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V. Sitaraman

Publications and source records attributed to V. Sitaraman.

8 recordsLinked to original sources

Direct measurement of $^{18}$F($\alpha,p$)$^{21}$Ne cross sections with ANASEN

The $^{18}$F($\alpha,p$)$^{21}$Ne reaction may impact Asymptotic Giant Branch nucleosynthesis and helium burning on accreting white dwarfs. This reaction has never been directly measured, and constraints from a previous time-inverse measurement leave large uncertainties in the reaction rate. We measured $^{18}$F($\alpha,p$)$^{21}$Ne cross sections directly for the first time covering from $2 \leq E_{cm} \leq 4$ MeV. Combining these results with previous work and comparisons to statistical model calculations results in a substantial improvement in uncertainties in the reaction rate. Cross sections were measured in inverse kinematics at TRIUMF-ISAC using a radioactive $^{18}$F beam and ANASEN with an extended $^{4}$He gas target. Protons were detected in arrays of silicon-strip detectors with the measured trajectories and energies allowing reconstruction of the center-of-mass energy and final state in $^{21}$Ne populated. We found the total cross section is in good agreement with statistical calculations, though population of the second excited state in $^{21}$Ne is greater than predicted. This direct measurement is combined with the previous time-inverse measurement and a new reaction rate is calculated for 0.1--3 GK. The uncertainties in the $^{18}$F($\alpha,p$)$^{21}$Ne reaction rate have been reduced to a sufficient level to allow robust predictions from AGB models. The new recommended rate leads to a 45\% increase in $^{19}$F production compared to the previous rate.

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Excited states of $^{148}$Nd studied via the $^{150}$Nd$(p,t){}^{148}$Nd reaction and the observation of possible low-spin two-phonon octupole states at $N=88$

We report new data from a $^{150}$Nd$(p,t){}^{148}$Nd experiment performed at the John D. Fox Accelerator Laboratory of Florida State University. In total, 54 excited states of $^{148}$Nd were observed up to an excitation energy of 3500 keV. In this work, we focus on $0^+$ states and their band members. In contrast to previous work, the $0^+_3$ band is proposed as the candidate for the two-phonon octupole vibrational band. Supporting $spdf$ IBM-1 calculations are presented. To test the robustness of the IBM calculations, several observables were interrogated and are discussed in this publication. In addition, we make the case that neither the $0^+_2$ nor the $0^+_3$ states of the other $N=88$ isotones are likely good candidates for two-phonon octupole states. Based on our new data for $^{148}$Nd, we propose candidates in $^{150}$Sm and $^{152}$Gd. Using available $\gamma$-decay data for states with moderate spins in the yrast sequence and a comparison to IBM calculations, we also show how the staggering of the $B(E1)/B(E2)$ ratios in the yrast sequence can possibly be used to probe the appearance of bands with multiple octupole phonons.

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The ICESPICE demonstrator for particle/$\gamma$-$e^{-}$ coincidence experiments at Florida State University

The Internal Conversion Electron SPectrometer In Coincidence Experiments (ICESPICE) demonstrator has been developed at Florida State University to enable particle/gamma-electron coincidence measurements in low-energy nuclear structure studies. ICESPICE is based on the mini-orange spectrometer concept and features a modular design using commercially available permanent magnets arranged in toroidal configurations to transport internal conversion electrons to room-temperature PIPS detectors while suppressing background from undesired particles. The system was optimized through SolidWorks modeling, COMSOL magnetic field simulations, and Geant4 particle tracking to maximize the magnetic transmission probability for electrons around 1 MeV. Commissioning tests using a calibrated 207Bi source demonstrated the performance of multiple spectrometer-detector configurations. Coincidence measurements between CeBr3 detectors from the CeBrA array and PIPS detectors revealed clear gamma-electron correlations. The first in-beam particle-electron measurements using ICESPICE were performed with the Super-Enge Split-Pole Spectrograph (SE-SPS) in the 208Pb(d,t)207Pb reaction. Prompt coincidences between tritons detected with the SE-SPS and electrons detected with ICESPICE were observed. The presented results show that ICESPICE is a promising ancillary detector system for in-beam internal conversion electron spectroscopy at the FSU SE-SPS.

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Properties of states in \textsuperscript{19}Ne important for the \textsuperscript{18}F$(p,\alpha)$\textsuperscript{15}O reaction rate

Observation of the 511-keV positron-annihilation line would be a powerful probe of classical novae, with the primary source of positrons likely from the $\beta^+$ decay of \textsuperscript{18}F. We have determined the properties of important resonances in $^{19}$Ne which govern the \textsuperscript{18}F($p,\alpha$)\textsuperscript{15}O reaction rate and the production of \textsuperscript{18}F in novae. Measured $\alpha$ and proton angular distributions from states populated in the \textsuperscript{19}F(\textsuperscript{3}He,$t$)\textsuperscript{19}Ne reaction identified six near-threshold proton $s$-wave \textsuperscript{18}F$+p$ ($L_p=0$) states, and the asymptotic normalization of these states was studied using the symmetry-adapted no-core shell model. We have improved our understanding of states contributing to the \textsuperscript{18}F($p,\alpha$)\textsuperscript{15}O reaction rate and show that earlier studies significantly underestimated the uncertainties.

