arXiv subjects

V. Grinenko

Publications and source records attributed to V. Grinenko.

35 records · Page 2Linked to original sources

arXiv2017

Macroscopic phase separation of superconductivity and ferromagnetism in Sr0.5Ce0.5FBiS2-xSex revealed by muSR

The compound Sr$_{0.5}$Ce$_{0.5}$FBiS$_{2}$ belongs to the intensively studied family of layered BiS$_2$ superconductors. It attracts special attention because superconductivity at $T_{sc} = 2.8$ K was found to coexist with local-moment ferromagnetic order with a Curie temperature $T_C = 7.5$ K. Recently it was reported that upon replacing S by Se $T_C$ drops and ferromagnetism becomes of an itinerant nature (Thakur et al., Sci. Reports 6, 37527 (2016)). At the same time $T_{sc}$ increases and it was argued superconductivity coexists with itinerant ferromagnetism. Here we report a muon spin rotation and relaxation study ($μ$SR) conducted to investigate the coexistence of superconductivity and ferromagnetic order in Sr$_{0.5}$Ce$_{0.5}$FBiS$_{2-x}$Se$_x$ with $x=0.5$ and $1.0$. By inspecting the muon asymmetry function we find that both phases do not coexist on the microscopic scale, but occupy different sample volumes. For $x=0.5$ and $x=1.0$ we find a ferromagnetic volume fraction of $\sim \, 8 \%$ and $\sim \, 30 \%$ at $T=0.25$ K, well below $T_{C} = 3.4$ K and $T_C = 3.3$ K, respectively. For $x=1.0$ ($T_{sc} = 2.9$ K) the superconducting phase occupies the remaining sample volume ($\sim \, 70 \%$), as shown by transverse field experiments that probe the Gaussian damping due to the vortex lattice. We conclude ferromagnetism and superconductivity are macroscopically phase separated.

cond-mat.supr-con↗

arXiv2017

Magnetic order and spin dynamics in the helical magnetic system Fe$_3$PO$_4$O$_3$

The 3$d$-electronic spin dynamics and the magnetic order in Fe$_3$PO$_4$O$_3$ were investigated by muon spin rotation and relaxation ($μ$SR) and $^{57}$Fe Mössbauer spectroscopy. Zero-field (ZF)-$μ$SR and $^{57}$Fe Mössbauer studies confirm static long range magnetic ordering below $T_{\mathrm{N}}$ $\approx$ 164\,K. Both transverse-field (TF) and ZF-$μ$SR results evidence 100\% magnetic volume fraction in the ordered state. The ZF-$μ$SR time spectra can be best described by a Bessel function, which is consistent with the helical magnetic structure proposed by neutron scattering experiments. The Mössbauer spectra are described in detail by considering the specific angular distribution of the local hyperfine field $B_{\mathrm{hyp}}$ with respect to the local electric field gradient. The $μ$SR spin-lattice relaxation rate exhibits two peaks: One at the magnetic ordering temperature related to critical magnetic fluctuations and another peak at 35\,K signaling the presence of a secondary low energy scale in Fe$_3$PO$_4$O$_3$.

cond-mat.str-el↗

arXiv2017

Selective mass enhancement close to the quantum critical point in BaFe$_2$(As$_{1-x}$P$_x$)$_2$

A quantum critical point (QCP) is currently being conjectured for the BaFe$_2$(As$_{1-x}$P$_x$)$_2$ system at the critical value $x_{\rm c} \approx$ 0.3. In the proximity of a QCP, all thermodynamic and transport properties are expected to scale with a single characteristic energy, given by the quantum fluctuations. Such an universal behavior has not, however, been found in the superconducting upper critical field $H_{\rm c2}$. Here we report $H_{\rm c2}$-data for epitaxial thin films extracted from the electrical resistance measured in very high magnetic fields up to 67 Tesla. Using a multi-band analysis we find that $H_{\rm c2}$ is sensitive to the QCP, implying a significant charge carrier effective mass enhancement at the doping-induced QCP that is essentially band-dependent. Our results point to two qualitatively different groups of electrons in BaFe$_2$(As$_{1-x}$P$_x$)$_2$. The first one (possibly associated to hot spots or whole Fermi sheets) has a strong mass enhancement at the QCP, and the second one is insensitive to the QCP. The observed duality could also be present in many other quantum critical systems.

cond-mat.supr-con↗

arXiv2017

Superconductivity with broken time reversal symmetry in ion irradiated Ba$_{0.27}$K$_{0.73}$Fe$_2$As$_2$ single crystals

