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Trinanjan Datta

Publications and source records attributed to Trinanjan Datta.

At least 37 records · Page 2Linked to original sources

Torque equilibrium spin wave theory study of anisotropy and Dzyaloshinskii-Moriya interaction effects on the indirect K$-$ edge RIXS spectrum of a triangular lattice antiferromagnet

We apply the recently formulated torque equilibrium spin wave theory (TESWT) to compute the $1/S$-order interacting $K$ -edge bimagnon resonant inelastic x-ray scattering (RIXS) spectra of an anisotropic triangular lattice antiferromagnet with Dzyaloshinskii-Moriya (DM) interaction. We extend the interacting torque equilibrium formalism, incorporating the effects of DM interaction, to appropriately account for the zero-point quantum fluctuation that manifests as the emergence of spin Casimir effect in a noncollinear spin spiral state. Using inelastic neutron scattering data from Cs$_2$CuCl$_4$ we fit the 1/S corrected TESWT dispersion to extract exchange and DM interaction parameters. We use these new fit coefficients alongside other relevant model parameters to investigate, compare, and contrast the effects of spatial anisotropy and DM interaction on the RIXS spectra at various points across the magnetic Brillouin zone. We highlight the key features of the bi- and trimagnon RIXS spectrum at the two inequivalent rotonlike points, $M(0,2 π/\sqrt{3})$ and $M^{\prime}(π,π/\sqrt{3})$, whose behavior is quite different from an isotropic triangular lattice system. While the roton RIXS spectrum at the $M$ point undergoes a spectral downshift with increasing anisotropy, the peak at the $M^\prime$ location loses its spectral strength without any shift. With the inclusion of DM interaction the spiral phase is more stable and the peak at both $M$ and $M^\prime$ point exhibits a spectral upshift. Our calculation offers a practical example of how to calculate interacting RIXS spectra in a non-collinear quantum magnet using TESWT. Our findings provide an opportunity to experimentally test the predictions of interacting TESWT formalism using RIXS, a spectroscopic method currently in vogue.

cond-mat.mtrl-sci↗

Spectroscopic signatures of next-nearest-neighbor hopping in the charge and spin dynamics of doped one-dimensional antiferromagnets

We study the impact of next-nearest-neighbor (nnn) hopping on the low-energy collective excitations of strongly correlated doped antiferromagnetic cuprate spin chains. Specifically, we use exact diagonalization and the density matrix renormalization group method to study the single-particle spectral function, the dynamical spin and charge structure factors, and the Cu $L$-edge resonant inelastic x-ray scattering (RIXS) intensity of the doped $t$-$t^\prime$-$J$ model for a set of $t^\prime$ values. We find evidence for the breakdown of spin-charge separation as $|t^\prime|$ increases and identify its fingerprints in the dynamical response functions. The inclusion of nnn hopping couples the spinon and holon excitations, resulting in the formation of a spin-polaron, where a ferromagnetic spin polarization cloud dresses the doped carrier. The spin-polaron manifests itself as additional spectral weight in the dynamical correlation functions, which appear simultaneously in the spin- and charge-sensitive channels. We also demonstrate that RIXS can provide a unique view of the spin-polaron, due to its sensitivity to both the spin and charge degrees of freedom.

cond-mat.str-el↗

$K$ -edge and $L_{3}$ -edge RIXS study of columnar and staggered quantum dimer phases of the square lattice Heisenberg model

We compute the $K$ and $L_{3}$ -edge resonant inelastic x-ray scattering (RIXS) spectrum of the columnar and the staggered quantum dimer states accessible to the square lattice Heisenberg magnet. Utilizing a bond operator representation mean field theory we investigate the RIXS features of the one- and two-triplon excitation spectrum supported by the quantum dimer model in the background of condensed singlet excitation. We find that the two-triplon excitation boundary lies within a 124 (78) meV to (414) 345 meV energy range for the columnar (staggered) phase. We estimated the two-triplon gap to be 124 (78) meV for the columnar (staggered) dimer phase. The highest intensity of the $K$ -edge RIXS spectrum is centralized approximately around the $(π/2,π/2)$ point for both the columnar and the staggered phases. At the $L_{3}$ -edge we study the one- and two- triplon signal considering experimental scattering geometry, polarization restriction, and experimental resolution effects. Our calculations find an additional contribution to the two-triplon RIXS signal, not previously reported in the literature, that originates from the local hard-core dimer constraint. This leads to a finite non-zero signal at the (0,0) momentum transfer which can offer an explanation for the existing ladder RIXS experiments and also predicts a non-zero signal for the two-dimensional quantum dimer system. We find that the $L_3$ edge RIXS response of the one- and two-triplon signal could exist in antiphase rung modulation for zero and $π$ as found in inelastic neutron scattering. We also consider static crystal twinning at the $L_3$ -edge RIXS signal to mimic realistic crystal effects. Since the disordered phase has the potential to harbor a variety of quantum paramagnetic states, our RIXS calculations provide useful signatures to identify the true nature of the ordering pattern.

