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V. Caracciolo

Publications and source records attributed to V. Caracciolo.

At least 37 records · Page 2Linked to original sources

Search for double beta decay of $^{106}$Cd with an enriched $^{106}$CdWO$_4$ crystal scintillator in coincidence with CdWO$_4$ scintillation counters

Studies on double beta decay processes in $^{106}$Cd were performed by using a cadmium tungstate scintillator enriched in $^{106}$Cd at 66% ($^{106}$CdWO$_4$) with two CdWO$_4$ scintillation counters (with natural Cd composition). No effect was observed in the data accumulated over 26033 h. New improved half-life limits were set on the different channels and modes of the $^{106}$Cd double beta decay at level of $\lim T_{1/2}\sim 10^{20}-10^{22}$ yr. The limit for the two neutrino electron capture with positron emission in $^{106}$Cd to the ground state of $^{106}$Pd, $T^{2ν\mathrm{EC}β^+}_{1/2}\geq2.1\times 10^{21}$ yr, was set by the analysis of the $^{106}$CdWO$_4$ data in coincidence with the energy release 511 keV in both CdWO$_4$ counters. The sensitivity approaches the theoretical predictions for the decay half-life that are in the range $T_{1/2}\sim10^{21}-10^{22}$ yr. The resonant neutrinoless double-electron capture to the 2718 keV excited state of $^{106}$Pd is restricted at the level of $T^{0ν\mathrm{2K}}_{1/2}\geq2.9\times10^{21}$ yr

nucl-ex↗

Search for alpha decay of naturally occurring osmium nuclides accompanied by gamma quanta

A search for $α$ decay of naturally occurring osmium isotopes to the lowest excited levels of daughter nuclei has been performed by using an ultra-low-background Broad-Energy Germanium $γ$-detector with a volume of 112 cm$^3$ and an ultra-pure osmium sample with a mass of 118 g at the Gran Sasso National Laboratory of the INFN (Italy). The isotopic composition of the osmium sample has been measured with high precision using Negative Thermal Ionisation Mass Spectrometry. After 15851 h of data taking with the $γ$-detector no effect has been detected, and lower limits on the $α$ decays were set at level of $\lim T_{1/2}\sim 10^{15}-10^{19}$ yr. The limits for the $α$ decays of $^{184}$Os and $^{186}$Os to the first excited levels of daughter nuclei, $T_{1/2}(^{184}$Os$)\geq 6.8\times10^{15}$ yr and $T_{1/2}(^{186}$Os$)\geq3.3\times10^{17}$ yr (at 90% C.L.), exceed the present theoretical estimates of the decays half-lives. For $^{189}$Os and $^{192}$Os also decays to the ground states of the daughter nuclei were searched for due to the instability of the daughter nuclides relative to $β$ decay.

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Search for $α$ decay of naturally occurring Hf-nuclides using a Cs$_2$HfCl$_6$ scintillator

Residual radioactive contaminants of a caesium hafnium chloride (Cs$_2$HfCl$_6$) crystal scintillator have been measured in a low background setup at the Gran Sasso National Laboratory of the INFN, Italy. The total alpha activity of the detector is at the level of 7.8(3) mBq/kg. The results of direct studies of the $α$ decay of naturally occurring Hf isotopes that have been performed using the "source=detector" approach are presented. In 2848 h of data taking, the $α$ decay of $^{174}$Hf was observed with T$_{1/2} = (7.0\pm1.2)\times10^{16} $ y.

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Developments and improvements of radiopure ZnWO$_{4}$ anisotropic scintillators

The ZnWO$_4$ is an anisotropic crystal scintillator; for its peculiar characteristics, it is a very promising detector to exploit the so-called directionality approach in the investigation of those Dark Matter (DM) candidates inducing nuclear recoils. Recently, in the framework of the ADAMO project, an R\&D to develop high quality and ultra-radiopure ZnWO$_4$ crystal scintillators has been carried out. In the present paper the measurements to study the anisotropic response of a ZnWO$_4$ to $α$ particles and to nuclear recoils induced by neutron scattering are reported. Monochromatic neutrons have been produced by a neutron generator at ENEA-CASACCIA. The quenching factor values for nuclear recoils along different crystallographic axes have been determined for three different nuclear recoils energies. These results open the possibility to realize a pioneer experiment to investigate the above mentioned DM candidates by means of the directionality.

