arXiv subjects

Toru Morishita

Publications and source records attributed to Toru Morishita.

15 recordsLinked to original sources

arXiv2026

Photoelectron spectroscopy of 3s3p doubly excited helium dressed with strong near-infrared laser fields

We report time-resolved photoelectron spectroscopy of the $3s3p$ doubly excited states of helium dressed by an intense near-infrared (NIR) laser field. Using synchronized XUV free-electron-laser and 800-nm NIR laser pulses, we observe a pronounced delay-dependent shift of resonance-related spectral minima together with the emergence of additional structures around the NIR sideband energy. \textit{Ab initio} theoretical calculations support these observations and identify the features as signatures of NIR-induced coupling of the bright ($3s3p {}^{1}P^{o}$) autoionizing state to nearby dark ($^{1}D^{e}$ and $^{1}S^{e}$) resonances below the $N = 3$ threshold. A multichannel Fano resonance analysis of the measured spectra yields delay-dependent line-shape parameters and resonance energies, establishing a quantitative route to characterize and control correlated two-electron resonances in strong laser fields.

physics.atom-ph↗

arXiv2026

Vortex photoelectron holography in strong-field tunneling ionization

Vortex electrons, characterized by a helical phase front, offer unique advantages for probing material structures. Such electrons can be generated via tunneling ionization in strong laser fields. In this paper, we investigate the rescattering dynamics of vortex photoelectrons by the parent ion. Specifically, we introduce vortex photoelectron holography, extending conventional strong-field photoelectron holography (SFPH) from plane-wave to vortex rescattering. By solving the time-dependent Schrödinger equation, we extract the vortex scattering phase from the SFPH fringes, showing excellent agreement with scattering calculations. Thus, our work provides direct access to the vortex scattering phase, paving the way for applying SFPH to structurally sensitive imaging with phase-engineered photoelectrons.

physics.atom-ph↗

arXiv2019

Quantization of Conductance in Quasi-Periodic Quantum Wires

We study charge transport in the Peierls-Harper model with a quasi-periodic cosine potential. We compute the Landauer-type conductance of the wire. Our numerical results show the following: (i) When the Fermi energy lies in the absolutely continuous spectrum that is realized in the regime of the weak coupling, the conductance is quantized to the universal conductance. (ii) For the regime of localization that is realized for the strong coupling, the conductance is always vanishing irrespective of the value of the Fermi energy. Unfortunately, we cannot make a definite conclusion about the case with the critical coupling. We also compute the conductance of the Thue-Morse model. Although the potential of the model is not quasi-periodic, the energy spectrum is known to be a Cantor set with zero Lebesgue measure. Our numerical results for the Thue-Morse model also show the quantization of the conductance at many locations of the Fermi energy, except for the trivial localization regime. Besides, for the rest of the values of the Fermi energy, the conductance shows a similar behavior to that of the Peierls-Harper model with the critical coupling.

cond-mat.mes-hall↗

arXiv2014

Probing dipole-forbidden autoionizing states by isolated attosecond pulses

We propose a general technique to retrieve the information of dipole-forbidden resonances in the autoionizing region. In the simulation, a helium atom is pumped by an isolated attosecond pulse in the extreme ultraviolet (EUV) combined with a few-femtosecond laser pulse. The excited wave packet consists of the $^1S$, $^1P$, and $^1D$ states, including the background continua, near the $2s2p(^1P)$ doubly excited state. The resultant electron spectra with various laser intensities and time delays between the EUV and laser pulses are obtained by a multilevel model and an ab initio time-dependent Schrödinger equation calculation. By taking the ab initio calculation as a "virtual measurement", the dipole-forbidden resonances are characterized by the multilevel model. We found that in contrast to the common assumption, the nonresonant coupling between the continua plays a significant role in the time-delayed electron spectra, which shows the correlation effect between photoelectrons before they leave the core. This technique takes the advantages of ultrashort pulses uniquely and would be a timely test for the current attosecond technology.

physics.atom-ph↗

arXiv2008

Quantitative rescattering theory for laser-induced high-energy plateau photoelectron spectra