cond-mat.str-el↗

Detecting Crystallographic Lattice Chirality using Resonant Inelastic X-ray Scattering

The control and detection of crystallographic chirality is an important and challenging scientific problem. Chirality has wide ranging implications from medical physics to cosmology including an intimate but subtle connection in magnetic systems, for example Mn$_{1-x}$Fe$_{x}$Si. X-ray diffraction techniques with resonant or polarized variations of the experimental setup are currently utilized to characterize lattice chirality. We demonstrate using theoretical calculations the feasibility of indirect $K$ -edge bimagnon resonant inelastic X-ray scattering (RIXS) spectrum as a viable experimental technique to distinguish crystallographic handedness. We apply spin wave theory to the recently discovered $\sqrt {5}\times\sqrt {5}$ vacancy ordered chalcogenide Rb$_{0.89}$Fe$_{1.58}$Se$_{2}$ for realistic X-ray experimental set up parameters (incoming energy, polarization, and Bragg angle) to show that the computed RIXS spectrum is sensitive to the underlying handedness (right or left) of the lattice. A Flack parameter definition that incorporates the right- and left- chiral lattice RIXS response is introduced. It is shown that the RIXS response of the multiband magnon system RbFeSe arises both from inter- and intra- band scattering processes. The extinction or survival of these RIXS peaks are sensitive to the underlying chiral lattice orientation. This in turn allows for the identification of the two chiral lattice orientations.

cond-mat.str-el↗

Magnon-phonon coupling effects on the indirect K-edge resonant inelastic X-ray scattering spectrum of a 2D Heisenberg antiferromagnet

We compute the effects of magnon-phonon coupling on the indirect K-edge bimagnon resonant inelastic x-ray scattering (RIXS) intensity spectrum of a square lattice Heisenberg antiferromagnet. We analyze the effects of competing nearest and next--nearest magnetic and magnon-phonon coupling interaction in the RIXS spectrum, for both the antiferromagnetic (AF) and the collinear antiferromagnetic (CAF) phases of the model. Utilizing the Dyson-Maleev representation of spin operators, the Bethe-Salpeter ladder approximation scheme for the bimagnon interacting channel, and considering the lowest order magnon-phonon-magnon scattering interaction we highlight distinct features in the X-ray spectrum. Considering damping effects, arising due to the presence of phonons, we find that in the AF phase the RIXS intensity spectrum attains a maximum value primarily localized around the K $\left(\pm\fracπ{2}, \pm \fracπ{2}\right)$ - point. For the CAF phase the intensity is broadly distributed with a significant scattering intensity located around the Y $\left(\pm\fracπ{2}, 0\right)$ - point. Furthermore, in the CAF phase for suitable anisotropy, nearest-, and next-nearest neighbor interaction parameters the phonon effects can manifest itself as a distinct peak both below and above the bimagnon peak. Such a feature is in contrast to the antiferromagnetic spectrum where the effect due to the phonon peak was located consistently beyond the bimagnon peak in the high energy end of the spectrum. Additionally, in the CAF phase we find the RIXS bimagnon-phonon spectrum to be more sensitive to anisotropy compared to its antiferromagnetic counterpart. We conclude that the ultimate effect of magnon-phonon effects in the indirect K-edge RIXS spectrum, in both the antiferromagnetic and the collinear antiferromagnetic phase, is an observable effect.

cond-mat.str-el↗

Indirect K-edge bimagnon resonant inelastic X-ray scattering spectrum of $α$-FeTe

