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Ulrich Schollwöck

Publications and source records attributed to Ulrich Schollwöck.

At least 37 records · Page 2Linked to original sources
arXiv2024

Quantifying hole-motion-induced frustration in doped antiferromagnets by Hamiltonian reconstruction

Unveiling the microscopic origins of quantum phases dominated by the interplay of spin and motional degrees of freedom constitutes one of the central challenges in strongly correlated many-body physics. When holes move through an antiferromagnetic spin background, they displace the positions of spins, which induces effective frustration in the magnetic environment. However, a concrete characterization of this effect in a quantum many-body system is still an unsolved problem. Here we present a Hamiltonian reconstruction scheme that allows for a precise quantification of hole-motion-induced frustration. We access non-local correlation functions through projective measurements of the many-body state, from which effective spin-Hamiltonians can be recovered after detaching the magnetic background from dominant charge fluctuations. The scheme is applied to systems of mixed dimensionality, where holes are restricted to move in one dimension, but SU(2) superexchange is two-dimensional. We demonstrate that hole motion drives the spin background into a highly frustrated regime, which can quantitatively be described by an effective $J_1-J_2-$type spin model. We exemplify the applicability of the reconstruction scheme to ultracold atom experiments by recovering effective spin-Hamiltonians of experimentally obtained 1D Fermi-Hubbard snapshots. Our method can be generalized to fully 2D systems, enabling promising microscopic perspectives on the doped Hubbard model.

cond-mat.quant-gas↗
arXiv2024

Photo-induced dynamics with continuous and discrete quantum baths

The ultrafast quantum dynamics of photophysical processes in complex molecules is an extremely challenging computational problem with a wide variety of fascinating applications in quantum chemistry and biology. Inspired by recent developments in open quantum systems, we introduce a pure-state unraveled hybrid-bath method that describes a continuous environment via a set of discrete, effective bosonic degrees of freedom using a Markovian embedding. Our method is capable of describing both, a continuous spectral density and sharp peaks embedded into it. Thereby, we overcome the limitations of previous methods, which either capture long-time memory effects using the unitary dynamics of a set of discrete vibrational modes or use memoryless Markovian environments employing a Lindblad or Redfield master equation. We benchmark our method against two paradigmatic problems from quantum chemistry and biology. We demonstrate that compared to unitary descriptions, a significantly smaller number of bosonic modes suffices to describe the excitonic dynamics accurately, yielding a computational speed-up of nearly an order of magnitude. Furthermore, we take into account explicitly the effect of a $δ$-peak in the spectral density of a light-harvesting complex, demonstrating the strong impact of the long-time memory of the environment on the dynamics.

quant-ph↗
arXiv2024

Probing a Modified Luttinger Sum Rule in the Strongly Interacting 1D Fermi-Hubbard Model

Fermi surface reconstruction in cuprates can lead to an abrupt change in the Fermi momentum $k_F$ between different phases. This phenomenon remains subject of debate and is at the heart of an ongoing discussion about the nature of the metallic state in the pseudogap regime. Here we study a minimal model of a $k_F$ changing crossover in the one-dimensional Fermi-Hubbard model, where a tuning of the onsite interaction leads to a crossover between a spin-$1/2$ Luttinger liquid with small Fermi momentum and a spinless chargon liquid with large Fermi momentum. We attribute this to an emergent $U(1)$ symmetry in the strongly correlated limit, which can be used to derive a modified Luttinger sum rule recovering the large Fermi momentum. We analyse Friedel oscillations at the edge of a system to directly probe the change of Fermi momentum at zero and non-zero temperature. This paves the way for a direct experimental observation of changes of the Fermi momentum using ultracold fermions in a quantum gas microscope, with possible extensions to higher dimensional systems.

cond-mat.str-el↗
arXiv2024

Antiferromagnetic bosonic $t$-$J$ models and their quantum simulation in tweezer arrays

The combination of optical tweezer arrays with strong interactions -- via dipole-exchange of molecules and van-der-Waals interactions of Rydberg atoms -- has opened the door for the exploration of a wide variety of quantum spin models. A next significant step will be the combination of such settings with mobile dopants: This will enable to simulate the physics believed to underlie many strongly correlated quantum materials. Here we propose an experimental scheme to realize bosonic t-J models via encoding the local Hilbert space in a set of three internal atomic or molecular states. By engineering antiferromagnetic (AFM) couplings between spins, competition between charge motion and magnetic order similar to that in high-$T_c$ cuprates can be realized. Since the ground states of the 2D bosonic AFM t-J model we propose to realize have not been studied extensively before, we start by analyzing the case of two dopants -- the simplest instance in which their bosonic statistics plays a role, and contrast our results to the fermionic case. We perform large-scale density matrix renormalization group (DMRG) calculations on six-legged cylinders, and find a strong tendency for bosonic holes to form stripes. This demonstrates that bosonic, AFM t-J models may contain similar physics as the collective phases in strongly correlated electrons.

