arXiv subjects

Tsuyoshi Tamegai

Publications and source records attributed to Tsuyoshi Tamegai.

At least 55 records · Page 3Linked to original sources

arXiv2018

Multiple topological states in iron-based superconductors

Topological insulators and semimetals as well as unconventional iron-based superconductors have attracted major recent attention in condensed matter physics. Previously, however, little overlap has been identified between these two vibrant fields, even though the principal combination of topological bands and superconductivity promises exotic unprecedented avenues of superconducting states and Majorana bound states (MBSs), the central building block for topological quantum computation. Along with progressing laser-based spin-resolved and angle-resolved photoemission spectroscopy (ARPES) towards high energy and momentum resolution, we have resolved topological insulator (TI) and topological Dirac semimetal (TDS) bands near the Fermi level ($E_{\text{F}}$) in the iron-based superconductors Li(Fe,Co)As and Fe(Te,Se), respectively. The TI and TDS bands can be individually tuned to locate close to $E_{\text{F}}$ by carrier doping, allowing to potentially access a plethora of different superconducting topological states in the same material. Our results reveal the generic coexistence of superconductivity and multiple topological states in iron-based superconductors, rendering these materials a promising platform for high-$T_{\text{c}}$ topological superconductivity.

cond-mat.supr-con↗

arXiv2018

Disorder-sensitive node-like small gap in FeSe

We investigate the band structure, nematic state and superconducting gap structure of two selected FeSe single crystals containing different amount of disorder. Transport and angle-resolved photoemission spectroscopy measurements show that the small amount of disorder has little effect to the band structure and the nematic state of FeSe. However, temperature and magnetic field dependencies of specific heat for the two samples are quite different. Wave-vector-dependent gap structure are obtained from the three dimensional field-angle-resolved specific heat measurements. A small gap with two vertical-line nodes or gap minima along the $k_z$ direction is found only in the sample with higher quality. Such symmetry-unprotected nodes or gap minima are found to be smeared out by small amount of disorder, and the gap becomes isotropic in the sample of lower quality. Our study reveals that the reported controversy on the gap structure of FeSe is due to the disorder-sensitive node-like small gap.

cond-mat.supr-con↗

arXiv2018

Topological Dirac semimetal phase in the iron-based superconductor Fe(Te,Se)

Topological Dirac semimetals (TDSs) exhibit bulk Dirac cones protected by time reversal and crystal symmetry, as well as surface states originating from non-trivial topology. While there is a manifold possible onset of superconducting order in such systems, few observations of intrinsic superconductivity have so far been reported for TDSs. We observe evidence for a TDS phase in FeTe$_{1-x}$Se$_x$ ($x$ = 0.45), one of the high transition temperature ($T_c$) iron-based superconductors. In angle-resolved photoelectron spectroscopy (ARPES) and transport experiments, we find spin-polarized states overlapping with the bulk states on the (001) surface, and linear magnetoresistance (MR) starting from 6 T. Combined, this strongly suggests the existence of a TDS phase, which is confirmed by theoretical calculations. In total, the topological electronic states in Fe(Te,Se) provide a promising high $T_c$ platform to realize multiple topological superconducting phases.

cond-mat.supr-con↗

arXiv2018

Field-driven transition in the Ba$_{1-x}$K$_x$Fe$_2$As$_2$ superconductor with splayed columnar defects

Through 2.6 GeV U irradiations, we have induced bimodal splayed columnar defects in Ba$_{1-x}$K$_x$Fe$_2$As$_2$ single crystals with splay angles, $\pm 5 ^\circ$, $\pm 10 ^\circ$, $\pm 15 ^\circ$, and $\pm 20 ^\circ$. Critical current densities through magnetization measurements were carefully evaluated, where a splay angle of $\pm 5 ^\circ$ brought about the highest $J_\mathrm{c}$. Mageto-optical images close to $T_\mathrm{c}$ indicates highly anisotropic discontinuity lines in the remnant state, and with anisotropy increasing with greater splay angles. Moreover, amongst those with splayed columnar defects, anomalous non-monotonic field dependences of $J_\mathrm{c}$ and $S$ with an extrema at some fraction of the matching field are observed. We discuss that such $J_\mathrm{c}$ enhancement arises from a field-driven coupling transition in which intervortex interactions reorganize the vortex structure to be accommodated into columnar defects, thereby increasing pinning at higher fields.

