arXiv subjects

V. M. Shalaev

Publications and source records attributed to V. M. Shalaev.

14 recordsLinked to original sources

arXiv2025

Quantum dots emission enhancement via coupling with an epsilon-near-zero sublayer

Quantum emitters operating at telecom wavelengths are essential for the advancement of quantum technologies, particularly in the development of integrated on-chip devices for quantum computing, communication, and sensing. Coupling resonant structures to a near-zero-index (NZI) environment has been shown to enhance their optical performance by both increasing spontaneous emission rates and improving emission directionality. In this work, we comparatively study emission characteristics of colloidal PbS/CdS (core/shell) quantum dots at telecom wavelengths on different substrates, where two different sets of quantum dots emitting within and outside the epsilon-near-zero region are deposited on both glass and indium tin oxide (ITO) substrates. Our results demonstrate that coupling quantum dots to the epsilon-near-zero spectral region results in a reduction of photoluminescence lifetime of 54~times, a 7.5-fold increase in saturation intensity, and a relative emission cone narrowing from 17.6° to 10.3°. These results underline the strong dependence of quantum dot emission properties on the spectral overlap with the epsilon-near-zero condition, highlighting the potential of transparent conducting oxides (TCOs), such as ITO, for integration into next-generation quantum photonic devices. Due to their CMOS compatibility, fabrication tunability, and high thermal and optical damage thresholds, TCO NZI materials offer a robust platform for scalable and high-performance quantum optical systems operating within the telecom bandwidth.

physics.optics↗

arXiv2024

Natural width of the superconducting transition in epitaxial TiN films

We investigate the effect of various fluctuation mechanisms on the DC resistance in superconducting devices based on epitaxial titanium nitride (TiN) films. The samples we studied show a relatively steep resistive transition (RT), with a transition width $ΔT/T_\mathrm{c} \sim 0.002-0.025$, depending on the film thickness (20 nm, 9 nm, and 5 nm) and device dimensions. This value is significantly broader than expected due to conventional superconducting fluctuations ($ΔT/T_\mathrm{c} \ll 10^{-3}$). The shape and width of the RT can be perfectly described by the well-known effective medium theory, which allows us to understand the origin of the inhomogeneity in the superconducting properties of TiN films. We propose that this inhomogeneity can have both dynamic and static origins. The dynamic mechanism is associated with spontaneous fluctuations in electron temperature (T-fluctuations), while the static mechanism is due to a random spatial distribution of surface magnetic disorder (MD). Our analysis has revealed clear correlations between the transition width and material parameters as well as device size for both proposed mechanisms. While T-fluctuations may contribute significantly to the observed transition width, our findings suggest that the dominant contribution comes from the MD mechanism. Our results provide new insights into the microscopic origin of broadening of the superconducting transition and inhomogeneity in thin superconducting films.

cond-mat.supr-con↗

arXiv2024

Slow electron-phonon relaxation controls the dynamics of the superconducting resistive transition

We investigate the temporal and spatial scales of resistance fluctuations ($R$-fluctuations) at the superconducting resistive transition accessed through voltage fluctuations measurements in thin epitaxial TiN films. This material is characterized by a slow electron-phonon relaxation, which puts it far beyond the applicability range of the textbook scenario of superconducting fluctuations. The measured Lorentzian spectrum of the $R$-fluctuations identifies their correlation time, which is nearly constant across the transition region and has no relation to the conventional Ginzburg-Landau time scale. Instead, the correlation time coincides with the energy relaxation time determined by a combination of the electron-phonon relaxation and the relaxation via diffusion into reservoirs. Our data is quantitatively consistent with the model of spontaneous temperature fluctuations and highlight the lack of understanding of the resistive transition in materials with slow electron-phonon relaxation.

cond-mat.supr-con↗

arXiv2019

Superconductivity behavior in epitaxial TiN films points at surface magnetic disorder