cond-mat.quant-gas↗
arXiv2024

Confinement in 1+1D $\mathbb{Z}_2$ Lattice Gauge Theories at Finite Temperature

Confinement is a paradigmatic phenomenon of gauge theories, and its understanding lies at the forefront of high-energy physics. Here, we study confinement in a simple one-dimensional $\mathbb{Z}_2$ lattice gauge theory at finite temperature and filling, which is within the reach of current cold-atom and superconducting-qubit platforms. By employing matrix product states (MPS) calculations, we investigate the decay of the finite-temperature Green's function and uncover a smooth crossover between the confined and deconfined regimes. Furthermore, using the Friedel oscillations and string length distributions obtained from snapshots sampled from MPS, both of which are experimentally readily available, we verify that confined mesons remain well-defined at arbitrary finite temperature. This phenomenology is further supported by probing quench dynamics of mesons with exact diagonalization. Our results shed new light on confinement at finite temperature from an experimentally relevant standpoint.

cond-mat.quant-gas↗
arXiv2024

Pairing dome from an emergent Feshbach resonance in a strongly repulsive bilayer model

A key to understanding unconventional superconductivity lies in unraveling the pairing mechanism of mobile charge carriers in doped antiferromagnets, yielding an effective attraction between charges even in the presence of strong repulsive Coulomb interactions. Here, we study pairing in a mixed-dimensional (mixD) $t-J$ model, featuring robust binding energies -- despite dominant repulsive interactions -- that are strongly enhanced in the finite doping regime. The single and coupled mixD ladders we study, corresponding to bilayers of width $w\leq 2$, feature a crossover from tightly bound pairs of holes (closed channel) at small repulsion, to more spatially extended, correlated pairs of individual holes (open channel) at large repulsion. We derive an effective model for the latter, in which the attraction is mediated by the closed channel, in analogy to atomic Feshbach resonances. Using density matrix renormalization group (DMRG) simulations we reveal a dome of large binding energies at around $30\%$ doping, accompanied by a change of the Fermi surface volume and a crossover from extended to tightly bound hole pairs. Our work provides a microscopic theory of pairing in the doped mixD system with dominant repulsion, closely related to bilayer, Ni-based superconductors, and our predictions can be tested in state-of-the-art quantum simulators.

cond-mat.str-el↗
arXiv2024

Growing Extended Laughlin States in a Quantum Gas Microscope: A Patchwork Construction

The study of fractional Chern insulators and their exotic anyonic excitations poses a major challenge in current experimental and theoretical research. Quantum simulators, in particular ultracold atoms in optical lattices, provide a promising platform to realize, manipulate, and understand such systems with a high degree of controllability. Recently, an atomic $ν=1/2$ Laughlin state has been realized experimentally for a small system of two particles on 4 by 4 sites. The next challenge concerns the preparation of Laughlin states in extended systems, ultimately giving access to anyonic braiding statistics or gapless chiral edge-states in systems with open boundaries. Here, we propose and analyze an experimentally feasible scheme to grow larger Laughlin states by connecting multiple copies of the already existing 4-by-4-system. First, we present a minimal setting obtained by coupling two of such patches, producing an extended 8-by-4-system with four particles. Then, we analyze different preparation schemes, setting the focus on two shapes for the extended system, and discuss their respective advantages: While growing strip-like lattices could give experimental access to the central charge, square-like geometries are advantageous for creating quasi-hole excitations in view of braiding protocols. We highlight the robust quantization of the fractional quasi-hole charge upon using our preparation protocol. We benchmark the performance of our patchwork preparation scheme by comparing it to a protocol based on coupling one-dimensional chains. We find that the patchwork approach consistently gives higher target-state fidelities, especially for elongated systems. The results presented here pave the way towards near-term implementations of extended Laughlin states in quantum gas microscopes and the subsequent exploration of exotic properties of topologically ordered systems in experiments.

cond-mat.quant-gas↗
arXiv2023

Feshbach resonance in a strongly repulsive bilayer model: a possible scenario for bilayer nickelate superconductors

