arXiv subjects

Uzi Landman

Publications and source records attributed to Uzi Landman.

At least 19 recordsLinked to original sources

arXiv2025

Wave-function microscopy: Derivation and anatomy of exact algebraic spinful wave functions and full Wigner-molecular spectra of a few highly correlated rapidly rotating ultracold fermionic atoms

Exploring strongly correlated spinful states of few fermionic ultracold atoms in a rapidly rotating trap, an example of which was recently realized for two fermionic $^6$Li atoms in an optical tweezer, we derive analytical (algebraic) total-spin-eigenstate wavefunctions through the development and employment of a theoretical platform that integrates exact numerical diagonalization (full configuration interaction, FCI) with symbolic language processing. For such rapid rotations, where the atoms occupy the lowest Landau level (LLL), the obtained algebraic expressions can address the full LLL spectrum in all its complexity, demonstrating that their spatial, spectral, and spin characteristics manifest formation of collectively rotating and vibrating Wigner molecules. The explicitly exhibited analytic wavefunctions (for two and three spinful $^6$Li atoms) reproduce precisely the corresponding numerical FCI results, and they are shown to reach beyond the limited range of applicability of previous Jastrow-type treatments. These results, and their extension to bosonic systems, provide the impetus and analysis tools for future experimental and theoretical simulations of larger mesoscopic systems

cond-mat.quant-gas↗

arXiv2024

Crystal-field effects in the formation of Wigner-molecule supercrystals in moir\'e TMD superlattices

For moir\'e bilayer TMD superlattices, full-configuration-interaction (FCI) calculations are presented that take into account both the intra-moir\'e-quantum-dot (MQD) charge-carrier Coulombic interactions, as well as the crystal-field effect from the surrounding moir\'e pockets (inter-moir\'e-QD interactions). The effective computational embedding strategy introduced here allows for an FCI methodogy that enables the complete interpretation of the counterintuitive experimental observations reported recently in the context of moir\'e TMD superlattices at integer fillings $\nu=2$ and 4. Two novel states of matter are reported: (i) a genuinely quantum-mechanical supercrystal of $sliding$ Wigner molecules (WMs) for unstrained moir\'e TMD materials (when the crystal field is commensurate with the trilobal symmetry of the confining potential in each embedded MQD) and (ii) a supercrystal of $pinned$ Wigner molecules when the crystal field is incommensurate with the trilobal symmetry or straining of the whole material is involved. The case of $\nu=3$ is an exception, in that even the unstrained case is associated with a supercrystal of pinned WMs, which is due to the congruence of intrinsic (that of the WM) and external (that of the confining potential of the MQD) $C_3$ point-group symmetries. Furthermore, it is shown that the unrestricted Hartree-Fock approach fails to describe the supercrystal of sliding WMs in the unstrained case, providing a qualitative agreement only in the case of a supercrystal of pinned WMs

cond-mat.mes-hall↗

arXiv2024

Electronic Wigner-Molecule Polymeric Chains in Elongated Silicon Quantum Dots and Finite-Length Quantum Wires

The spectral properties of electrons confined in a wire-like quasi-one-dimensional (1D) elongated quantum dot (EQD) coupler between silicon qubits, are investigated with a newly developed valley-augmented unrestricted Hartree-Fock (va-UHF) method, generalized to include the valley degree of freedom treated as an isospin, allowing calculations for a large number of electrons. The lower energy symmetry-broken solutions of the self-consistent generalized Pople-Nesbet equations exhibit, for a confinement that has been modeled after an experimentally fabricated one in silicon, formation of Wigner-molecular polymeric (longitudinal) chains, initiating through charge accumulation at the edges of the finite-length quasi-1D wire. An increasing number of parallel zig-zag chains form as the number of electrons loaded into the confinement is increased, with the formation of newly added chains determined by the strength of the transverse harmonic confinement. The broken-symmetry va-UHF solutions, subsequently augmented by the quantum-mechanically required parity-restoration, go beyond the va-UHF single-determinant solution, predicting formation of entangled Wigner-molecular chains whose charge distributions obliterate the zig-zag organization of the broken-symmetry solutions. The symmetry-restored va-UHF methodology enables systematic investigations of multi-electron complex nano-scale confined structures that could be targeted for future imaging microscopy experiments in silicon and other materials (e.g., 1D domain walls in TMD materials), and quantum information utilization.

