arXiv subjects

V. D. Grigorieva

Publications and source records attributed to V. D. Grigorieva.

At least 19 recordsLinked to original sources

arXiv2026

A study of neutrinoless double electron capture in $^{40}$Ca from the AMoRE experiment

The search for neutrinoless double electron capture ($0ν\mathrm{2EC}$) provides a sensitive probe of lepton-number violation and the Majorana nature of neutrinos. We investigate the $0ν\mathrm{2EC}$ decay of $^{40}$Ca using cryogenic detectors equipped with metallic magnetic calorimeters in the AMoRE-I experiment. The analysis is based on a physics dataset corresponding to a total exposure of 7.32 kg$\cdot$yr from thirteen $^{40}$Ca$^{100}$MoO$_4$ crystals. No significant excess is observed, and a lower limit on the half-life is obtained as $T^{0ν}_{1/2} > 1.7 \times 10^{22}$ yr at 90$\%$ confidence level. An improved sensitivity is expected for the upcoming AMoRE-II experiment. These results demonstrate the potential of CaMoO$_4$ detectors to explore rare decay processes beyond the primary $^{100}$Mo $0νββ$ search program.

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arXiv2025

Characterization of the Li$_2$WO$_4$ crystal as a cryogenic scintillating calorimeter

A wide range of scintillating bolometers is under investigation for applications in the search for rare events and processes beyond the Standard Model. In this work, we report the first measurement of a natural, non-molybdenum-doped, lithium tungstate (LWO) crystal operated underground as a scintillating cryogenic calorimeter. The detector achieved a baseline energy resolution of 0.5 keV RMS with a low-energy threshold of about 1.5 keV. The simultaneous readout of heat and light enabled particle identification, revealing a clear separation between $β/γ$, $α$, and nuclear recoil populations above 300 keV, with a light-yield-based particle discrimination better than $6σ$. These results, fully comparable with those achieved with other compounds in the field, demonstrate that LWO is a promising candidate for rare-event searches. In particular, the combination of excellent radio-purity (with U/Th levels below 0.5 mBq/kg) and sensitivity to neutron interactions via the $^6$Li(n,$α$)$^3$H reaction makes this material an attractive option for next-generation experiments on dark matter, coherent elastic neutrino-nucleus scattering, and spin-dependent interactions.

physics.ins-det↗

arXiv2025

Improved limit on neutrinoless double beta decay of $^{100}$Mo from AMoRE-I

AMoRE searches for the signature of neutrinoless double beta decay of $^{100}$Mo with a 100 kg sample of enriched $^{100}$Mo. Scintillating molybdate crystals coupled with a metallic magnetic calorimeter operate at milli-Kelvin temperatures to measure the energy of electrons emitted in the decay. As a demonstration of the full-scale AMoRE, we conducted AMoRE-I, a pre-experiment with 18 molybdate crystals, at the Yangyang Underground Laboratory for over two years. The exposure was 8.02 kg$\cdot$year (or 3.89 kg$_{\mathrm{^{100}Mo}}\cdot$year) and the total background rate near the Q-value was 0.025 $\pm$ 0.002 counts/keV/kg/year. We observed no indication of $0νββ$ decay and report a new lower limit of the half-life of $^{100}$Mo $0νββ$ decay as $ T^{0ν}_{1/2}>2.9\times10^{24}~\mathrm{yr}$ at 90\% confidence level. The effective Majorana mass limit range is $m_{ββ}<$(210--610) meV using nuclear matrix elements estimated in the framework of different models, including the recent shell model calculations.

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arXiv2025

Development of MMC-based lithium molybdate cryogenic calorimeters for AMoRE-II

The AMoRE collaboration searches for neutrinoless double beta decay of $^{100}$Mo using molybdate scintillating crystals via low temperature thermal calorimetric detection. The early phases of the experiment, AMoRE-pilot and AMoRE-I, have demonstrated competitive discovery potential. Presently, the AMoRE-II experiment, featuring a large detector array with about 90 kg of $^{100}$Mo isotope, is under construction. This paper discusses the baseline design and characterization of the lithium molybdate cryogenic calorimeters to be used in the AMoRE-II detector modules. The results from prototype setups that incorporate new housing structures and two different crystal masses (316 g and 517 - 521 g), operated at 10 mK temperature, show energy resolutions (FWHM) of 7.55 - 8.82 keV at the 2.615 MeV $^{208}$Tl $γ$ line, and effective light detection of 0.79 - 0.96 keV/MeV. The simultaneous heat and light detection enables clear separation of alpha particles with a discrimination power of 12.37 - 19.50 at the energy region around $^6$Li(n, $α$)$^3$H with Q-value = 4.785 MeV. Promising detector performances were demonstrated at temperatures as high as 30 mK, which relaxes the temperature constraints for operating the large AMoRE-II array.