Since the discovery of superconductivity in cuprate materials, the minimal ingredients for high-T$_c$ superconductivity have been an outstanding puzzle. Motivated by the recently discovered nickelate bilayer superconductor La$_3$Ni$_2$O$_3$ under pressure, we study a minimal bilayer model, in which, as in La$_3$Ni$_2$O$_3$, inter- and intralayer magnetic interactions but no interlayer hopping are present: a mixed-dimensional (mixD) $t-J$ model. In the setting of a mixD ladder, we show that the system exhibits a crossover associated with a Feshbach resonance: from a closed-channel dominated regime of tightly bound bosonic pairs of holes to an open-channel dominated regime of spatially more extended Cooper pairs. The crossover can be tuned by varying doping, or by a nearest-neighbor Coulomb repulsion $V$ that we include in our model. Using density matrix renormalization group (DMRG) simulations and analytical descriptions of both regimes, we find that the ground state is a Luther-Emery liquid, competing with a density wave of tetraparton plaquettes at commensurate filling $δ=0.5$ at large repulsion, and exhibits a pairing dome where binding is facilitated by doping. Our observations can be understood in terms of pairs of correlated spinon-chargon excitations constituting the open channel, which are subject to attractive interactions mediated by the closed channel of tightly bound chargon-chargon pairs. When the closed channel is lowered in energy by doping or tuning $V$, a Feshbach resonance is realized, associated with a dome in the binding energy. Our predictions can be directly tested in state-of-the art quantum simulators, and we argue that the pairing mechanism we describe may be realized in the nickelate bilayer superconductor La$_3$Ni$_2$O$_3$.

cond-mat.str-el↗
arXiv2023

Adaptive Quantum State Tomography with Active Learning

Recently, tremendous progress has been made in the field of quantum science and technologies: different platforms for quantum simulation as well as quantum computing, ranging from superconducting qubits to neutral atoms, are starting to reach unprecedentedly large systems. In order to benchmark these systems and gain physical insights, the need for efficient tools to characterize quantum states arises. The exponential growth of the Hilbert space with system size renders a full reconstruction of the quantum state prohibitively demanding in terms of the number of necessary measurements. Here we propose and implement an efficient scheme for quantum state tomography using active learning. Based on a few initial measurements, the active learning protocol proposes the next measurement basis, designed to yield the maximum information gain. We apply the active learning quantum state tomography scheme to reconstruct different multi-qubit states with varying degree of entanglement as well as to ground states of the XXZ model in 1D and a kinetically constrained spin chain. In all cases, we obtain a significantly improved reconstruction as compared to a reconstruction based on the exact same number of measurements and measurement configurations, but with randomly chosen basis configurations. Our scheme is highly relevant to gain physical insights in quantum many-body systems as well as for benchmarking and characterizing quantum devices, e.g. for quantum simulation, and paves the way for scalable adaptive protocols to probe, prepare, and manipulate quantum systems.

quant-ph↗
arXiv2023

Detecting Hidden Order in Fractional Chern Insulators

Topological phase transitions go beyond Ginzburg and Landau's paradigm of spontaneous symmetry breaking and occur without an associated local order parameter. Instead, such transitions can be characterized by the emergence of non-local order parameters, which require measurements on extensively many particles simultaneously - an impossible venture in real materials. On the other hand, quantum simulators have demonstrated such measurements, making them prime candidates for an experimental confirmation of non-local topological order. Here, building upon the recent advances in preparing few-particle fractional Chern insulators using ultracold atoms and photons, we propose a realistic scheme for detecting the hidden off-diagonal long-range order (HODLRO) characterizing Laughlin states. Furthermore, we demonstrate the existence of this hidden order in fractional Chern insulators, specifically for the $ν=\frac{1}{2}$-Laughlin state in the isotropic Hofstadter-Bose-Hubbard model. This is achieved by large-scale numerical density matrix renormalization group (DMRG) simulations based on matrix product states, for which we formulate an efficient sampling procedure providing direct access to HODLRO in close analogy to the proposed experimental scheme. We confirm the characteristic power-law scaling of HODLRO, with an exponent $\frac{1}ν = 2$, and show that its detection requires only a few thousand snapshots. This makes our scheme realistically achievable with current technology and paves the way for further analysis of non-local topological orders, e.g. in topological states with non-Abelian anyonic excitations.

cond-mat.quant-gas↗
arXiv2023

Cooper-Paired Bipolaronic Superconductors

Light-mass bipolarons in off-diagonally coupled electron-phonon systems provide a potential route to bipolaronic high-Tc superconductivity. While there has been numerical progress in the physically relevant limit of slow phonons, more insights are needed to fully understand to what extent this mechanism survives at finite densities and in different regimes. We address these questions using advanced tensor-network methods applied to the Su-Schrieffer-Heeger model. Studying both the spectral properties of isolated bipolarons as well as the pairing correlations at small finite densities, we find evidence that the conventional picture of bipolarons as molecular bound states which undergo Bose-Einstein condensation may need to be reconsidered. Instead, our findings suggest correlation-driven formation of a fragmented condensate with spatially separated polaron pairs, stabilized by strong repulsive electron-electron interactions at moderate values of the electron-phonon coupling. These spatially modulated charge clouds exhibit pairing with a typical length-scale set by the Fermi momentum.

