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Umakanta Patra

Publications and source records attributed to Umakanta Patra.

4 recordsLinked to original sources

Si-Ga2O3/p-GaN epitaxial heterostructure based self-powered and visible-blind UV photodetectors with fast and electrically tuneable response time

n-Ga2O3/p-GaN heterojunction based photodetector devices are fabricated on Si-doped (-201) \beta-Ga2O3 epitaxial layers grown by pulsed laser deposition (PLD) technique on p-type c-GaN/sapphire templates. These devices demonstrate the ability to act as highly efficient self-powered visible blind UV-photodetectors with fast response time. It has been found that the optimum performance of the detector in terms of its responsivity, detectivity and response time could be achieved by adjusting the Si doping level and the thickness of the Ga2O3 layer. Our best performing device showing the peak responsivity and detectivity of 56.8 mA/W and 3*10^12 Jones, respectively, is achieved for 660 nm thick Ga2O3 layer with Si-concentration of 8*10^18 cm^-3. Moreover, as low as a few nW of optical signal can be sensed by the detector. The response time of the detector is found to be only a few tens of nanoseconds, which highlights their potential for application in ultrafast detection of UV light. These devices also exhibit a slower component of photoresponse with a timescale of a few tens of milliseconds. Interestingly, the time-scale of the slower response can be prolongated by several orders of magnitude through enhancing the applied reverse bias. Such an electrical tuneability of the response time is highly desirable for neuromorphic device applications.

cond-mat.mtrl-sci

CVD grown bilayer MoS2 based artificial optoelectronic synapses for arithmetic computing and image recognition applications

Demand for lower computing power has rapidly increased. In this context, brain-inspired neuromorphic computing, which integrate data storage and processing, has attracted significant attention. Here, our study reveals that field effect transistors fabricated on chemical vapor deposited bilayer (2L) MoS2 films can mimic the functions of biological synapse. These devices demonstrate high level of pair pulse facilitation (PPF), short term to long term memory (STM-to-LTM) transition as well as learning-forgetting-relearning properties. Effect of light intensity, pulse number, pulse width and photon energy on the STM-to-LTM transition is studied. It has been found that the rate of depression of the memory state can be controlled using the gate bias. Electrical and optical energy consumptions per synaptic event are estimated to be as low as 280 fJ and 20 nJ, respectively. Furthermore, photocurrent in these devices is observed to increase linearly with the number of the excitation pulses. This property has been exploited to demonstrate different arithmetic operations by the device. Moreover, these devices show great potential for image recognition. Artificial neural network simulation has returned an image recognition accuracy of ~85%. All these findings show a great prospect of 2L-MoS2 for developing low power, transparent and flexible neuromorphic devices.

cond-mat.mtrl-sci

Spontaneous growth of perfectly circular domains of MoS2 monolayers using chemical vapour deposition technique

Very large-scale integration of devices in a circular pattern has several advantages over the commonly used rectangular grid layout. For the development of such integrated circuits on a 2D semiconductor platform, spontaneous growth of the material in the form of circular islands is desirable. Here, we report the natural formation of 1L-MoS2 circular islands of diameter as large as a few hundreds of micrometer on SiO2/Si substrates by chemical vapor deposition (CVD) technique without the use of any seeding layer. The size of the circles is found to increase with the amount of sulphur used during growth. The study reveals that these circular islands are formed with a less-defective interior and a more-defective outer part that is dominated by a large density of grain boundaries and twists. Due to the lower defect density, the interior region yields much higher photoluminescence than the peripheral part. Field effect transistors (FETs) are fabricated on inner and outer portions of a circle to estimate the mobility and concentration of the background carriers in the two regions. The study shows that the maximum mobility is more than double in the interior than the outer part. While the carrier concentration remains practically unchanged in the two regions. The natural tendency to minimize the strain energy resulting from the mismatch between the thermal expansion coefficients of the monolayer and the substrate as well as the edge energy that originates from the boundary tension are thought to be the driving forces behind the formation of these circular domains.

cond-mat.mtrl-sci

Controlled Growth of large area bilayer MoS$_2$ films on SiO$_2$ substrates by chemical vapour deposition technique

Bilayer (2L) transition metal dichalcogenides (TMD) have the ability to host interlayer excitons, where electron and hole parts are spatially separated that leads to much longer lifetime as compared to direct excitons. This property can be utilized for the development of exciton-based logic devices, which are supposed to be superior in terms of energy efficiency and optical communication compatibility as compared to their electronic counterparts. However, obtaining uniformly thick bilayer epitaxial films with large area coverage is challenging. Here, we have engineered the flow pattern of the precursors over the substrate surface to obtain large area (mm2) covered strictly bilayer MoS$_2$ films on SiO$_2$ by chemical vapour deposition (CVD) technique without any plasma treatment of the substrate prior to the growth. Bilayer nature of these films is confirmed by Raman, low-frequency Raman, atomic force microscopy (AFM) and photoluminescence (PL) studies. The uniformity of the film has been checked by Raman peak separation and PL intensity map. High resolution transmission electron microscopy (HRTEM) reveals that crystalline and twisted bilayer islands coexist within the layer. Back gated field-effect transistor (FET) structures fabricated on the bilayers show on/off ratio of 10^6 and subthreshold swings (SS) of 2.5 V/Decade.

cond-mat.mtrl-sci