physics.ins-det↗

Measurements of ZnWO$_4$ anisotropic response to nuclear recoils for the ADAMO project

Anisotropic scintillators can offer a unique possibility to exploit the so-called directionality approach in order to investigate the presence of those Dark Matter (DM) candidates inducing nuclear recoils. In fact, their use can overcome the difficulty of detecting extremely short nuclear recoil traces. In this paper we present recent measurements performed on the anisotropic response of a ZnWO$_4$ crystal scintillator to nuclear recoils, in the framework of the ADAMO project. The anisotropic features of the ZnWO$_4$ crystal scintillators were initially measured with $α$ particles; those results have been also confirmed by the additional measurements presented here. The experimental nuclear recoil data were obtained by using a neutron generator at ENEA-CASACCIA and neutron detectors to tag the scattered neutrons; in particular, the quenching factor values for nuclear recoils along different crystallographic axes have been determined for three different neutron scattering angles (i.e. nuclear recoils energies). From these measurements, the anisotropy of the light response for nuclear recoils in the ZnWO$_4$ crystal scintillator has been determined at 5.4 standard deviations.

physics.ins-det↗

Improved model-dependent corollary analyses after the first six annual cycles of DAMA/LIBRA-phase2

Several of the many proposed Dark Matter candidate particles, already investigated with lower exposure and a higher software energy threshold, are further analyzed including the first DAMA/LIBRA--phase2 data release, with an exposure of 1.13 ton $\times$ yr and a lower software energy threshold (1 keV). The cumulative exposure above 2 keV considering also DAMA/NaI and DAMA/LIBRA--phase1 results is now 2.46 ton $\times$ yr. The analysis permits to constraint the parameters' space of the considered candidates restricting their values -- with respect to previous analyses -- thanks to the increase of the exposure and to the lower energy threshold.

hep-ph↗

First direct search for $2ε$ and $εβ^+$ decay of $^{144}$Sm and $2β^-$ decay of $^{154}$Sm

The first direct search for the double electron capture ($2ε$) and the electron capture with positron emission ($εβ^+$) in $^{144}$Sm to the ground state and to the excited levels of $^{144}$Nd was realized by measuring - over 1899 h - a 342 g sample of highly purified samarium oxide (Sm$_2$O$_3$) with the ultra-low background HP-Ge $γ$ spectrometer GeCris (465 cm$^3$) at the STELLA facility of the Gran Sasso National Laboratory (LNGS). No effect was observed and half-life limits were estimated at the level of $T_{1/2} \sim (0.1-1.3) \times 10^{20}$ yr (90% C.L.). Moreover, for the first time half-life limits of the double beta ($2β^-$) decay of $^{154}$Sm to several excited levels of $^{154}$Gd have been set; they are at the level of $T_{1/2} \sim (0.06-8) \times 10^{20}$ yr (90% C.L.).

nucl-ex↗

First search for 2$\varepsilon$ and $\varepsilonβ^+$ processes in $^{168}$Yb

The double-electron capture and the electron capture with positron emission in $^{168}$Yb have been investigated for the first time at the STELLA facility of the Gran Sasso underground laboratory (Italy) measuring 371 g of highly purified ytterbium oxide placed on the end-cap of a 465 cm$^3$ ultra-low-background high purity Germanium detector (HPGe). No gamma associated to double beta processes in $^{168}$Yb have been observed after 2074 h of data taking. This has allowed setting the half-life limits on the level of $\lim T_{1/2}\sim$ $10^{14}-10^{18}$ yr at 90\% C.L. Particularly, a lower half-life limit on a possible resonant neutrinoless double-electron capture in $^{168}$Yb to the $(2)^-$ 1403.7 keV excited state of $^{168}$Er is set as $T_{1/2}\geq1.9\times 10^{18}$ yr at 90\% C.L. Half-life limits $T_{1/2}^{2ν(0ν)}\geq 4.5(4.3)\times10^{16}$ yr were set on the $2ν(0ν)2β^-$ decay of $^{176}$Yb to the $2^+$ 84.3 keV first excited level of $^{176}$Hf.

