arXiv subjects

V. O. Nesterenko

Publications and source records attributed to V. O. Nesterenko.

72 records · Page 4Linked to original sources

arXiv2005

Self-Consistent Separable Rpa Approach for Skyrme Forces: Axial Nuclei

The self-consistent separable RPA (random phase approximation) method is formulated for Skyrme forces with pairing. The method is based on a general self-consistent procedure for factorization of the two-body interaction. It is relevant for various density- and current-dependent functionals. The contributions of the time-even and time-odd Skyrme terms as well as of the Coulomb and pairing terms to the residual interaction are taken self-consistently into account. Most of the expression have a transparent analytical form, which makes the method convenient for the treatment and analysis. The separable character of the residual interaction allows to avoid diagonalization of high-rank RPA matrices and thus to minimize the calculation effort. The previous studies have demonstrated high numerical accuracy and efficiency of the method for spherical nuclei. In this contribution, the method is specified for axial nuclei. We provide systematic and detailed presentation of formalism and discuss different aspects of the model.

nucl-th↗

arXiv2005

Practicable factorized TDLDA for arbitrary density- and current-dependent functionals

We propose a practicable method for describing linear dynamics of different finite Fermi systems. The method is based on a general self-consistent procedure for factorization of the two-body residual interaction. It is relevant for diverse density- and current-dependent functionals and, in fact, represents the self-consistent separable random-phase approximation (RPA), hence the name SRPA. SRPA allows to avoid diagonalization of high-rank RPA matrices and thus dwarfs the calculation expense. Besides, SRPA expressions have a transparent analytical form and so the method is very convenient for the analysis and treatment of the obtained results. SRPA demonstrates high numerical accuracy. It is very general and can be applied to diverse systems. Two very different cases, the Kohn-Sham functional for atomic clusters and Skyrme functional for atomic nuclei, are considered in detail as particular examples. SRPA treats both time-even and time-odd dynamical variables and, in this connection, we discuss the origin and properties of time-odd currents and densities in initial functionals. Finally, SRPA is compared with other self-consistent approaches for the excited states, including the coupled-cluster method.

physics.atm-clus↗

arXiv2005

Electronic excitations in atomic clusters: beyond dipole plasmon

Multipole electron modes beyond the Mie plasmon in atomic clusters are investigated within the time-dependent local density approximation theory (TDLDA). We consider the origin of the modes, their connection with basic cluster properties and possible routes of experimental observation. Particular attention is paid to infrared magnetic orbital modes, scissors and twist, and electric quadrupole mode. The scissors and twist modes determine orbital magnetism of clusters while the electric quadrupole mode provides direct access to the single electron spectra of the cluster. We examine two-photon processes (Raman scattering, stimulated emission pumping and stimulated adiabatic Raman passage) as the most promising tools for experimental investigation of the modes.

physics.atm-clus↗

arXiv2005

Two-Photon Excitation of Low-Lying Electronic Quadrupole States in Atomic Clusters

A simple scheme of population and detection of low-lying electronic quadrupole modes in free small deformed metal clusters is proposed. The scheme is analyzed in terms of the TDLDA (time-dependent local density approximation) calculations. As test case, the deformed cluster $Na^+_{11}$ is considered. Long-living quadrupole oscillations are generated via resonant two-photon (two-dipole) excitation and then detected through the appearance of satellites in the photoelectron spectra generated by a probe pulse. Femtosecond pump and probe pulses with intensities $I = 2\cdot 10^{10} - 2\cdot 10^{11} W/cm^2$ and pulse duration $T = 200 - 500$ fs are found to be optimal. The modes of interest are dominated by a single electron-hole pair and so their energies, being combined with the photoelectron data for hole states, allow to gather new information about mean-field spectra of valence electrons in the HOMO-LUMO region. Besides, the scheme allows to estimate the lifetime of electron-hole pairs and hence the relaxation time of electronic energy into ionic heat.

physics.atm-clus↗

arXiv2004

Momentum distribution in heavy deformed nuclei: role of effective mass

The impact of nuclear deformation on the momentum distributions (MD) of occupied proton states in $^{238}$U is studied with a phenomenological Woods-Saxon (WS) shell model and the self-consistent Skyrme-Hartree-Fock (SHF) scheme. Four Skyrme parameterizations (SkT6, SkM*, SLy6, SkI3) with different effective masses are used. The calculations reveal significant deformation effects in the low-momentum domain of $K^π=1/2^{\pm}$ states, mainly of those lying near the Fermi surface. For other states, the deformation effect on MD is rather small and may be neglected. The most remarkable result is that the very different Skyrme parameterizations and the WS potential give about identical MD. This means that the value of effective mass, being crucial for the description of the spectra, is not important for the spatial shape of the wave functions and thus for the MD. In general, it seems that, for the description of MD at $0\le k \le 300$ MeV/c, one may use any single-particle scheme (phenomenological or self-consistent) fitted properly to the global ground state properties.