We calculate the K-edge indirect bimagnon resonant inelastic X-ray scattering (RIXS) intensity spectra of the bicollinear antiferromagnetic order known to occur in the $α$-FeTe chalcogenide system. Utilizing linear spin wave theory for this large-S spin system we find that the bimagnon spectrum contains four scattering channels (two intraband and two interband). We find from our calculations that for suitable energy-momentum combination the RIXS spectra can exhibit a one-, two- or three- peak structure. The number of peaks provides a clue on the various bimagnon excitation processes that can be supported both in and within the acoustic and optical magnon branches of the bicollinear antiferromagnet. Unlike the RIXS response of the antiferromagnetic or the collinear antiferromagnetic spin ordering, the RIXS intensity spectrum of the bicollinear antiferromagnet does not vanish at the magnetic ordering wave vector $(π/2,-π/2)$. It is also sensitive to next-next nearest neighbor and biquadratic coupling interactions. Our predicted RIXS spectrum can be utilized to understand the role of multi-channel bimagnon spin excitations present in the $α$-FeTe chalcogenide.

cond-mat.mtrl-sci↗

Spin and quadrupolar orders in the spin-1 bilinear-biquadratic model for iron-based superconductors

Motivated by recent experimental and theoretical progresses of the magnetic properties of iron-based superconductors, we provide a comprehensive analysis of the spin-1 bilinear-biquadratic (BBQ) model on the square lattice. Using variational approach in the mean-field level, we identify the existence of various magnetic phases, including conventional spin dipolar orderings (ferro- or antiferromagnet), novel quadrupolar (spin nematic) orderings and mixed dipolar-quadrupolar orderings. In contrast to the usual Heisenberg model, the elementary excitations of the spin-1 BBQ model are described by the flavor-wave theory within the SU(3) representation. By fitting the experimental spin-wave dispersion, we determine the refined exchange couplings corresponding to the collinear antiferromagnetic iron pnictides. We also present the dynamic structure factors of both spin dipolar and quadrupolar components with connections to the future experiments.

cond-mat.str-el↗

Signatures of indirect K-edge resonant inelastic x-ray scattering on magnetic excitations in triangular lattice antiferromagnet

We compute the K-edge indirect resonant inelastic x-ray scattering (RIXS) spectrum of a triangular lattice antiferromagnet in its ordered coplanar 3- sublattice 120 degree magnetic state. By considering the first order self$-$energy corrections to the spin wave spectrum, magnon decay rate, bimagnon interactions within the ladder approximation Bethe-Salpeter scheme, and the effect of three-magnon contributions up to 1/S- order we find that the RIXS spectra is non-trivially affected. For a purely isotropic triangular lattice model, the peak splitting mechanism and the appearance of a multipeak RIXS structure is primarily dictated by the damping of magnon modes. At a scattering wavevector corresponding to the zone center Γpoint and at the roton point q=M, where the magnon decay rate is zero, a stable single peak forms. At the $Γ$ point, the contribution is purely trimagnon at the 1/S level and occurs approximately at the trimagnon energy of 6JS. The roton peak occurs at a lower energy of 4JS. The K-edge single peak RIXS spectra at the roton momentum can be utilized as an experimental signature to detect the presence of roton excitations. A unique feature of the triangular lattice K-edge RIXS spectra is the nonvanishing RIXS intensity at both the zone center $Γ$ point and the antiferromagnetic wavevector K point. This result is in sharp contrast to the vanishing K-edge RIXS intensity of the collinear magnetic phases on the square lattice. We find that including XXZ anisotropy leads to additional peak splitting, including at the roton scattering wavevector where the single peak destabilizes towards a two-peak structure. The observed splitting is consistent with our earlier theoretical prediction of the effects of spatial anisotropy on the RIXS spectra of a frustrated quantum magnet [Luo, Datta, and Yao, Phys. Rev. B 89, 165103 (2014)].

cond-mat.mtrl-sci↗

Spectrum splitting of bimagnon excitations in a spatially frustrated Heisenberg antiferromagnet revealed by resonant inelastic x-ray scattering

We perform a comprehensive analysis of the bimagnon resonant inelastic x-ray scattering (RIXS) intensity spectra of the spatially frustrated Jx-Jy-J2 Heisenberg model on a square lattice in both the antiferromagnetic and the collinear antiferromagnetic phase. We study the model for strong frustration and significant spatial anisotropy to highlight the key signatures of RIXS spectrum splitting which may be experimentally discernible. Based on an interacting spin wave theory study within the ladder approximation Bethe-Salpeter scheme, we find the appearance of a robust two-peak structure over a wide range of the transferred momenta in both magnetically ordered phases. The unfrustrated model has a single-peak structure with a two-peak splitting originating due to spatial anisotropy and frustrated interactions. Our predicted two-peak structure from both magnetically ordered regime can be realized in iron pnictides.