Over the last years a lot of theoretical and experimental efforts have been made to find states with broken time reversal symmetry (BTRS) in multi-band superconductors. In particular, it was theoretically proposed that in the Ba$_{1-x}$K$_{x}$Fe$_2$As$_2$ system either an $s+is$ or an $s+id$ BTRS state may exist at high doping levels in a narrow region of the phase diagram. Here we report the observation of an enhanced zero field muon spin relaxation rate below the superconducting transition temperature for a high quality crystalline sample with $x \approx$ 0.73. This indicates that indeed the time reversal symmetry is broken in superconducting Ba$_{1-x}$K$_{x}$Fe$_2$As$_2$ at this doping level.

cond-mat.supr-con↗

arXiv2017

Constraints on the total coupling strength to bosons in iron based superconductors

At present, there is still no consistent interpretation of the normal and superconducting properties of Fe-based superconductors (FeSCs). The strength of the el-el interaction and the role of correlation effects are under debate. Here, we examine several common materials and illustrate various problems and concepts that are generic for all FeSCs. Based on empirical observations and qualitative insight from density functional theory, we show that the superconducting and low-energy thermodynamic properties of the FeSCs can be described semi-quantitively within multiband Eliashberg theory. We account for an important high-energy mass renormalization phenomenologically,and in agreement with constraints provided by thermodynamic, optical, and angle-resolved photoemission data. When seen in this way, all FeSCs with $T_\mathrm{c} <$ 40~K studied so far are found to belong to an {\it intermediate} coupling regime. This finding is in contrast to the strong coupling scenarios proposed in the early period of the FeSC history.We also discuss several related issues, including the role of band shifts as measured by the positions of van Hove singularities, and the nature of a recently suggested quantum critical point in the strongly hole-doped systems AFe$_2$As$_2$ (A = K, Rb, Cs). Using high-precision full relativistic GGA-band structure calculations, we arrive at a somewhat milder mass renormalization in comparison with previous studies. From the calculated mass anisotropies of all Fermi surface sheets, only the $\varepsilon$-pocket near the corner of the BZ is compatible with the experimentally observed anisotropy of the upper critical field. pointing to its dominant role in the superconductivity of these three compounds.

cond-mat.supr-con↗

arXiv2016

Advanced surface characterization of Ba(Fe$_{0.92}$Co$_{0.08}$)$_2$As$_2$ epitaxial thin films

We report on the systematic characterization of Ba(Fe$_{0.92}$Co$_{0.08}$)$_2$As$_2$ epitaxial thin films on CaF$_2$ substrate in view of their possible use for superconducting electronic applications. By using different and complementary techniques we studied the morphological characteristics of the surface, the structural properties, the magnetic response, and the superconducting properties in terms of critical temperature, critical current, and energy gaps. Particular attention was paid to the homogeneity of the films and to the comparison of their superconducting properties with those of single crystals of the same compound.

cond-mat.supr-con↗

arXiv2015

Coexistence of superconductivity and itinerant ferromagnetism in Sr0.5Ce0.5FBiS2-xSex (x = 0.5 and 1.0), the first non-U material with Tc < TFM

We have carried out detailed magnetic and transport studies of the new Sr0.5Ce0.5FBiS2-xSex (x = 0.5, 1) superconductors derived by doping Se in Sr0.5Ce0.5FBiS2. Se-doping produces several effects: it suppresses semiconducting like behavior observed in the undoped Sr0.5Ce0.5FBiS2, ferromagnetic ordering temperature, TFM, decreases considerably from 7.5 K (in Sr0.5Ce0.5FBiS2) to 3.5 K and superconducting transition temperature, Tc, gets enhanced slightly to 2.9 - 3.3 K. Thus in these Se-doped materials, TFM is just marginally higher than Tc. Magnetization studies provide an evidence of bulk superconductivity in Sr0.5Ce0.5FBiS2-xSex. Quite remarkably, as compared with the effective paramagnetic Ce-moment (~ 2.2 muB), the ferromagnetically ordered Ce-moment in the superconducting state is rather small (~ 0.1 muB). To the best of our knowledge, the title compounds are the first Ce-based superconducting itinerant ferromagnetic materials (Tc < TFM). We stress that Ce-4f electrons are responsible for both superconductivity and ferromagnetism just as U-5f electrons are in UCoGe. Furthermore, a novel feature of these materials is a dual hysteresis loop corresponding to both the ferromagnetism and the coexisting superconductivity. Such features of Sr0.5Ce0.5FBiS2-xSex put these materials apart from the well known U-containing superconducting ferromagnets reported so far.