cond-mat.mes-hall↗

arXiv2024

Wigner-molecule supercrystal in transition-metal dichalcogenide moiré superlattices: Lessons from the bottom-up approach

The few-body problem for $N=4$ fermionic charge carriers in a double-well moiré quantum dot (MQD), representing the first step in a bottom-up strategy to investigate formation of molecular supercrystals in transition metal dichalcogenide (TMD) moiré superlattices with integral fillings, $ν> 1$, is solved exactly by employing large-scale exact-diagonalization via full configuration interaction (FCI) computations. A comparative analysis with the mean-field solutions of the often used spin-and-space unrestricted Hartree Fock (sS-UHF) demonstrates the limitations of the UHF method (by itself) to provide a proper description of the influence of the interdot Coulomb interaction. In particular, it is explicitly shown for $ν=2$ that the exact charge densities (CDs) within each MQD retain the ring-like shape characteristic (for a wide range of relevant parameters) of a fully isolated MQD, as was found for sliding Wigner molecules (WMs). This deeply quantum-mechanical behavior contrasts sharply with the UHF CDs that portray solely orientationally pinned and well localized dumbbell dimers. An improved CD, which agrees with the FCI-calculated one, derived from the restoration of the sS-UHF broken parity symmetries is further introduced, suggesting a beyond-mean-field methodological roadmap for correcting the sS-UHF results. It is conjectured that the conclusions for the $ν=2$ moiré TMD superlattice case extend to all cases with integral fillings that are associated with sliding WMs in isolated MQDs. The case of $ν=3$, associated with a pinned WM in isolated MQDs, is an exception.

cond-mat.str-el↗

arXiv2023

Quantum Wigner molecules in moiré materials

The few-body problem (with $N \leq 6$ fermionic charge carriers) in isolated moiré quantum dots (MQDs) in transition metal dichalcogenide (TMD) bilayer materials with integer fillings, $ν\geq 2$, is investigated by employing large-scale full configuration interaction (FCI, also termed exact-diagonalization) computations, and by performing a comparative analysis of the ensuing first-order (charge densities, CDs) and second-order (conditional probability distributions, CPDs) correlation functions. With parameters representative of bilayer experimental TMD setups, our investigations reveal the determining role of the strong inter-particle Coulombic repulsion in bringing about Wigner molecularization, which is associated with many-body physics beyond both that described by the Aufbau principle of natural atoms, as well as by the widely used Hubbard model for strongly-interacting condensed-matter systems. In particular, for weak and moderate trilobal crystal-field deformations of the MQDs, the imperative employment of the CPDs brings to light the geometrical polygonal-ring configurations underlying the Wigner molecules (WMs) that remain hidden at the level of a charge-density analysis, apart from the case of $N=3$ when a pinned WM emerges in the charge density due to the coincidence of the $C_3$ symmetries associated with both the intrinsic geometry of the $N=3$ WM and the TMD trilobal crystal-field of the confining pocket potential. The FCI numerically exact-diagonalization results provide critical benchmarks for assessing and guiding the development of future computational methodologies of interacting strongly-correlated fermions in isolated MQDs and their superlattices in TMD materials.

cond-mat.str-el↗

arXiv2022

Valleytronic full configuration-interaction approach: An application to the excitation spectra of Si double-dot qubits

