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V. Dziom

Publications and source records attributed to V. Dziom.

17 recordsLinked to original sources

Universal transparency and fine band structure near the Dirac point in HgTe quantum wells

Spin-orbit coupling in thin HgTe quantum wells results in a relativistic-like electron band structure, making it a versatile solid state platform to observe and control non-trivial electrodynamic phenomena. Here we report an observation of universal terahertz (THz) transparency determined by fine-structure constant $\alpha \approx 1/137$ in 6.5 nm-thick HgTe layer, close to the critical thickness separating phases with topologically different electronic band structure. Using THz spectroscopy in magnetic field we obtain direct evidence of asymmetric spin splitting of the Dirac cone. This particle-hole asymmetry facilitates optical control of edge spin currents in the quantum wells.

cond-mat.mes-hall

Optical Shubnikov - de Haas oscillations in 2D electron systems

We report on dynamic Shubnikov - de Haas (SdH) oscillations that are measured in the optical response, sub - terahertz transmittance of two-dimensional systems, and reveal two distinct types of oscillation nodes: "universal" nodes at integer ratios of radiation and cyclotron frequencies and "tunable" nodes at positions sensitive to all parameters of the structure. The nodes in both real and imaginary parts of the measured complex transmittance are analyzed using a dynamic version of the static Lifshitz-Kosevich formula. These results demonstrate that the node structure of the dynamic SdH oscillations provides an all-optical access to quantization- and interaction-induced renormalization effects, in addition to parameters one can obtain from the static SdH oscillations.

cond-mat.mes-hall

Band structure of a HgTe-based three-dimensional topological insulator

From the analysis of the cyclotron resonance, we experimentally obtain the band structure of the three-dimensional topological insulator based on a HgTe thin film. Top gating was used to shift the Fermi level in the film, allowing us to detect separate resonance modes corresponding to the surface states at two opposite film interfaces, the bulk conduction band, and the valence band. The experimental band structure agrees reasonably well with the predictions of the $\mathbf{k\cdot p}$ model. Due to the strong hybridization of the surface and bulk bands, the dispersion of the surface states is close to parabolic in the broad range of the electron energies.

cond-mat.mes-hall

Sign change of polarization rotation under either time or space inversion in magnetoelectric YbAl3(BO3)4

Materials with optical activity can rotate the polarization plane of transmitted light. The most typical example is the natural optical activity, which has the symmetry property of changing sign after space inversion but being invariant to time inversion. Faraday rotation exhibits the opposite: it is invariant to space inversion but changes sign after time reversal. Here, we demonstrate that in a magnetoelectric material, another type of polarization rotation is possible. This effect is investigated in magnetoelectric YbAl3(BO3)4 under the viewpoint of time and space inversion symmetry arguments. We observe the sign change of the rotation sense under either time or space reversal. This investigation proves that the polarization rotation in YbAl3(BO3)4 must be classified as gyrotropic birefringence, which has been discussed within the idea of time-reversal breaking in underdoped cuprates. The diagonal terms in the magnetoelectric susceptibility are responsible for the observed signal of gyrotropic birefringence. Further analysis of the experimental spectra reveals a substantial contribution of the natural optical activity to the polarization rotation. We also demonstrate that the observed activity originates from the magnetoelectric susceptibility.

cond-mat.mtrl-sci

Superradiant and transport lifetimes of the cyclotron resonance in the topological insulator HgTe

We investigate the superradiance effects in three-dimensional topological insulator HgTe with conducting surface states. We demonstrate that the superradiance can be explained using the classical electrodynamic approach. Experiments using the continuous-wave spectroscopy allowed to separate the energy losses in the system into intrinsic and radiation losses, respectively. These results demonstrate that the superradiance effects are not sensitive to the details of the band structure of the material.

cond-mat.mes-hall

High-frequency breakdown of the integer QHE in GaAs/AlGaAs heterojunctions

The integer quantum Hall effect is a well-studied phenomenon at frequencies below about 100 Hz. The plateaus in high-frequency Hall conductivity were experimentally proven to retain up to 33 GHz, but the behavior at higher frequencies has remained largely unexplored. Using continuous wave THz spectroscopy, the complex Hall conductivity of GaAs/AlGaAs heterojunctions was studied in the range of 69-1100 GHz. Above 100 GHz, the quantum plateaus are strongly smeared out and replaced by weak quantum oscillations in the real part of the conductivity. The amplitude of the oscillations decreases with increasing frequency. Near 1 THz, the Hall conductivity does not reveal any features related to the filling of Landau levels. Similar oscillations are observed in the imaginary part as well, this effect has no analogy at zero frequency. This experimental picture is in disagreement with existing theoretical considerations of the high-frequency quantum Hall effect.