cond-mat.supr-con↗

arXiv2015

Unusually high critical current of clean P-doped BaFe2As2 single crystalline thin film

Microstructura lly clean, isov alently P-doped BaFe2As2 (Ba-122) single crystalline thin films have been prepared on MgO (001) substrates by molecular beam epitaxy. These films show a superconducting transition temperature (Tc) of over 30 K although P content is around 0.22, which is lower than the optimal one for single crystals (i.e., 0.33). The enhanced Tc at this doping level is attributed to the in-plane tensile strain. The strained film shows high transport self-field critical current densities (Jc) of over 6 MA/cm2 at 4.2 K, which are among the highest for Fe based superconductors (FeSCs). In-field Jc exceeds 0.1 MA/cm2 at m0H = 35 T for H||ab and m0H = 18 T for H||c at 4.2 K, respectively, in spite of moderate upper critical fields compared to other FeSCs with similar Tc. Structural investigations reveal no defects or misoriented grains pointing to strong pinning centers. We relate this unexpected high Jc to a strong enhancement of the vortex core energy at optimal Tc, driven by in-plane strain and doping. These unusually high Jc make P-doped Ba-122 very favorable for high-field magnet applications.

cond-mat.supr-con↗

arXiv2014

Superconducting properties of K$_{1-x}$Na$_x$Fe$_2$As$_2$ under pressure

The effect of hydrostatic pressure and partial Na substitution on the normal-state properties and the superconducting transition temperature ($T_c$) of K$_{1-x}$Na$_x$Fe$_2$As$_2$ single crystals were investigated. It was found that a partial Na substitution leads to a deviation from the standard $T^2$ Fermi-liquid behavior in the temperature dependence of the normal-state resistivity. It was demonstrated that non-Fermi liquid like behavior of the resistivity for K$_{1-x}$Na$_{x}$Fe$_2$As$_2$ and some KFe$_2$As$_2$ samples can be explained by disorder effect in the multiband system with rather different quasiparticle effective masses. Concerning the superconducting state our data support the presence of a shallow minimum around 2 GPa in the pressure dependence of $T_c$ for stoichiometric KFe$_2$As$_2$. The analysis of $T_c$ in the K$_{1-x}$Na$_{x}$Fe$_2$As$_2$ at pressures below 1.5 GPa showed, that the reduction of $T_c$ with Na substitution follows the Abrikosov-Gor'kov law with the critical temperature $T_{c0}$ of the clean system (without pair-breaking) which linearly depends on the pressure. Our observations, also, suggest that $T_c$ of K$_{1-x}$Na$_x$Fe$_2$As$_2$ is nearly independent of the lattice compression produced by the Na substitution. Further, we theoretically analyzed the behavior of the band structure under pressure within the generalized gradient approximation (GGA). A qualitative agreement between the calculated and the recently in de Haas-van Alphen experiments [T. Terashima et al., Phys.Rev.B89, 134520(2014)] measured pressure dependencies of the Fermi-surface cross-sections has been found. These calculations, also, indicate that the observed minimum around 2~GPa in the pressure dependence of $T_c$ may occur without a change of the pairing symmetry.

cond-mat.supr-con↗

arXiv2014

Specific heat of K071Na0.29Fe2As2 at very low temperatures

A commercially available calorimeter has been used to investigate the specific heat of a high-quality \kn\ single crystal. The addenda heat capacity of the calorimeter is determined in the temperature range $0.02 \, \mathrm{K} \leq T \leq 0.54 \, \mathrm{K}$. The data of the \kn\ crystal imply the presence of a large $T^2$ contribution to the specific heat which gives evidence of $d$-wave order parameter symmetry in the superconducting state. To improve the measurements, a novel design for a calorimeter with a paramagnetic temperature sensor is presented. It promises a temperature resolution of $ΔT \approx 0.1 \, \mathrm{μK}$ and an addenda heat capacity less than $200 \, \mathrm{pJ/K}$ at $ T < 100 \, \mathrm{mK}$.

cond-mat.supr-con↗

arXiv2014

Superconducting specific heat jump $ΔC_{\rm el} \propto T_c^β\ (β\approx 2)$ for K$_{1-x}$Na$_x$Fe$_2$As$_2$

