arXiv subjects

Tsutomu Momoi

Publications and source records attributed to Tsutomu Momoi.

At least 19 recordsLinked to original sources

arXiv2026

Antisymmetric Dynamical Spin Correlations: Spin-Space-Group Constraints and Frequency-Moment Sum Rules

Polarized inelastic neutron scattering probes the handedness of magnetic excitations through the spin-component-antisymmetric part of the dynamical spin-structure-factor tensor. We derive its symmetry constraints under unitary and antiunitary residual operations of magnetic space groups and spin-space groups. These constraints determine the allowed tensor components, their parity under momentum reversal, and symmetry-enforced nodes. We then introduce the corresponding antisymmetric commutator spectral function and derive exact zero-temperature sum rules for its frequency moments. The zeroth moment is fixed by the uniform magnetization. For Heisenberg or XXZ exchange Hamiltonians, the first moment of the $xy$ component is fixed by a momentum-weighted static vector chirality. For compensated collinear antiferromagnets, the antisymmetric dynamical structure factor is forbidden when inversion or a translation relates the opposite-spin sublattices. In rotation-related altermagnets, however, an $xy$ component that is even under momentum reversal is allowed at generic wave vectors. Finite antisymmetric spectral weight can therefore coexist with vanishing zeroth and first moments of the commutator spectral function. In a planar helix, by contrast, a residual antiunitary spin-space-group symmetry makes the allowed $xy$ component odd under momentum reversal. Its first moment is generally nonzero and is fixed by a momentum-weighted static vector chirality through the first-moment sum rule. Linear spin-wave calculations for representative altermagnetic and helical models explicitly realize these symmetry and sum-rule constraints.

cond-mat.str-el↗

arXiv2026

Numerical Block Diagonalization and Linked-Cluster Expansion for Deriving Effective Hamiltonians: Applications to Spin Excitations

We present a numerical, non-perturbative framework for constructing effective Hamiltonians that describe the dynamics of low-energy degrees of freedom within a restricted Hilbert space in quantum many-body systems. The approach is based on block diagonalization guided by a minimal-deformation principle imposed within a selected target sector. The formulation is designed to remain compatible with the numerical linked-cluster expansion. For gapped systems, the relation between minimal deformation and cluster additivity requires careful treatment when excited eigenstates contain finite admixtures of the ground state. After establishing a cluster-additive basis that reproduces the Hörmann-Schmidt construction, the minimal-deformation criterion uniquely determines the effective Hamiltonian within each excitation sector. The same criterion also provides a practical numerical procedure for selecting relevant low-energy eigenstates, including regimes characterized by strong level mixing and avoided crossings. The framework is illustrated using two spin models: the one-dimensional transverse-field Ising model as a benchmark and the two-dimensional Shastry-Sutherland model with Dzyaloshinskii-Moriya interactions, relevant to SrCu$_2$(BO$_3$)$_2$. In both cases, the resulting effective Hamiltonians accurately capture the excitation dynamics and the associated band structures.

cond-mat.str-el↗

arXiv2024

Dynamics of quantum spin-nematics: Comparisons with canted antiferromagnets

The identification of spin-nematic states is challenging due to the absence of Bragg peaks. However, the study of dynamical physical quantities provides a promising avenue for characterizing these states. In this study, we investigate the dynamical properties of spin-nematic states in three-dimensional quantum spin systems in a magnetic field, using a two-component boson theory that incorporates magnons and bi-magnons. Our particular focus lies on the dynamical spin structure factor at zero temperature and the nuclear magnetic resonance (NMR) relaxation rate at finite temperatures. Our findings reveal that the dynamical structure factor does not exhibit any diverging singularity across momentum and frequency while providing valuable information about the form factor of bi-magnon states and the underlying structure of spin-nematic order. Furthermore, we find a temperature dependence in the NMR relaxation rate proportional to $T^3$ at low temperatures, similar to canted antiferromagnets. A clear distinction arises as there is no critical divergence of the NMR relaxation rate at the spin-nematic transition temperature. Our theoretical framework provides a comprehensive understanding of the excitation spectrum and the dynamical properties of spin-nematic states, covering arbitrary spin values $S$ and encompassing site and bond nematic orders. Additionally, we apply the same methodology to analyze these dynamical quantities in a canted antiferromagnetic state and compare the results with those in the spin-nematic states.