The influence of strong electron-electron interactions and Wigner-molecule (WM) formation on the spectra of $2e$ singlet-triplet double-dot Si qubits is presented based on a full configuration interaction (FCI) approach that incorporates the valley degree of freedom (VDOF) in the context of the continuous (effective mass) description of semiconductor materials. Our FCI treats the VDOF as an isospin in addition to the regular spin. Our treatment is able to assign to each energy curve in the qubit's spectrum a complete set of good quantum numbers for both the spin and the valley isospin. This reveals an underlying SU(4) $\supset$ SU(2) $\times$ SU(2) group-chain organization in the Si double-dot spectra. With parameters in the range of actual experimental situations, we demonstrate in a double-dot qubit that, in the (2,0) charge configuration and compared to the expected large, and dot-size determined, single-particle (orbital) energy gap, the strong $e-e$ interactions drastically quench the spin-singlet$-$spin-triplet energy gap, $E_{\rm ST}$, within the same valley, making it competitive to the small energy gap, $E_V$, between the two valleys. We present results for both the $E_{\rm ST} < E_V$ and $E_{\rm ST} > E_V$ cases. We investigate the spectra as a function of detuning and demonstrate the strengthening of the avoided crossings due to a lowering of the interdot barrier and/or the influence of valley-orbit coupling. We further demonstrate, as a function of an applied magnetic field, the emergence of avoided crossings in the (1,1) charge configuration due to the spin-valley coupling. The valleytronic FCI formulated here, and implementeded for two electrons confined in a tunable double quantum dot, offers also a most effective tool for analyzing the spectra of Si qubits with more than two wells and/or more than two electrons.

cond-mat.mes-hall↗

arXiv2022

Wigner molecules and hybrid qubits

It is demonstrated that exact diagonalization of the microscopic many-body Hamiltonian via systematic full configuration-interaction (FCI) calculations is able to predict the spectra as a function of detuning of three-electron hybrid qubits based on GaAs asymmetric double quantum dots. It is further shown that, as a result of strong inter-electron correlations, these spectroscopic patterns, including avoided crossings between states associated with different electron occupancies of the left and right wells, are inextricably related to the formation of Wigner molecules. These physical entities cannot be captured by the previously employed independent-particle or Hubbard-type theoretical modeling of the hybrid qubit. We report remarkable agreement with recent experimental results. Moreover, the present FCI methodology for multi-well quantum dots can be straightforwardly extended to treat Si/SiGe hybrid qubits, where the central role of Wigner molecules was recently experimentally confirmed as well.

cond-mat.mes-hall↗

arXiv2022

Molecular formations and spectra due to electron correlations in three-electron hybrid double-well qubits

We show that systematic full configuration-interaction (FCI) calculations enable prediction of the energy spectra and the intrinsic spatial and spin structures of the many-body wave functions as a function of the detuning parameter for the case of three-electron hybrid qubits based on GaAs asymmetric double quantum dots. Specifically, in comparison with the case of weak interactions and treating the entire three-electron double-dot hybrid qubit as an integral unit, it is shown that the predicted spectroscopic patterns, originating from strong electron correlations, manifest the formation of Wigner molecules (WMs). Signatures of WM formation include: (1) a strong suppression of the energy gaps relative to the non-interacting-electrons modeling, and (2) the appearance of a pair of avoided crossings arising between states associated with two-electron occupancies in the left and right wells. The Wigner molecule is a physical entity associated with electron localization within each well and it cannot be captured by the previously employed independent-particle or two-site-Hubbard theoretical modeling of the hybrid qubits. The emergence of strong WMs is investigated in depth through the concerted use of FCI-adapted diagnostic tools like charge and spin densities, as well as conditional probability distributions. Furthermore, the energy spectrum as a function of the strength of the Coulomb repulsion (at constant detuning) is calculated in order to complement the thorough analysis of the factors contributing to WM emergence. We report remarkable agreement with recent experimental measurements. The present FCI methodology for multi-well quantum dots can be straightforwardly extended to treat valleytronic two-band Si/SiGe hybrid qubits, where the central role of the WMs was confirmed recently.

