arXiv subjects

V. Ara Apkarian

Publications and source records attributed to V. Ara Apkarian.

3 recordsLinked to original sources

arXiv2025

Coherent Field Emission Upon Ultrafast Laser Irradiation of the Tip Plasmon

Irradiation of sharp silver tips with femtosecond laser pulses leads to photoassisted coherent field emission without a static field. We reconstruct the time profile of the emission, and show that the process is entirely governed by the collective response of the tip plasmon and its field emission. Weak-field optical excitation leads to multiphoton absorption and field emission from the tip apex due to the enhanced local field. The attendant sharp field gradient ensures ponderomotive acceleration of emitted electrons and non-local light-matter interaction. The crossover regime in which simultaneous multiphoton absorption and optical field emission take place is evidenced by the time profile of electron emission correlation, laser power dependence, and polarization angle dependence of each harmonic current.

physics.optics↗

arXiv2025

Overcoming the indirect bandgap: efficient silicon emission via momentum-expanded photonic states

Silicon's inherently indirect bandgap severely limits its radiative efficiency, posing a fundamental challenge to the development of practical silicon-based light sources. While strategies such as nanoscale confinement of electrons and holes (quantum dots), Mie resonators, and hybrid plasmonic structures have improved emission, they typically require complex fabrication workflows. Here, we demonstrate a conceptually distinct and scalable approach to enable light emission from a bulk silicon wafer by decorating its surface with gold or copper nanoparticles. Remarkably, the effect is nearly identical for Au and Cu, with particle size emerging as the dominant factor. We show that strong luminescence from the bulk wafer emerges only when the nanoparticle diameter is below 2 nm. We attribute this effect to the formation of spatially confined photonic states with broadened momentum distributions, which must enable diagonal, phonon-independent optical transitions that bypass the limitations imposed by silicon's indirect bandgap. This mechanism yields broadband emission across the visible and near-infrared spectrum, with quantum efficiencies comparable to direct bandgap semiconductors, representing a 10^5-fold increase in integrated spectral intensity. This discovery challenges the conventional understanding of silicon's optical constraints and opens a practical pathway toward high-performance silicon-based optical and optoelectronic components.

physics.optics↗

arXiv2002

An Implementation of the Deutsch-Jozsa Algorithm on Molecular Vibronic Coherences Through Four-Wave Mixing: a Theoretical Study

Time-Frequency Resolved Coherent Anti-Stokes Raman Scattering (TFRCARS) was recently proposed as a means to implement quantum logic using the molecular ro-vibrational manifold as a quantum register [R. Zadoyan et al., Chem. Phys. 266, 323 (2001)]. We give a concrete example of how this can be accomplished through an illustrative algorithm that solves the Deutsch-Jozsa problem. We use realistic molecular parameters to recognize that, as the problem size expands, shaped pulses must be tailored to maintain fidelity of the algorithm.

quant-ph↗