cond-mat.supr-con↗

arXiv2017

Gap structure of FeSe determined by field-angle-resolved specific heat measurements

Quasiparticle excitations in FeSe were studied by means of specific heat ($C$) measurements on a high-quality single crystal under rotating magnetic fields. The field dependence of $C$ shows three-stage behavior with different slopes, indicating the existence of three gaps ($Δ_1$, $Δ_2$, and $Δ_3$). In the low-temperature and low-field region, the azimuthal-angle ($ϕ$) dependence of $C$ shows a four-fold symmetric oscillation with sign change. On the other hand, the polar-angle ($θ$) dependence manifests as an anisotropy-inverted two-fold symmetry with unusual shoulder behavior. Combining the angle-resolved results and the theoretical calculation, the smaller gap $Δ_1$ is proved to have two vertical-line nodes or gap minima along the $k_z$ direction, and is determined to reside on the electron-type $\varepsilon$ band. $Δ_2$ is found to be related to the electron-type $δ$ band, and is isotropic in the $ab$-plane but largely anisotropic out of the plane. $Δ_3$ residing on the hole-type $α$ band shows a small out-of-plane anisotropy with a strong Pauli-paramagnetic effect.

cond-mat.supr-con↗

arXiv2017

Symmetry-unprotected nodes or gap minima in $s_{++}$ state of FeSe single crystal

We report the study on superconducting pairing mechanism of FeSe via the pair-breaking effects induced by H$^+$-irradiation combined with low-temperature specific heat measurements. A multi-gap structure with nodes or gap minima is suggested in a clean FeSe by the specific heat results. The suppression of critical temperature $T_c$ with increasing the defect density manifests a two-step behavior. When the increase in the residual resistivity is small, $Δρ_0$ $<$ $\sim$4.5 $μΩ$cm, $T_c$ is gradually suppressed with increasing the density of scattering centers, suggesting the presence of symmetry-unprotected nodes or gap minima. However, for $Δρ_0$ $>$ $\sim$4.5 $μΩ$cm, $T_c$ is almost independent of the scattering, which indicates that the nodes or gap minima are lifted and the order parameter becomes almost isotropic without sign change. Thus, the superconductivity in FeSe is found to be realized in symmetry-unprotected nodal or highly anisotropic $s_{++}$ state.

cond-mat.supr-con↗

arXiv2017

Exfoliation and van der Waals heterostructure assembly of intercalated ferromagnet Cr1/3TaS2

Ferromagnetic van der Waals (vdW) materials are in demand for spintronic devices with all-two-dimensional-materials heterostructures. Here, we demonstrate mechanical exfoliation of magnetic-atom-intercalated transition metal dichalcogenide Cr1/3TaS2 from its bulk crystal; previously such intercalated materials were thought difficult to exfoliate. Magnetotransport in exfoliated tens-of-nanometres-thick flakes revealed ferromagnetic ordering below its Curie temperature TC ~ 110 K as well as strong in-plane magnetic anisotropy; these are identical to its bulk properties. Further, van der Waals heterostructure assembly of Cr1/3TaS2 with another intercalated ferromagnet Fe1/4TaS2 is demonstrated using a dry-transfer method. The fabricated heterojunction composed of Cr1/3TaS2 and Fe1/4TaS2 with a native Ta2O5 oxide tunnel barrier in between exhibits tunnel magnetoresistance (TMR), revealing possible spin injection and detection with these exfoliatable ferromagnetic materials through the vdW junction.