cond-mat.str-el↗

arXiv2022

Magnetically hidden state on the ground floor of the magnetic Devil's staircase

We investigated the low-temperature and high-field thermodynamic and ultrasonic properties of SrCu2(BO3)2, which exhibits various plateaux in its magnetization curve above 27~T, called a magnetic Devil's staircase. The results of the present study confirm that magnetic crystallization, the first step of the staircase, occurs above 27~T as a 1st-order transition accompanied by a sharp singularity in heat capacity $C_p$ and a kink in the elastic constant. In addition, we observe a thermodynamic anomaly at lower fields around 26~T, which has not been previously detected by any magnetic probes. At low temperatures, this magnetically hidden state has a large entropy and does not exhibit Schottky-type gapped behavior, which suggests the existence of low-energy collective excitations. Based on our observations and theoretical predictions, we propose that magnetic quadrupoles form a spin-nematic state around 26~T as a hidden state on the ground floor of the magnetic Devil's staircase.

cond-mat.str-el↗

arXiv2022

Novel quantum phase of the chromium spinel oxide HgCr$_{\rm 2}$O$_{\rm 4}$ in high magnetic fields

In this study, we have performed the magnetocaloric effect and the specific heat measurements of chromium spinel oxide HgCr$_2$O$_4$, wherein the magnetic Cr$^{3+}$ ions form a highly frustrated pyrochlore lattice with significant spin-lattice coupling. In addition to the known magnetic-field-induced phases, our thermodynamic measurements detect a novel quantum phase just before the saturation of the magnetization, which has not been expected from the classical theories of the pyrochlore lattice antiferromagnet with spin-lattice coupling. Based on recent theoretical model calculation, we discuss the possibility of a spin nematic state appearing for this quantum phase.

cond-mat.str-el↗

arXiv2020

Anomalies of kagome antiferromagnets on magnetization plateaus

We discuss the ground-state degeneracy of spin-$1/2$ kagome-lattice quantum antiferromagnets on magnetization plateaus by employing two complementary methods: the adiabatic flux insertion in closed boundary conditions and a 't Hooft anomaly argument on inherent symmetries in a quasi-one-dimensional limit. The flux insertion with a tilted boundary condition restricts the lower bound of the ground-state degeneracy on $1/9$, $1/3$, $5/9$, and $7/9$ magnetization plateaus under the $\mathrm{U(1)}$ spin-rotation and the translation symmetries: $3$, $1$, $3$, and $3$, respectively. This result motivates us further to develop an anomaly interpretation of the $1/3$ plateau. Taking advantage of the insensitivity of anomalies to spatial anisotropies, we examine the existence of the unique gapped ground state on the $1/3$ plateau from a quasi-one-dimensional viewpoint. In the quasi-one-dimensional limit, kagome antiferromagnets are reduced to weakly coupled three-leg spin tubes. Here, we point out the following anomaly description of the $1/3$ plateau. While a simple $S=1/2$ three-leg spin tube cannot have the unique gapped ground state on the $1/3$ plateau because of an anomaly between a $\mathbb Z_3\times \mathbb Z_3$ symmetry and the translation symmetry at the $1/3$ filling, the kagome antiferromagnet breaks explicitly one of the $\mathbb Z_3$ symmetries related to a $\mathbb Z_3$ cyclic transformation of spins in the unit cell. Hence the kagome antiferromagnet can have the unique gapped ground state on the $1/3$ plateau.

cond-mat.str-el↗

arXiv2020

Effects of Dzyaloshinskii-Moriya interactions in volborthite: Magnetic orders and thermal Hall effect

