arXiv subjects

V. Manea

Publications and source records attributed to V. Manea.

17 recordsLinked to original sources

arXiv2026

Constraining the trend of the $N = 50$ shell gap towards $^{100}$Sn with the masses of $^{96-98}$Cd

We present the first determination of the $N = 50$ empirical shell gap at $Z = 48$ by precise mass measurements of the neutron-deficient cadmium isotopes $^{96-98}$Cd with the ISOLTRAP mass spectrometer at ISOLDE-CERN, including the first precise determination of the excitation energy of the $25/2^+$ isomer in $^{97}$Cd. Through the systematics of Coulomb Displacement Energies, we further deduce the empirical shell gap in the higher-$Z$ isotopic chains, tightly constraining the $^{100}$Sn mass-surface region. The new experimental data suggest an enhancement of the gap towards $^{100}$Sn, which is discussed in comparison to state-of-the-art calculations using energy-density functional and new ab initio approaches.

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arXiv2026

Mass spectrometry of $^{75}$Zn ground and isomeric states from in-trap decay of $^{75}$Cu

We report on high-precision mass measurements of the ground and first isomeric state of $^{75}$Zn, performed using the time-of-flight ion-cyclotron-resonance technique at the ISOLTRAP Penning-trap mass spectrometer at ISOLDE/CERN. The isomeric state was produced using in-trap decay of $^{75}$Cu. This marks the first direct investigation of the isomeric state of $^{75}$Zn via mass spectrometry. The isomer was observed at an excitation energy of 123.7(20) keV, in 2$\,\sigma$ agreement with the value previously determined through decay spectroscopy. In addition, our measurements correct a misassignment of the ground-state mass excess based on a previous measurement by Baruah et al., revising the value to -62681.0(21) keV. To further investigate the earlier discrepancy, we explored the spin-parity assignments of the ground and isomeric states in $^{75}$Zn using Skyrme Hartree-Fock plus Bardeen-Cooper-Schrieffer theoretical calculations, given the absence of definitive experimental data. In light of the laser spectroscopy results from Wraith et al., our results add strong evidence for a spin-1/2 ground state, which would agree with large-scale shell-model predictions as well as explaining disagreements with the Monte Carlo Shell Model.

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arXiv2026

A prototype gas cell for the stopping, extraction and neutralization of radioactive nuclei from the SPIRAL2 Super Separator Spectrometer (S$^3$)

We present the design and simulation of a prototype gas cell for in-gas-jet laser-ionization and spectroscopy studies using the low energy branch of the SPIRAL2-S$^3$ radioactive-ion-beam facility. The prototype aims to demonstrate the possibility to reduce the extraction time of radioactive ions from the gas cell, while implementing a controlled neutralization mechanism, necessary for laser-spectroscopy studies. Different simulation methods of ion processes in gas are comparatively discussed. Design considerations and detailed simulations of the ion extraction time and efficiency are presented. A study of the dynamics of electrons obtained in the gas cell by ionization is also performed to assess the achievable electron densities.

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arXiv2025

Extending the low-$Z$ "border'' of the $A=100$ region of deformation with precision mass spectrometry of $^{96-98}$Kr

The onset of collective nuclear behavior in the ${N=60}$, ${A\sim100}$, region is examined through high-precision mass measurements of $^{96-98}$Kr, performed with the ISOLTRAP mass spectrometer at ISOLDE, CERN. Our results for $^{96-97}$Kr agree with previous measurements, with our new $^{97}$Kr Penning-trap mass value three times more precise. The mass value of $^{98}$Kr is measured for the first time. The new mass surface, together with comparisons to beyond-mean-field theoretical predictions, suggests that collectivity persists for the ${Z=36}$ isotopes, blurring the apparent ``low-$Z$ boundary'' of this deformed region.