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arXiv2024

Projected background and sensitivity of AMoRE-II

AMoRE-II aims to search for neutrinoless double beta decay with an array of 423 Li$_2$$^{100}$MoO$_4$ crystals operating in the cryogenic system as the main phase of the Advanced Molybdenum-based Rare process Experiment (AMoRE). AMoRE has been planned to operate in three phases: AMoRE-pilot, AMoRE-I, and AMoRE-II. AMoRE-II is currently being installed at the Yemi Underground Laboratory, located approximately 1000 meters deep in Jeongseon, Korea. The goal of AMoRE-II is to reach up to $T^{0νββ}_{1/2}$ $\sim$ 6 $\times$ 10$^{26}$ years, corresponding to an effective Majorana mass of 15 - 29 meV, covering all the inverted mass hierarchy regions. To achieve this, the background level of the experimental configurations and possible background sources of gamma and beta events should be well understood. We have intensively performed Monte Carlo simulations using the GEANT4 toolkit in all the experimental configurations with potential sources. We report the estimated background level that meets the 10$^{-4}$counts/(keV$\cdot$kg$\cdot$yr) requirement for AMoRE-II in the region of interest (ROI) and show the projected half-life sensitivity based on the simulation study.

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arXiv2024

Searching for Beyond the Standard Model physics using the improved description of $^{100}$Mo $2νββ$ decay spectral shape with CUPID-Mo

The current experiments searching for neutrinoless double-$β$ ($0νββ$) decay also collect large statistics of Standard Model allowed two-neutrino double-$β$ ($2νββ$) decay events. These can be used to search for Beyond Standard Model (BSM) physics via $2νββ$ decay spectral distortions. $^{100}$Mo has a natural advantage due to its relatively short half-life, allowing higher $2νββ$ decay statistics at equal exposures compared to the other isotopes. We demonstrate the potential of the dual read-out bolometric technique exploiting a $^{100}$Mo exposure of 1.47 kg $\times$ y, acquired in the CUPID-Mo experiment at the Modane underground laboratory (France). We set limits on $0νββ$ decays with the emission of one or more Majorons, on $2νββ$ decay with Lorentz violation, and $2νββ$ decay with a sterile neutrino emission. In this analysis, we investigate the systematic uncertainty induced by modeling the $2νββ$ decay spectral shape parameterized through an improved model, an effect never considered before. This work motivates searches for BSM processes in the upcoming CUPID experiment, which will collect the largest amount of $2νββ$ decay events among the next-generation experiments.

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arXiv2024

Background study of the AMoRE-pilot experiment

We report a study on the background of the Advanced Molybdenum-Based Rare process Experiment (AMoRE), a search for neutrinoless double beta decay (\znbb) of $^{100}$Mo. The pilot stage of the experiment was conducted using $\sim$1.9 kg of \CAMOO~ crystals at the Yangyang Underground Laboratory, South Korea, from 2015 to 2018. We compared the measured $β/γ$ energy spectra in three experimental configurations with the results of Monte Carlo simulations and identified the background sources in each configuration. We replaced several detector components and enhanced the neutron shielding to lower the background level between configurations. A limit on the half-life of $0νββ$ decay of $^{100}$Mo was found at $T_{1/2}^{0ν} \ge 3.0\times 10^{23}$ years at 90\% confidence level, based on the measured background and its modeling. Further reduction of the background rate in the AMoRE-I and AMoRE-II are discussed.