Volborthite offers an interesting example of a highly frustrated quantum magnet in which ferromagnetic and antiferromagnetic interactions compete on anisotropic kagome lattices. A recent density functional theory calculation has provided a magnetic model based on coupled trimers, which is consistent with a broad 1/3-magnetization plateau observed experimentally. Here we study the effects of Dzyaloshinskii-Moriya (DM) interactions in volborthite. We derive an effective model in which pseudospin-1/2 moments emerging on trimers form a network of an anisotropic triangular lattice. Using the effective model, we show that for a magnetic field perpendicular to the kagome layer, magnon excitations from the 1/3-plateau feel a Berry curvature due to the DM interactions, giving rise to a thermal Hall effect. Our magnon Bose gas theory can explain qualitative features of the magnetization and the thermal Hall conductivity measured experimentally. A further quantitative comparison with experiment poses constraints on the coupling constants in the effective model, promoting a quasi-one-dimensional picture. Based on this picture, we analyze low-temperature magnetic phase diagrams using effective field theory, and point out their crucial dependence on the field direction.

cond-mat.str-el↗

arXiv2019

Spin nematics in frustrated spin-dimer systems with bilayer structure

We study frustrated spin-1/2 dimer systems in two dimensions with a bilayer structure, where spins are ferromagnetically coupled in dimers. Our model includes frustrated two-spin exchange interactions as well as four-spin interaction. We pay particular attention to the spin nematic phase, which does not exhibit any magnetic (spin-dipole) order but has a spin-quadrupolar long-range order. Employing a perturbation calculation, a mean-field approximation, and a numerical many-variable variational Monte Carlo method, we determine ground-state phase diagrams on various two-dimensional lattices. It is found that the model exhibits the spin nematic phase with ferro-quadrupolar order in a wide parameter region, in addition to conventional magnetically-ordered phases. In particular, it is shown that even when the four-spin interactions are absent, frustrated two-spin exchange interactions can realize the spin nematic phase as a result of strong interdimer correlations. It is also found that the phase transitions between the spin nematic phase and antiferromagnetic phases can be continuous. Furthermore, we present some exact arguments that various phases including the spin nematic phase and the vector chiral (p-type nematic) phase emerge from an SU(4) symmetric point in the model by the addition of appropriate perturbative interactions. The spin nematic phase generated from the SU(4) point is connected with the spin nematic phase found numerically in the system with only two-spin interactions.

cond-mat.str-el↗

arXiv2019

Spin-Wave Theory for the Scalar Chiral Phase in the Multiple-Spin Exchange Model on a Triangular Lattice

We study the effects of quantum fluctuations on a non-coplanar tetrahedral spin structure, which has a scalar chiral order, in the spin-1/2 multiple-spin exchange model with up to the six-spin exchange interactions on a triangular lattice. We find that, in the linear spin-wave approximation, the tetrahedral structure survives the quantum fluctuations because spin waves do not soften in the whole parameter region of the tetrahedral-structure phase evaluated for the classical system. In the quantum corrections to the ground-state energy, sublattice magnetization, and scalar chirality, the effects of the quantum fluctuations are small for the ferromagnetic nearest-neighbor interactions and for the strong five-spin interactions. The six-spin interactions have little effect on the quantum corrections in the tetrahedral-structure phase. This calculation also corrects an error in the previously reported value of scalar chirality for the spin-1/2 multiple-spin exchange model with up to the four-spin exchange interactions.