We present a systematic study of the electronic specific heat jump ($ΔC_{\rm el}$) at the superconducting transition temperature $T_c$ of K$_{1-x}$Na$_x$Fe$_2$As$_2$. Both $T_c$ and $ΔC_{\rm el}$ monotonously decrease with increasing $x$. The specific heat jump scales approximately with a power-law, $ΔC_{\rm el} \propto T_c^β$, with $β\approx 2$ determined by the impurity scattering rate, in contrast to most iron-pnictide superconductors, where the remarkable Bud'ko-Ni-Canfield (BNC) scaling $ΔC_{\rm el} \propto T^3$ has been found. Both the $T$ dependence of $C_{\rm el}(T)$ in the superconducting state and the nearly quadratic scaling of $ΔC_{\rm el}$ at $T_c$ are well described by the Eliashberg-theory for a two-band $d$-wave superconductor with weak pair-breaking due to nonmagnetic impurities. The disorder induced by the Na substitution significantly suppresses the small gaps leading to gapless states in the slightly disordered superconductor, which results in a large observed residual Sommerfeld coefficient in the superconducting state for $x > 0$.

cond-mat.supr-con↗

arXiv2013

Strain induced superconductivity in the parent compound BaFe2As2

The discovery of superconductivity (SC) with a transition temperature, Tc, up to 65K in single-layer FeSe (bulk Tc =8K) films grown on SrTiO3 substrates has attracted special attention to Fe-based thin films. The high Tc is a consequence of the combined effect of electron transfer from the oxygen-vacant substrate to the FeSe thin film and lattice tensile strain. Here we demonstrate the realization of SC in the parent compound BaFe2As2 (no bulk Tc) just by tensile lattice strain without charge doping. We investigate the interplay between strain and SC in epitaxial BaFe2As2 thin films on Fe-buffered MgAl2O4 single crystalline substrates. The strong interfacial bonding between Fe and the FeAs sublattice increases the Fe-Fe distance due to the lattice misfit which leads to a suppression of the antiferromagnetic spin density wave and induces SC with bulk-Tc ?10K. These results highlight the role of structural changes in controlling the phase diagram of Fe-based superconductors.

cond-mat.supr-con↗

arXiv2013

Specific heat of Ca$_{0.32}$Na$_{0.68}$Fe$_2$As$_2$ single crystals: unconventional s$_\pm$ multi-band superconductivity with intermediate repulsive interband coupling and sizable attractive intraband couplings

We report a low-temperature specific heat study of high-quality single crystals of the heavily hole doped superconductor Ca$_{0.32}$Na$_{0.68}$Fe$_2$As$_2$. This compound exhibits bulk superconductivity with a transition temperature $T_c \approx 34$\,K, which is evident from the magnetization, transport, and specific heat measurements. The zero field data manifests a significant electronic specific heat in the normal state with a Sommerfeld coefficient $γ\approx 53$ mJ/mol K$^{2}$. Using a multi-band Eliashberg analysis, we demonstrate that the dependence of the zero field specific heat in the superconducting state is well described by a three-band model with an unconventional s$_\pm$ pairing symmetry and gap magnitudes $Δ_i$ of approximately 2.35, 7.48, and -7.50 meV. Our analysis indicates a non-negligible attractive intraband coupling,which contributes significantly to the relatively high value of $T_c$. The Fermi surface averaged repulsive and attractive coupling strengths are of comparable size and outside the strong coupling limit frequently adopted for describing high-$T_c$ iron pnictide superconductors. We further infer a total mass renormalization of the order of five, including the effects of correlations and electron-boson interactions.

cond-mat.supr-con↗

arXiv2013

Evidence of d-wave Superconductivity in K_(1-x)Na_xFe_2As_2 (x = 0, 0.1) Single Crystals from Low-Temperature Specific Heat Measurements

From the measurement and analysis of the specific heat of high-quality K_(1-x)Na_xFe_2As_2 single crystals we establish the presence of large T^2 contributions with coefficients alpha_sc ~ 30 mJ/mol K^3 at low-T for both x=0 and 0.1. Together with the observed square root field behavior of the specific heat in the superconducting state both findings evidence d-wave superconductivity on almost all Fermi surface sheets with an average gap amplitude of Delta_0 in the range of 0.4 - 0.8 meV. The derived Delta_0 and the observed T_c agree well with the values calculated within the Eliashberg theory, adopting a spin-fluctuation mediated pairing in the intermediate coupling regime.