cond-mat.mes-hall↗

arXiv2021

Excitation spectra of two correlated electrons in a quantum dot

Measurements and a theoretical interpretation of the excitation spectrum of a two-electron quantum dot fabricated on a parabolic Ga[Al]As quantum well are reported. Experimentally, excited states are found beyond the well-known lowest singlet- and triplet states. These states can be reproduced in an exact diagonalization calculation of a parabolic dot with moderate in-plane anisotropy. The calculated spectra are in reasonable quantitative agreement with the measurement, and suggest that correlations between the electrons play a significant role in this system. Comparison of the exact results with the restricted Hartree-Fock and the generalized Heitler-London approach shows that the latter is more appropriate for this system because it can account for the spatial correlation of the electron states.

cond-mat.mes-hall↗

arXiv2021

Exact closed-form analytic wave functions in two dimensions: Contact-interacting fermionic spinful ultracold atoms in a rapidly rotating trap

Exact two-dimensional analytic wave functions for an arbitrary number $N$ of contact-interacting lowest-Landau-level (LLL) spinful fermions are derived with the use of combined numerical and symbolic computational approaches via analysis of exact Hamiltonian numerical diagonalization data. Closed-form analytic expressions are presented for two families of zero-interaction-energy states at given total angular momentum and total spin $0 \leq S \leq N/2$ in the neighborhood of the $ν=1$ filling, covering the range from the maximum density droplet to the first quasihole. Our theoretical predictions for higher-order spatial and momentum correlations reveal intrinsic polygonal, multi-ring crystalline-type structures, which can be tested with ultracold-atom experiments in rapidly rotating traps, simulating quantum Hall physics (including quantum LLL skyrmions).

cond-mat.quant-gas↗

arXiv2020

Highly Ordered Boron Nitride/Epigraphene Epitaxial Films on Silicon Carbide by Lateral Epitaxial Deposition

Realizing high-performance nanoelectronics requires control of materials at the nanoscale. Methods to produce high quality epitaxial graphene (EG) nanostructures on silicon carbide are known. The next step is to grow Van der Waals semiconductors on top of EG nanostructures. Hexagonal boron nitride (h-BN) is a wide bandgap semiconductor with a honeycomb lattice structure that matches that of graphene, making it ideally suited for graphene-based nanoelectronics. Here, we describe the preparation and characterization of multilayer h-BN grown epitaxially on EG using a migration-enhanced metalorganic vapor phase epitaxy process. As a result of the lateral epitaxial deposition (LED) mechanism, the grown h-BN/EG heterostructures have highly ordered epitaxial interfaces, as desired in order to preserve the transport properties of pristine graphene. Atomic scale structural and energetic details of the observed row-by-row, growth mechanism of the 2D epitaxial h-BN film are analyzed through first-principles simulations, demonstrating one-dimensional nucleation-free-energy-barrierless growth. This industrially relevant LED process can be applied to a wide variety of van der Waals materials.

cond-mat.mtrl-sci↗

arXiv2020

Fractional quantum Hall physics and higher-order momentum correlations in a few spinful fermionic contact-interacting ultracold atoms in rotating traps

The fractional quantum Hall effect (FQHE) is theoretically investigated, with numerical and algebraic approaches, in assemblies of a few spinful ultracold neutral fermionic atoms, interacting via repulsive contact potentials and confined in a single rapidly rotating two-dimensional harmonic trap. Going beyond the commonly used second-order correlations in the real configuration space, the methodology in this paper will assist the analysis of experimental observations by providing benchmark results for $N$-body spin-unresolved, as well as spin-resolved, momentum correlations measurable in time-of-flight experiments with individual particle detection. Our analysis shows that the few-body lowest-Landau-level (LLL) states with good magic angular momenta exhibit inherent ordered quantum structures in the $N$-body correlations, similar to those associated with rotating Wigner molecules (WMs), familiar from the field of semiconductor quantum dots under high magnetic fields. The application of a small perturbing stirring potential induces, at the ensuing avoided crossings, formation of symmetry broken states exhibiting ordered polygonal-ring structures, explicitly manifest in the single-particle density profile of the trapped particles. Away from the crossings, an LLL state obtained from exact diagonalization of the microscopic Hamiltonian, found to be well-described by a (1,1,1) Halperin two-component variational wavefunction, represents also a spinful rotating WM. Analysis of the calculated LLL wavefunction enables a two-dimensional generalization of the Girardeau one-dimensional 'fermionization' scheme, originally invoked for mapping of bosonic-type wave functions to those of spinless fermions.