cond-mat.mes-hall↗

arXiv2017

Effects of heavy-ion irradiation on FeSe

We report the effects of heavy-ion irradiation on FeSe single crystals by irradiating Uranium up to a dose equivalent matching field of $B_ϕ$ = 16 T. Almost continuous columnar defects along the $c$-axis with a diameter $\sim$10 nm are confirmed by high-resolution transmission electron microscopy. $T_c$ is found to be suppressed by introducing columnar defects at a rate of d$T_c$/d$B_ϕ$ $\sim$ -0.29KT$^{-1}$, which is much larger than those observed in iron pnictides. This unexpected large suppression of $T_c$ in FeSe is discussed in relation to the large diameter of the columnar defects as well as its unique band structure with a remarkably small Fermi energy. The critical current density is first dramatically enhanced with irradiation reaching a value over $\sim$2$\times$10$^5$ A/cm$^2$ ($\sim$5 times larger than that of the pristine sample) at 2 K (self-field) with $B_ϕ$ = 2 T, then gradually suppressed with increasing $B_ϕ$. The $δ$$l$-pinning associated with charge-carrier mean free path fluctuations, and the $δ$$T_c$-pinning associated with spatial fluctuations of the transition temperature are found to coexist in the pristine FeSe, while the irradiation increases the contribution from $δ$$l$-pinning, and makes it dominant over $B_ϕ$ = 4 T.

cond-mat.supr-con↗

arXiv2016

Structural-transition-induced quasi two-dimensional Fermi surface in FeSe

We report detailed study of angular-dependent magnetoresistance (AMR) with tilting angel $θ$ from $c$-axis ranging from 0$^\circ$ to 360$^\circ$ on a high-quality FeSe single crystal. A pronounced AMR with twofold symmetry is observed, which is caused by the quasi two-dimensional (2D) Fermi surface. The pronounced AMR is observed only in the orthorhombic phase, indicating that the quasi-2D Fermi surface is induced by the structural transition. Details about the influence of the multiband effect to the AMR are also discussed. Besides, the angular response of a possible Dirac-cone-like band structure is investigated by analyzing the detailed magnetoresistance at different $θ$. The obtained characteristic field ($B^*$) can be also roughly scaled in the 2D approximation, which indicates that the Dirac-cone-like state is also 2D in nature.

cond-mat.supr-con↗

arXiv2016

Enhancement of critical current densities in (Ba,K)Fe2As2 wires and tapes using HIP technique

(Ba,K)Fe2As2 superconducting wires and tapes are fabricated by using hot isostatic pressing (HIP) technique, and their superconducting properties are studied. In the HIP round wire, transport critical current density (Jc) at 4.2 K has achieved record-high value of 175 kA/cm2 at zero field, and exceeds 20 kA/cm2 even at 100 kOe. Improvement of polycrystalline powder synthesis may play a key role for the enhancement of Jc. In the HIP tape, even larger transport Jc of 380 kA/cm2 is realized at zero field. Based on magnetization and magneto-optical measurements, possible further enhancement of Jc is discussed.

cond-mat.supr-con↗

arXiv2016

Effects of Iodine Annealing on Fe1+yTe0.6Se0.4

Effects of iodine annealing to induce bulk superconductivity in Fe1+yTe0.6Se0.4 have been systematically studied by changing the molar ratio of iodine to the sample and annealing temperature. The optimal condition to induce bulk superconductivity with Tc ~14.5 K and self-field Jc(2 K) ~ 5x10^5 A/cm2 is found to be a molar ratio of iodine of 5-7 % at the annealing temperature of 400 C. Furthermore, the fact that no compounds containing iodine are detected in the crystal and a significant amount of FeTe2 is produced after the iodine annealing strongly indicate that the excess iron is consumed to form FeTe2 and iodine works as a catalyst in this process.

cond-mat.supr-con↗

arXiv2016

Influence of interstitial Fe to the phase diagram of Fe$_{1+y}$Te$_{1-x}$Se$_x$ single crystals