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arXiv2025

An experimental setup for the study of gas-cell processes for the S$^3$-Low Energy Branch

We present an experimental setup dedicated to the study of in-gas ion processes and characterization of gas stopping cells for the Low Energy Branch of the Super Separator Spectrometer (S$^3$) at SPIRAL2-GANIL. The first application is the development of a new gas stopper with a neutralization mechanism designed for faster extraction of the radioactive ions. This development should enable in-gas-jet laser spectroscopy and other low-energy experiments with shorter lived radioactive isotopes. We discuss in detail the motivation and objectives of these developments and we present the results of simulations performed in the design phase, as well as the first experimental results.

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arXiv2024

Refining the nuclear mass surface with the mass of $^{103}$Sn

Mass measurements with the ISOLTRAP mass spectrometer at CERN-ISOLDE improve mass uncertainties of neutron-deficient tin isotopes towards doubly-magic $^{100}$Sn. The mass uncertainty of $^{103}$Sn was reduced by a factor of 4, and the new value for the mass excess of -67104(18) keV is compared with nuclear \textit{ab initio} and density functional theory calculations. Based on these results and local trends in the mass surface, the masses of $^{101,103}$Sn, as determined through their $Q_{\textrm{EC}}$ values, were found to be inconsistent with the new results. From our measurement for $^{103}$Sn, we extrapolate the mass excess of $^{101}$Sn to -60005(300) keV, which is significantly more bound than previously suggested. By correcting the mass values for $^{101,103}$Sn, we also adjust the values of $^{104}$Sb, $^{105,107}$Te, $^{108}$I, $^{109,111}$Xe, and $^{112}$Cs near the proton drip line which are connected through their $\alpha$- and proton $Q$-values. The results show an overall smoothening of the mass surface, suggesting the absence of deformation energy above the ${N=50}$ shell closure.

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arXiv2023

Isomeric excitation energy for $^{99}$In$^{m}$ from mass spectrometry reveals constant trend next to doubly magic $^{100}$Sn

The excitation energy of the 1/2$^-$ isomer in $^{99}$In at ${N=50}$ is measured to be 671(37) keV and the mass uncertainty of the 9/2$^+$ ground state is significantly reduced using the ISOLTRAP mass spectrometer at ISOLDE/CERN. The measurements exploit a major improvement in the resolution of the multi-reflection time-of-flight mass spectrometer. The results reveal an intriguing constancy of the $1/2^-$ isomer excitation energies in neutron-deficient indium that persists down to the $N = 50$ shell closure, even when all neutrons are removed from the valence shell. This trend is used to test large-scale shell model, \textit{ab initio}, and density functional theory calculations. The models have difficulties describing both the isomer excitation energies and ground-state electromagnetic moments along the indium chain.

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arXiv2021

Charge radii, moments and masses of mercury isotopes across the N = 126 shell closure

Combining laser spectroscopy in a Versatile Arc Discharge and Laser Ion Source, with Penning-trap mass spectrometry at the CERN-ISOLDE facility, this work reports on mean-square charge radii of neutron-rich mercury isotopes across the $N = 126$ shell closure, the electromagnetic moments of $^{207}$Hg and more precise mass values of $^{206-208}$Hg. The odd-even staggering (OES) of the mean square charge radii and the kink at $N = 126$ are analyzed within the framework of covariant density functional theory (CDFT), with comparisons between different functionals to investigate the dependence of the results on the underlying single-particle structure. The observed features are defined predominantly in the particle-hole channel in CDFT, since both are present in the calculations without pairing. However, the magnitude of the kink is still affected by the occupation of the $1i_{11/2}$ and $2g_{9/2}$ orbitals with a dependence on the relative energies as well as pairing.

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arXiv2021

Mass measurements of 99-101In challenge ab initio nuclear theory of the nuclide 100Sn

100Sn is of singular interest for nuclear structure. Its closed-shell proton and neutron configuration exhibit exceptional binding and 100Sn is the heaviest nucleus comprising protons and neutrons in equal number, a feature that enhances the contribution of the short-range, proton-neutron pairing interaction and strongly influences its decay via the weak interaction. Decays studies in the region of 100Sn have attempted to prove its doubly magic character but few have studied it from the ab initio theoretical perspective and none have addressed the odd-proton nuclear forces. Here we present, the first direct measurement of the exotic odd-proton nuclide 100In - the beta-decay daughter of 100Sn - and 99In, only one proton below 100Sn. The most advanced mass spectrometry techniques were used to measure 99In, produced at a rate of only a few ions per second, and to resolve the ground and isomeric states in 101In. The experimental results are confronted with new ab initio many-body approaches. The 100-fold improvement in precision of the 100In mass value exarcebates a striking discrepancy in the atomic mass values of 100Sn deduced from recent beta-decay results.