A comprehensive quantitative rescattering (QRS) theory for describing the production of high-energy photoelectrons generated by intense laser pulses is presented. According to the QRS, the momentum distributions of these electrons can be expressed as the product of a returning electron wave packet with the elastic differential cross sections (DCS) between free electrons with the target ion. We show that the returning electron wave packets are determined mostly by the lasers only, and can be obtained from the strong field approximation. The validity of the QRS model is carefully examined by checking against accurate results from the solution of the time-dependent Schrödinger equation for atomic targets within the single active electron approximation. We further show that experimental photoelectron spectra for a wide range of laser intensity and wavelength can be explained by the QRS theory, and that the DCS between electrons and target ions can be extracted from experimental photoelectron spectra. By generalizing the QRS theory to molecular targets, we discuss how few-cycle infrared lasers offer a promising tool for dynamic chemical imaging with temporal resolution of a few femtoseconds.

physics.atom-ph↗

arXiv2008

Origin of Plateau and Species dependence of Laser-Induced High-Energy Photoelectron Spectra

We analyzed the energy and momentum distributions of laser-induced high-energy photoelectrons of alkali and rare gas atoms. For the plateau electrons with energies above $4U_p$, ($U_p$ is the ponderomotive energy), in the tunneling ionization regime, we showed that they originate from the backscattering of laser-induced returning electrons. Using the differential elastic scattering cross sections between the target ion with \emph{free} electrons, we explain experimental observations of whether the plateau electron spectra is flat or steeply descending, and their dependence on species and laser intensity. This quantitative rescattering theory can be used to obtain energy and momentum distributions of plateau electrons without the need of solving the time-dependent Schrödinger equation, but with similar accuracy.

physics.atom-ph↗

arXiv2007

Extraction of the species dependent dipole moment from high-order harmonic spectra in rare gas atoms

Based on high-order harmonic generation (HHG) spectra obtained from solving the time-dependent Schrodinger equation for atoms, we established quantitatively that the HHG yield can be expressed as the product of a returning electron wave packet and the photo-recombination cross sections, and the shape of the returning wave packet is shown to be largely independent of the species. By comparing the HHG spectra generated from different targets under identical laser pulses, accurate structural information, including the phase of the recombination amplitude, can be retrieved. This result opens up the possibility of studying the target structure of complex systems, including their time evolution, from the HHG spectra generated by short laser pulses.

physics.atom-ph↗

arXiv2007

Retrieval of electron-atom scattering cross sections from laser-induced electron rescattering of atomic negative ions in intense laser fields

We investigated the two-dimensional electron momentum distributions of atomic negative ions in an intense laser field by solving the time-dependent Schrodinger equation (TDSE) and using the first- and 2nd-order strong-field approximations (SFA). We showed that photoelectron energy distributions and low-energy photoelectron momentum spectra predicted from SFA are in reasonable agreement with the solutions from the TDSE. More importantly, we showed that accurate electron-atom elastic scattering cross sections can be retrieved directly from high-energy electron momentum spectra of atomic negative ions in the laser field. This opens up the possibility of measuring electron-atom and electron-molecule scattering cross sections from the photodetachment of atomic and molecular negative ions by intense short lasers, respectively, with temporal resolutions in the order of femtoseconds.

physics.atom-ph↗

arXiv2007

Analysis of two-dimensional high-energy photoelectron momentum distributions in single ionization of atoms by intense laser pulses

We analyzed the two-dimensional (2D) electron momentum distributions of high-energy photoelectrons of atoms in an intense laser field using the second-order strong field approximation (SFA2). The SFA2 accounts for the rescattering of the returning electron with the target ion to first order and its validity is established by comparing with results obtained by solving the time-dependent Schrödinger equation (TDSE) for short pulses. By analyzing the SFA2 theory, we confirmed that the yield along the back rescattered ridge (BRR) in the 2D momentum spectra can be interpreted as due to the elastic scattering in the backward directions by the returning electron wave packet. The characteristics of the extracted electron wave packets for different laser parameters are analyzed, including their dependence on the laser intensity and pulse duration. For long pulses we also studied the wave packets from the first and the later returns.

physics.atom-ph↗

arXiv2007

Improved Lewenstein model for high-order harmonic generation of atoms and molecules with scattering wavefunctions