cond-mat.str-el↗

Exact solution and high temperature series expansion study of the 1/5-th depleted square lattice Ising model

The critical behavior of the 1/5-depleted square-lattice Ising model with nearest neighbor ferromagnetic interaction has been investigated by means of both an exact solution and a high-temperature series expansion study of the zero-field susceptibility. For the exact solution we employ a decoration transformation followed by a mapping to a staggered 8-vertex model. This yields a quartic equation for the critical coupling giving $K_{c} (\equivβJ_{c}) =0.695$. The series expansion for the susceptibility, to $\mathcal{O}(K^{18})$, when analyzed via standard Padé approximant methods gives an estimate of K$_{c}$, consistent with the exact solution result to at least four significant figures. The series expansion is also analyzed for the leading amplitude and subdominant terms.

cond-mat.stat-mech↗

Spin transport in the Neel and collinear antiferromagnetic phase of the two dimensional spatial and spin anisotropic Heisenberg model on a square lattice

We analyze and compare the effect of spatial and spin anisotropy on spin conductivity in a two dimensional S=1/2 Heisenberg quantum magnet on a square lattice. We explore the model in both the Neel antiferromagnetic (AF) phase and the collinear antiferromagnetic (CAF) phase. We find that in contrast to the effects of spin anisotropy in the Heisenberg model, spatial anisotropy in the AF phase does not suppress the zero temperature regular part of the spin conductivity in the zero frequency limit - rather it enhances it. We also explore the finite temperature effects on the Drude weight in the AF phase for various spatial and spin anisotropy parameters. We find that the Drude weight goes to zero as the temperature approaches zero. At finite temperatures (within the collision less approximation) enhancing spatial anisotropy increases the Drude weight value and increasing spin anisotropy decreases the Drude weight value. In the CAF phase (within the non-interacting approximation) the zero frequency spin conductivity has a finite value for non-zero values of the spatial anisotropy parameter. In the CAF phase increasing the spatial anisotropy parameter suppresses the regular part of the spin conductivity response at zero frequency. Furthermore, we find that the CAF phase displays a spike in the spin conductivity not seen in the AF phase. Inclusion of the smallest amount of spin anisotropy causes a gap to develop in the spin conductivity response of both the AF and CAF phase. Based on these studies we conclude that materials with spatial anisotropy are better spin conductors than those with spin anisotropy both at zero and finite temperatures. We utilize exchange parameter ratios for real material systems as inputs to the computation of spin conductivity.

cond-mat.str-el↗

Spin wave theory study of neutron intensity, magnetic field, and anisotropy of Type IIA FCC antiferromagnet

We study the spin dynamics in a 3D quantum antiferromagnet on a face-centered cubic (FCC) lattice. The effects of magnetic field, single-ion anisotropy, and biquadratic interactions are investigated using linear spin wave theory with spins in a canted basis about the Type IIA FCC antiferromagnetic ground state structure which is known to be stable. We calculate the expected finite frequency neutron scattering intensity and give qualitative criteria for typical FCC materials MnO and CoO. The magnetization reduction due to quantum zero point fluctuations is also analyzed.

cond-mat.mtrl-sci↗

Effect of next-nearest neighbor interactions on the dynamic order parameter of the Kinetic Ising model in an oscillating field

We study the effects of next-nearest neighbor (NNN) interactions in the two-dimensional ferromagnetic kinetic Ising model exposed to an oscillating field. By tuning the interaction ratio (p = JNNN/JNN) of the NNN (JNNN) to the nearest-neighbor (NN) interaction (JNN) we find that the model undergoes a transition from a regime in which the dynamic order parameter Q is equal to zero to a phase in which Q is not equal to zero. From our studies we conclude that the model can exhibit an interaction induced transition from a deterministic to a stochastic state. Furthermore, we demonstrate that the systems' metastable lifetime is sensitive not only to the lattice size, external field amplitude, and temperature (as found in earlier studies) but also to additional interactions present in the system.

cond-mat.stat-mech↗

Dynamic phase transition and hysteresis dispersion law of the kinetic Ising model with next-nearest neighbor interaction