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arXiv2020

Laser spectroscopy of neutron-rich $^{207,208}$Hg isotopes: Illuminating the kink and odd-even staggering in charge radii across the $N=126$ shell closure

The mean-square charge radii of $^{207,208}$Hg ($Z=80, N=127,128$) have been studied for the first time and those of $^{202,203,206}$Hg ($N=122,123,126$) remeasured by the application of in-source resonance-ionization laser spectroscopy at ISOLDE (CERN). The characteristic \textit{kink} in the charge radii at the $N=126$ neutron shell closure has been revealed, providing the first information on its behavior below the $Z=82$ proton shell closure. A theoretical analysis has been performed within relativistic Hartree-Bogoliubov and non-relativistic Hartree-Fock-Bogoliubov approaches, considering both the new mercury results and existing lead data. Contrary to previous interpretations, it is demonstrated that both the kink at $N=126$ and the odd-even staggering (OES) in its vicinity can be described predominately at the mean-field level, and that pairing does not need to play a crucial role in their origin. A new OES mechanism is suggested, related to the staggering in the occupation of the different neutron orbitals in odd- and even-$A$ nuclei, facilitated by particle-vibration coupling for odd-$A$ nuclei.

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arXiv2020

Masses of short-lived $^{49}Sc$, $^{50}Sc$, $^{70}As$, $^{73}Br$ and stable $^{196}Hg$ nuclides

Mass measurements of $^{49,50}$Sc, $^{70}$As, $^{73}$Br and $^{196}$Hg nuclides produced at CERN's radioactive-ion beam facility ISOLDE are presented. The measurements were performed at the ISOLTRAP mass spectrometer by use of the multi-reflection time-of-flight and the Penning-trap mass spectrometry techniques. The new results agree well with previously known literature values. The mass accuracy for all cases has been improved.

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arXiv2020

First glimpse of the $N=82$ shell closure below $Z=50$ from masses of neutron-rich cadmium isotopes and isomers

We probe the $N=82$ nuclear shell closure by mass measurements of neutron-rich cadmium isotopes with the ISOLTRAP spectrometer at ISOLDE-CERN. The new mass of $^{132}$Cd offers the first value of the $N=82$, two-neutron shell gap below $Z=50$ and confirms the phenomenon of mutually enhanced magicity at $^{132}$Sn. Using the recently implemented phase-imaging ion-cyclotron-resonance method, the ordering of the low-lying isomers in $^{129}$Cd and their energies are determined. The new experimental findings are used to test large-scale shell-model, mean-field and beyond-mean-field calculations, as well as the ab initio valence-space in-medium similarity renormalization group.

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arXiv2019

An alternative approach to populate and study the $^{229}$Th nuclear clock isomer

A new approach to observe the radiative decay of the $^{229}$Th nuclear isomer, and to determine its energy and radiative lifetime, is presented. Situated at a uniquely low excitation energy, this nuclear state might be a key ingredient for the development of a nuclear clock, a nuclear laser and the search for time variations of the fundamental constants. The isomer's $\gamma$ decay towards the ground state will be studied with a high-resolution VUV spectrometer after its production by the $\beta$ decay of $^{229}$Ac. The novel production method presents a number of advantages asserting its competitive nature with respect to the commonly used $^{233}$U $\alpha$-decay recoil source. In this paper, a feasibility analysis of this new concept, and an experimental investigation of its key ingredients, using a pure $^{229}$Ac ion beam produced at the ISOLDE radioactive beam facility, is reported.