Superconductivity (SC) with the suppression of long-range antiferromagnetic (AFM) order is observed in the parent compounds of both iron-based and cuprate superconductors. The AFM wave vectors are bicollinear ($π$, 0) in the parent compound FeTe different from the collinear AFM order ($π$, $π$) in most iron pnictides. Study of the phase diagram of Fe$_{1+y}$Te$_{1-x}$Se$_x$ is the most direct way to investigate the competition between bicollinear AFM and SC. However, presence of interstitial Fe affects both magnetism and SC of Fe$_{1+y}$Te$_{1-x}$Se$_x$, which hinders the establishment of the real phase diagram. Here, we report the comparison of doping-temperature ($x$-$T$) phase diagrams for Fe$_{1+y}$Te$_{1-x}$Se$_x$ (0 $\leq$ $x$ $\leq$ 0.43) single crystals before and after removing interstitial Fe. Without interstitial Fe, the AFM state survives only for $x$ $<$ 0.05, and bulk SC emerges from $x$ = 0.05, and does not coexist with the AFM state. The previously reported spin glass state, and the coexistence of AFM and SC may be originated from the effect of the interstitial Fe. The phase diagram of Fe$_{1+y}$Te$_{1-x}$Se$_x$ is found to be similar to the case of the "1111" system such as LaFeAsO$_{1-x}$F$_x$, and is different from that of the "122" system.

cond-mat.supr-con↗

arXiv2016

Electron carriers with possible Dirac-cone-like dispersion in FeSe$_{1-x}$S$_x$ ($x$ = 0 and 0.14) single crystals triggered by structural transition

We report detailed study of the transport properties of FeSe$_{1-x}$S$_x$ ($x$ = 0 and 0.14) single crystals grown by vapor transport method. 14\% S doping is found significantly suppress the structural transition from $T_s$ $\sim$ 86 K in FeSe to $\sim$ 49 K, although the superconducting transition temperature, $T_c$, is only slightly affected. A pronounced linear magnetoresistance (MR) is observed in both FeSe and FeSe$_{0.86}$S$_{0.14}$ single crystals, which is found to be triggered by the structural transition. The linear MR and related discussion indicate the possible existence of Dirac-cone-like state, which may come from the band shift induced by ferro-orbital order. The mobility of the Dirac-cone-like band is found to decrease after S doping. Besides, the invalid Kohler's scaling of MR is found for temperature below $T_s$ in both crystals, however the re-establishment of the Kohler's scaling at temperatures below 30 K is observed in FeSe, but not in FeSe$_{0.86}$S$_{0.14}$. All these observations above support that the orbital ordering causes the band reconstruction in FeSe, and also that the orbital ordering in FeSe is suppressed by the chemical pressure from S doping.

cond-mat.supr-con↗

arXiv2016

Effects of Pnictogen Atmosphere Annealing in Fe$_{1+y}$Te$_{0.6}$Se$_{0.4}$

It has been clarified that bulk superconductivity in Fe$_{1+y}$Te$_{0.6}$Se$_{0.4}$ can be induced by annealing in an appropriate atmosphere to remove the harmful effects of excess iron. In order to clarify the details of the annealing process, we studied the changes in the physical properties and reaction products of Fe$_{1+y}$Te$_{0.6}$Se$_{0.4}$ annealed in pnictogen (P, As, Sb) atmospheres. Crystals annealed in a pnictogen atmosphere show bulk superconductivity and the values of $T_{c}$ and $J_{c}$ are about $14~$K and 2-4 $\times 10{^5}~$A/cm$^2$ ($2~$K, self-field), respectively. It is also found that the reaction rate increases with the increase in the saturated vapor pressure of the pnictogen. Unexpectedly, the reaction products of Fe$_{1+y}$Te$_{0.6}$Se$_{0.4}$ after annealing in a P atmosphere mainly consist of FeTe$_2$. In addition, the amount of P required to obtain the optimal $T_{c}$ is much smaller than the amount of excess iron, which is similar to the case of oxygen annealing. P, oxygen, and to some extent As could serve as catalysts to form FeTe$_2$ to remove excess iron.

cond-mat.supr-con↗

arXiv2015

Enhancement of critical current density and mechanism of vortex pinning in H$^+$-irradiated FeSe single crystal

