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V. A. Sautenkov

Publications and source records attributed to V. A. Sautenkov.

9 recordsLinked to original sources

Influence of Many-Body Dipole-Dipole Interactions on Excitation Transfer in a Dense Gas

We study non-radiative dipole-dipole induced excitation transfer in dense Rb vapour. We show that density dependence of characteristic time of the excitation diffusion changes from linear to non-linear for high Rb density. It is attributed to the breakdown of binary collisions approach to the dipole-dipole excitation transfer. It is shown that the observed result can be qualitatively described if the mean free path is replaced by mean interatomic distance for the chracteristic diffusion length.

physics.atom-ph↗

Optical-field-induced dips and splits in nonlinear spectra of selective reflection from high-density atomic vapor

We discuss nonlinear spectra of selective reflection from high-density rubidium atomic vapor, where the self-broadening of the resonant transition $5S_{1/2}-5P_{3/2}$ dominates over the Doppler width. In the experiments, the hole-burning technique with probe and pump lasers is used. The reflection of weak probe beam is investigated at four atomic densities in the range $(1.2\text{--}3.6)\times10^{17}$~cm$^{-3}$ and various pump beam intensities. To enhance the spectral resolution, the frequency derivative $\text{d}R/\text{d}ν$ of the reflection coefficient $R$ is analyzed. Increasing the atomic number density changes the character of self-broadening from inhomogeneous to homogeneous. At the highest density, the strong pump field splits the observed spectra into two homogeneously broadened symmetric resonances. The appearance of the optical-field-induced resonances can be explained within the framework of "dressed atomic states" approach. At lower densities the spectral profiles are inhomogeneously broadened. Spectral profiles of the frequency derivative are separated by optically saturated dips. The width of such dips is a combination of the homogeneous component of self-broadening and intensity-dependent field broadening. Careful study of the transition from inhomogeneous to homogeneous broadening may initiate further development of the theory of interatomic interactions in high density atomic gas media.

physics.atom-ph↗

Pump-probe studies of resonantly saturated selective reflection from high-density rubidium vapor

Nonlinear selective reflection from the interface YAG window-high density rubidium vapor in the high-temperature cell is studied at the transition 5S$_{1/2}$-5P$_{3/2}$. In the experiment tunable pump and probe lasers are used. The selective reflection spectra for the laser probe beam are investigated at four different rubidium atomic densities and five different pump beam intensities. The estimated dipole-dipole interaction-induced line broadening varies from $13.2$ to $39.6$ GHz, the measured pumped intensities change from $1.2$ to $8.8$ kW$\cdot$cm$^{-2}$. Growth of the pump intensity causes reduction of the magnitude and the width of the recorded selective reflection resonance. We suggest developing all-optical modulators on the basis of nonlinear selective reflection.

physics.atom-ph↗

Self-focusing of CW Laser Beam with Variable Radius in Rubidium Atomic Vapor

Self-focusing of a cw laser beam in rubidium atomic vapor was studied. The beam power and beam spot size at entrance of a glass cell with the rubidium vapor were variable parameters. A steep grow of the threshold power of self-focusing for the small beam radii (< 30 μm) was observed. Our experimental data are in an agreement with the theoretical results published by Semak and Shneider in 2013. Additional experiments in resonance and transparent media are suggested in order to check and extend our measurements.

physics.optics↗

Photoluminescence studies study of a phenyl-substituted PPV

We report on the photophysics of a phenyl-substituted PPV both in solution and as a film. For both systems we have studied the decay of the photoluminescence and of the emission anisotropy for a large set of wavelengths spanning the entire photoluminescence spectrum. At long wavelengths the decay behavior is that of an interchain species. At the shortest wavelengths the decay of the photoluminescence from the film is observed to have a long-lived component, in addition to the rapidly decaying component usually associated with energy transfer. We attribute this slow component to emission by isolated intrachain excitons with reduced nonradiative relaxation.

physics.chem-ph↗

Measuring the gain dynamics in a conjugated polymer film

We present a simple method for measuring the gain decay time in a conjugated polymer film by optically exciting the film with two mutually delayed ultrashort pump pulses. When the pump is set at such a power level that amplified spontaneous emission marginally develops along the polymer waveguide, the total output emitted from its edge decays exponentially as a function of the interpulse delay. The corresponding decay time represents the decay time of the gain of the polymer material.

physics.chem-ph↗

Enhancement of field generation via maximal atomic coherence prepared by fast adiabatic passage in Rb vapor

We have experimentally demonstrated the enhancement of coherent Raman scattering in Rb atomic vapor by exciting atomic coherence with fractional stimulated Raman adiabatic passage. Experimental results are in good agreement with numerical simulations. The results support the possibility of increasing the sensitivity of CARS by preparing atomic or molecular coherence using short pulses.

quant-ph↗

Nonlinear optics via double dark resonances

Double dark resonances originate from a coherent perturbation of a system displaying electromagnetically induced transparency. We experimentally show and theoretically confirm that this leads to the possibility of extremely sharp resonances prevailing even in the presence of considerable Doppler broadening. A gas of 87Rb atoms is subjected to a strong drive laser and a weak probe laser and a radio frequency field, where the magnetic coupling between the Zeeman levels leads to nonlinear generation of a comb of sidebands.

quant-ph↗

Enhancement of Magneto-Optic Effects via Large Atomic Coherence

We utilize the generation of large atomic coherence to enhance the resonant nonlinear magneto-optic effect by several orders of magnitude, thereby eliminating power broadening and improving the fundamental signal-to-noise ratio. A proof-of-principle experiment is carried out in a dense vapor of Rb atoms. Detailed numerical calculations are in good agreement with the experimental results. Applications such as optical magnetometry or the search for violations of parity and time reversal symmetry are feasible.

quant-ph↗