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Cryogenic light detectors with enhanced performance for rare events physics

We have developed and tested a new way of coupling bolometric light detectors to scintillating crystal bolometers based upon simply resting the light detector on the crystal surface, held in position only by gravity. This straightforward mounting results in three important improvements: (1) it decreases the amount of non-active materials needed to assemble the detector, (2) it substantially increases the light collection efficiency by minimizing the light losses induced by the mounting structure, and (3) it enhances the thermal signal induced in the light detector thanks to the extremely weak thermal link to the thermal bath. We tested this new technique with a 16 cm$^2$ Ge light detector with thermistor readout sitting on the surface of a large TeO$_2$ bolometer. The light collection efficiency was increased by greater than 50\% compared to previously tested alternative mountings. We obtained a baseline energy resolution on the light detector of 20~eV RMS that, together with increased light collection, enabled us to obtain the best $α$ vs $β/γ$ discrimination ever obtained with massive TeO$_2$ crystals. At the same time we achieved rise and decay times of 0.8 and 1.6 ms, respectively. This superb performance meets all of the requirements for the CUPID (CUORE Upgrade with Particle IDentification) experiment, which is a 1-ton scintillating bolometer follow up to CUORE.

physics.ins-det↗

First model independent results from DAMA/LIBRA-phase2

The first model independent results obtained by the DAMA/LIBRA-phase2 experiment are presented. The data have been collected over 6 annual cycles corresponding to a total exposure of 1.13 ton $\times$ yr, deep underground at the Gran Sasso National Laboratory (LNGS) of the I.N.F.N. The DAMA/LIBRA-phase2 apparatus, $\simeq$ 250 kg highly radio-pure NaI(Tl), profits from a second generation high quantum efficiency photomultipliers and of new electronics with respect to DAMA/LIBRA-phase1. The improved experimental configuration has also allowed to lower the software energy threshold. New data analysis strategies are presented. The DAMA/LIBRA-phase2 data confirm the evidence of a signal that meets all the requirements of the model independent Dark Matter (DM) annual modulation signature, at 9.5 $σ$ C.L. in the energy region (1-6) keV. In the energy region between 2 and 6 keV, where data are also available from DAMA/NaI and DAMA/LIBRA-phase1 (exposure $1.33$ ton $\times$ yr, collected over 14 annual cycles), the achieved C.L. for the full exposure (2.46 ton $\times$ yr) is 12.9 $σ$; the modulation amplitude of the single-hit scintillation events is: $(0.0103 \pm 0.0008)$ cpd/kg/keV, the measured phase is $(145 \pm 5)$ days and the measured period is $(0.999 \pm 0.001)$ yr, all these values are well in agreement with those expected for DM particles. No systematics or side reaction able to mimic the exploited DM signature (i.e. to account for the whole measured modulation amplitude and to simultaneously satisfy all the requirements of the signature), has been found or suggested by anyone throughout some decades thus far.

hep-ex↗

Half-life measurements of $^{212}$Po with thorium-loaded liquid scintillator

Precise measurement of half-life of $^{212}$Po (one of the daughter nuclides in radioactive chain of $^{232}$Th) was realized by means of liquid scintillator based on toluene doped by complex of thorium and trioctylphosphine oxide with concentration of Th $\sim0.1$ mass %. Fast photomultiplier tube and high frequency oscilloscope were used to acquire the scintillation signals waveforms. The algorithms were developed to find pairs of $^{212}$Bi beta-decays and subsequent $^{212}$Po alpha-decays, to calculate time differences between the events in the pair, and to build $^{212}$Bi beta-decay and $^{212}$Po alpha-decay energy spectra. Preliminary the $^{212}$Po half-life is $T_{1/2} = (294.8 \pm 1.9)$ ns. The experiment is in progress aiming at reduction of the statistical and systematic uncertainties.