cond-mat.supr-con↗
arXiv2023

Stable bipolarons in open quantum systems

Recent advances in numerical methods significantly pushed forward the understanding of electrons coupled to quantized lattice vibrations. At this stage, it becomes increasingly important to also account for the effects of physically inevitable environments. In particular, we study the transport properties of the Hubbard-Holstein Hamiltonian that models a large class of materials characterized by strong electron-phonon coupling, in contact with a dissipative environment. Even in the one-dimensional and isolated case, simulating the quantum dynamics of such a system with high accuracy is very challenging due to the infinite dimensionality of the phononic Hilbert spaces. For this reason, the effects of dissipation on the conductance properties of such systems have not been investigated systematically so far. We combine the non-Markovian hierarchy of pure states method and the Markovian quantum jumps method with the newly introduced projected purified density-matrix renormalization group, creating powerful tensor-network methods for dissipative quantum many-body systems. Investigating their numerical properties, we find a significant speedup up to a factor $\sim 30$ compared to conventional tensor-network techniques. We apply these methods to study dissipative quenches, aiming for an in-depth understanding of the formation, stability, and quasi-particle properties of bipolarons. Surprisingly, our results show that in the metallic phase dissipation localizes the bipolarons, which is reminiscent of an indirect quantum Zeno effect. However, the bipolaronic binding energy remains mainly unaffected, even in the presence of strong dissipation, exhibiting remarkable bipolaron stability. These findings shed light on the problem of designing real materials exhibiting phonon-mediated high-$T_\mathrm{C}$ superconductivity.

cond-mat.str-el↗
arXiv2023

Coexistence of superconductivity with partially filled stripes in the Hubbard model

Combining the complementary capabilities of two of the most powerful modern computational methods, we find superconductivity in both the electron- and hole-doped regimes of the two-dimensional Hubbard model (with next nearest neighbor hopping). In the electron-doped regime, superconductivity is weaker and is accompanied by antiferromagnetic Néel correlations at low doping. The strong superconductivity on the hole-doped side coexists with stripe order, which persists into the overdoped region with weaker hole density modulation. These stripe orders, neither filled as in the pure Hubbard model (no next nearest neighbor hopping) nor half-filled as seen in previous state-of-the-art calculations, vary in fillings between 0.6 and 0.8. The resolution of the tiny energy scales separating competing orders requires exceedingly high accuracy combined with averaging and extrapolating with a wide range of system sizes and boundary conditions. These results validate the applicability of this iconic model for describing cuprate high-$T_c$ superconductivity.

cond-mat.supr-con↗
arXiv2023

Ferromagnetism and Skyrmions in the Hofstadter-Fermi-Hubbard Model

Strongly interacting fermionic systems host a variety of interesting quantum many-body states with exotic excitations. For instance, the interplay of strong interactions and the Pauli exclusion principle can lead to Stoner ferromagnetism, but the fate of this state remains unclear when kinetic terms are added. While in many lattice models the fermions' dispersion results in delocalization and destabilization of the ferromagnet, flat bands can restore strong interaction effects and ferromagnetic correlations. To reveal this interplay, here we propose to study the Hofstadter-Fermi-Hubbard model using ultracold atoms. We demonstrate, by performing large-scale DMRG simulations, that this model exhibits a lattice analog of the quantum Hall ferromagnet at magnetic filling factor $ν=1$. We reveal the nature of the low energy spin-singlet states around $ν\approx1$ and find that they host quasi-particles and quasi-holes exhibiting spin-spin correlations reminiscent of skyrmions. Finally, we predict the breakdown of flat-band ferromagnetism at large fields. Our work paves the way towards experimental studies of lattice quantum Hall ferromagnetism, including prospects to study many-body states of interacting skyrmions and explore the relation to high-$T_{\rm c}$ superconductivity.

cond-mat.quant-gas↗
arXiv2023

Formation of CuO$_2$ sublattices by suppression of interlattice correlations in tetragonal CuO