cond-mat.mes-hall

Switching of magnons by electric and magnetic fields in multiferroic borates

Electric manipulation of magnetic properties is a key problem of materials research. To fulfil the requirements of modern electronics, these processes must be shifted to high frequencies. In multiferroic materials this may be achieved by electric and magnetic control of their fundamental excitations. Here we identify magnetic vibrations in multiferroic iron-borates which are simultaneously sensitive to external electric and magnetic fields. Nearly 100% modulation of the terahertz radiation in an external field is demonstrated for SmFe3(BO3)4. High sensitivity can be explained by a modification of the spin orientation which controls the excitation conditions in multiferroic borates. These experiments demonstrate the possibility to alter terahertz magnetic properties of materials independently by external electric and magnetic fields.

cond-mat.mtrl-sci

Band Structure of Two-dimensional Dirac Semimetal from Cyclotron Resonance

Knowing the band structure of materials is one of the prerequisites to understand their properties. Therefore, especially in the last decades, angle-resolved photoemission spectroscopy (ARPES) has become a highly demanded experimental tool to investigate the band structure. However, especially in thin film materials with a layered structure and several capping layers, access to the electronic structure by ARPES is limited. Therefore, several alternative methods to obtain the required information have been suggested. Here, we directly invert the results by cyclotron resonance experiments to obtain the band structure of a two-dimensional (2D) material. This procedure is applied to the mercury telluride quantum well with critical thickness which is characterized by a 2D electron gas with linear dispersion relations. The Dirac-like band structure in this material could be mapped both on the electron and on the hole side of the band diagram. In this material, purely linear dispersion of the hole-like carriers is in contrast to detectable quadratic corrections for the electrons.

cond-mat.mtrl-sci

Giant gigahertz optical activity in multiferroic ferroborate

In contrast to well studied multiferroic manganites with a spiral structure, the electric polarization in multiferroic borates is induced within collinear antiferromagnetic structure and can easily be switched by small static fields. Because of specific symmetry conditions, static and dynamic properties in borates are directly connected, which leads to giant magnetoelectric and magnetodielectric effects. Here we prove experimentally that the giant magnetodielectric effect in samarium ferroborate SmFe3(BO3)4 is of intrinsic origin and is caused by an unusually large electromagnon situated in the microwave range. This electromagnon reveals strong optical activity exceeding 120 degrees of polarization rotation in a millimeter thick sample.

cond-mat.str-el

Terahertz spectroscopy of crystal-field transitions in magnetoelectric TmAl3(BO3)4

Dynamic magnetic properties of magnetoelectric TmAl3(BO3)4 borate have been investigated by terahertz spectroscopy. Crystal field (CF) transitions within the ground multiplet 3H6 of Tm3+ ions are observed and they are identified as magnetic-dipole transitions from the ground singlet A1 to the next excited doublet E of Tm3+ ions. Unexpected fine structure of the transitions is detected at low temperatures. The new modes are assigned to local distortions of the sites with D3 symmetry by Bi3+ impurities, which resulted in the splitting of A1 -> E transition. Two types of locally distorted sites are identified and investigated. The main contribution to the static magnetic susceptibility is shown to be determined by the matrix elements of the observed magnetic transitions. We demonstrate that even in case of local distortions the symmetry of the undistorted crystal is recovered for magnetic and for quadratic magnetoelectric susceptibilities.

cond-mat.str-el

Electric field control of terahertz polarization in a multiferroic manganite with electromagnons

All-electrical control of a dynamic magnetoelectric effect is demonstrated in a classical multiferroic manganite DyMnO3, a material containing coupled antiferromagnetic and ferroelectric orders. Due to intrinsic magnetoelectric coupling with electromagnons a linearly polarized terahertz light rotates upon passing through the sample. The amplitude and the direction of the polarization rotation are defined by the orientation of ferroelectric domains and can be switched by static voltage. These experiments allow the terahertz polarization to be tuned using the dynamic magnetoelectric effect.

cond-mat.str-el

Universal Faraday rotation in HgTe wells with critical thickness

The universal value of Faraday rotation angle close to the fine structure constant is experimentally observed in thin HgTe quantum wells with thickness on the border between trivial insulating and the topologically non-trivial Dirac phases. The quantized value of the Faraday angle remains robust in the broad range of magnetic fields and gate voltages. Dynamic Hall conductivity of the hole-like carriers extracted from the analysis of the transmission data shows theoretically predicted universal value of consistent with the doubly degenerate Dirac state. On shifting the Fermi level by the gate voltage the effective sign of the charge carriers changes from positive (holes) to negative (electrons). The electron-like part of the dynamic response does not show quantum plateaus and is well described within the classical Drude model.

