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V. Bhartiya

Publications and source records attributed to V. Bhartiya.

2 recordsLinked to original sources

Observation of multipartite spin entanglement in a cuprate chain

Quantum materials are believed to host highly entangled states of matter, but probing and quantifying such entanglement has long remained experimentally elusive. Here, we use resonant inelastic X-ray scattering (RIXS) as a probe of multipartite spin entanglement. By projecting the RIXS cross section onto the appropriate spin excitation channel, we show that the Quantum Fisher Information can be extracted directly from the measured spin fluctuation spectrum. We detect at least 7-partite spin entanglement in the model one-dimensional cuprate Sr$_2$CuO$_3$, revealing one of the largest entanglement depths yet reported in a solid. The observed entanglement depth agrees with Hubbard-model expectations and persists to elevated temperatures. Our results establish RIXS as an experimental probe of many-body spin entanglement and provide a platform for extensions to charge and orbital sectors and nonequilibrium settings.

cond-mat.str-el

Capping effects on spin and charge excitations in parent and superconducting Nd1-xSrxNiO2

Superconductivity in infinite layer nickelates Nd1-xSrxNiO2 has so far been achieved only in thin films raising questions on the role of substrates and interfaces. Given the challenges associated with their synthesis it is imperative to identify their intrinsic properties. We use Resonant Inelastic X-ray Scattering (RIXS) to investigate the influence of the SrTiO3 capping layer on the excitations of Nd1-xSrxNiO2 (x = 0 and 0.2). Spin excitations are observed in parent and 20% doped Nd1-xSrxNiO2 regardless of capping, proving that magnetism is intrinsic to infinite-layer nickelates and appears in a significant fraction of their phase diagram. In parent and superconducting Nd1-xSrxNiO2, the spin excitations are slightly hardened in capped samples compared to the non-capped ones. Additionally, a weaker Ni - Nd charge transfer peak at ~ 0.6 eV suggests that the hybridization between Ni 3d and Nd 5d orbitals is reduced in capped samples. From our data, capping induces only minimal differences in Nd1-xSrxNiO2 and we phenomenologically discuss these differences based on the reconstruction of the SrTiO3 - NdNiO2 interface and other mechanisms such as crystalline disorder.

cond-mat.supr-con