetic topological states. The magnetic ground state of MnBi$_2$Te$_4$ is an antiferromagnetic phase which leads to an antiferromagetic topological insulator state with a large topologically non-trivial energy gap ($\sim$0.2~eV). It is the parent state for the axion state, which has gapped bulk and surface states, and quantized topological magnetoelectric effect. The ferromagnetic phase of MnBi$_2$Te$_4$ leads to an ideal minimal type-II Weyl semimetal with two Weyl points accompanied by one hole-type and one electron-type Fermi pocket at the Fermi level, which has never been discovered elsewhere. We further present a simple and unified continuum model to capture the salient topological features of this kind of materials.

cond-mat.mes-hall↗