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arXiv2023

Measurement of the $2νββ$ decay rate and spectral shape of $^{100}$Mo from the CUPID-Mo experiment

Neutrinoless double beta decay ($0νββ$) is a yet unobserved nuclear process which would demonstrate Lepton Number violation, a clear evidence of beyond Standard Model physics. The process two neutrino double beta decay ($2νββ)$ is allowed by the Standard Model and has been measured in numerous experiments. In this letter, we report a measurement of $2νββ$ decay half-life of $^{100}$Mo to the ground state of $^{100}$Ru of $(7.07~\pm~0.02~\text{(stat.)}~\pm~0.11~\text{(syst.)})~\times~10^{18}$~yr by the CUPID-Mo experiment. With a relative precision of $\pm~1.6$ \% this is the most precise measurement to date of a $2νββ$ decay rate in $^{100}$Mo. In addition, we constrain higher-order corrections to the spectral shape which provides complementary nuclear structure information. We report a novel measurement of the shape factor $ξ_{3,1}=0.45~\pm 0.03~\text{(stat.)} \ \pm 0.05 \ \text{(syst.)}$, which is compared to theoretical predictions for different nuclear models. We also extract the first value for the effective axial vector coupling constant obtained from a spectral shape study of $2νββ$ decay.

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arXiv2023

The background model of the CUPID-Mo $0νββ$ experiment

CUPID-Mo, located in the Laboratoire Souterrain de Modane (France), was a demonstrator for the next generation $0νββ$ decay experiment, CUPID. It consisted of an array of 20 enriched Li$_{2}$$ ^{100}$MoO$_4$ bolometers and 20 Ge light detectors and has demonstrated that the technology of scintillating bolometers with particle identification capabilities is mature. Furthermore, CUPID-Mo can inform and validate the background prediction for CUPID. In this paper, we present a detailed model of the CUPID-Mo backgrounds. This model is able to describe well the features of the experimental data and enables studies of the $2νββ$ decay and other processes with high precision. We also measure the radio-purity of the Li$_{2}$$^{100}$MoO$_4$ crystals which are found to be sufficient for the CUPID goals. Finally, we also obtain a background index in the region of interest of 3.7$^{+0.9}_{-0.8}$(stat)$^{+1.5}_{-0.7}$(syst)$\times10^{-3}$counts/$Δ$E$_{FWHM}$/mol$_{iso}$/yr, the lowest in a bolometric $0νββ$ decay experiment.

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arXiv2023

Li$_2$$^{100\textrm{depl}}$MoO$_4$ Scintillating Bolometers for Rare-Event Search Experiments

We report on the development of scintillating bolometers based on lithium molybdate crystals containing molybdenum depleted in the double-$β$ active isotope $^{100}$Mo (Li$_2$$^{100\textrm{depl}}$MoO$_4$). We used two Li$_2$$^{100\textrm{depl}}$MoO$_4$ cubic samples, 45 mm side and 0.28 kg each, produced following purification and crystallization protocols developed for double-$β$ search experiments with $^{100}$Mo-enriched Li$_2$MoO$_4$ crystals. Bolometric Ge detectors were utilized to register scintillation photons emitted by the Li$_2$$^{100\textrm{depl}}$MoO$_4$ crystal scintillators. The measurements were performed in the CROSS cryogenic set-up at the Canfranc underground laboratory (Spain). We observed that the Li$_2$$^{100\textrm{depl}}$MoO$_4$ scintillating bolometers are characterized by excellent spectrometric performance ($\sim$3--6 keV FWHM at 0.24--2.6 MeV $γ$'s), moderate scintillation signal ($\sim$0.3--0.6 keV/MeV depending on light collection conditions) and high radiopurity ($^{228}$Th and $^{226}$Ra activities are below a few $μ$Bq/kg), comparable to the best reported results of low-temperature detectors based on Li$_2$MoO$_4$ with natural or $^{100}$Mo-enriched molybdenum content. Prospects of Li$_2$$^{100\textrm{depl}}$MoO$_4$ bolometers for use in rare-event search experiments are briefly discussed.

physics.ins-det↗

arXiv2022

Final results on the $0νββ$ decay half-life limit of $^{100}$Mo from the CUPID-Mo experiment

The CUPID-Mo experiment to search for 0$νββ$ decay in $^{100}$Mo has been recently completed after about 1.5 years of operation at Laboratoire Souterrain de Modane (France). It served as a demonstrator for CUPID, a next generation 0$νββ$ decay experiment. CUPID-Mo was comprised of 20 enriched Li$_2$$^{100}$MoO$_4$ scintillating calorimeters, each with a mass of $\sim$ 0.2 kg, operated at $\sim$20 mK. We present here the final analysis with the full exposure of CUPID-Mo ($^{100}$Mo exposure of 1.47 kg$\times$yr) used to search for lepton number violation via 0$νββ$ decay. We report on various analysis improvements since the previous result on a subset of data, reprocessing all data with these new techniques. We observe zero events in the region of interest and set a new limit on the $^{100}$Mo 0$νββ$ decay half-life of $T^{0ν}_{1/2} > 1.8 \times 10^{24}$ year (stat.+syst.) at 90% CI. Under the light Majorana neutrino exchange mechanism this corresponds to an effective Majorana neutrino mass of $\left < (0.28$--$0.49)$ eV, dependent upon the nuclear matrix element utilized.

