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Uroš Delić

Publications and source records attributed to Uroš Delić.

At least 19 recordsLinked to original sources

Engineering recoil heating in coherent-scattering levitated optomechanics

Recoil heating from photon scattering is a fundamental source of decoherence in optical trapping, severely limiting the preparation of nonclassical motional states. In cavity setups in the coherent scattering configuration, a predictive theory of recoil heating rate is missing, as usual perturbative approaches fail in the presence of sharp optical resonances. Hence, current works assume that the recoil heating rate is approximately equal to its free-space value. Here we show that this is not the case, as the electromagnetic environment can strongly modify recoil heating rate by the Purcell effect. Specifically, we predict that this rate can be significantly suppressed in state-of-the-art microcavities, for both center-of-mass and librational motion. To establish these results, we develop a general theoretical framework based on macroscopic quantum electrodynamics and on the few-mode quantization approach developed in nanophotonics. Our method applies to particles trapped in the presence of arbitrary electromagnetic structures, thus providing a route to engineering motional decoherence in levitated optomechanics by photonic structure design.

quant-ph↗

Floquet engineering of nonreciprocal light-induced dipolar interactions

Tweezer arrays of polarizable objects are a promising platform for assembling quantum matter and building next-generation quantum sensors. Light-induced dipolar interactions have emerged as a method to couple their motion, thereby establishing a new paradigm for controlling collective mechanical degrees of freedom. Here, we extend these into the regime of Floquet-driven interactions, combined with the intrinsic nonreciprocity of optical forces. We demonstrate beamsplitter, single-, and two-mode squeezing operations, as well as signatures of a negative-mass-like oscillator arising from the nonreciprocity. Moreover, we show that a programmable combination of these operations enables continuous tuning of complex eigenfrequencies. These results establish a toolbox of quantum operations of nonreciprocal interactions that are essential for investigating non-Hermitian many-body physics and collective quantum optomechanics.

quant-ph↗

Steady-state entanglement of interacting masses in free space through optimal feedback control

We develop a feedback strategy based on optimal quantum feedback control for Gaussian systems to maximise the likelihood of steady-state entanglement detection between two directly interacting masses. We employ linear quadratic Gaussian (LQG) control to engineer the phase space dynamics of the two masses and propose Einstein-Podolsky-Rosen (EPR)-type variance minimisation constraints for the feedback to facilitate unconditional entanglement generation. This scheme allows for stationary entanglement in parameter regimes where strategies based on total energy minimisation cooling would fail.

quant-ph↗

Controlling Rydberg atom-polariton interactions: from exceptional points to fast readout

Rydberg atoms represent a platform underpinning many recent developments in quantum computation, simulation, sensing, and metrology. They further facilitate optical nonlinearity at the single-photon level when coupled to photons propagating in atomic clouds, which form collective atomic excitations called Rydberg polaritons, strongly interacting with each other. Here, we experimentally explore interactions between a Rydberg polariton in an atomic ensemble and a single, adjacent, Rydberg atom. We discover three different regimes of quantum dynamics corresponding to polariton blockade, coherent exchange, and probabilistic hopping, which are defined by their distinct transmission characteristics, with a transition through an exceptional point occurring between blockade and coherent exchange. We investigate the applications of such interactions for fast, non-destructive detection of Rydberg atoms and present proof-of-principle demonstrations for their potential application in nonlinear photonic networks.

physics.atom-ph↗

Quantum ground-state cooling of two librational modes of a nanorotor

Controlling the motion of nanoscale objects at the quantum limit promises new tests of quantum mechanics and advanced sensors. Rotational motion is of particular interest, as it follows nonlinear dynamics in a compact, closed configuration space, which opens up a plethora of phenomena and applications beyond the possibilities of free or trapped linear motion. A prerequisite for such experiments is the capability to trap nanorotors and initialize them in a quantum ground state of libration. Here, we demonstrate the reliable, repetitive laser-induced loading of silica nanodimers and trimers into an optical tweezer. Coherent scattering in a high-finesse cavity allows us to cool two different librational modes to the quantum ground state with occupation numbers as low as $n_β=0.54\pm0.32$ and $n_α=0.21\pm0.03$. By simultaneously cooling both degrees of freedom ($n_β=0.73\pm0.22$, $n_α=1.02\pm0.08$) we align nanorotors to a space-fixed axis with precision better than 20$\,μ$rad, close to the zero-point amplitude of librations.

