Searcharxiv⌕ Search

arXiv subjects

V. I. Belotelov

Publications and source records attributed to V. I. Belotelov.

At least 19 recordsLinked to original sources

Superconductivity-Enabled Conversion of Ferromagnetic Resonance into Standing Spin Waves

Superconductors can transport spin without Joule dissipation, yet their coherent coupling to short-wavelength magnons in insulating magnets remains largely unexplored. Here we demonstrate experimentally and theoretically that a conventional diffusive superconductor can enable the conversion of the uniform ferromagnetic resonance (FMR) mode into perpendicular standing spin waves (PSSWs) in an adjacent ferrimagnetic insulator. In Bi-substituted iron-garnet/Nb bilayers, the microwave transmission develops an additional resonance feature that appears only below the Nb superconducting transition temperature and lies close to the uniform FMR peak. A microscopic theory that self-consistently couples the quasiclassical Keldysh--Usadel description of the superconducting condensate to the Landau--Lifshitz--Gilbert dynamics shows that the conversion relies on two ingredients: (i) an interfacial spin-transfer torque mediated by spin-polarized triplet Cooper pairs and (ii) a depth-dependent effective field produced by Abrikosov vortices (electromagnetic proximity). The resulting susceptibility reproduces the measured lineshapes and establishes superconductivity as an active control parameter for exchange standing-wave modes in magnetic insulators.

cond-mat.supr-con↗

Degeneracy and trajectory control of spin eigenmodes excited by fs-optical pulses in a nearly compensated ferrimagnet

We investigate optically excited spin dynamics in a uniaxial ferrimagnet near the magnetization compensation point under a magnetic field applied along the magnetic anisotropy axis. Experiment and numerical modeling reveal an unusual regime where the frequencies of two spin eigenmodes approach each other and become highly field sensitive. The modes, corresponding to opposite rotations of the Neel vector, simultaneously reverse their handedness at a critical field where their frequencies become degenerate. At this point, the two-frequency precessional dynamics collapses into a linear oscillations directed along the inverse-Faraday-effect excitation induced by a single pump pulse. We further show that a double-pulse excitation scheme enables control of the spin trajectory. These results uncover an unconventional dynamical regime in ferrimagnets and establish new opportunities for manipulating spin motion in magnonic systems and devices.

cond-mat.mtrl-sci↗

Enhanced magneto-optical intensity effect in a helicity-preserving all-dielectric metasurface at Mie resonances and the anapole state

Nanophotonic structures provide an efficient route to enhancing magneto-optical effects by concentrating electromagnetic fields at subwavelength scales. In this work, we propose and experimentally demonstrate a helicity-preserving all-dielectric metasurface for enhancing magnetization-induced transmission modulation under circularly polarized excitation. The optical response of the structure is governed by the Mie resonances of silicon nanodisks and by a spectral feature associated with the anapole state. In the spectral regions of the Mie resonances, the metasurface exhibits a pronounced enhancement of the magneto-optical intensity response relative to a bare magnetic film of the same thickness, with the normalized magneto-optical intensity effect increased by a factor of about 2-3. A strong response is also observed in the spectral region associated with the anapole state, manifested as a local transmission maximum. In this regime, the normalized magneto-optical intensity effect exceeds that of the bare magnetic film by about 30%, while the metasurface transmission remains as high as around 80%. The enhanced response in this spectral region is preserved over a broad range of incidence angles. These results demonstrate that all-dielectric metasurfaces combining Mie resonances with the spectral feature associated with the anapole state provide an efficient platform for magneto-optical intensity modulation of circularly polarized light at high transmission.

physics.optics↗

The prospects of nonthermal magnetization switching in near-compensated rare earth iron garnets

Ultrafast spin dynamics in a magnetically compensated rare earth iron garnet film driven by femtosecond optical pulses through the inverse Faraday effect is theoretically investigated. Numerical simulations based on the equations of motion for the Néel vector reveal the temporal evolution of the system and its trajectories in the effective potential landscape tuned by external field and temperature. The results demonstrate a clear threshold behavior: weak pulses induce only oscillations around the initial equilibrium state, while a stronger excitation results in a deterministic magnetization switching. The switching threshold is determined by the magnetic state of the sample on its phase diagramme as well as on the laser pulse helicity. This mechanism demonstrates a non-thermal and even non-absorptive pathway towards optomagnonic logic and memory devices.