cond-mat.str-el↗

arXiv2018

Symmetry protected topological phases in two-orbital SU(4) fermionic atoms

We study one-dimensional systems of two-orbital SU(4) fermionic cold atoms. In particular, we focus on an SU(4) spin model [named SU(4) $e$-$g$ spin model] that is realized in a low-energy state in the Mott insulator phase at the filling $n_g=3, n_e=1$ ($n_g, n_e$: numbers of atoms in ground and excited states, respectively). Our numerical study with the infinite-size density matrix renormalization group shows that the ground state of SU(4) $e$-$g$ spin model is a nontrivial symmetry protected topological (SPT) phase protected by $Z_4 \times Z_4$ symmetry. Specifically, we find that the ground state belongs to an SPT phase with the topological index $2\in\mathbb{Z}_4$ and show sixfold degenerate edge states. This is topologically distinct from SPT phases with the index $1\in\mathbb{Z}_4$ that are realized in the SU(4) bilinear model and the SU(4) Affleck-Kennedy-Lieb-Tasaki (AKLT) model. We explore the phase diagram of SU(4) spin models including $e$-$g$ spin model, bilinear-biquadratic model, and AKLT model, and identify that antisymmetrization effect in neighboring spins (that we quantify with Casimir operators) is the driving force of the phase transitions. Furthermore, we demonstrate by using the matrix product state how the $\mathbb{Z}_4$ SPT state with six edge states appears in the SU(4) $e$-$g$ spin model.

cond-mat.str-el↗

arXiv2018

Kinetic frustration induced supersolid in the $S=1/2$ kagome lattice antiferromagnet in a magnetic field

We examine instabilities of the plateau phases in the spin-1/2 kagome-lattice antiferromagnet in an applied field by means of degenerate perturbation theory, and find some emergent supersolid phases below the $m=5/9$ plateau. The wave functions of the plateau phases in a magnetic field have the particular construction based on the building blocks of resonating hexagons and their surrounding sites. Magnon excitations on each of these blocks suffer from a kinetic frustration effect, namely, they cannot hop easily to the others since the hopping amplitudes through the two paths destructively cancel out with each other. The itineracy is thus weakened, and the system is driven toward the strong coupling regime, which together with the selected paths allowed in real space bears a supersolid phase. This mechanism is contrary to that proposed in lattice-Bose gases, where the strong competing interactions suppress with each other, allowing a small kinetic energy scale to attain the itinerancy. Eventually, we find a supersolid state in which the pattern of resonating hexagons are preserved from the plateau crystal state and only one-third of the originally polarized spins outside the hexagons dominantly join the superfluid component, or equivalently, participate in the magnetization process.

cond-mat.str-el↗

arXiv2018

Electron spin resonance for the detection of long-range spin nematic order

In this paper we propose that electron spin resonance (ESR) measurements enable us to detect the long-range spin nematic order. We show that the frequency of the paramagnetic resonance peak in the ESR spectrum is shifted by the ferroquadrupolar order parameter together with other quantities. The ferroquadrupolar order parameter is extractable from the angular dependence of the frequency shift. In contrast, the antiferroquadrupolar order parameter is usually invisible in the frequency shift. Instead, the long-range antiferroquadrupolar order yields a characteristic resonance peak in the ESR spectrum, which we call a magnon-pair resonance peak. This resonance corresponds to the excitation of the bound magnon pair at the wave vector $\bm k={\bm 0}$. Reflecting the condensation of bound magnon pairs, the field dependence of the magnon-pair resonance frequency shows a singular upturn at the saturation field. Moreover, the intensity of the magnon-pair resonance peak shows a characteristic angular dependence and it vanishes when the magnetic field is parallel to one of the axes that diagonalize the weak anisotropic interactions. We confirm these general properties of the magnon-pair resonance peak in the spin nematic phase by studying an $S=1$ bilinear-biquadratic model on the square lattice in the linear flavor-wave approximation. In addition, we argue applications to the $S=1/2$ frustrated ferromagnets and also the $S=1/2$ orthogonal dimer spin system SrCu$_2$(BO$_3$)$_2$, both of which are candidate materials of spin nematics. Our theory for the antiferroquadrupolar ordered phase is consistent with many features of the magnon-pair resonance peak experimentally observed in the low-magnetization regime of SrCu$_2$(BO$_3$)$_2$.