cond-mat.supr-con↗

arXiv2012

Disordered magnetism in superconducting KFe2As2 single crystals

High-quality KFe2As2 (K122) single crystals synthesized by different techniques have been studied by magnetization and specific heat (SH) measurements. There are 2 types of samples both affected by disordered magnetic phases: (i) cluster-glass (CG) like or (ii) Griffiths phase (G) like. For (i) at low applied magnetic fields the T-dependence of the zero field cooled (ZFC) linear susceptibility (chi_l) exhibits an anomaly with an irreversible behavior in ZFC and field cooled (FC) data. This anomaly is related to the freezing temperature T_f. The extrapolated T_f to B=0 varies between 50 K and 90 K. Below T_f we observed a magnetic hysteresis in the field dependence of the isothermal magnetization (M(B)). The frequency shift of the freezing temperature delta T_f=Delta T_f/[T_fΔ(\ln ν)]\sim 0.05$ has an intermediate value, which provides evidence for the formation of a CG-like state in the K122 samples of type (i). The frequency dependence of their T_f follows a conventional power-law divergence of critical slowing down: tau=tau_0 [T_f(nu)/T_f(0)-1]^{-zν^{'}} with the critical exponent zν^{'}=10(2) and a relatively long characteristic time constant tau_0 =6.9 x10^{-11}$s also supporting a CG behavior. The large value of the Sommerfeld coefficient was related to magnetic contribution from a CG. Samples from (ii) did not show a hysteresis behavior for chi_l(T) and M(B). Below a crossover temperature T^* sim 40 K a power-law dependence in the chi_l propto T^[lambda_G-1}], with a non-universal lambda_G was observed, suggesting a quantum G-like behavior. In this case chi_l and M(B) can be scaled using the scaling function M_s(T,B)= B^{1-λ_{\tiny G}}Y(mu B/k_BT) with the scaling moment mu of the order of 3.5mu_b. The same non-universal exponent was found also in SH measurements, where the magnetic contribution C/T propto T^(lambda_G-1).

cond-mat.dis-nn↗

arXiv2012

Specific heat and upper critical field in KFe2As2 single crystals

We report low-temperature specific heat measurements for high-quality single crystalline KFe2As2 (T_c about 3.5 K). The investigated zero-field specific heat data yields an unusually large nominal Sommerfeld coefficient gamma_n of 94(3) mJ/mol K^2 which is however significantly affected by extrinsic contributions as evidenced by a sizable residual linear specific heat and various theoretical considerations including also an analysis of Kadowaki-Woods relations. Then KFe2As2 should be classified as a weak to intermediately strong coupling superconductor with a total electron-boson coupling constant lambda_tot near 1 (including a calculated weak electron-phonon coupling constant of lambda_el-ph =0.17. From specific heat and ac susceptibility studies in external magnetic fields the magnetic phase diagram has been constructed. We confirm the high anisotropy of the upper critical fields B_c2(T) ranging from a factor of 5 near T_c to a slightly reduced value approaching T=0 for fields B || ab$ and || c and show that their ratio Gamma slightly exceeds the mass anisotropy of 4.35 derived from our full-relativistic LDA-band structure calculations. Its slight reduction when approaching T=0 is not a consequence of Pauli-limiting as in less perfect samples but point likely to a multiband effect. We also report irreversibility field data obtained from ac susceptibility measurements. The double-maximum in the T-dependence of its imaginary part for fields B || c indicates a peak-effect in the T-dependence of critical currents.

cond-mat.supr-con↗

arXiv2012

KFe2As2: coexistence of superconductivity and local moment derived spin-glass

High-quality KFe2As2 single crystals have been studied by transport, magnetization and low-T specific heat measurements. Their analysis shows that superconductivity occurs (in some cases coexists) in the vicinity of disordered magnetic phases (Griffiths and spin-glass type) depending of the amount of local magnetic moments (probably excess Fe derived)and sample inhomogeneity. The achieved phenomenological description of our data including also data from the literature provides a consistent explanation of the observed non-Fermi-liquid behavior and of the nominally large experimental Sommerfeld coefficient gamma_n about 94 mJ/mol K^2. We suggest that the intrinsic value (directly related to the itinerant quasi-particles) gamma_el about 60(10)mJ/mol K^2 is significantly reduced compared with gamma_n. Then an enhanced relative jump of the electronic specific heat Delta C_el/gamma_el T_c about 0.8 and a weak total electron-boson coupling constant lambda less or about 1 follow.

cond-mat.supr-con↗