We demonstrate a simple method to improve the Lewenstein model for the description of high-order harmonic generation (HHG). It is shown that HHG spectra can be expressed as the product of a returning electron wave packet and the photo-recombination cross sections, where the former can be extracted from the Lewenstein model. By replacing plane waves with scattering waves in the calculation of recombination matrix elements, we showed that the resulting HHG spectra agree well with those from solving the time-dependent Schrödinger equation. The improved model can be used for quantitative calculations of high harmonics generated by molecules.

physics.atom-ph↗

arXiv2007

Accurate retrieval of structural information from laser-induced photoelectron and high-harmonic spectra by few-cycle laser pulses

By analyzing ``exact'' theoretical results from solving the time-dependent Schrödinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross sections of the target ion with {\em free} electrons can be extracted accurately from laser-generated high-energy electron momentum spectra and high-order harmonic spectra, respectively. Since both electron scattering and photoionization (the inverse of photo-recombination) are the conventional means for interrogating the structure of atoms and molecules, this result shows that existing few-cycle infrared lasers can be implemented for ultrafast imaging of transient molecules with temporal resolution of a few femtoseconds.

physics.atom-ph↗

arXiv2006

Dynamical stabilization of matter-wave solitons revisited

We consider dynamical stabilization of Bose-Einstein condensates (BEC) by time-dependent modulation of the scattering length. The problem has been studied before by several methods: Gaussian variational approximation, the method of moments, method of modulated Townes soliton, and the direct averaging of the Gross-Pitaevskii (GP) equation. We summarize these methods and find that the numerically obtained stabilized solution has different configuration than that assumed by the theoretical methods (in particular a phase of the wavefunction is not quadratic with $r$). We show that there is presently no clear evidence for stabilization in a strict sense, because in the numerical experiments only metastable (slowly decaying) solutions have been obtained. In other words, neither numerical nor mathematical evidence for a new kind of soliton solutions have been revealed so far. The existence of the metastable solutions is nevertheless an interesting and complicated phenomenon on its own. We try some non-Gaussian variational trial functions to obtain better predictions for the critical nonlinearity $g_{cr}$ for metastabilization but other dynamical properties of the solutions remain difficult to predict.

cond-mat.other↗

arXiv2005

Attosecond light pulses to reveal the time-dependent rovibrational motion of the correlated electron pair in helium

We illustrate how attosecond light pulses can be used to directly mapping out the time-dependence of the correlated motion of two excited atomic electrons, discuss how the two-electron correlations manifest themselves in realistic attosecond measurements, and propose the following for experimental exploration: (a) The single ionization signals which directly reveal bending-vibrational motion of the correlated electron pair, (b) and also its rotational motion. (c) The double ionization signals which directly reveal the two-electron density in momentum space. To facilitate the description of the above points, use is made of simple wave packets of doubly-excited states of helium.

physics.atom-ph↗

arXiv2005

Gyroscopic effects in interference of matter waves

A new gyroscopic interference effect stemming from the Galilean translational factor in the matter wave function is pointed out. In contrast to the well-known Sagnac effect that stems from the geometric phase and leads to a shift of interference fringes, this effect causes slanting of the fringes. We illustrate it by calculations for two split cigar-shaped Bose-Einstein condensates under the conditions of a recent experiment, see Y.Shin et al., Phys. Rev. Lett. 92, 050405 (2004). Importantly, the measurement of slanting obviates the need of a third reference cloud.

cond-mat.other↗

arXiv2005

Siegert pseudostate perturbation theory: one- and two-threshold cases

Perturbation theory for the Siegert pseudostates (SPS) [Phys.Rev.A 58, 2077 (1998) and Phys.Rev.A 67, 032714 (2003)] is studied for the case of two energetically separated thresholds. The perturbation formulas for the one-threshold case are derived as a limiting case whereby we reconstruct More's theory for the decaying states [Phys.Rev.A 3,1217(1971)] and amend an error. The perturbation formulas for the two-threshold case have additional terms due to the non-standard orthogonality relationship of the Siegert Pseudostates. We apply the theory to a 2-channel model problem, and find the rate of convergence of the perturbation expansion should be examined with the aide of the variance $D= ||E-\sum_{n}λ^n E^{(n)}||$ instead of the real and imaginary parts of the perturbation energy individually.

physics.atom-ph↗