In this report, we comprehensively study the effect of H$^+$ irradiation on the critical current density, $J_c$, and vortex pinning in FeSe single crystal. It is found that the value of $J_c$ for FeSe is enhanced more than twice after 3-MeV H$^+$ irradiation. The scaling analyses of the vortex pinning force based on the Dew-Hughes model reveal that the H$^+$ irradiation successfully introduce point pinning centers into the crystal. We also find that the vortex creep rates are strongly suppressed after irradiation. Detailed analyses of the critical current dependent pinning energy based on the collective creep theory and extend Maley's method show that the H$^+$ irradiation enhances the value of $J_c$ before the flux creep, and also reduces the size of flux bundle, which will further reduce the field dependence of $J_c$ due to vortex motion.

cond-mat.supr-con↗

arXiv2015

Critical current density, vortex dynamics, and phase diagram of FeSe single crystal

We present a comprehensive study of the vortex pinning and dynamics in a high-quality FeSe single crystal, which is free from doping introduced inhomogeneities and charged quasi-particle-scattering because of its innate superconductivity. Critical current density, $J_c$, is found to be almost isotropic, and reaches a value $\sim$ 3 $\times$ 10$^4$ A/cm$^2$ at 2 K (self-field) for both $H$ $\|$ $c$ and $ab$. The normalized magnetic relaxation rate $S$ (= $\mid$dln$M$/dln$t$$\mid$) shows a temperature insensitive plateau behavior in the intermediate temperature range with a relatively high creep rate ($S$ $\sim$ 0.02 under zero field), which is interpreted in the framework of the collective creep theory. A crossover from the elastic to plastic creep is observed, while the fish-tail effect is absent for both $H$ $\|$ $c$ and $ab$. Based on this observation, the origin of the fish-tail effect is also discussed. Combining the results of $J_c$ and $S$, vortex motion in FeSe single crystal is found to be dominated by sparse strong point-like pinning from nm-sized defects or imperfections. The weak collective pinning is also observed and proved in the form of large bundles. Besides, the vortex phase diagram of FeSe is also constructed and discussed.

cond-mat.supr-con↗

arXiv2015

Evolution of superconducting and transport properties in annealed FeTe$_{1-x}$Se$_x$ (0.1 $\leq$ $x$ $\leq$ 0.4) multiband superconductors

We investigated the superconducting and transport properties in FeTe$_{1-x}$Se$_{x}$ (0.1 $\leq$ $x$ $\leq$ 0.4) single crystals prepared by O$_2$-annealing. Sharp superconducting transition width observed in magnetization measurement and the small residual resistivity prove the high quality of the crystals. All the crystals manifest large, homogeneous, and isotropic critical current density \emph{J}$_c$ with self-field value over 10$^5$ A/cm$^2$ at 2 K. The large and field-robust critical current densities prove that the superconductivity in FeTe$_{1-x}$Se$_{x}$ (0.1 $\leq$ $x$ $\leq$ 0.4) is in bulk nature. The values of anisotropy parameter close to $T_c$ for crystals with different Se doping levels all reside in the range of 2 - 3. Hall coefficients $R_H$ keeps positive and almost constant value at high temperatures, followed by a sudden decreases before reaching $T$$_c$, which indicates that the electron-type charge carriers become dominant at low temperatures. Furthermore, the characteristic temperature for the sudden decrease in $R_H$ gradually increases with Se doping.

cond-mat.supr-con↗

arXiv2014

Magneto-optical characterizations of FeTe$_{0.5}$Se$_{0.5}$ thin films with critical current density over 1 MA/cm$^2$

We performed magneto-optical (MO) measurements on FeTe$_{0.5}$Se$_{0.5}$ thin films grown on LaAlO$_3$ (LAO) and Yttria-stabilized zirconia (YSZ) single-crystalline substrates. These thin films show superconducting transition temperature, ${T_c}$ $\sim$ 19 K, 4 K higher than the bulk sample. Typical roof-top patterns can be observed in the MO images of thin films grown on LAO and YSZ, from which a large and homogeneous critical current density, ${J_c}$, over 1 $\times$ 10$^6$ A/cm$^2$ at 5 K was obtained. Magnetic flux penetration measurement reveals that the current is almost isotropically distributed in the two thin films. Compared with bulk crystals, FeTe$_{0.5}$Se$_{0.5}$ thin film demonstrates not only higher ${T_c}$, but also much larger ${J_c}$, which is attractive for applications.

cond-mat.supr-con↗