nucl-th↗

arXiv2004

Infrared electron modes in light deformed clusters

Infrared quadrupole modes (IRQM) of the valence electrons in light deformed sodium clusters are studied by means of the time-dependent local-density approximation (TDLDA). IRQM are classified by angular momentum components $λμ=$20, 21 and 22 whose $μ$ branches are separated by cluster deformation. In light clusters with a low spectral density, IRQM are unambiguously related to specific electron-hole excitations, thus giving access to the single-electron spectrum near the Fermi surface (HOMO-LUMO region). Most of IRQM are determined by cluster deformation and so can serve as a sensitive probe of the deformation effects in the mean field. The IRQM branch $λμ=$21 is coupled with the magnetic scissors mode, which gives a chance to detect the latter. We discuss two-photon processes, Raman scattering (RS), stimulated emission pumping (SEP), and stimulated adiabatic Raman passage (STIRAP), as the relevant tools to observe IRQM. A new method to detect the IRQM population in clusters is proposed.

physics.atm-clus↗

arXiv2003

Low-energy quadrupole modes in deformed clusters

Properties of low-energy (infra-red) quadrupole modes (LEQM) of multipolarity $+AFw-lambda+AFw-mu =$20, 21 and 22 in deformed sodium clusters are studied within the Kohn-Sham LDA RPA approach. Possible manifestations of LEQM in stimulated Raman adiabatic passage (STIRAP) reaction are discussed. It is shown that, in free light clusters, where the low-energy spectrum is delute, LEQM can be unambiguously identified as particular electron-hole pairs. This gives a chance to reconstruct the mean field level scheme near the Fermi surface. Moreover, due to the connection with electric $+AFw-lambda+AFw-mu =$21 mode, the scissors mode can be detected. In heavy (supported) oblate clusters, LEQM are in general rather involved. Nevertheless, some interesting $+AFw-lambda+AFw-mu =$21 and 22 structures determined by specific deformation effects can be resolved. The origin of the structures is discussed in detail.

physics.atm-clus↗

arXiv2003

Deformation effects in low-momentum distributions of heavy nuclei

Momentum distributions (MD) of deep hole proton states in $^{238}$U are studied paying particular attention to the influence of deformation. Two essentially different mean-field models, Woods-Saxon (WS) and Skyrme-Hartree-Fock with the SkM$^*$ force, are used. Noticeable deviations between the WS and SkM$^*$ results are found. They are mainly due to the difference in effective nucleon mass. In particular, SkM$^*$ gives much weaker deformation effects at low momenta than WS. It is shown that, in spite of the deformation mixing, MD at low momenta can serve for identification of $K^π=1/2^+$ hole states originating from $s_{1/2}$ spherical sub-shells. Moreover, following the WS calculations, the deformation results in additional $K^π=1/2^+$ states with strong $l=0$ contributions. A possibility to probe such states in knock-out experiments is discussed.

nucl-th↗

arXiv2002

Orbital magnetism in axially deformed sodium clusters: From scissors mode to dia-para magnetic anisotropy

Low-energy orbital magnetic dipole excitations, known as scissors mode (SM), are studied in alkali metal clusters. Subsequent dynamic and static effects are explored. The treatment is based on a self-consistent microscopic approach using the jellium approximation for the ionic background and the Kohn-Sham mean field for the electrons. The microscopic origin of SM and its main features (structure of the mode in light and medium clusters, separation into low- and high-energy plasmons, coupling high-energy M1 scissors and E2 quadrupole plasmons, contributions of shape isomers, etc) are discussed. The scissors M1 strength acquires large values with increasing cluster size. The mode is responsible for the van Vleck paramagnetism of spin-saturated clusters. Quantum shell effects induce a fragile interplay between Langevin diamagnetism and van Vleck paramagnetism and lead to a remarkable dia-para anisotropy in magnetic susceptibility of particular light clusters. Finally, several routes for observing the SM experimentally are discussed.

physics.atm-clus↗

arXiv2002

Separable RPA for self-consistent nuclear models

Self-consistent factorization of two-body residual interaction is proposed for arbitrary density- and current-dependent energy functionals. Following this procedure, a separable RPA (SRPA) method is constructed. SRPA considerably simplifies the calculations and demonstrates quick convergence to exact results. The method is tested for SkI3 and SkM* forces.