cond-mat.quant-gas↗

arXiv2020

All-order momentum correlations of three ultracold bosonic atoms confined in triple-well traps: Signatures of emergent many-body quantum phase transitions and analogies with three-photon quantum-optics interference

All-order momentum correlation functions associated with the time-of-flight spectroscopy of three spinless ultracold bosonic interacting neutral atoms confined in a linear three-well optical trap are presented. The underlying Hamiltonian employed for the interacting atoms is an augmented three-site Hubbard model. Our investigations target matter-wave interference of massive particles, aiming at the establishment of experimental protocols for characterizing the quantum states of trapped attractively or repulsively interacting ultracold particles, with variable interaction strength. The manifested advantages and deep physical insights that can be gained through the employment of the results of our study for a comprehensive understanding of the nature of the quantum states of interacting many-particle systems, via analysis of the all-order (that is 1st, 2nd and 3rd) momentum correlation functions for three bosonic atoms in a three well confinement, are illustrated and discussed in the context of time-of-flight inteferometric interrogations of the interaction-strength-induced emergent quantum phase transition from the Mott insulating phase to the superfluid one. Furthermore, we discuss that our inteferometric interrogations establish strong analogies with the quantum-optics interference of three photons, including the aspects of genuine three-photon interference, which are focal to explorations targeting the development and implementation of quantum information applications and quantum computing.

cond-mat.quant-gas↗

arXiv2019

Third-order momentum correlation interferometry maps for entangled quantal states of three singly trapped massive ultracold fermions

Analytic higher-order momentum correlation functions associated with the time-of-flight spectroscopy of three ultracold fermionic atoms singly-confined in a linear three-well optical trap are presented, corresponding to the W- and Greenberger-Horne-Zeilinger-type (GHZ) states that belong to characteristic classes of tripartite entanglement and represent the strong-interaction regime captured by a three-site Heisenberg Hamiltonian. The methodology introduced here contrasts with and goes beyond that based on the standard Wick's factorization scheme; it enables determination of both third-order and second-order spin-resolved and spin-unresolved momentum correlations, aiming at matter-wave interference investigations with trapped massive particles in analogy with, and having the potential for expanding the scope of, recent three-photon quantum-optics interferometry.

cond-mat.quant-gas↗

arXiv2019

Anyon optics with time-of-flight two-particle interference of double-well-trapped interacting ultracold atoms

The subject of bianyon interference with ultracold atoms is introduced through theoretical investigations pertaining to the second-order momentum correlation maps of two anyons (built upon spinless and spin-1/2 bosonic, as well as spin-1/2 fermionic ultracold atoms) trapped in a double-well optical trap. The two-particle system is modeled according to the recently proposed protocols for emulating an anyonic Hubbard Hamiltonian in ultracold-atom one-dimensional lattices. Because the second-order momentum correlations are mirrored in the time-of-flight second-order interference patterns in space, our findings provide impetus for time-of-flight experimental protocols for detecting anyonic statistics via interferometry measurements of massive particles that broaden the scope of the biphoton interferometry of quantum optics.

cond-mat.quant-gas↗

arXiv2019

Interference, spectral momentum correlations, entanglement, and Bell inequality for a trapped interacting ultracold atomic dimer: Analogies with biphoton interferometry