cond-mat.mtrl-sci↗

Unusual sign-changing Faraday effect in nanometer-thick magnetic films

It is generally believed that the magneto-optical Faraday effect appears in the the bulk of a magnetic material and its sign is fully determined by the sign of the non-diagonal permittivity element. Here we reveal an additional contribution to the Faraday effect from the film interfaces. It becomes notable for films with a thickness of a few tens of nanometers. As a result, in the absorption band of the film a novel feature of the Faraday effect is experimentally observed and numerically confirmed: sign of the Faraday rotation at a fixed wavelength becomes dependent on the film thickness and therefore is ambiguously related to the sign of the gyration and magnetization of the film. We elaborated an analytical model taking into account an interplay between the bulk and surface contributions which nicely describes the experimental data. Moreover, the Faraday rotation coming purely from interfaces without any bulk contribution is demonstrated. Possible applications of the observed unusual Faraday rotation behavior include hardware data encryption and other devices performing polarization control at nanoscale.

physics.optics↗

Micrometer thick single crystal iron-garnet films on a diamagnetic buffer layer for cryogenic applications

This work advances the frontier of low-damping magnetic materials, directly addressing the demand for ultra-low-loss components in quantum computing and cryogenic electronics. Here we demonstrate a new approach to get single crystal micrometer-thick yttrium iron garnet (YIG) films with low damping through isolating and mitigating interfacial paramagnetic contributions of a paramagnetic substrate by a buffer-layer. The YIG films with the diamagnetic yttrium scandium gallium garnet buffer layer grown by liquid phase epitaxy on a gadolinium gallium substrate demonstrate homogeneity unprecedented for the thin planar YIG structures, yielding ferromagnetic resonance linewidths of 4.9 MHz at 4 K and 5.9 MHz at 16 mK, the lowest values reported to date. These results underscore the critical role of interfacial engineering in overcoming intrinsic material limitations, opening avenues for further optimization in spin-based technologies.

cond-mat.mtrl-sci↗

Magnon-photon coupling in the YIG-based disk and ring microcavities

Optomagnonic dielectric resonators offer a promising platform for the bidirectional conversion of microwave and optical photons at the single quantum level. Current implementation of such a conversion lacks from low magneto-optical interaction strength, limiting its practical utilization in quantum technologies. The main bottleneck is the small spatial overlap between optical and magnon modes. Here, we show that utilization of a disk and ring geometries notably increases the mode overlap. We analyze the interaction volume of optical whispering gallery and magnon Kittel modes inside yttrium iron garnet disk and ring microcavities of various sizes and found a significant improvement in modes coupling up to $\sim4.5~kHz$ . Maximal theoretical conversion efficiency for small disks with radius $5~μm$ can reach unity for optimal optical power $\sim100~μW$, which is experimentally feasible. Strategies for further improvements of interactions are discussed.

physics.optics↗

Thermally-controlled magnetooptical metasurface for tunable Faraday rotation

We present novel type of tunable magneto-optical metasurfaces performing Faraday rotation, the sign and value of which are not fixed after the structure fabrication but can be tuned in a wide range via heating of the metasurface. We demonstrate both experimentally and theoretically that the Faraday rotation angle is enhanced in the vicinity of the magnetodipole and electrodipole Mie resonances and can be changed in a wide range from -0.3 degrees to +0.1 degrees for the same metasurface at fixed wavelength of incident light under the temperature changes from the 294~K to 488~K. Such thermal heating can be performed by an external control laser. As laser radiation can be focused at the spots of $~\sim 1μ$m diameter, the magneto-optical response can also be tuned locally. Thus one may obtain the inhomogeneous magnetooptically-induced polarization rotation distributions across the metasurface by the creation of the laser beam patterns with the desired intensity profiles. Another possibility opened by the proposed merasurface is self-modulation of polarization of laser light performed depending on its intensity.