cond-mat.str-el↗

arXiv2017

Exact diagonalization and cluster mean-field study of triangular-lattice XXZ antiferromagnets near saturation

Quantum magnetic phases near the magnetic saturation of triangular-lattice antiferromagnets with XXZ anisotropy have been attracting renewed interest since it has been suggested that a nontrivial coplanar phase, called the $π$-coplanar or $Ψ$ phase, could be stabilized by quantum effects in a certain range of anisotropy parameter $J/J_z$ besides the well-known 0-coplanar (known also as $V$) and umbrella phases. Recently, Sellmann $et$ $al$. [Phys. Rev. B {\bf 91}, 081104(R) (2015)] claimed that the $π$-coplanar phase is absent for $S=1/2$ from an exact-diagonalization analysis in the sector of the Hilbert space with only three down-spins (three magnons). We first reconsider and improve this analysis by taking into account several low-lying eigenvalues and the associated eigenstates as a function of $J/J_z$ and by sensibly increasing the system sizes (up to 1296 spins). A careful identification analysis shows that the lowest eigenstate is a chirally antisymmetric combination of finite-size umbrella states for $J/J_z\gtrsim 2.218$ while it corresponds to a coplanar phase for $J/J_z\lesssim 2.218$. However, we demonstrate that the distinction between 0-coplanar and $π$-coplanar phases in the latter region is fundamentally impossible from the symmetry-preserving finite-size calculations with fixed magnon number.} Therefore, we also perform a cluster mean-field plus scaling analysis for small spins $S\leq 3/2$. The obtained results, together with the previous large-$S$ analysis, indicate that the $π$-coplanar phase exists for any $S$ except for the classical limit ($S\rightarrow \infty$) and the existence range in $J/J_z$ is largest in the most quantum case of $S=1/2$.

cond-mat.str-el↗

arXiv2016

Geometrically Frustrated Coarsening Dynamics in Spinor Bose-Fermi Mixtures

Coarsening dynamics theory has successfully described the equilibration of a broad class of systems.By studying the relaxation of a periodic array of microcondensates immersed in a Fermi gas which can mediate long-range spin interactions to simulate frustrated classical magnets, we show that coarsening dynamics can be suppressed by geometrical frustration. The system is found to eventually approach a metastable state which is robust against random field noise and characterized by finite correlation lengths with the emergence of topologically stable Z2 vortices. We find universal scaling laws with no thermal-equilibrium analog that relate the correlation lengths and the number of vortices to the degree of frustration in the system.

cond-mat.quant-gas↗

arXiv2016

Novel phases in a square-lattice frustrated ferromagnet : 1/3-magnetisation plateau, helicoidal spin-liquid and vortex crystal

A large part of the interest in magnets with frustrated antiferromagnetic interactions comes from the many new phases found in applied magnetic field. In this Article, we explore some of the new phases which arise in a model with frustrated ferromagnetic interactions, the $J_1-J_2-J_3$ Heisenberg model on a square lattice. Using a combination of classical Monte-Carlo simulation and spin-wave theory, we uncover behaviour reminiscent of some widely-studied frustrated antiferromagnets, but with a number of new twists. We first demonstrate that, for a suitable choice of parameters, the phase diagram as a function of magnetic field and temperature is nearly identical to that of the Heisenberg antiferromagnet on a triangular lattice, including the celebrated 1/3-magnetisation plateau. We then examine how this phase diagram changes when the model is tuned to a point where the classical ground--state is highly degenerate. In this case, two new phases emerge; a classical, finite-temperature spin-liquid, characterised by a "ring" in the spin structure--factor $\mathcal{S}({\mathbf q})$; and a vortex crystal, a multiple-Q state with finite magnetisation, which can be viewed as an ordered lattice of magnetic vortices. All of these new phases persist for a wide range of magnetic field. We discuss the relationship between these results and published studies of frustrated antiferromagnets, together with some of the materials where these new phases might be observed in experiment.

