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V. Sechovsky

Publications and source records attributed to V. Sechovsky.

14 recordsLinked to original sources
arXiv2025

Strange metallicity encompasses high magnetic field-induced superconductivity in UTe2

A strange metallic state - characterized by an electrical resistivity that rises linearly in temperature $T$ at a rate governed by Planckian energetic dissipation - is present in a number of unconventional superconductors. Despite widespread investigative efforts, the microscopic properties of strange metallicity continue to defy elementary description. Here we investigate heavy fermion UTe$_2$, which hosts a suite of exotic spin-triplet superconducting phases, the most extreme of which resides in a narrow angular window of intense magnetic fields $>$ 40 T. Through angle-dependent magnetotransport measurements in pulsed magnetic fields, we find that this superconductive phase emerges from a strange metallic state with Planckian $T$-linear resistivity confined to a small region of phase space where the field-induced superconductivity is strongest, suggesting a shared underlying mechanism. These findings reveal a novel setting for strange metallicity - in contrast to the general case of singlet superconductivity emerging on the border of antiferromagnetism, here strange metallicity accompanies field-induced triplet superconductivity within a spin-polarized magnetic state. This result demonstrates the remarkable ubiquity of strange metallicity across diverse materials settings, and highlights UTe$_2$ as a unique platform for exploring the interplay between unconventional superconductivity and quantum criticality.

cond-mat.str-el↗
arXiv2025

Suppression of ferromagnetism in van der Waals insulator due to pressure-induced layer stacking variation

Ferromagnetism in van der Waals insulators like CrBr3 is highly sensitive to structural modifications. We explore the pressure-driven structural and magnetic transformations of the van der Waals magnet CrBr3, establishing it as a model platform for phenomena emerging in layered vdW systems. Single-crystal X-ray diffraction revealed intrinsic trimorphism with two known phases (monoclinic and rhombohedral) and a so-far unreported trigonal phase. The paracrystal model well captures the coexistence of the rhombohedral and trigonal phases at ambient conditions. Increasing pressure drives the growth of the AA-stacked trigonal phase at the expense of the rhombohedral phase, which becomes undetectable above 8.4 GPa. Magnetization measurements provided the first direct evidence of a collapse of ferromagnetism above 5.8 GPa. This behavior is attributed to the increasing number of AFM-coupled Cr moments in AA stackings. Ab initio DFT calculations of electronic structure and atomistic simulations of finite-temperature magnetism corroborate the scenario.

cond-mat.mtrl-sci↗
arXiv2024

Pressure-enhanced $f$-electron orbital weighting in UTe2 mapped by quantum interferometry

The phase landscape of UTe$_2$ features a remarkable diversity of superconducting phases under applied pressure and magnetic field. Recent quantum oscillation studies at ambient pressure have revealed the quasi-2D Fermi surface of this material. However, the pressure-dependence of the Fermi surface remains an open question. Here we track the evolution of the UTe$_2$ Fermi surface as a function of pressure up to 19.5 kbar by measuring quantum interference oscillations. We find that in sufficient magnetic field to suppress both superconductivity at low pressures and incommensurate antiferromagnetism at higher pressures, the quasi-2D Fermi surface found at ambient pressure smoothly connects to that at 19.5 kbar, with no signs of a reconstruction over this pressure interval. We observe a smooth increase in oscillatory frequency with increasing pressure, indicating that the warping of the cylindrical Fermi sheets continuously increases with pressure. By computing a tight-binding model, we show that this enhanced warping indicates increased $f$-orbital contribution at the Fermi level - up to and beyond the critical pressure at which superconductivity is truncated. These findings highlight the value of high-pressure quantum interference measurements as a new probe of the electronic structure in heavy fermion materials.

cond-mat.supr-con↗
arXiv2024

A quantum critical line bounds the high field metamagnetic transition surface in UTe$_2$

Quantum critical phenomena are widely studied across various materials families, from high temperature superconductors to magnetic insulators. They occur when a thermodynamic phase transition is suppressed to zero temperature as a function of some tuning parameter such as pressure or magnetic field. This generally yields a point of instability - a so-called quantum critical point - at which the phase transition is driven exclusively by quantum fluctuations. Here we show that the heavy fermion metamagnet UTe$_2$ possesses a quantum phase transition at extreme magnetic field strengths of over 70 T. Rather than terminating at one singular point, we find that the phase boundary is sensitive to magnetic field components in each of the three Cartesian axes of magnetic field space. This results in the three-dimensional transition surface being bounded by a continuous ring of quantum critical points, the locus of which forms an extended line of quantum criticality - a novel form of quantum critical phase boundary. Within this quantum critical line sits a magnetic field-induced superconducting state in a toroidal shape, which persists to fields over 70~T. We model our data by a phenomenological free energy expansion, and show how a three-dimensional quantum critical phase boundary - rather than a more conventional singular point of instability - anchors the remarkable high magnetic field phase landscape of UTe$_2$.