physics.optics↗

Asymmetric Faraday effect caused by a break of spatial symmetry

It is widely known that the magneto-optical Faraday effect is linear in magnetization, and therefore the Faraday angles for the states with opposite magnetizations are of opposite sign but equal in modulus. Here we demonstrate that under certain spatial symmetry-breaking conditions, an asymmetric Faraday effect (AFE) arises, meaning that the Faraday angles for opposite magnetic states differ not only in sign but in absolute value as well. Experimental investigations of AFE are performed in a one-dimensional all-garnet magnetophotonic crystal, where AFE appears in the vicinity of the cavity resonance for an oblique incidence of light with an inclined light polarization plane. The magnitude of the observed asymmetry between Faraday rotations for the two opposite magnetizations is very large and reaches 30$\%$ of the absolute value of the Faraday effect. We confirm the generality of the suggested effect by the numerical analysis of several different configurations in which AFE arises. The discovered AFE is of prime importance for nanoscale magnonics and optomagnetism.

physics.optics↗

Unconventional spin dynamics in the non-collinear phase of a ferrimagnet

Ferrimagnets containing several partially compensated magnetic sublattices are considered the most promising materials for all-optical data storage and for ultrafast communications based on spin waves. There are two magnetic phases of the ferrimagnets: collinear and non-collinear ones. Up to now spin dynamics in ferrimagnets has been studied mostly in the collinear state without paying much attention to the kind of the magnetic phase. Here we investigate laser induced ultrafast spin dynamics in a rare-earth iron garnet film in the noncollinear phase as well. We identify a crucial influence of the magnetic phase on the excited spin modes which allowed us to discover several prominent effects previously overlooked. In particular, the non-collinearity makes the quasi-antiferromagnetic mode sensitive to the external magnetic field and brings its frequency close to the frequency of the quasiferromagnetic mode. The latter maximizes near the magnetization compensation point and vanishes towards the collinear phase. Spectacularly, at the phase transition the quasiferromagnetic mode becomes soft and its amplitude significantly increases reaching 7°. This opens new opportunities for the ultrafast control of spins in ferrimagnets for nonthermal data storage and data processing.

cond-mat.mtrl-sci↗

Direct observation of magnon BEC in an out-of-plane magnetized yttrium iron garnet film

Bose-Einstain condensation occurs at an appropriate density of bosonic particles, depending on their mass and temperature. We were able to experimentally observe the transition from the spin wave regime to the magnon Bose-Einstein condensed state (mBEC) with increasing magnon density by a microwave pumping. We used optical methods to register the spatial distribution of the magnon density and phase. For the first time, a coherent state of stationary magnons was demonstrated far from the region of their excitation.

cond-mat.mes-hall↗

Superconducting spin valves based on a single spiral magnetic layer

A detailed investigation of a superconducting spin-triplet valve is presented. This spin-valve consists of a superconducting film covering a metal with an intrinsic spiral magnetic order, which could result from competing isotropic exchanges or, if the crystal lattice breaks central symmetry, from asymmetric Dzyaloshinskii-Moriya exchange. Depending on the anisotropy, such a metal may change its magnetization either from a spiral to uniform order, as seen in Ho and Er, or in the direction of the spiral itself, as in crystals of the B20-type structure (such as MnSi, (Fe,Co)Si, FeGe, etc.). The nonuniform magnetic order controls the appearance of long-range triplet superconducting correlations at strong exchange fields, affecting the detailed character of the proximity effect. We show that the magnetic control of the spin-valve behavior can also be obtained from moderately low exchange fields (typically associated to negligible long-range triplet correlations), thanks to an orientation-dependent averaging mechanism of the magnetic inhomogeneity on the scale of the Cooper pairs. Our numerical calculations reveal that the spin-valve effect is in fact magnified at moderately low exchange fields, when the exchange splitting in the spiral magnet is comparable to the superconducting gap, and the spiral period is less than or equal to the superconducting coherence length in the magnet multiplied by $2π$.

cond-mat.supr-con↗

The Faraday effect in magnetoplasmonic nanostructures with spatial modulation of magnetization