cond-mat.str-el↗

arXiv2015

Nematic ordering in pyrochlore antiferromagnets: high-field phase of chromium spinel oxides

Motivated by recent observation of a new high field phase near saturation in chromium spinels $A$Cr$_2$O$_4$ ($A=$ Zn, Cd, Hg), we study the $S = 3/2$ pyrochlore Heisenberg antiferromagnet with biquadratic interactions. Magnon instability analysis at the saturation field reveals that a very small biquadratic interaction can induce magnon pairing in pyrochlore antiferromagnets, which leads to the emergence of a ferro-quadrupolar phase, or equivalently a spin nematic phase, below the saturation field. We present the magnetic phase diagram in an applied field, studying both $S=3/2$ and $S=1$ spin systems. The relevance of our result to chromium spinels is discussed.

cond-mat.str-el↗

arXiv2014

Z_3 symmetry-protected topological phases in the SU(3) AKLT model

We study $\mathbb{Z}_3$ symmetry-protected topological (SPT) phases in one-dimensional spin systems with $Z_3 \times Z_3$ symmetry. We construct ground-state wave functions of the matrix product form for nontrivial $\mathbb{Z}_3$ phases and their parent Hamiltonian from a cocycle of the group cohomology $H^2(Z_3\times Z_3,U(1))$. The Hamiltonian is an SU(3) version of the Affleck-Kennedy-Lieb-Tasaki (AKLT) model, consisting of bilinear and biquadratic terms of su(3) generators in the adjoint representation. A generalization to the SU($N$) case, the SU($N$) AKLT Hamiltonian, is also presented which realizes nontrivial $\mathbb{Z}_N$ SPT phases. We use the infinite-size variant of the density matrix renormalization group (iDMRG) method to determine the ground-state phase diagram of the SU(3) bilinear-biquadratic model as a function of the parameter $θ$ controlling the ratio of the bilinear and biquadratic coupling constants. The nontrivial $\mathbb{Z}_3$ SPT phase is found for a range of the parameter $θ$ including the point of vanishing biquadratic term ($θ=0$) as well as the SU(3) AKLT point [$θ=\arctan(2/9)$]. A continuous phase transition to the SU(3) dimer phase takes place at $θ\approx -0.027π$, with a central charge $c\approx3.2$. For SU(3) symmetric cases we define string order parameters for the $\mathbb{Z}_3$ SPT phases in a similar way to the conventional Haldane phase. We propose simple spin models that effectively realize the SU(3) and SU(4) AKLT models.

cond-mat.str-el↗

arXiv2014

Magnon condensation with finite degeneracy on the triangular lattice

We study the spin 1/2 triangular-lattice $J_1$-$J_2$-$J_3$ antiferromagnet close to the saturation field using the dilute Bose gas theory, where the magnetic structure is determined by the condensation of magnons. We focus on the case of ferromagnetic $J_1$ and antiferromagnetic $J_2,J_3$, that is particularly rich because frustration effects allow the single-magnon energy dispersion to have six-fold degenerate minima at incommensurate momenta. Our calculation also includes an interlayer coupling $J_0$, which covers both antiferromagnetic and ferromagnetic cases including negligibly small regime (two-dimensional case). Besides the spiral and fan phases, we find a new double-$q$ phase (superposition of two modes), dubbed "${\bf Q}_0$-${\bf Q}_1$" (or simply "01") phase, that enjoys a new type of multiferroic character. Certain phase boundaries have a singular $J_0$ dependence for $J_0\to 0$, implying that even a very small interlayer coupling drastically changes the ground state. A mechanism for this singularity is presented. Moreover, in some regions of the parameter space, we show that a dilute gas of magnons can not be stable, and phase separation (corresponding to a magnetization jump) is expected. In the $J_1$-$J_2$ model ($J_3=0$), formation of two-magnon bound states is observed, which can lead to a quadrupolar (spin-nematic) ordered phase. Exact diagonalization analysis is also applied to the search of bound states.

cond-mat.str-el↗