arXiv subjects

Utpal Chatterjee

Publications and source records attributed to Utpal Chatterjee.

6 recordsLinked to original sources

arXiv2025

Tunable Electronic Interactions and Weak Antilocalization in Bulk Ge$_2$Sb$_2$Te$_{5-5x}$Se$_{5x}$ Phase Change Materials

Phase change materials (PCMs) are well-known for their reversible and rapid switching between crystalline and amorphous phases through thermal excitations mediated by strong electrical or laser pulses. This crystal-to-amorphous transition is accompanied by a remarkable contrast in optical and electronic properties, making PCMs useful in nonvolatile data storage applications. Here, we combine electrical transport and angle resolved photoemission spectroscopy (ARPES) measurements to study the electronic structure of bulk Ge$_2$Sb$_2$Te$_{5-5x}$Se$_{5x}$ (GSST) for $0\le x \le 0.8$, where $x$ represents the amount of Se substituting Te in Ge$_2$Sb$_2$Te$_5$ (GST)-- a prototypical PCM. The single-particle density of states (SDOS) derived from the integrated ARPES data displays metallic behavior for all $x$, as evidenced by the presence of a finite density of states in the vicinity of the chemical potential. Transport measurements also display clear signatures of metallic transport, consistent with the SDOS data. The temperature dependence of the resistance indicates the onset of moderate electron-electron Coulomb interaction effects at low temperatures for $x\geq 0.6$. At the same time, the magnetoresistance data shows signatures of weak antilocalization for $x\geq 0.6$. An analysis on the temperature dependence of the phase coherence length suggests that electron dephasing is primarily due to inelastic electron-electron scattering. We find that these effects are enhanced with increasing $x$, portraying GSST as a novel PCM where electronic interactions can be tuned via chemical doping.

cond-mat.mtrl-sci↗

arXiv2025

Particle-hole symmetry in the pseudogap phase of moderately underdoped cuprate high temperature superconductors evidenced from joint density of states analysis

In conventional superconductors, the energy scale associated with the superfluid stiffness is much larger compared to the pairing energy and hence, the superconducting transition temperature (Tc) is entirely dictated by the superconducting (SC) energy gap. The phase rigidity of the SC condensate in unconventional superconductors, on the other hand, can be low enough to enable destruction of superconductivity via phase incoherence and persistence of an energy gap even at the absence of macroscopic superconductivity above Tc. This is considered a possible mechanism of the pseudogap (PG) state of cuprate high temperature superconductors (HTSCs). We have investigated the electronic energy ({\omega}) and momentum-separation vector (q) dependence of the joint density of states (JDOS), derived from the autocorrelated Angle Resolved Photoemission Spectroscopy (ARPES) data, from moderately underdoped Bi2Sr2CaCu2O8+{\delta}HTSC samples at temperatures below and above Tc. We found that q-space structure of the constant {\omega} JDOS intensity maps and the dispersions of the JDOS peaks are essentially the same both below and above Tc. Furthermore, the dispersions of the JDOS peaks above Tc are particle-hole symmetric. These observations evince similarity between the nature of the energy gap below and above Tc, which supports preformed pairing scenario for the PG state at least in the moderately underdoped regime.

cond-mat.supr-con↗

arXiv2022

Coupled electronic and magnetic excitations in the cuprates and their role in the superconducting transition

The formation of Cooper pairs, a bound state of two electrons of opposite spin and momenta by exchange of a phonon [1], is a defining feature of conventional superconductivity. In the cuprate high temperature superconductors, even though it has been established that the superconducting state also consists of Cooper pairs, the pairing mechanism remains intensely debated. Here we investigate superconducting pairing in the Bi2Sr2CaCu2O8+\delta (Bi2212) cuprate by employing spectral functions obtained directly from angle-resolved photoemission (ARPES) experiments as input to the Bethe-Salpeter gap equation. Assuming that Cooper pairing is driven solely by spin fluctuations, we construct the single-loop spin-fluctuation-mediated pairing interaction, and use it to compute the eigenfunctions and eigenvalues of the Bethe-Salpeter equation in the particle-particle channel for multiple Bi2212 samples. The key point of our results is that, as the temperature is reduced, the leading eigenvalue increases upon approaching Tc, reaching a value of approximately 1 at the Tc corresponding to each doping value, indicating a superconducting transition with d-wave eigenfunctions. This suggests that spin fluctuations can approximately account for Tc and, consequently, mediate pairing in the cuprate high temperature superconductors.

cond-mat.supr-con↗

arXiv2022

Denoising and feature extraction in photoemission spectra with variational auto-encoder neural networks

In recent years, distinct machine learning (ML) models have been separately used for feature extraction and noise reduction from energy-momentum dispersion intensity maps obtained from raw angle-resolved photoemission spectroscopy (ARPES) data. In this work, we employ a shallow variational auto-encoder (VAE) neural network to demonstrate the prospect of using ML for both denoising of as well as feature extraction from ARPES dispersion maps.

physics.ins-det↗

arXiv2019

Metal-to-insulator transition in Pt-doped TiSe$_2$ driven by emergent network of narrow transport channels

Metal-to-insulator transitions (MIT) can be driven by a number of different mechanisms, each resulting in a different type of insulator -- Change in chemical potential can induce a transition from a metal to a band insulator; strong correlations can drive a metal into a Mott insulator with an energy gap; an Anderson transition, on the other hand, due to disorder leads to a localized insulator without a gap in the spectrum. Here we report the discovery of an alternative route for MIT driven by the creation of a network of narrow channels. Transport data on Pt substituted for Ti in TiSe$_2$ shows a dramatic increase of resistivity by five orders of magnitude for few % of Pt substitution, with a power-law dependence of the temperature-dependent resistivity $\rho(T)$. Our scanning tunneling microscopy data show that Pt induces an irregular network of nanometer-thick domain walls (DWs) of charge density wave (CDW) order, which pull charge carriers out of the bulk and into the DWs. While the CDW domains are gapped, the charges confined to the narrow DWs interact strongly, with pseudogap-like suppression in the local density of states, even when they were weakly interacting in the bulk, and scatter at the DW network interconnects thereby generating the highly resistive state. Angle-resolved photoemission spectroscopy spectra exhibit pseudogap behavior corroborating the spatial coexistence of gapped domains and narrow domain walls with excess charge carriers.

cond-mat.str-el↗

arXiv2005

Evidence of Class Transitions in GRS 1915+105 from IXAE Data

GRS 1915+105 shows at least twelve distinct classes of light curves. By analysing the data obtained from Indian X-ray Astronomy Experiment (IXAE) instrument aboard IRS-P3 satellite, we show that in at least two days, transitions between one class to another were observed. In these days the so-called $κ$ class went to $ρ$ class and $χ$ class went to $ρ$ class. In the frequency-time plane such transitions exhibited change in quasi-periodic oscillation (QPO) frequency. We could detect that low-frequency QPOs can occur in anticipation of a class transition several hundred minutes before the actual transition

astro-ph↗