quant-ph↗

Programmable few-atom Bragg scattering and ground-state cooling in a cavity

By integrating tweezer arrays with a high-cooperativity ring cavity with chiral atom-cavity coupling, we demonstrate highly directional Bragg scattering from a programmable number of atoms. Through accurate control of the interatomic distance, we observe a narrowing-down of the Bragg peak as we increase the atom number one by one. The observed high-contrast Bragg interference is enabled by cavity sideband cooling of both the radial and axial motions to near the ground state with phonon occupation numbers below 0.17 and 3.4, respectively. This new platform that integrates strong and controlled atom-light coupling into atomic arrays enables applications from programmable quantum optics to quantum metrology and computation.

quant-ph↗

Nonequilibrium entanglement between levitated masses under optimal control

We present a protocol that maximizes unconditional entanglement generation between two masses interacting directly through $1/r^{n}$ potential. The protocol combines optimal quantum control of continuously measured masses with their non-equilibrium dynamics, driven by a time-dependent interaction strength. Applied to a pair of optically trapped sub-micron particles coupled via electrostatic interaction, our protocol enables unconditional entanglement generation at the fundamental limit of the conditional state and with an order of magnitude smaller interaction between the masses compared to the existing steady-state approaches.

quant-ph↗

Quantum theory of non-Hermitian optical binding between nanoparticles

Recent experiments demonstrate highly tunable nonreciprocal coupling between levitated nanoparticles due to optical binding [Rieser et al., Science 377, 987 (2022)]. In view of recent experiments cooling nanoparticles to the quantum regime, we here develop the quantum theory of small dielectric objects interacting via the forces and torques induced by scattered tweezer photons. The interaction is fundamentally non-Hermitian and accompanied by correlated quantum noise. We present the corresponding Markovian quantum master equation and show how to reach nonreciprocal and unidirectional coupling. Our work provides the theoretical tools for exploring and exploiting the rich quantum physics of nonreciprocally coupled nanoparticle arrays.

quant-ph↗

Quantum Optical Binding of Nanoscale Particles

Optical binding refers to the light-induced interaction between two or more objects illuminated by laser fields. The high tunability of the strength, sign, and reciprocity of this interaction renders it highly attractive for controlling nanoscale mechanical motion. Here, we discuss the quantum theory of optical binding and identify unique signatures of this interaction in the quantum regime. We show that these signatures are observable in near-future experiments with levitated nanoparticles. In addition, we prove the impossibility of entanglement induced by far-field optical binding in free space and identify strategies to circumvent this no-go theorem.

quant-ph↗

Exponentially Enhanced non-Hermitian Cooling

Certain non-Hermitian systems exhibit the skin effect, whereby the wavefunctions become exponentially localized at one edge of the system. Such exponential amplification of wavefunction has received significant attention due to its potential applications in e.g., classical and quantum sensing. However, the opposite edge of the system, featured by the exponentially suppressed wavefunctions, remains largely unexplored. Leveraging this phenomenon, we introduce a non-Hermitian cooling mechanism, which is fundamentally distinct from traditional refrigeration or laser cooling techniques. Notably, non-Hermiticity will not amplify thermal excitations, but rather redistribute them. Hence, thermal excitations can be cooled down at one edge of the system, and the cooling effect can be exponentially enhanced by the number of auxiliary modes, albeit with a lower bound that depends on the dissipative interaction with the environment. Non-Hermitian cooling does not rely on intricate properties such as exceptional points or non-trivial topology, and it can apply to a wide range of Bosonic modes such as photons, phonons, magnons, etc.

quant-ph↗

Fluctuation-induced Forces on Nanospheres in External Fields

We analyze the radiative forces between two dielectric nanospheres mediated via the quantum and thermal fluctuations of the electromagnetic field in the presence of an external drive. We generalize the scattering theory description of fluctuation forces to include external quantum fields, allowing them to be in an arbitrary quantum state. The known trapping and optical binding potentials are recovered for an external coherent state. We demonstrate that an external squeezed vacuum state creates similar potentials to a laser, despite its zero average intensity. Moreover, Schrödinger cat states of the field can enhance or suppress the optical potential depending on whether they are odd or even. Considering the nanospheres trapped by optical tweezers, we examine the total interparticle potential as a function of various experimentally relevant parameters, such as the field intensity, polarization, and phase of the trapping lasers. We demonstrate that an appropriate set of parameters could produce mutual bound states of the two nanospheres with potential depth as large as $\sim200$ K. Our results are pertinent to ongoing experiments with trapped nanospheres in the macroscopic quantum regime, paving the way for engineering interactions among macroscopic quantum systems.

quant-ph↗

Non-Hermitian dynamics and nonreciprocity of optically coupled nanoparticles

Non-Hermitian dynamics, as observed in photonic, atomic, electrical, and optomechanical platforms, holds great potential for sensing applications and signal processing. Recently, fully tunable nonreciprocal optical interaction has been demonstrated between levitated nanoparticles. Here, we use this tunability to investigate the collective non-Hermitian dynamics of two nonreciprocally and nonlinearly interacting nanoparticles. We observe parity-time symmetry breaking and, for sufficiently strong coupling, a collective mechanical lasing transition, where the particles move along stable limit cycles. This work opens up a research avenue of nonequilibrium multi-particle collective effects, tailored by the dynamic control of individual sites in a tweezer array.