cond-mat.supr-con↗
arXiv2023

Quantum interference between quasi-2D Fermi surface sheets in UTe2

UTe$_2$ is a spin-triplet superconductor candidate for which high quality samples with long mean free paths have recently become available, enabling quantum oscillation measurements to probe its Fermi surface and effective carrier masses. It has recently been reported that UTe$_2$ possesses a 3D Fermi surface component [Phys. Rev. Lett. 131, 036501 (2023)]. The distinction between 2D and 3D Fermi surface sections in triplet superconductors can have important implications regarding the topological properties of the superconductivity. Here we report the observation of oscillatory components in the magnetoconductance of UTe$_2$ at high magnetic fields. We find that these oscillations are well described by quantum interference between quasiparticles traversing semiclassical trajectories spanning magnetic breakdown networks. Our observations are consistent with a quasi-2D model of this material's Fermi surface based on prior dHvA-effect measurements. Our results strongly indicate that UTe$_2$ -- which exhibits a multitude of complex physical phenomena -- possesses a remarkably simple Fermi surface consisting exclusively of two quasi-2D cylindrical sections.

cond-mat.supr-con↗
arXiv2023

Enhanced triplet superconductivity in next generation ultraclean UTe2

The unconventional superconductor UTe$_2$ exhibits numerous signatures of spin-triplet superconductivity -- a rare state of matter which could enable quantum computation protected against decoherence. UTe$_2$ possesses a complex phase landscape comprising two magnetic field-induced superconducting phases, a metamagnetic transition to a field-polarised state, along with pair- and charge-density wave orders. However, contradictory reports between studies performed on UTe$_2$ specimens of varying quality have severely impeded theoretical efforts to understand the microscopic origins of the exotic superconductivity. Here, we report a comprehensive suite of high magnetic field measurements on a new generation of pristine quality UTe$_2$ crystals. Our experiments reveal a significantly revised high magnetic field superconducting phase diagram in the ultraclean limit, showing a pronounced sensitivity of field-induced superconductivity to the presence of crystalline disorder. We employ a Ginzburg-Landau model that excellently captures this acute dependence on sample quality. Our results suggest that in close proximity to a field--induced metamagnetic transition the enhanced role of magnetic fluctuations -- that are strongly suppressed by disorder -- is likely responsible for tuning UTe$_2$ between two distinct spin-triplet superconducting phases.

cond-mat.supr-con↗
arXiv2023

Quasi-2D Fermi surface in the anomalous superconductor UTe2

The heavy fermion paramagnet UTe$_2$ exhibits numerous characteristics of spin-triplet superconductivity. Efforts to understand the microscopic details of this exotic superconductivity have been impeded by uncertainty regarding the underlying electronic structure. Here we directly probe the Fermi surface of UTe$_2$ by measuring magnetic quantum oscillations in pristine quality crystals. We find an angular profile of quantum oscillatory frequency and amplitude that is characteristic of a quasi-2D Fermi surface, which we find is well described by two cylindrical Fermi sheets of electron- and hole-type respectively. Additionally, we find that both cylindrical Fermi sheets possess considerable undulation but negligible small-scale corrugation, which may allow for their near-nesting and therefore promote magnetic fluctuations that enhance the triplet pairing mechanism. Importantly, we find no evidence for the presence of any 3D Fermi surface sections. Our results place strong constraints on the possible symmetry of the superconducting order parameter in UTe$_2$.

cond-mat.supr-con↗
arXiv2021

Magnetic anisotropy in van-der-Waals ferromagnet VI3

A comprehensive study of magnetocrystalline anisotropy of a layered van-der-Waals ferromagnet VI3 was performed. We measured angular dependences of the torque and magnetization with respect to the direction of the applied magnetic field within the "ac" plane perpendicular to and within the basal ab plane, respectively. A two-fold butterfly-like signal was detected by magnetization in the perpendicular "ac" plane. This signal symmetry remains conserved throughout all magnetic regimes as well as through the known structural transition down to the lowest temperatures. The maximum of the magnetization signal and the resulting magnetization easy axis is significantly tilted from the principal c axis by ~40{\deg}. The close relation of the magnetocrystalline anisotropy to the crystal structure was documented. In contrast, a two-fold-like angular signal was detected in the paramagnetic region within the ab plane in the monoclinic phase, which transforms into a six-fold-like signal below the Curie temperature TC. With further cooling, another six-fold-like signal with an angular shift of ~30{\deg} grows approaching TFM. Below TFM, in the triclinic phase, the original six-fold-like signal vanishes, being replaced by a secondary six-fold-like signal with an angular shift of ~30{\deg}.