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arXiv2002

Scissors modes in triaxial metal clusters

We study the scissors mode (orbital M1 excitations) in small Na clusters, triaxial metal clusters ${\rm Na}_{12}$ and ${\rm Na}_{16}$ and the close-to-spherical ${{\rm Na}_9}^+$, all described in DFT with detailed ionic background. The scissors modes built on spin-saturated ground and spin-polarized isomeric states are analyzed in virtue of both macroscopic collective and microscopic shell-model treatments. It is shown that the mutual destruction of Coulomb and the exchange-correlation parts of the residual interaction makes the collective shift small and the net effect can depend on details of the actual excited state. The crosstalk with dipole and spin-dipole modes is studied in detail. In particular, a strong crosstalk with spin-dipole negative-parity mode is found in the case of spin-polarized states. Triaxiality and ionic structure considerably complicate the scissors response, mainly at expense of stronger fragmentation of the strength. Nevertheless, even in these complicated cases the scissors mode is mainly determined by the global deformation. The detailed ionic structure destroys the spherical symmetry and can cause finite M1 response (transverse optical mode) even in clusters with zero global deformation. But its strength turns out to be much smaller than for the genuine scissors modes in deformed systems.

physics.atm-clus↗

arXiv2002

Quasi free electro fission of 238U

We present the result of a theoretical study of the quasi free electrofission of $^{238}$U. The exclusive differential cross sections for the quasi free scattering reaction stage have been calculated in PWIA, using a Macroscopic-Microscopic approach for the description of the proton bound states. The nuclear shape was parametrized in terms of cassinian ovaloids. The equilibrium deformation parameters have been calculated by minimizing the total nuclear energy. In the calculation the axially deformed Woods-Saxon single particle potential was used. The obtained single particle momentum distributions were averaged over the nuclear symmetry axis direction. The occupation numbers were calculated in the BCS approach. The fissility for the single hole excited states of the residual nucleus $^{237}$% Pa was calculated on the statistical theory grounds both without taking into account the pre-equilibrium emission of the particle, and with preequilibrium emission in the framework of the exciton model.

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arXiv2001

Electric multipole plasmons in deformed sodium clusters

The random-phase-approximation (RPA) method with separable residual forces (SRPA) is proposed for the description of multipole electric oscillations of valence electrons in deformed alkali metal clusters. Both the deformed mean field and residual interaction are derived self-consistently from the Kohn-Sham functional. SRPA drastically simplifies the computational effort which is urgent if not decisive for deformed systems. The method is applied to the description of dipole, quadrupole and octupole plasmons in deformed sodium clusters of a moderate size. We demonstrate that, in clusters with the size N>50, Landau damping successfully competes with deformation splitting and even becomes decisive in forming the width and gross structure of the dipole plasmon. Besides, the plasmon is generated by excitations from both ground state and shape isomers. In such clusters familiar experimental estimates for deformation splitting of dipole plasmon are useless.

physics.atm-clus↗

arXiv2001

Self-Consistent Separable RPA For Density- and Current-Dependent Forces

Self-consistent factorization of two-body residual interaction is proposed for arbitrary density- and current-dependent energy functionals. Following this procedure, a separable RPA (SRPA) method is constructed. SRPA dramatically simplifies the calculations and demonstrates quick convergence to exact results. The method is tested for SkM* forces.

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arXiv2000

Twist Mode in Spherical Alkali Metal Clusters

A remarkable orbital quadrupole magnetic resonance, so-called twist mode, is predicted in alkali metal clusters where it is represented by $I^π=2^-$ low-energy excitations of valence electrons with strong M2 transitions to the ground state. We treat the twist by both macroscopic and microscopic ways. In the latter case, the shell structure of clusters is fully exploited, which is crucial for the considered size region ($8\le N_e\le 1314$). The energy-weighted sum rule is derived for the pseudo-Hamiltonian. In medium and heavy spherical clusters the twist dominates over its spin-dipole counterpart and becomes the most strong multipole magnetic mode.

cond-mat.mes-hall↗

arXiv1999

Orbital Magnetic Dipole Mode in Deformed Clusters: A Fully Microscopic Analysis

The orbital M1 collective mode predicted for deformed clusters in a schematic model is studied in a self-consistent random-phase-approximation approach which fully exploits the shell structure of the clusters. The microscopic mechanism of the excitation is clarified and the close correlation with E2 mode established. The study shows that the M1 strength of the mode is fragmented over a large energy interval. In spite of that, the fraction remaining at low energy, well below the overwhelming dipole plasmon resonance, is comparable to the strength predicted in the schematic model. The importance of this result in view of future experiments is stressed.

physics.atm-clus↗

arXiv1999

A Variety of Giant Resonances in Metal Clusters

Multipole electric and magnetic giant resonances in metal clusters are reviewed and compared with their counterparts in atomic nuclei. The main attention is paid to E1 resonance (dipole plasmon).

physics.atm-clus↗

arXiv1999

Electromagnetic Modes in Deformed Nuclei

A strength function method is adopted to describe a coupling between electric and magnetic modes of different multipolarity. The collective vibrations are analysed for a separable residual interaction in the framework of the random-phase approximation. The coupling between $M2$ and $E1$ giant resonances is considered as an illustrative example.

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