arXiv subjects

V. Cros

Publications and source records attributed to V. Cros.

At least 19 recordsLinked to original sources

arXiv2025

Orbital torque and efficient magnetization switching using ultrathin Co|Al light-metal interfaces: Experiments and modeling

The emergence of the orbital degree of freedom in modern orbitronics offers a promising alternative to heavy metals for the efficient control of magnetization. In this context, identifying interfaces that exhibit orbital-momentum locking and an orbital Rashba-Edelstein response to an external electric field is of primary importance. In this work, we experimentally investigate the Co/Al system and extend the study to Co/Pt/Al structures. We show that inserting ultrathin Pt layers between Co and Al can significantly modify the orbital properties, highlighting the critical role of Co/Al orbital bonding in generating orbital polarization. We further model the orbital response of these systems using semi-phenomenological approaches and linear-response theory within the framework of density-functional theory.

cond-mat.mtrl-sci↗

arXiv2025

Quantum Kinetic Anatomy of Electron Angular Momenta Edge Accumulation

Controlling electron's spin and orbital degrees of freedom has been a major research focus over the past two decades, as it underpins the electrical manipulation of magnetization. Leveraging a recently introduced quantum kinetic theory of multiband systems [T. Valet and R. Raimondi, Phys. Rev. B 111, L041118 (2025)], we outline how the intrinsic angular momenta linear response is partitioned into intraband and interband contributions. Focusing on time reversal and inversion symmetric metals, we show that the spin and orbital Hall currents are purely intraband. We also reveal that the intrinsic edge densities originate partially, and in the orbital case probably mostly, from a new interband mechanism. We discuss how this profoundly impacts the interpretation of orbital edge accumulation observations, and has broader implications for current induced torques.

cond-mat.mes-hall↗

arXiv2025

Anatomy of torques from orbital Rashba textures: the case of Co/Al interfaces

In the context of orbitronics, the rising of the orbital angular momentum generated at light metal interfaces from orbital textures via orbital Rashba-Edelstein effects nowadays represent extraordinary alternatives to the usual heavy-metal spin-based materials. In the light of very recent experimental results [\textcolor{blue}{S. Krishnia \textit{et al.}, Nanoletters 2023, 23, 6785}], starting from state-of-the-art density functional theory simulations, we provide theoretical insights into the emergence of very strong orbital torques at the Co/Al interface location a strong orbital Rashba texture. By using linear response theory, we calculate the exerted orbital torque amplitudes, mainly of field-like intraband character, acting onto the ultrathin Co. Moreover, we show that an insertion of a single atomic plane of Pt between Co and Al is enough to suppress the effect which questions about the anatomy of the torque action clearly behaving differently than in the standard way. This work opens new routes to the engineering of spintronic devices.

cond-mat.mtrl-sci↗

arXiv2025

Quantitative analysis of vectorial torques in thin 3d Co ferromagnet using orbital-spin conversion

Recent findings in orbitronics pointed out large current-induced torques originating, in the current understanding, from incident orbital currents. These are generated by orbital Rashba-Edelstein effect (OREE) produced at the interface between some light metal and oxides films e.g. by naturally oxidized copper layer (Cu*). In the present work, by using second harmonic Hall techniques, we determine the ratio of orbital vs spin currents exerting torques on thin transition metals Co ferromagnet in systems using an orbit-to-spin Pt converter as interlayer with Cu*. Our results quantifying damping like torques show that both orbital and spin currents are enhanced in these systems. Moreover, the experimental determination of the decoherence length in a sample series with varying Co thickness clearly demonstrates the interfacial generation of the orbital currents in Cu* by Orbital Rashba-Edelstein effects (REE) leading to subsequent magnetic torque in Co over a typical lengthscale of several nanometers

cond-mat.mtrl-sci↗

arXiv2024

Alternative harmonic detection approach for quantitative determination of spin and orbital torques

In this study, the spin-orbit torque (SOT) in light metal oxide systems is investigated using an experimental approach based on harmonic Hall voltage techniques in out-of-plane (OOP) angular geometry for samples with in-plane magnetic anisotropy. In parallel, an analytical derivation of this alternative OOP harmonic Hall detection geometry has been developed, followed by experimental validation to extract SOT effective fields. In addition, to accurately quantifying SOT, this method allows complete characterization of thermoelectric effects, opening promising avenues for accurate SOT characterization in related systems. In particular, this study corroborates the critical role of naturally oxidized copper interfaced with metallic Cu in the generation of orbital current in Co(2)|Pt(4)|CuOx(3), demonstrating a two-fold increase in damping-like torques compared to a reference sample with an oxidized Al capping layer. These findings offer promising directions for future research on the application aspect of non-equilibrium orbital angular momentum.

