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Ueli Töpfer

Publications and source records attributed to Ueli Töpfer.

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Universal transport of active colloids with sensory delay in motility landscapes

We experimentally, numerically and analytically explore the diffusive transport of active colloidal particles with sensory delay, navigating motility landscapes in which the self-propulsion speed depends on space. We show how the transport properties can be obtained by replacing the space dependence of the self-propulsion speed by a dynamical stochastic switching process in the absence of delay, and extend the theory for systems with finite delayed responses. We obtain analytical results for the mean square displacement and the effective diffusion coefficient which accurately predict experimental measurements and numerical simulations across multiple scales. We show how, within the regime of validity of the delay-extended theory, density patterns and effective diffusion obey universal scaling forms. Our work provides minimal framework describing the transport properties of active swimmers with internal adaptation dynamics in motility landscapes.

cond-mat.stat-mech

Density modulations in active colloidal systems through orthogonal propulsion control and sensory delays

Recent advancements in active colloidal systems aim to mimic key characteristics of biological microswimmers, particularly their adaptive motility in response to environmental changes. While many approaches rely on externally imposing a propulsive force, achieving true autonomous and self-regulating adaptation to the environment remains limited. In this study, we develop and analyze Janus microswimmers driven by electrohydrodynamic flows that autonomously adjust their propulsion dynamics in response to varying illumination conditions. Our Janus particles are silica colloids partially coated with titania, which self-propel via induced-charge electrophoresis (ICEP) under uniform AC electric fields. Since titania is photoconductive, it increases its conductivity under UV illumination, which thereby regulates the propulsion velocity independently of and orthogonally to the applied electric field. Crucially, the velocity adaptation requires a finite time. This sensory delay, which we systematically characterize, leads to enhanced microswimmer localization in response to spatiotemporal light modulations compared to the typical case of instantaneous response considered for synthetic microswimmers. By harnessing these dynamics, akin to those of biological microswimmers, we exert precise control over both local and global particle behavior, presenting novel opportunities for adaptive active matter systems.

cond-mat.soft