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arXiv2022

New measurement of double beta decays of $^{100}$Mo to excited states of $^{100}$Ru with the CUPID-Mo experiment

The CUPID-Mo experiment, located at Laboratoire Souterrain de Modane (France), was a demonstrator experiment for CUPID. It consisted of an array of 20 Li$_2^{100}$MoO$_4$ (LMO) calorimeters each equipped with a Ge light detector (LD) for particle identification. In this work, we present the result of a search for two-neutrino and neutrinoless double beta decays of $^{100}$Mo to the first 0$^+$ and $2^+$ excited states of $^{100}$Ru using the full CUPID-Mo exposure (2.71 kg$\times$yr of LMO). We measure the half-life of $2νββ$ decay to the $0^{+}_1$ state as $T_{1/2}^{2ν\rightarrow 0_1^+}=7.5\pm 0.8 \ \text{(stat.)} \ ^{+ 0.4}_{-0.3} \ \text{(syst.)} )\times 10^{20} \ \mathrm{yr}$. The bolometric technique enables measurement of the electron energies as well as the gamma rays from nuclear de-excitation and this allows us to set new limits on the two-neutrino decay to the $2_1^+$ state of $T^{2ν\rightarrow 2_1^+}_{1/2}>4.4\times 10^{21} \ \mathrm{yr} \ \text{(90 % c.i.)}$ and on the neutrinoless modes of $T_{1/2}^{0ν\rightarrow 2_1^+}>2.1\times10^{23} \ \mathrm{yr}\ \text{(90 % c.i.)}$, $T_{1/2}^{0ν\rightarrow 0_1^+}>1.2\times10^{23} \ \mathrm{yr}\ \text{(90 % c.i.)}$. Information on the electrons spectral shape is obtained which allows us to make the first comparison of the single state (SSD) and higher state (HSD) $2νββ$ decay models for the $0_1^+$ excited state of $^{100}$Ru.

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arXiv2021

New Limit for Neutrinoless Double-Beta Decay of $^{100}$Mo from the CUPID-Mo Experiment

The CUPID-Mo experiment at the Laboratoire Souterrain de Modane (France) is a demonstrator for CUPID, the next-generation ton-scale cryogenic $0νββ$ experiment. It consists of a 4.2 kg array of 20 enriched Li$_{2}$$^{100}$MoO$_4$ scintillating bolometers to search for the lepton number violating process of $0νββ$ decay in $^{100}$Mo. With more than one year of operation (2.16 kg$\times$yr of physics data), no event in the region of interest and hence no evidence for $0νββ$ is observed. We report a new limit on the half-life of $0νββ$ decay in $^{100}$Mo of $T_{1/2} > 1.5 \times 10^{24}\,$yr at 90 % C.I. The limit corresponds to an effective Majorana neutrino mass $\langle m_{ββ} \rangle$ $<$ (0.31--0.54)$\,$eV, dependent on the nuclear matrix element in the light Majorana neutrino exchange interpretation.

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arXiv2021

Pulse Shape Discrimination in CUPID-Mo using Principal Component Analysis

CUPID-Mo is a cryogenic detector array designed to search for neutrinoless double-beta decay ($0νββ$) of $^{100}$Mo. It uses 20 scintillating $^{100}$Mo-enriched Li$_2$MoO$_4$ bolometers instrumented with Ge light detectors to perform active suppression of $α$ backgrounds, drastically reducing the expected background in the $0νββ$ signal region. As a result, pileup events and small detector instabilities that mimic normal signals become non-negligible potential backgrounds. These types of events can in principle be eliminated based on their signal shapes, which are different from those of regular bolometric pulses. We show that a purely data-driven principal component analysis based approach is able to filter out these anomalous events, without the aid of detector response simulations.