cond-mat.mtrl-sci↗

arXiv2024

Controlling encirclement of an exceptional point using coupled spintronic nano-oscillators

Exceptional points (EPs), branch singularities parameter space of non-Hermitian eigenvalue manifolds, display unique topological phenomena linked to eigenvalue and eigenvector switching: the parameter space states are highly sensitive to the system's parameter changes. Therefore, we suggest investigating the parameter space in the presence of an EP by experimentally accessing and exploiting the topological nature of the coupled system around an EP. We demonstrate control over exceptional points in coupled vortex spin-transfer torque oscillators by adjusting the system's damping through the spin-transfer torque effect and their relative phase. This approach allows for precise manipulation of the coupling behavior in the vicinity of an exceptional point. We report the presence of both level attraction/repulsion by adjusting the system's parameters. Moreover, we evidence the topological nature of the EP by dynamically encircling it in the phase-current parameter space, leading to a switch of the eigenstates. Our study introduces a new method for exploring non-Hermitian physics in spintronic systems at room temperature.

cond-mat.mes-hall↗

arXiv2024

Probing nonlinear spin dynamics in canted easy-plane antiferromagnets using spin-rectification effects

We investigate spin-rectification phenomena in canted antiferromagnets, closely connected to the family of altermagnetic materials. Our results show that excitation efficiency is significantly enhanced by the Dzyaloshinskii-Moriya interaction. Antiferromagnetic dynamics can be detected through spin-Hall magnetoresistance and bolometric effects, with an efficiency reaching up to mV/W. The rectified voltage shape is influenced by both the symmetry of the exciting torques, detection mechanisms (continuous spin-pumping and spin-Hall magnetoresistance), and the antiferromagnetic crystalline axis. Under high pumping power, we observe a saturation effect related to Suhl-like spin-wave instabilities and a nonlinear redshift of the antiferromagnetic resonance. These findings open new avenues for studying nonlinear dynamics in antiferromagnetic and altermagnetic spintronic devices.

cond-mat.mes-hall↗

arXiv2023

Quantifying the large contribution from orbital Rashba effect to the effective damping-like torque on magnetization

The generation of large spin currents, and the associated spin torques, which are at the heart of modern spintronics, have long been achieved by charge-to-spin conversion mechanisms, i.e. the spin Hall effect and/or the Rashba effect, intrinsically linked to a strong spin-orbit coupling. Recently, a novel path has been predicted and observed for achieving significant current-induced torques originating from light elements, hence possessing a weak spin-orbit interaction. These findings point out to the potential involvement of the orbital counterpart of electrons, namely the orbital Hall and orbital Rashba effects. In this study, we aim at quantifying these orbital-related contributions to the effective torques acting on a thin Co layer in different systems. First, in Pt|Co|Cu|AlOx stacking, we demonstrate a comparable torque strength coming from the conversion due to the orbital Rashba effect at the Cu|AlOx interface and the one from the effective spin Hall effect in bottom Pt|Co system. Secondly, in order to amplify the orbital-to-spin conversion, we investigate the impact of an intermediate Pt layer in Co|Pt|Cu|CuOx. From the Pt thickness dependence of the effective torques determined by harmonic Hall measurements complemented by spin Hall magneto-resistance and THz spectroscopy experiments, we demonstrate that a large orbital Rashba effect is present at the Cu|CuOx interface, leading to a twofold enhancement of the net torques on Co for the optimal Pt thickness. Our findings not only demonstrate the crucial role that orbital currents can play in low-dimensional systems with weak spin-orbit coupling, but also reveal that they enable more energy efficient manipulation of magnetization in spintronic devices.

cond-mat.mtrl-sci↗

arXiv2023

X-ray holography of skyrmionic cocoons in aperiodic magnetic multilayers

The development and characterization of three-dimensional (3D) topological magnetic textures has become an important topic in modern magnetism both for fundamental and technological perspectives. Among the novel 3D spin textures, skyrmionic cocoons have been successfully stabilized in magnetic multilayers having a variable thickness of the ferromagnet in the vertical direction of the stack. These ellipsoidal 3D magnetic textures remain vertically confined in a fraction of the total thickness while coexisting with fully columnar skyrmions. Here, we use X-ray holography with about 15 nm lateral resolution to investigate how their properties depend on the field and temperature. We observe circular objects with different amplitude of contrast which evidences the presence of different 3D objects located in various vertical parts of the multilayer. Moreover, we witness during out-of-plane cycling an attractive interaction between cocoons located at various heights, mainly due to the stray field, which impacts their horizontal positioning. The X-ray holography measurements also allow to determine the size of the cocoons at remanence which, at room temperature, possess diameter close to 100 nm in average. Combining this transmission technique with magnetic force microscopy and micromagnetic simulations gives a precise insight into the 3D distribution of the magnetization which demonstrate the 3D nature of skyrmionic cocoons.