We analyze the evolution of the normal and superconducting electronic properties in epitaxial TiN films, characterized by high Ioffe-Regel parameter values, as a function of the film thickness. As the film thickness decreases, we observe an increase of in the residual resistivity, which becomes dominated by diffusive surface scattering for $d\leq20\,$nm. At the same time, a substantial thickness-dependent reduction of the superconducting critical temperature is observed compared to the bulk TiN value. In such a high quality material films, this effect can be explained by a weak magnetic disorder residing in the surface layer with a characteristic magnetic defect density of $\sim10^{12}\,\mathrm{cm}^{-2}$. Our results suggest that surface magnetic disorder is generally present in oxidized TiN films.

cond-mat.mtrl-sci↗

arXiv2019

Negative refraction in time-varying, strongly-coupled plasmonic antenna-ENZ systems

Time-varying metasurfaces are emerging as a powerful instrument for the dynamical control of the electromagnetic properties of a propagating wave. Here we demonstrate an efficient time-varying metasurface based on plasmonic nano-antennas strongly coupled to an epsilon-near-zero (ENZ) deeply sub-wavelength film. The plasmonic resonance of the metal resonators strongly interacts with the optical ENZ modes, providing a Rabi level spitting of ~30%. Optical pumping at frequency ω induces a nonlinear polarisation oscillating at 2ω responsible for an efficient generation of a phase conjugate and a negative refracted beam with a conversion efficiency that is more than four orders of magnitude greater compared to the bare ENZ film. The introduction of a strongly coupled plasmonic system therefore provides a simple and effective route towards the implementation of ENZ physics at the nanoscale

physics.optics↗

arXiv2017

Controlling hybrid nonlinearities in transparent conducting oxides via two-colour excitation

Nanophotonics and metamaterials have revolutionised the way we think about optical space (epsilon, mu), enabling us to engineer the refractive index almost at will, to confine light to the smallest of the volumes, and to manipulate optical signals with extremely small footprints and energy requirements. Significant efforts are now devoted to finding suitable materials and strategies for the dynamic control of the optical properties. Transparent conductive oxides exhibit large ultrafast nonlinearities under both interband and intraband excitations. Here, we show that combining these two effects in aluminium-doped zinc oxide via a two colour laser field discloses new material functionalities. Owing to the independence of the two nonlinearities the ultrafast temporal dynamics of the material permittivity can be designed by acting on the amplitude and delay of the two fields. We demonstrate the potential applications of this novel degree of freedom by dynamically addressing the modulation bandwidth and optical spectral tuning of a probe optical pulse.

physics.optics↗

arXiv2016

Superconducting detector for visible and near-infrared quantum emitters

Further development of quantum emitter based communication and sensing applications intrinsically depends on the availability of robust single-photon detectors. Here, we demonstrate a new generation of superconducting single-photon detectors specifically optimized for the 500-1100 nm wavelength range, which overlaps with the emission spectrum of many interesting solid-state atom-like systems, such as nitrogen-vacancy and silicon-vacancy centers in diamond. The fabricated detectors have a wide dynamic range (up to 350 million counts per second), low dark count rate (down to 0.1 counts per second), excellent jitter (62 ps), and the possibility of on-chip integration with a quantum emitter. In addition to performance characterization, we tested the detectors in real experimental conditions involving nanodiamond nitrogen-vacancy emitters enhanced by a hyperbolic metamaterial.

quant-ph↗

arXiv2016

Enhanced nonlinear refractive index in epsilon-near-zero materials

New propagation regimes for light arise from the ability to tune the dielectric permittivity to extremely low values. Here we demonstrate a universal approach based on the low linear permittivity values attained in the epsilon-near-zero (ENZ) regime for enhancing the nonlinear refractive index, which enables remarkable light-induced changes of the material properties. Experiments performed on Al-doped ZnO (AZO) thin films show a six-fold increase of the Kerr nonlinear refractive index ($n_2$) at the ENZ wavelength, located in the 1300 nm region. This in turn leads to ultrafast light-induced refractive index changes of the order of unity, thus representing a new paradigm for nonlinear optics.

physics.optics↗

arXiv2015

Epsilon-Near-Zero Al-Doped ZnO for Ultrafast Switching at Telecom Wavelengths: Outpacing the Traditional Amplitude-Bandwidth Trade-Off