The magneto-optical Faraday effect in the magnetoplasmonic nanostructures with nonuniform, periodically modulated spatial distribution of the magnetization is considered. It is shown that in such nanostructures the Faraday effect can experience the resonant enhancement in the spectral range of the plasmonic and waveguide optical modes excitation. It happens both for $s$ and $p$-polarized light. Such an effect can serve for the spectrally selective detection of the short spin waves in the magnetic materials.

physics.optics↗

Birefringence-mediated enhancement of the magneto-optical activity in anisotropic magnetic crystals

Optical anisotropy is usually treated as an unfavorable condition for the magneto-optical measurements since it is known to diminish the Faraday rotation concerning the case of the isotropic medium. Here we show that the situation could be quite opposite: a phenomenon of birefringence mediated enhancement of the magneto-optical activity appears if the incident light polarization and angle of incidence are set properly. The present study relies on the experimental, analytical, and numerical studies of iron borate $\mathrm{FeBO_3}$ crystals. We demonstrate a significant increase of the magneto-optical activity resulting in nearly $100\%$ magneto-optical light modulation magnitude. The approach applies to other types of birefringent crystals with the magneto-optical response that makes it crucial for various practical applications, including magneto-optical microscopy, pump-probe studies, and others.

physics.optics↗

Accumulation and control of spin waves in magnonic dielectric microresonators by a comb of ultrashort laser pulses

Spin waves in magnetic microresonators are at the core of modern magnonics. Here we demonstrate a new method of tunable excitation of different spin wave modes in magnetic microdisks by using a train of laser pulses coming at a repetition rate higher than the decay rate of spin precession. The microdisks are etched in a transparent bismuth iron garnet film and the light pulses influence the spins nonthermally through the inverse Faraday effect. The high repetition rate of the laser stimulus of 10 GHz establishes an interplay between the spin wave resonances in the frequency and momentum domains. As a result, scanning of the focused laser spot near the disk boarder changes interference pattern of the magnons and leads to a resonant dependence of the spin wave amplitude on the external magnetic field. Apart from that, we achieved a switching between volume and surface spin waves by a small variation of the external magnetic field.

physics.optics↗

Optical excitation and probing of the antiferromagnetic modes with non-uniform in-depth distribution in birefringent antiferromagnetic crystals

Optical pump-probe setups are commonly used for excitation and investigation of the spin dynamics in various types of magnetic materials. However, usually the spatially homogeneous excitation is considered. In the present study we describe an approach for optical excitation of the nonuniform THz spin dynamics and for probing its spatial distribution inside a magnetic crystal. We propose to illuminate a crystal with laser pulses of properly adjusted polarization to benefit from a strong optical birefringence inherent to the crystal. It results in an unusual behavior of the effective magnetic field generated by the pulses due to the inverse Faraday effect and the peculiar sign-changing dependence of the direct Faraday effect inside the crystal. The study is performed exemplary for yttrium orthoferrite crystal although the proposed approach is applicable for various magnetic materials with optical anisotropy.

physics.optics↗

Valley polarization of trions in monolayer MoSe$_2$ interfaced with bismuth iron garnet

Interfacing atomically thin van der Waals semiconductors with magnetic substrates enables additional control on their intrinsic valley degree of freedom and provides a promising platform for the development of novel valleytronic devices for information processing and storage. Here we study circularly polarized photoluminescence in heterostructures of monolayer MoSe$_2$ and thin films of ferrimagnetic bismuth iron garnet. We observe strong emission from charged excitons with negative valley polarization, which switches sign with increasing temperature, and demonstrate contrasting response to left and right circularly polarized excitation, associated with finite out-of-plane magnetization in the substrate. We propose a theoretical model accounting for magnetization-induced imbalance of charge carriers in the two valleys of MoSe$_2$, as well as for valley-switching scattering from B to A excitons and fast formation of trions with extended valley relaxation times, which shows excellent agreement with the experimental data. Our results provide new insights into valley physics in 2D semiconductors interfaced with magnetic substrates.

cond-mat.mes-hall↗