cond-mat.mes-hall↗

arXiv2023

Antiferromagnetic magnon spintronic based on non-reciprocal and non-degenerated ultra-fast spin-waves in the canted antiferromagnet {\alpha}-Fe2O3

Spin-waves in antiferromagnets hold the prospects for the development of faster, less power-hungry electronics, as well as promising physics based on spin-superfluids and coherent magnon-condensates. For both these perspectives, addressing electrically coherent antiferromagnetic spin-waves is of importance, a prerequisite that has so far been elusive, because unlike ferromagnets,antiferromagnets couple weakly to radiofrequency fields. Here, we demonstrate the detection of ultra-fast non-reciprocal spin-waves in the dipolar-exchange regime of a canted antiferromagnet using both inductive and spintronic transducers. Using time-of-flight spin-wave spectroscopy on hematite ({\alpha}-Fe2O3), we find that the magnon wave packets can propagate as fast as 20 km/s for reciprocal bulk spin-wave modes and up to 6 km/s for surface-spin waves propagating parallel to the antiferromagnetic Neel vector. We finally achieve efficient electrical detection of non-reciprocal spin-wave transport using non-local inverse spin-Hall effects. The electrical detection of coherent non-reciprocal antiferromagnetic spin waves paves the way for the development of antiferromagnetic and altermagnet-based magnonic devices.

cond-mat.mes-hall↗

arXiv2022

Large interfacial Rashba interaction and giant spin-orbit torques in atomically thin metallic heterostructures

The ability of spin-orbit interactions to convert charge current into spin current, most often in the bulk of heavy metal thin films, has been the hallmark of spintronics in the last decade. In this study, we demonstrate how the insertion of light metal element interface profoundly affects both the nature of spin-orbit torque and its efficiency in terms of damping-like ($H_{\text{DL}}$) and field-like ($H_{\text{FL}}$) effective fields in ultrathin Co ferromagnet. Indeed, we measure unexpectedly large $H_{\text{FL}}$/$H_{\text{DL}}$ ratio ($\sim$2.5) upon inserting a 1.4 nm thin Al layer in Pt|Co|Al|Pt as compared to a similar stacking including Cu instead of Al. From our modelling, these results strongly evidence the presence of large Rashba interaction at Co|Al interface producing a giant $H_{\text{FL}}$, which was not expected from a metallic interface. The occurrence of such enhanced torques from an interfacial origin is further validated by demonstrating current-induced magnetization reversal showing a significant decrease of the critical current for switching.

cond-mat.mes-hall↗

arXiv2021

Evidence for spin current driven Bose-Einstein condensation of magnons

The quanta of magnetic excitations - magnons - are known for their unique ability to undergo Bose-Einstein condensation at room temperature. This fascinating phenomenon reveals itself as a spontaneous formation of a macroscopic coherent state under the influence of incoherent stimuli. Spin currents have been predicted to offer electronic control of magnon Bose-Einstein condensates, but this phenomenon has not been experimentally evidenced up to now. Here we experimentally show that current-driven Bose-Einstein condensation can be achieved in nanometer-thick films of magnetic insulators with tailored dynamic magnetic nonlinearities and minimized magnon-magnon interactions. We demonstrate that, above a certain threshold, magnons injected by the spin current overpopulate the lowest-energy level forming a highly coherent spatially extended state. By accessing magnons with essentially different energies, we quantify the chemical potential of the driven magnon gas and show that, at the critical current, it reaches the energy of the lowest magnon level. Our results pave the way for implementation of integrated microscopic quantum magnonic and spintronic devices.

cond-mat.mes-hall↗

arXiv2021

Dispersionless propagation of ultra-short spin-wave pulses in ultrathin yttrium iron garnet waveguides

We study experimentally the propagation of nanosecond spin-wave pulses in microscopic waveguides made of nanometer-thick yttrium iron garnet films. For these studies, we use micro-focus Brillouin light scattering spectroscopy, which provides the possibility to observe propagation of the pulses with high spatial and temporal resolution. We show that, for most spin-wave frequencies, dispersion leads to broadening of the pulse by several times at propagation distances of 10 micrometers. However, for certain frequency interval, the dispersion broadening is suppressed almost completely resulting in a dispersionless pulse propagation. We show that the formation of the dispersion-free region is caused by the competing effects of the dipolar and the exchange interaction, which can be controlled by the variation of the waveguide geometry. These conclusions are supported by micromagnetic simulations and analytical calculations. Our findings provide a simple solution for the implementation of high-speed magnonic systems that require undisturbed propagation of short information-carrying spin-wave pulses.