physics.optics↗

Force-Gradient Sensing and Entanglement via Feedback Cooling of Interacting Nanoparticles

We show theoretically that feedback-cooling of two levitated, interacting nanoparticles enables differential sensing of forces and the observation of stationary entanglement. The feedback drives the two particles into a stationary, non-thermal state which is susceptible to inhomogeneous force fields and which exhibits entanglement for sufficiently strong inter-particle couplings. We predict that force-gradient sensing at the zepto-Newton per micron range is feasible and that entanglement due to the Coulomb interaction between charged particles can be realistically observed in state-of-the-art setups.

quant-ph↗

Linear Ultrastrong Optomechanical Interaction

Light-matter interaction in the ultrastrong coupling regime can be used to generate exotic ground states with two-mode squeezing and may be of use for quantum enhanced sensing. Current demonstrations of ultrastrong coupling have been performed in fundamentally nonlinear systems. We report a cavity optomechanical system that operates in the linear coupling regime, reaching a maximum coupling of $g_x/Ω_x=0.55\pm 0.02$. Such a system is inherently unstable, which may in the future enable strong mechanical squeezing.

quant-ph↗

Dry launching of silica nanoparticles in vacuum

Clean loading of silica nanoparticles with a radius as small as ~50 nm is required for experiments in levitated optomechanics that operate in ultra-high vacuum. We present a cheap and simple experimental method for dry launching of silica nanoparticles by shaking from a polytetrafluoroethylene (PTFE) surface. We report on the successful launching of single silica nanoparticles with a minimum radius of 43 nm, which is enabled by the low stiction to the launching surface. Nanoparticles with radii of 43 nm and 71.5 nm are launched with a high flux and small angular spread of $\sim \pm 10^\circ$, which allows for trapping in a tightly focused optical tweezer within a couple of minutes. The measured velocities are significantly smaller than 1 m/s. The demonstrated launching method allows for controlled loading of dry nanoparticles with radii as small as 43 nm into optical traps in (ultra-)high vacuum, although we anticipate that loading of smaller sizes is equally feasible.

physics.app-ph↗

Dissipative phase transitions in optomechanical systems

We show that optomechanical quantum systems can undergo dissipative phase transitions within the limit of small nonlinear interaction and strong external drive. In such a defined thermodynamical limit, the nonlinear interaction stabilizes optomechanical dynamics in strong and ultrastrong coupling regimes. As a consequence optomechanical systems possess a rich phase diagram consisting of periodic orbits, discontinuous, and continuous dissipative phase transitions with and without bifurcation. We also find a critical point where continuous and discontinuous dissipative phase transition lines meet. Our analysis demonstrates that optomechanical systems are valuable for understanding the rich physics of dissipative phase transitions and ultrastrong coupling regimes.

quant-ph↗

Observation of strong and tunable light-induced dipole-dipole interactions between optically levitated nanoparticles

Arrays of optically trapped nanoparticles have emerged as a promising platform for the study of complex non-equilibrium phenomena. Analogous to atomic many-body systems, one of the crucial ingredients is the ability to precisely control the interactions between particles. However, the optical interactions studied thus far only provide conservative optical binding forces of limited tunability. Here we demonstrate a coupling mechanism that is orders of magnitude stronger and has new qualitative features. These effects arise from the previously unexplored phase coherence between the optical fields that drive the light-induced dipole-dipole interaction. In addition, polarization control allows us to observe electrostatic coupling between charged particles in the array. Our results pave the way for a fully programmable many-body system of interacting nanoparticles with tunable dissipative and nonreciprocal interactions, which are instrumental for exploring entanglement and topological phases in arrays of levitated nanoparticles.

physics.optics↗

MAQRO -- BPS 2023 Research Campaign Whitepaper

The objective of the proposed MAQRO mission is to harness space for achieving long free-fall times, extreme vacuum, nano-gravity, and cryogenic temperatures to test the foundations of physics in macroscopic quantum experiments. This will result in the development of novel quantum sensors and a means to probe the foundations of quantum physics at the interface with gravity. Earlier studies showed that the proposal is feasible but that several critical challenges remain, and key technologies need to be developed. These new technologies will open up the potential for achieving additional science objectives. The proposed research campaign aims to advance the state of the art and to perform the first macroscopic quantum experiments in space. Experiments on the ground, in micro-gravity, and in space will drive the proposed research campaign during the current decade to enable the implementation of MAQRO within the subsequent decade.

quant-ph↗