nucl-ex↗

Final results of the Aurora experiment to study 2$β$ decay of $^{116}$Cd with enriched $^{116}$CdWO$_4$ crystal scintillators

The double-beta decay of $^{116}$Cd has been investigated with the help of radiopure enriched $^{116}$CdWO$_4$ crystal scintillators (mass of 1.162 kg) at the Gran Sasso underground laboratory. The half-life of $^{116}$Cd relatively to the $2\nu2β$ decay to the ground state of $^{116}$Sn was measured with the highest up-to-date accuracy as $T_{1/2}=(2.63^{+0.11}_{-0.12})\times10^{19}$ yr. A new improved limit on the 0$ν$2$β$ decay of $^{116}$Cd to the ground state of $^{116}$Sn was set as $T_{1/2}\geq 2.2 \times 10^{23}$ yr at 90\% C.L., which is the most stringent known restriction for this isotope. It corresponds to the effective Majorana neutrino mass limit in the range $\langle m_ν\rangle\le(1.0-1.7)$ eV, depending on the nuclear matrix elements used in the estimations. New improved half-life limits for the 0$ν$2$β$ decay with majoron(s) emission, Lorentz-violating $2\nu2β$ decay and $2β$ transitions to excited states of $^{116}$Sn were set at the level of $T_{1/2}\geq 10^{20}-10^{22}$ yr. New limits for the hypothetical lepton-number violating parameters (right-handed currents admixtures in weak interaction, the effective majoron-neutrino coupling constants, R-parity violating parameter, Lorentz-violating parameter, heavy neutrino mass) were set.

nucl-ex↗

Double beta decay of $^{150}$Nd to the first excited $0^+$ level of $^{150}$Sm: preliminary results

The double beta decay of $^{150}$Nd to the first excited 0$^+$ level of $^{150}$Sm ($E_{exc}$ = 740.5 keV) has been investigated with the help of the ultra-low-background setup consisting of four HP Ge (high-purity germanium) detectors (${\approx}$ 225 cm$^3$ volume each one) at the Gran Sasso underground laboratory of INFN (Italy). A highly purified 2.381-kg sample of neodymium oxide (Nd$_2$O$_3$) was used as a source of $γ$ quanta expected in the decays. Gamma quanta with energies 334.0 keV and 406.5 keV emitted after deexcitation of the $0_1^+$ 740.5 keV level of $^{150}$Sm are observed in the coincidence spectra accumulated over 16375 h. The half-life relatively to the two neutrino double beta decay $^{150}$Nd $\rightarrow$ $^{150}$Sm(0$_1^+$) is measured as $T_{1/2} = [4.7_{-1.9}^{+4.1}\text{(stat)} {\pm} 0.5\text{(syst)}] {\times} 10^{19} y$, in agreement with results of previous experiments.

nucl-ex↗

First search for $2\varepsilon$ and $\varepsilonβ^+$ decay of $^{162}$Er and new limit on $2β^{-}$ decay of $^{170}$Er to the first excited level of $^{170}$Yb

The first search for double electron capture ($2\varepsilon$) and electron capture with positron emission ($\varepsilonβ^+$) of $^{162}$Er to the ground state and to several excited levels of $^{162}$Dy was realized with 326 g of highly purified erbium oxide. The sample was measured over 1934 h by the ultra-low background HP Ge $γ$ spectrometer GeCris (465 cm$^3$) at the Gran Sasso underground laboratory. No effect was observed, the half-life limits were estimated at the level of $\lim T_{1/2}\sim 10^{15}-10^{18}$ yr. A possible resonant $0νKL_1$ capture in $^{162}$Er to the $2^+$ 1782.7 keV excited state of $^{162}$Dy is restricted as $T_{1/2}\geq5.0\times 10^{17}$ yr at 90% C.L. A new improved half-life limit $T_{1/2}\geq4.1\times 10^{17}$ yr was set on the $2β^-$ decay of $^{170}$Er to the $2^+$ 84.3 keV first excited state of $^{170}$Yb.

nucl-ex↗

Investigation of 2$β$ Decay of $^{116}$Cd with the Help of Enriched $^{116}$CdWO$_4$ Crystal Scintillators