cond-mat.mes-hall↗

arXiv2020

Spin-orbit-torque magnonics

The field of magnonics, which utilizes propagating spin waves for nano-scale transmission and processing of information, has been significantly advanced by the advent of the spin-orbit torque. The latter phenomenon can allow one to overcome two main drawbacks of magnonic devices - low energy efficiency of conversion of electrical signals into spin wave signals, and fast spatial decay of spin waves in thin-film waveguiding structures. At first glance, the excitation and amplification of spin waves by spin-orbit torques can seem to be straightforward. Recent research indicates, however, that the lack of the mode-selectivity in the interaction of spin currents with dynamic magnetic modes and the onset of dynamic nonlinear phenomena represent significant obstacles. Here, we discuss the possible route to overcoming these limitations, based on the suppression of nonlinear spin-wave interactions in magnetic systems with perpendicular magnetic anisotropy. We show that this approach enables efficient excitation of coherent magnetization dynamics and propagating spin waves in extended spatial regions, and is expected to enable practical implementation of complete compensation of spin-wave propagation losses.

cond-mat.mes-hall↗

arXiv2020

The 2020 Skyrmionics Roadmap

The notion of non-trivial topological winding in condensed matter systems represents a major area of present-day theoretical and experimental research. Magnetic materials offer a versatile platform that is particularly amenable for the exploration of topological spin solitons in real space such as skyrmions. First identified in non-centrosymmetric bulk materials, the rapidly growing zoology of materials systems hosting skyrmions and related topological spin solitons includes bulk compounds, surfaces, thin films, heterostructures, nano-wires and nano-dots. This underscores an exceptional potential for major breakthroughs ranging from fundamental questions to applications as driven by an interdisciplinary exchange of ideas between areas in magnetism which traditionally have been pursued rather independently. The skyrmionics roadmap provides a review of the present state of the art and the wide range of research directions and strategies currently under way. These are, for instance, motivated by the identification of the fundamental structural properties of skyrmions and related textures, processes of nucleation and annihilation in the presence of non-trivial topological winding, an exceptionally efficient coupling to spin currents generating spin transfer torques at tiny current densities, as well as the capability to purpose-design broad-band spin dynamic and logic devices.

cond-mat.str-el↗

arXiv2020

Tailored flux pinning in superconductor/ferromagnet multilayers with engineered magnetic domain morphology from stripes to skyrmions

Superconductor/Ferromagnet (S/F) hybrid systems show interesting magneto-transport behaviors that result from the transfer of properties between both constituents. For instance, magnetic memory can be transferred from the F into the S through the pinning of superconducting vortices by the ferromagnetic textures. The ability to tailor this type of induced behavior is important to broaden its range of applications. Here we show that engineering the F magnetization reversal allows tuning the strength of the vortex pinning (and memory) effects, as well as the field range in which they appear. This is done by using magnetic multilayers in which Co thin films are combined with different heavy metals (Ru, Ir, Pt). By choosing the materials, thicknesses, and stacking order of the layers, we can design the characteristic domain size and morphology, from out-of-plane magnetized stripe domains to much smaller magnetic skyrmions. These changes strongly affect the magneto-transport properties. The underlying mechanisms are identified by comparing the experimental results to a magnetic pinning model.

cond-mat.supr-con↗

arXiv2019

Temporal pattern recognition with delayed feedback spin-torque nano-oscillators

The recent demonstration of neuromorphic computing with spin-torque nano-oscillators has opened a path to energy efficient data processing. The success of this demonstration hinged on the intrinsic short-term memory of the oscillators. In this study, we extend the memory of the spin-torque nano-oscillators through time-delayed feedback. We leverage this extrinsic memory to increase the efficiency of solving pattern recognition tasks that require memory to discriminate different inputs. The large tunability of these non-linear oscillators allows us to control and optimize the delayed feedback memory using different operating conditions of applied current and magnetic field.

physics.app-ph↗

arXiv2019

Analog and digital phase modulation of spin torque nano-oscillators

Spin torque nano-oscillators (STNO) are nanoscale devices with wide band frequency tunability. Their multifunctional RF properties are well suited to define novel schemes for wireless communications that use basic protocols for data transmission such as amplitude, frequency and phase shift keying (ASK, FSK, PSK). In contrast to ASK and FSK, implementation of PSK is more challenging for STNOs because of their relatively high phase noise. Here we introduce a special PSK technique by combining their modulation and injection locking functionality. The concept is validated using magnetic tunnel junction based vortex STNOs for injection locking at 2f and f/2 showing phase shifts up to 2.1rad and data transmission rates up to 4Mbit/s. Quadrature phase shift keying and analog phase modulation are also implemented, where the latter is employed for voice transmission over a distance of 10 meters. This demonstrates that STNO phase noise and output power meet the requested performances for operation in existing communication schemes.

physics.app-ph↗