Elucidating similarities and differences between quantum-optics biphoton interference phenomena and the quantum physics of quasi-one-dimensional double-well optically-trapped ultracold neutral bosonic or fermionic atoms, we show that the analog of the optical biphoton joint-coincidence spectral correlations, studied with massless non-interacting biphotons emanating from EPR-Bell-Bohm single-occupancy sources, corresponds to a distinct contribution in the total second-order momentum correlations of the massive, interacting, and time-evolving ultracold atoms. This single-occupancy contribution can be extracted from the total second-order momentum correlation function measured in time-of-flight experiments, which for the trapped atomic system contains, in general, a double-occupancy, NOON, component. The dynamics of the two-particle system are modeled by a Hubbard Hamiltonian. This partial coincidence spectrum is a cosine-square quantum beating dependent on the difference of the momenta of the two particles, while the corresponding coincidence probability proper, familiar from its role in describing the Hong-Ou-Mandel coincidence dip of overlapping photons, results from an integration over the particle momenta. Because the second-order momentum correlations are mirrored in the time-of-flight spectra in space, our theoretical findings provide impetus for time-of-flight experimental protocols for emulating with (massive) ultracold atoms venerable optical interferometries that use two space-time separated and entangled (massless) photons or double-slit optical sources. The implementation of such developments will facilitate testing of fundamental aspects and enable applications of quantum physics with trapped massive ultracold atoms, that is, investigations of nonlocality and violation of Bell inequalities, entanglement, and quantum information science.

cond-mat.quant-gas↗

arXiv2018

Interatomic interaction effects on second-order momentum correlations and Hong-Ou-Mandel interference of double-well-trapped ultracold fermionic atoms

Identification and understanding of the evolution of interference patterns in two-particle momentum correlations as a function of the strength of interatomic interactions are important in explorations of the nature of quantum states of trapped particles. Together with the analysis of two-particle spatial correlations, they offer the prospect of uncovering fundamental symmetries and structure of correlated many-body states, as well as opening vistas into potential control and utilization of correlated quantum states as quantum information resources. With the use of the second-order density matrix constructed via exact diagonalization of the microscopic Hamiltonian, and an analytic Hubbard-type model, we explore here the systematic evolution of characteristic interference patterns in the two-body momentum and spatial correlation maps of two entangled ultracold fermionic atoms in a double well, for the entire attractive- and repulsive-interaction range. We uncover statistics-governed bunching and antibunching, as well as interaction-dependent interference patterns, in the ground and excited states, and interpret our results in light of the Hong-Ou-Mandel interference physics, widely exploited in photon indistinguishability testing and quantum information science.

cond-mat.quant-gas↗

arXiv2017

Two-point momentum correlations of few ultracold quasi-one-dimensional trapped fermions: Diffraction patterns

Spatial and momentum correlations are important in the analysis of the quantum states and different phases of trapped ultracold atom systems as a function of the strength of interatomic interactions. Identification and understanding of spin-resolved patterns exhibited in two-point correlations, accessible directly by experiments, are key for uncovering the symmetry and structure of the many-body wave functions of the trapped system. Using the configuration interaction method for exact diagonalization of the many-body Hamiltonian of $N=2-4$ fermionic atoms trapped in single, double, triple, and quadruple wells, we analyze both two-point momentum and space correlations, as well as associated noise distributions, for a broad range of interparticle contact repulsion strengths and interwell separations, unveiling characteristics allowing insights into the transition, via an intermediate phase, from the non-interacting Bose-Einstein condensate to the weakly interacting quasi-Bose-Einstein regime, and from the latter to the strong-repulsion Tonks-Girardeau (TG) one. The ab-initio numerical predictions are shown to agree well with the results of a constructed analytical model employing localized displaced Gaussian functions to represent the $N$ fermions. The two-point momentum correlations are found to exhibit damped oscillatory diffraction behavior. This diffraction behavior develops fully for atoms trapped in a single well with strong interatomic repulsion in the TG regime, or for atoms in well-separated multi-well traps. Additionally, the two-body momentum correlation and noise distributions are found to exhibit "shortsightedness", with the main contribution coming from nearest-neighboring particles.

cond-mat.quant-gas↗