arXiv subjects

V. Sandoghdar

Publications and source records attributed to V. Sandoghdar.

28 records · Page 2Linked to original sources

arXiv2007

Controlled coupling of counterpropagating whispering-gallery modes by a single Rayleigh scatterer: a classical problem in a quantum optical light

We present experiments where a single subwavelength scatterer is used to examine and control the back-scattering induced coupling between counterpropagating high-Q modes of a microsphere resonator. Our measurements reveal the standing wave character of the resulting symmetric and antisymmetric eigenmodes, their unbalanced intensity distributions, and the coherent nature of their coupling. We discuss our findings and the underlying classical physics in the framework common to quantum optics and provide a particularly intuitive explanation of the central processes.

quant-ph↗

arXiv2007

Near-field imaging and frequency tuning of a high-Q photonic crystal membrane microcavity

We discuss experimental studies of the interaction between a nanoscopic object and a photonic crystal membrane resonator of quality factor Q=55000. By controlled actuation of a glass fiber tip in the near-field of a photonic crystal, we constructed a complete spatio-spectral map of the resonator mode and its coupling with the fiber-tip. On the one hand, our findings demonstrate that scanning probes can profoundly influence the optical characteristics and the near-field images of photonic devices. On the other hand, we show that the introduction of a nanoscopic object provides a low-loss method for on-command tuning of a photonic crystal resonator frequency. Our results are in a very good agreement with the predictions of a combined numerical/analytical theory.

cond-mat.other↗

arXiv2007

Scanning Near-Field Optical Coherent Spectroscopy of Single Molecules at 1.4 Kelvin

We present scanning near-field extinction spectra of single molecules embedded in a solid matrix. By varying the molecule-tip separation, we modify the line shape of the spectra, demonstrating the coherent nature of the interaction between the incident laser light and the excited state of the molecule. We compare the measured data with the outcome of numerical calculations and find a very good agreement.

physics.optics↗

arXiv2006

Strong extinction of a laser beam by a single molecule

We present an experiment where a single molecule strongly affects the amplitude and phase of a laser field emerging from a subwavelength aperture. We achieve a visibility of -6% in direct and +10% in cross-polarized detection schemes. Our analysis shows that a close to full extinction should be possible using near-field excitation.

quant-ph↗

arXiv2006

On-command enhancement of single molecule fluorescence using a gold nanoparticle as an optical nano-antenna

We investigate the coupling of a single molecule to a single spherical gold nanoparticle acting as a nano-antenna. Using scanning probe technology, we position the particle in front of the molecule with nanometer accuracy and measure a strong enhancement of more than 20 times in the fluorescence intensity simultaneous to a 20-fold shortening of the excited state lifetime. Direct comparison with three-dimensional calculations allow us to decipher the contributions of the excitation enhancement, spontaneous emission modification, and quenching. Furthermore, we provide direct evidence for the role of the particle plasmon resonance in the modification of the molecular emission.

cond-mat.other↗

arXiv2006

Controlled photon transfer between two individual nanoemitters via shared high-Q modes of a microsphere resonator

We realize controlled cavity-mediated photon transfer between two single nanoparticles over a distance of several tens of micrometers. First, we show how a single nanoscopic emitter attached to a near-field probe can be coupled to high-Q whispering-gallery modes of a silica microsphere at will. Then we demonstrate transfer of energy between this and a second nanoparticle deposited on the sphere surface. We estimate the photon transfer efficiency to be about six orders of magnitude higher than that via free space propagation at comparable separations.

quant-ph↗

arXiv2005

Spontaneous emission rates of dipoles in photonic crystal membranes

We show theoretically that finite two-dimensional (2D) photonic crystals in thin semiconductor membranes strongly modify the spontaneous emission rate of embedded dipole emitters. Three-dimensional Finite-Difference Time-Domain calculations show over 7 times inhibition and 15 times enhancement of the emission rate compared to the vacuum emission rate for judiciously oriented and positioned dipoles. The vertical index confinement in membranes strongly enhances modifications of the emission rate as compared to vertically unconfined 2D photonic crystals. The emission rate modifications inside the membrane mimic the local electric field mode density in a simple 2D model. The inhibition of emission saturates exponentially as the crystal size around the source is increased, with a $1/e$ length that is inversely proportional to the bandwidth of the emission gap. We obtain inhibition of emission only close to the slab center. However, enhancement of emission persists even outside the membrane, with a distance dependence which dependence can be understood by analyzing the contributions to the spontaneous emission rate of the different vertically guided modes of the membrane. Finally we show that the emission changes can even be observed in experiments with ensembles of randomly oriented dipoles, despite the contribution of dipoles for which no gap exists.

cond-mat.other↗

arXiv2005

Optical microscopy via spectral modifications of a nano-antenna

The existing optical microscopes form an image by collecting photons emitted from an object. Here we report on the experimental realization of microscopy without the need for direct optical communication with the sample. To achieve this, we have scanned a single gold nanoparticle acting as a nano-antenna in the near field of a sample and have studied the modification of its intrinsic radiative properties by monitoring its plasmon spectrum.

physics.optics↗

arXiv2005

Measuring the quantum efficiency of single radiating dipoles using a scanning mirror

Using scanning probe techniques, we show the controlled manipulation of the radiation from single dipoles. In one experiment we study the modification of the fluorescence lifetime of a single molecular dipole in front of a movable silver mirror. A second experiment demonstrates the changing plasmon spectrum of a gold nanoparticle in front of a dielectric mirror. Comparison of our data with theoretical models allows determination of the quantum efficiency of each radiating dipole.

physics.optics↗

arXiv2004

Tuning of High-Q Photonic Crystal Microcavities by a Subwavelength Near-field Probe

We demonstrate that the resonance frequencies of high-Q microcavities in two-dimensional photonic crystal membranes can be tuned over a wide range by introducing a subwavelength dielectric tip into the cavity mode. Three-dimensional finite-difference time-domain (FDTD) simulations show that by varying the lateral and vertical positions of the tip, it is possible to tune the resonator frequency without lowering the quality factor. Excellent agreement with a perturbative theory is obtained, showing that the tuning range is limited by the ratio of the cavity mode volume to the effective polarizability of the nano-perturber.

cond-mat.other↗