cond-mat.mtrl-sci↗
arXiv2020

Magnetic and electronic phases of U$_\mathbf{2}$Rh$_\mathbf{3}$Si$_\mathbf{5}$

We present a detailed study of the magnetic and electronic properties of U$_2$Rh$_3$Si$_5$, a material that has been demonstrated to exhibit a first order antiferromagnetic phase transition. From a high magnetic field study, together with extensive experiments in moderate fields, we establish the magnetic phase diagrams for all crystallographic directions. The possibility of an electronic phase in a narrow interval above the N\'eel temperature as a precursor of a magnetic phase is discussed.

cond-mat.str-el↗
arXiv2016

Topological insulator homojunctions including magnetic layers: the example of n-p type ($n$-QLs Bi$_2$Se$_3$/Mn-Bi$_2$Se$_3$) heterostructures

Homojunctions between Bi$_2$Se$_3$ and its Mn-doped phase are investigated as a sample geometry to study the influence of spin degrees of freedom on topological insulator properties. $n$ quintuple layers (QLs) of Bi$_2$Se$_3$ are grown ontop of Mn-doped Bi$_2$Se$_3$ by molecular beam epitaxy for $0\le n \le 30\,$QLs, allowing to unhamperedly monitor the development of electronic and topological properties by surface sensitive techniques like angle resolved photoemission spectroscopy. With increasing $n$, a Mn-induced gap at the Dirac point is gradually filled in an "hourglass" fashion to reestablish a topological surface state at $n \sim 9\,$QLs. Our results suggest a competition of upwards and downwards band bending effects due to the presence of an n-p type interface, which can be used to tailor topological and quantum well states independently.

cond-mat.mtrl-sci↗
arXiv2012

Magnetic Phase Diagram of the new Heavy Fermion Compound Ce2PtIn8

We report on the discovery and investigation of a new 218 heavy fermion compound. Crystals have been synthesized from In-flux. Structurally, Ce2PtIn8 is located between the cubic CeIn3 and the more two-dimensional CeTIn5 (T = transition metal) type of compounds. The weak anisotropy of the paramagnetic susceptibility suggests rather 3D magnetic correlations. Specific heat, electrical resistivity and magnetization measurements revealed that Ce2PtIn8 orders antiferromagnetically below Tn = 2.1 K. An order-to-order transition is observed at Tm = 2 K. Similarities in the H - T phase diagram to other CenTmIn3n+2m (T = Rh, Pt) compounds point to a pressure-induced quantum phase transition (QPT) which, according to the tentative location of Ce2PtIn8 in the recent proposed global phase diagram for QPT, would be of spin density wave type.

cond-mat.str-el↗
arXiv2010

Samarium Magnetism Studied on SmPd2Al3 Single Crystal

In this paper, specific features of Sm magnetism in an intermetallic compound have been studied. For this purpose, a high-quality single crystal of SmPd2Al3 was grown and subjected to detailed measurements of specific heat, magnetization, ac susceptibility, and electrical resistivity with respect to temperature and a magnetic field applied along the principal crystallographic directions. SmPd2Al3 magnetism was found to be strongly anisotropic with the easy-magnetization direction along the c axis where the main magnetic features are concentrated. The a-axis response remains weak, paramagneticlike, even in the magnetically ordered state. Ferromagnetism with TC=12.4 K has been indicated by all the measured physical properties. At lower temperatures, three successive order-order phase transitions have been observed on the temperature dependence of the specific heat as three anomalies: at 3.4, 3.9, and 4.4 K, respectively. The low-temperature magnetization data can be understood within a scenario that considers the antiferromagnetic ground state as being gradually destroyed through a series of four metamagnetic transitions at 0.03, 0.35, 0.5, and 0.75 T, as detected in the 1.8 K magnetization data. The experimental data are discussed together with the results of electronic-structure and crystal-field calculations from first principles, which were performed as an important part of the study for comprehension and explanation of the observed behavior of the SmPd2Al3 compound.

cond-mat.str-el↗
arXiv2007

Anomalous magnetoresistance of EuB$_{5.99}$C$_{0.01}$: Enhancement of magnetoresistance in systems with magnetic polarons

We present results of measurements of electrical, magnetic and thermal properties of EuB$_{5.99}$C$_{0.01}$. The observed anomalously large negative magnetoresistance as above, so below the Curie temperature of ferromagnetic ordering $T_C$ is attributed to fluctuations in carbon concentration. Below $T_C$ the carbon richer regions give rise to helimagnetic domains, which are responsible for an additional scattering term in the resistivity, which can be suppressed by a magnetic field. Above $T_C$ these regions prevent the process of percolation of magnetic polarons (MPs), acting as "spacers" between MPs. We propose that such "spacers", being in fact volumes incompatible with existence of MPs, may be responsible for the decrease of the percolation temperature and for the additional (magneto)resistivity increase in systems with MPs.

cond-mat.mtrl-sci↗