Double beta decay of $^{116}$Cd has been investigated with the help of radiopure enriched $^{116}$CdWO$_4$ crystal scintillators in the experiment Aurora. The half-life of $^{116}$Cd relatively to the 2$ν$2$β$ decay of $^{116}$Cd to the ground level of $^{116}$Sn is measured with the highest up-to-date accuracy as $T_{1/2}$ = [2.69 $\pm$ 0.02 (stat.) $\pm$ 0.14 (syst.)] $\times$ 10$^{19}$ yr. A new improved limit on the 0$ν$2$β$ decay of $^{116}$Cd to the ground state of $^{116}$Sn is set as $T_{1/2}\geq 2.4 \times 10^{23}$ yr at 90\% C.L., that corresponds to the effective Majorana neutrino mass limit in the range $\langle$$m_ν$$\rangle$ $\le$ $(1.1-1.6)$ eV, depending on the nuclear matrix elements used in the estimations. New improved limits on other $2β$ processes in $^{116}$Cd (decays with majoron emission, transitions to excited levels of $^{116}$Sn) were set at the level of $T_{1/2}\geq 10^{21}-10^{22}$ yr.

nucl-ex↗

DAMA/LIBRA results and perspectives

The DAMA/LIBRA experiment ($\sim$ 250 kg of highly radio-pure NaI(Tl)) is running deep underground at the Gran Sasso National Laboratory (LNGS) of the I.N.F.N. Here we briefly recall the results obtained in its first phase of measurements (DAMA/LIBRA--phase1, total exposure: 1.04 ton $\times$ yr). DAMA/LIBRA--phase1 and the former DAMA/NaI (cumulative exposure: $1.33$ ton $\times$ yr) give evidence at 9.3 $σ$ C.L. for the presence of DM particles in the galactic halo by exploiting the model-independent DM annual modulation signature. No systematic or side reaction able to mimic the exploited DM signature has been found or suggested by anyone over more than a decade. At present DAMA/LIBRA--phase2 is running with increased sensitivity.

hep-ex↗

Improvement of radiopurity level of enriched $^{116}$CdWO$_4$ and ZnWO$_4$ crystal scintillators by recrystallization

As low as possible radioactive contamination of a detector plays a crucial role to improve sensitivity of a double beta decay experiment. The radioactive contamination of a sample of $^{116}$CdWO$_4$ crystal scintillator by thorium was reduced by a factor $\approx 10$, down to the level 0.01 mBq/kg ($^{228}$Th), by exploiting the recrystallization procedure. The total alpha activity of uranium and thorium daughters was reduced by a factor $\approx 3$, down to 1.6 mBq/kg. No change in the specific activity (the total $α$ activity and $^{228}$Th) was observed in a sample of ZnWO$_4$ crystal produced by recrystallization after removing $\approx 0.4$ mm surface layer of the crystal.

physics.ins-det↗

Search for $2β$ decay of $^{106}$Cd with enriched $^{106}$CdWO$_4$ crystal scintillator in coincidence with four HPGe detectors

A radiopure cadmium tungstate crystal scintillator, enriched in $^{106}$Cd to 66%, with mass of 216 g ($^{106}$CdWO$_4$), was used to search for double beta decay processes in $^{106}$Cd in coincidence with four ultra-low background high purity germanium detectors in a single cryostat. New improved limits on the double beta processes in $^{106}$Cd have been set on the level of $10^{20}- 10^{21}$ yr after 13085 h of data taking. In particular, the half-life limit on the two neutrino electron capture with positron emission, $T_{1/2}^{2ν\varepsilonβ^+}\geq 1.1\times 10^{21}$ yr, has reached the region of theoretical predictions. With this half-life limit the effective nuclear matrix element for the $2ν\varepsilonβ^+$ decay is bounded as $M^{2ν\varepsilonβ^+}_{eff}\le 1.1$. The resonant neutrinoless double electron captures to the 2718 keV, 2741 keV and 2748 keV excited states of $^{106}$Pd are restricted at the level of $T_{1/2} \geq (8.5\times10^{20}-1.4\times10^{21}$) yr.

nucl-ex↗