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arXiv2019

Shape staggering of mid-shell mercury isotopes from in-source laser spectroscopy compared with Density Functional Theory and Monte Carlo Shell Model calculations

Neutron-deficient $^{177-185}$Hg isotopes were studied using in-source laser resonance-ionization spectroscopy at the CERN-ISOLDE radioactive ion-beam facility, in an experiment combining different detection methods tailored to the studied isotopes. These include either alpha-decay tagging or Multi-reflection Time-of-Flight gating to identify the isotopes of interest. The endpoint of the odd-even nuclear shape staggering in mercury was observed directly by measuring for the first time the isotope shifts and hyperfine structures of $^{177-180}$Hg. Changes in the mean-square charge radii for all mentioned isotopes, magnetic dipole and electric quadrupole moments of the odd-A isotopes and arguments in favor of $I = 7/2$ spin assignment for $^{177,179}$Hg were deduced. Experimental results are compared with Density Functional Theory (DFT) and Monte-Carlo Shell Model (MCSM) calculations. DFT calculations with several Skyrme parameterizations predict a large jump in the charge radius around the neutron $N = 104$ mid shell, with an odd-even staggering pattern related to the coexistence of nearly-degenerate oblate and prolate minima. This near-degeneracy is highly sensitive to many aspects of the effective interaction, a fact that renders perfect agreement with experiment out of reach for current functionals. Despite this inherent diffculty, the SLy5s1 and a modified UNEDF1^{SO} parameterization predict a qualitatively correct staggering that is off by two neutron numbers. MCSM calculations of states with the experimental spins and parities show good agreement for both electromagnetic moments and the observed charge radii. A clear mechanism for the origin of shape staggering within this context is identified: a substantial change in occupancy of the proton $πh_{9/2}$ and neutron $νi_{13/2}$ orbitals.

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arXiv2017

Study of the long-lived excited state in the neutron deficient nuclides $^{195,197,199}$Po by precision mass measurement

Direct mass measurements of the low-spin $3/2^{(-)}$ and high-spin $13/2^{(+)}$ states in the neutron-deficient isotopes $^{195}$Po, $^{197}$Po, and high-spin $13/2^{(+)}$ state in $^{199}$Po were performed with the Penning-trap mass spectrometer ISOLTRAP at ISOLDE-CERN. These measurements allow the determination of the excitation energy of the isomeric state arising from the $ν$i$_{13/2}$ orbital in $^{195,197}$Po. Additionally, the excitation energy of isomeric states of lead, radon, and radium isotopes in this region were obtained from $α$-decay chains. The new excitation energies complete the knowledge of the energy systematics in the region and confirm for the first time that the $13/2^{(+)}$ states remain isomeric, independent of the number of valence neutrons.

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arXiv2015

Precision Mass Measurements of 129-131Cd and Their Impact on Stellar Nucleosynthesis via the Rapid Neutron Capture Process

Masses adjacent to the classical waiting-point nuclide 130Cd have been measured by using the Penning- trap spectrometer ISOLTRAP at ISOLDE/CERN. We find a significant deviation of over 400 keV from earlier values evaluated by using nuclear beta-decay data. The new measurements show the reduction of the N = 82 shell gap below the doubly magic 132Sn. The nucleosynthesis associated with the ejected wind from type-II supernovae as well as from compact object binary mergers is studied, by using state-of-the-art hydrodynamic simulations. We find a consistent and direct impact of the newly measured masses on the calculated abundances in the A = 128 - 132 region and a reduction of the uncertainties from the precision mass input data.

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arXiv2015

Probing the N = 32 shell closure below the magic proton number Z = 20: Mass measurements of the exotic isotopes 52,53K

The recently confirmed neutron-shell closure at N = 32 has been investigated for the first time below the magic proton number Z = 20 with mass measurements of the exotic isotopes 52,53K, the latter being the shortest-lived nuclide investigated at the online mass spectrometer ISOLTRAP. The resulting two-neutron separation energies reveal a 3 MeV shell gap at N = 32, slightly lower than for 52Ca, highlighting the doubly-magic nature of this nuclide. Skyrme-Hartree-Fock-Boguliubov and ab initio Gorkov-Green function calculations are challenged by the new measurements but reproduce qualitatively the observed shell effect.

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