We investigate the tetragonal phase of the binary transition metal oxide CuO (t-CuO) within the context of cellular dynamical mean-field theory. Due to its strong antiferromagnetic correlations and simple structure, analysing the physics of t-CuO is of high interest as it may pave the way towards a more complete understanding of high temperature superconductivity in hole-doped antiferromagnets. In this work we give a formal justification for the weak coupling assumption that has previously been made for the interconnected sublattices within a single layer of t-CuO by studying the non-local self-energies of the system. We compute momentum-resolved spectral functions using a Matrix Product State (MPS)-based impurity solver directly on the real axis, which does not require any numerically ill-conditioned analytic continuation. The agreement with photoemission spectroscopy indicates that a single band Hubbard model is sufficient to capture the material's low energy physics. We perform calculations on a range of different temperatures, finding two magnetic regimes, for which we identify the driving mechanism behind their respective insulating state. Finally, we show that in the hole-doped regime the sublattice structure of t-CuO has interesting consequences on the symmetry of the superconducting state.

cond-mat.str-el↗
arXiv2023

Confinement Induced Frustration in a One-Dimensional $\mathbb{Z}_2$ Lattice Gauge Theory

Coupling dynamical charges to gauge fields can result in highly non-local interactions with a linear confining potential. As a consequence, individual particles bind into mesons which, in one dimension, become the new constituents of emergent Luttinger liquids. Furthermore, at commensurate fillings, different Mott-insulating states can be stabilized by including nearest-neighbour (NN) interactions among charges. However, rich phase diagrams expected in such models have not been fully explored and still lack comprehensive theoretical explanation. Here, by combining numerical and analytical tools, we study a simple one-dimensional $\mathbb{Z}_2$ lattice gauge theory at half-filling, where U$(1)$ matter is coupled to gauge fields and interacts through NN repulsion. We uncover a rich phase diagram where the local NN interaction stabilizes a Mott state of individual charges (or partons) on the one hand, and a Luttinger liquid of confined mesons on the other. Furthermore, at the interface between these two phases, we uncover a highly frustrated regime arising due to the competition between the local NN repulsion and the non-local confining interactions, realizing a pre-formed parton plasma. Our work is motivated by the recent progress in ultracold atom experiments, where such simple model could be readily implemented. For this reason we calculate the static structure factor which we propose as a simple probe to explore the phase diagram in an experimental setup.

cond-mat.quant-gas↗
arXiv2022

Snapshot-based detection of $\frac{1}{2}$-Laughlin states: coupled chains and central charge

Experimental realizations of topologically ordered states of matter, such as fractional quantum Hall states, with cold atoms are now within reach. In particular, optical lattices provide a promising platform for the realization and characterization of such states, where novel detection schemes enable an unprecedented microscopic understanding. Here we show that the central charge can be directly measured in current cold atom experiments using the number entropy as a proxy for the entanglement entropy. We perform density-matrix renormalization-group simulations of Hubbard-interacting bosons on coupled chains subject to a magnetic field with $α=\frac{1}{4}$ flux quanta per plaquette. Tuning the inter-chain hopping, we find a transition from a trivial quasi-one dimensional phase to the topologically ordered Laughlin state at magnetic filling factor $ν=\frac{1}{2}$ for systems of three or more chains. We resolve the transition using the central charge, on-site correlations, momentum distributions and the many-body Chern number. Additionally, we propose a scheme to experimentally estimate the central charge from Fock basis snapshots. The model studied here is experimentally realizable with existing cold atom techniques and the proposed observables pave the way for the detection and classification of a larger class of interacting topological states of matter.

cond-mat.quant-gas↗
arXiv2021

Stochastic Adaptive Single-Site Time-Dependent Variational Principle

In recent years, the time-dependent variational principle (TDVP) method based on the matrix product state (MPS) wave function formulation has shown its great power in performing large-scale quantum dynamics simulations for realistic chemical systems with strong electron-vibration interactions. In this work, we propose a new stochastic adaptive single-site TDVP (SA-1TDVP) scheme to evolve the bond-dimension adaptively, which can integrate the tra-ditional advantages of both the high efficiency of single-site TDVP (1TDVP) variant and the high accuracy of the two-site TDVP (2TDVP) variant. Based on the assumption that the level statistics of entanglement Hamiltonians, which originate from the reduced density matrices of the MPS method, follows a Poisson or Wigner distribution, as generically predicted by random matrix theory, addi-tional random singular values are generated to expand the bond-dimension automatically. Tests on simulating the vibrationally-resolved quantum dynamics and absorption spectra in the pyrazine molecule and perylene bisimide (PBI) J-aggregate trimer as well as a spin-1/2 Heisenberg chain show that it can be automatic and as accurate as 2TDVP but reduce the computational time remarkably.

cond-mat.str-el↗