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arXiv2019

Precise measurement of $2νββ$ decay of $^{100}$Mo with the CUPID-Mo detection technology

We report the measurement of the two-neutrino double-beta ($2νββ$) decay of $^{100}$Mo to the ground state of $^{100}$Ru using lithium molybdate (\crystal) scintillating bolometers. The detectors were developed for the CUPID-Mo program and operated at the EDELWEISS-III low background facility in the Modane underground laboratory. From a total exposure of $42.235$ kg$\times$d, the half-life of $^{100}$Mo is determined to be $T_{1/2}^{2ν}=[7.12^{+0.18}_{-0.14}\,\mathrm{(stat.)}\pm0.10\,\mathrm{(syst.)}]\times10^{18}$ years. This is the most accurate determination of the $2νββ$ half-life of $^{100}$Mo to date. We also confirm, with the statistical significance of $>3σ$, that the single-state dominance model of the $2νββ$ decay of $^{100}$Mo is favored over the high-state dominance model.

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arXiv2019

Na-based crystal scintillators for next-generation rare event searches

The growing interest in clarifying the controversial situation in the Dark Matter sector has driven the experimental efforts towards new ways to investigate the long-standing DAMA/LIBRA result. Among them, low-temperature calorimeters based on Na-containing scintillating crystals offer the possibility to clarify the nature of the measured signal via particle identification. Here we report the first measurement of Na-containing crystals, based on material different from NaI, i.e. Na$_2$Mo$_2$O$_7$ and Na$_2$W$_2$O$_7$, pointing out their excellent performance in term of energy resolution, light yield, and particle identification.

physics.ins-det↗

arXiv2019

First data from the CUPID-Mo neutrinoless double beta decay experiment

The CUPID-Mo experiment is searching for neutrinoless double beta decay in $^{100}$Mo, evaluating the technology of cryogenic scintillating Li$_{2}^{100}$MoO$_4$ detectors for CUPID (CUORE Upgrade with Particle ID). CUPID-Mo detectors feature background suppression using a dual-readout scheme with Li$_{2}$MoO$_4$ crystals complemented by Ge bolometers for light detection. The detection of both heat and scintillation light signals allows the efficient discrimination of $α$ from $γ$&$β$ events. In this proceedings, we discuss results from the first 2 months of data taking in spring 2019. In addition to an excellent bolometric performance of 6.7$\,$keV (FWHM) at 2615$\,$keV and an $α$ separation of better than 99.9\% for all detectors, we report on bulk radiopurity for Th and U. Finally, we interpret the accumulated physics data in terms of a limit of $T_{1/2}^{0ν}\,> 3\times10^{23}\,$yr for $^{100}$Mo and discuss the sensitivity of CUPID-Mo until the expected end of physics data taking in early 2020.

hep-ex↗

arXiv2019

The CUPID-Mo experiment for neutrinoless double-beta decay: performance and prospects

CUPID-Mo is a bolometric experiment to search for neutrinoless double-beta decay ($0νββ$) of $^{100}$Mo. In this article, we detail the CUPID-Mo detector concept, assembly, installation in the underground laboratory in Modane in 2018, and provide results from the first datasets. The demonstrator consists of an array of 20 scintillating bolometers comprised of $^{100}$Mo-enriched 0.2 kg Li$_2$MoO$_4$ crystals. The detectors are complemented by 20 thin cryogenic Ge bolometers acting as light detectors to distinguish $α$ from $γ$/$β$ events by the detection of both heat and scintillation light signals. We observe good detector uniformity, facilitating the operation of a large detector array as well as excellent energy resolution of 5.3 keV (6.5 keV) FWHM at 2615 keV, in calibration (physics) data. Based on the observed energy resolutions and light yields a separation of $α$ particles at much better than 99.9\% with equally high acceptance for $γ$/$β$ events is expected for events in the region of interest for $^{100}$Mo $0νββ$. We present limits on the crystals' radiopurity ($\leq$3 $μ$Bq/kg of $^{226}$Ra and $\leq$2 $μ$Bq/kg of $^{232}$Th). Based on these initial results we also discuss a sensitivity study for the science reach of the CUPID-Mo experiment, in particular, the ability to set the most stringent half-life limit on the $^{100}$Mo $0νββ$ decay after half a year of livetime. The achieved results show that CUPID-Mo is a successful demonstrator of the technology - developed in the framework of the LUMINEU project - selected for the CUPID experiment, a proposed follow-up of CUORE, the currently running first tonne-scale cryogenic $0νββ$ experiment.

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