cond-mat.mtrl-sci

Terahertz properties of Dirac fermions in HgTe films with optical doping

Terahertz properties of mercury telluride (HgTe) films with critical thickness are presented and discussed. The density of the charge carriers is controlled using contact-free optical doping by visible light. In the magneto-optical response of HgTe the contribution of two types of carriers (electrons and holes) can be identified. The density of the electrons can be modified by light illumination by more than one order of magnitude. As the hole density is roughly illuminationindependent, the terahertz response of the illuminated samples becomes purely electronic. In some cases, light illumination may switch the qualitative electrodynamic response from hole-like to the electron-like. The cyclotron mass of the electrons could be extracted from the data and shows a square root dependence upon the charge concentration in the broad range of parameters. This can be interpreted as a clear proof of a linear dispersion relations, i.e. Dirac-type charge carriers.

cond-mat.mtrl-sci

Observation of the universal magnetoelectric effect in a 3D topological insulator

The electrodynamics of topological insulators (TIs) is described by modified Maxwell's equations, which contain additional terms that couple an electric field to a magnetization and a magnetic field to a polarization of the medium, such that the coupling coefficient is quantized in odd multiples of $e^2 / 2 h c $ per surface. Here, we report on the observation of this so-called topological magnetoelectric (TME) effect. We use monochromatic terahertz (THz) spectroscopy of TI structures equipped with a semi-transparent gate to selectively address surface states. In high external magnetic fields, we observe a universal Faraday rotation angle equal to the fine structure constant $α= e^2 / \hbar c$ when a linearly polarized THz radiation of a certain frequency passes through the two surfaces of a strained HgTe 3D TI. These experiments give insight into axion electrodynamics of TIs and may potentially be used for a metrological definition of the three basic physical constants.

cond-mat.str-el

Giant directional birefringence in multiferroic ferroborate

Many technological applications are based on electric or magnetic order of materials, for instance magnetic memory. Multiferroics are materials which exhibit electric and magnetic order simultaneously. Due to the coupling of electric and magnetic effects, these materials show a strong potential to control electricity and magnetism and, more generally, the properties and propagation of light. One of the most fascinating and counter-intuitive recent results in multiferroics is directional anisotropy, the asymmetry of light propagation with respect to the direction of propagation. The absorption in the material can be different for forward and backward propagation of light, which in extreme case may lead to complete suppression of absorption in one direction. Another remarkable effect in multiferroics is directional birefringence, i.e. different velocities of light for different directions of propagation. In this paper, we demonstrate giant directional birefringence in a multiferroic samarium ferroborate. The effect is easily observed for linear polarization of light in the range of millimeter-wavelengths, and survives down to very low frequencies. The dispersion and absorption close to the electromagnon resonance can be controlled and fully suppressed in one direction. Therefore, samarium ferroborate is a universal tool for optical control: with a magnetic field as an external parameter it allows switching between two functionalities: polarization rotation and directional anisotropy.

cond-mat.mtrl-sci

Order-disorder type critical behaviour at the magnetoelectric phase transition in multiferroic DyMnO$_3$

We present the results of detailed dielectric investigations of the relaxation dynamics in DyMnO$_3$ multiferroic manganite. Strong low-frequency relaxation process near the paraelectric-ferroelectric phase transition is observed. The high frequency mode is directly to the relaxational motion of multiferroic domain walls. We provide an experimental evidence that this relaxation mode corresponds to a chirality switching of the spin cycloid in DyMnO$_3$. We demonstrate that the relaxation dynamics in DyMnO$_3$ is typical for an order-disorder phase transition and may be understood within a simple model with a double well potential. DyMnO$_3$ follows an order-disorder transition scenario implicating that a short range cycloidal order of Mn-spins exists above $T_C$. These results suggest the interpretation of the paraelectric sinusoidal phase in manganites as a dynamical equilibrium of magnetic cycloids with opposite chiralities.

cond-mat.mtrl-sci

ESR of the quasi-two-dimensional antiferromagnet with a triangular lattice CuCrO2

Using electron-spin-resonance (ESR) technique we investigate the magnetic structure of CuCrO2, quasi-two-dimensional antiferromagnet with weakly distorted triangular lattice. Resonance frequencies and the excitation conditions in CuCrO2 at low temperatures are well described in the frame of cycloidal spin structure, defined by two susceptibilities parallel and perpendicular to the spin plane and by a biaxial crystal-field anisotropy. In agreement with the calculations, the character of the eigenmodes changes drastically at the spin-flop transition. The splitting of the observed modes can be well attributed to the resonances from different domains. The domain structure in CuCrO2 can be controlled by annealing of the sample in magnetic field.

cond-mat.str-el