We study the effects of next-nearest neighbor (NNN) interaction on the dynamic phase transition (DPT) and hysteresis loop area law in the two-dimensional ferromagnetic kinetic Ising model. We find that inclusion of the NNN interaction causes the DPT boundary of the NN kinetic Ising model to shift to larger values of magnetic field and temperature. The NNN kinetic Ising model can therefore exhibit an interaction induced DPT. Also in the low frequency limit (f$\to$0) the hysteresis loop area law, A(h$_{o}$,f), changes from h$^{0.70}_{o}$f$^{0.36}$ (NN) to h$^{0.14\pm 0.01}_{o}$f$^{0.13\pm0.01}$ (NNN) where h$_o$ is the external field amplitude and f is the frequency. DPT and hysteresis in the kinetic Ising model arises as a competition between the system's metastable lifetime and the time period of the external field. Including the NNN interaction changes the system's metastable lifetime. This causes the DPT and the hysteretic properties to change. We conclude that the systems metastable lifetime is sensitive not only to the lattice size, external field amplitude, and temperature but also to additional interactions present in the system. Furthermore by tracking the probability density P(Q) of the dynamic order parameter Q we conclude that the DPT is of second order.

cond-mat.stat-mech↗

Zero temperature phases of the frustrated J1-J2 antiferromagnetic spin-1/2 Heisenberg model on a simple cubic lattice

At zero temperature magnetic phases of the quantum spin-1/2 Heisenberg antiferromagnet on a simple cubic lattice with competing first and second neighbor exchanges (J1 and J2) is investigated using the non-linear spin wave theory. We find existence of two phases: a two sublattice Neel phase for small J2 (AF), and a collinear antiferromagnetic phase at large J2 (CAF). We obtain the sublattice magnetizations and ground state energies for the two phases and find that there exists a first order phase transition from the AF-phase to the CAF-phase at the critical transition point, pc = 0.28. Our results for the value of pc are in excellent agreement with results from Monte-Carlo simulations and variational spin wave theory. We also show that the quartic 1/S corrections due spin-wave interactions enhance the sublattice magnetization in both the phases which causes the intermediate paramagnetic phase predicted from linear spin wave theory to disappear.

cond-mat.str-el↗

Non-linear spin wave theory results for the frustrated S = 1/2 Heisenberg antiferromagnet on a body-centered cubic lattice

At zero temperature the sublattice magnetization of the quantum spin-1/2 Heisenberg antiferromagnet on a body-centered cubic lattice with competing first and second neighbor exchange (J1 and J2) is investigated using the non-linear spin wave theory. The zero temperature phases of the model consist of a two sublattice Néel phase for small J_2 (AF_1) and a collinear phase at large J_2 (AF_2). We show that quartic corrections due to spin-wave interactions enhance the sublattice magnetization in both the AF_1 and the AF_2 phase. The magnetization corrections are prominent near the classical transition point of the model and in the J_2> J_1 regime. The ground state energy with quartic interactions is also calculated. It is found that up to quartic corrections the first order phase transition (previously observed in this model) between the AF_1 and the AF_2 phase survives.

cond-mat.str-el↗

Impurity effects in multiferroic compounds

We investigate the effect of impurities in multiferroic materials using an equation of motion approach for the spin dynamics of the host multiferroic compound. We model the impurities as a two-level system and focus on the regime where the impurity spins relax slowly. When the impurity strength is weak the host spins oscillate with no decay and the electric polarization is not affected. However as the impurity strength is increased the host spin components get damped and the electrion polarization is suppressed. Since polarization in multiferroic materials is driven by magnetic ordering we conclude that the presence of impurities is detrimental to multiferroicity.

cond-mat.str-el↗

1D-FFLO state in the absence of time-reversal symmetry breaking

A novel route to a one-dimensional Fulde-Ferrell-Larkin-Ovchinnikov (1D-FFLO) state in the absence of broken time-reversal symmetry is proposed in this paper. At present such a state may be encouraged in a clean AlAs quantum wire. Using the AlAs quantum wire as an example it is shown using bosonization and the renormalization group approach that the 1D-FFLO state can arise due to a combination of Coulomb interactions and the unique bandstructure arrangement of the AlAs quantum wire. The present theoretical proposal is very general and is applicable to other systems with similar fermionic interaction terms.

cond-mat.str-el↗