Transparent conducting oxides have recently gained great attention as CMOS-compatible materials for applications in nanophotonics due to their low optical loss, metal-like behavior, versatile/tailorable optical properties, and established fabrication procedures. In particular, aluminum doped zinc oxide (AZO) is very attractive because its dielectric permittivity can be engineered over a broad range in the near infrared and infrared. However, despite all these beneficial features, the slow (> 100 ps) electron-hole recombination time typical of these compounds still represents a fundamental limitation impeding ultrafast optical modulation. Here we report the first epsilon-near-zero AZO thin films which simultaneously exhibit ultra-fast carrier dynamics (excitation and recombination time below 1 ps) and an outstanding reflectance modulation up to 40% for very low pump fluence levels (< 4 mJ/cm2) at the telecom wavelength of 1.3 μm. The unique properties of the demonstrated AZO thin films are the result of a low temperature fabrication procedure promoting oxygen vacancies and an ultra-high carrier concentration. As a proof-of-concept, an all-optical AZO-based plasmonic modulator achieving 3 dB modulation in 7.5 μm and operating at THz frequencies is numerically demonstrated. Our results overcome the traditional "modulation depth vs. speed" trade-off by at least an order of magnitude, placing AZO among the most promising compounds for tunable/switchable nanophotonics.

physics.optics↗

arXiv2013

Broadband enhancement of spontaneous emission from nitrogen-vacancy centers in nanodiamonds by hyperbolic metamaterials

We experimentally demonstrate a broadband enhancement of emission from nitrogen vacancy centers in nanodiamonds. The enhancement is achieved by using a multilayer metamaterial with hyperbolic dispersion. The metamaterial is fabricated as a stack of alternating gold and alumina layers. Our approach paves the way towards the construction of efficient single-photon sources as planar on-chip devices.

physics.optics↗

arXiv2009

Experimental observation of the trapped rainbow

We report on the first experimental demonstration of the broadband "trapped rainbow" in the visible frequency range using an adiabatically tapered waveguide. Being a distinct case of the slow light phenomenon, the trapped rainbow effect could be applied to optical computing and signal processing, and to providing enhanced light-matter interactions.

physics.optics↗

arXiv2006

Effect of an Optical Negative Index Thin Film on Optical Bistability

We investigate nonlinear transmission in a layered structure consisting of a slab of positive index material (PIM) with Kerr-type nonlinearity and a sub-wavelength layer of linear negative index material (NIM) sandwiched between semi-infinite linear dielectrics. We find that a thin layer of NIM leads to significant changes in the hysteresis width when the nonlinear slab is illuminated at an angle near that of total internal reflection. Unidirectional diode-like transmission with enhanced operational range is demonstrated. These results may be useful for NIMs characterization and for designing novel NIMs based devices.

physics.optics↗

arXiv2005

Enhancement and suppression of surface plasmon resonance in Ag aggregate by optical gain and absorption in surrounding dielectric medium

We have observed the compensation of loss in metal by gain in interfacing dielectric in the mixture of aggregated silver nanoparticles and rhodamine 6G dye. The demonstrated six-fold enhancement of the Rayleigh scattering is the evidence of the increase of the quality factor of the surface plasmon (SP) resonance. The reported experimental observation paves the road to many practical applications of nanoplasmonics. We have also predicted and experimentally observed a suppression of the surface SP resonance in metallic nanoparticles embedded in a dielectric host with absorption.

physics.optics↗

arXiv2005

Negative Refractive Index in Optics of Metal-Dielectric Composites

Specially designed metal-dielectric composites can have a negative refractive index in the optical range. Specifically, it is shown that arrays of single and paired nanorods can provide such negative refraction. For pairs of metal rods, a negative refractive index has been observed at 1.5 micrometer. The inverted structure of paired voids in metal films may also exhibit a negative refractive index. A similar effect can be accomplished with metal strips in which the refractive index can reach -2. The refractive index retrieval procedure and the critical role of light phases in determining the refractive index is discussed.

physics.optics↗