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Experimental study of $^{53}$Cr via the $(d,p\gamma)$ reaction

Excited states in $^{53}$Cr were studied via the $^{52}$Cr$(d,p\gamma)$ reaction up to the neutron-separation threshold. Proton-$\gamma$ angular correlations and $\gamma$ decay branching ratios were measured in particle-$\gamma$ coincidences between the Super-Enge Split-Pole Spectrograph (SE-SPS) and CeBr$_3$ Array (CeBrA) demonstrator of the John D. Fox Accelerator Laboratory at Florida State University. Previous spin-parity assignments from a $(d,p)$ singles experiment at the SE-SPS are supported and $\gamma$-ray transitions in $^{53}$Cr reported. We firmly assign higher-lying excited states to $^{53}$Cr because overlapping excited states and contaminants could be identified better due to the complementary $\gamma$-decay information. We also correct some of the previously reported excitation energies and present a reanalysis of previously measured $^{52}$Cr$(d,p){}^{53}${Cr} angular distributions guided by the complementary $\gamma$-ray information. Based on this reanalysis, the fragmentation of the neutron $2p_{3/2}$, $2p_{1/2}$, $1f_{5/2}$, $1g_{9/2}$, and $2d_{5/2}$ single-particle strengths is reassessed for $^{53}$Cr. A comparison to the corresponding strengths in $^{55}$Fe is presented.

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Single-Neutron Adding on $^{34}$S

Purpose: Single-neutron adding data was collected in order to determine the distribution of the single-neutron strength of the $0f_{7/2}$, $1p_{3/2}$, $1p_{1/2}$ and $0f_{5/2}$ orbitals outside of $Z=16, N=18$, $^{34}$S. Methods: The $^{34}$S($d$,$p$)$^{35}$S reaction has been measured at 8 MeV/u to investigate cross sections to excited states in $^{35}$S. Outgoing proton yields and momenta were analyzed by the Super-Enge Split-Pole Spectrograph in conjunction with the CeBrA demonstrator located at the John D. Fox Laboratory at Florida State University. Angular distributions were compared with Distorted Wave Born Approximation calculations in order to extract single-neutron spectroscopic overlaps. Results: Spectroscopic overlaps and strengths were determined for states in $^{35}$S up through 6 MeV in excitation energy. Each orbital was observed to have fragmented strength where a single level carried the majority. The single-neutron centroids of the $0f_{7/2}$, $1p_{3/2}$, $1p_{1/2}$ and $0f_{5/2}$ orbitals were determined to be $2360^{+90}_{-40}$ keV, $3280^{+80}_{-50}$ keV, $4780^{+60}_{-40}$ keV, and $\gtrsim7500$ keV, respectively. Conclusion: A previous discrepancy in the literature with respect to distribution of the neutron $1p_{1/2}$ strength was resolved. The integration of the normalized spectroscopic strengths, up to 5.1 MeV in excitation energy, revealed fully-vacant occupancies for the $0f_{7/2}$, $1p_{3/2}$, and $1p_{1/2}$ orbitals, as expected. The spacing in the single-neutron energies highlighted a reduction in the traditional $N=28$ shell-gap, relative to both the $1p$ spin-orbit energy difference ($N=32$) and the lower limit on the $N=34$ shell spacing.

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Suppressed Electric Quadrupole Collectivity in $^{49}$Ti

Single-step Coulomb excitation of $^{46,48,49,50}$Ti is presented. A complete set of $E2$ matrix elements for the quintuplet of states in $^{49}$Ti, centered on the $2^+$ core excitation, was measured for the first time. A total of nine $E2$ matrix elements are reported, four of which were previously unknown. $^{49}_{22}$Ti$_{27}$ shows a $20\%$ quenching in electric quadrupole transition strength as compared to its semi-magic $^{50}_{22}$Ti$_{28}$ neighbour. This $20\%$ quenching, while empirically unprecedented, can be explained with a remarkably simple two-state mixing model, which is also consistent with other ground-state properties such as the magnetic dipole moment and electric quadrupole moment. A connection to nucleon transfer data and the quenching of single-particle strength is also demonstrated. The simplicity of the $^{49}$Ti-$^{50}$Ti pair (i.e., approximate single-$j$ $0f_{7/2}$ valence space and isolation of yrast states from non-yrast states) provides a unique opportunity to disentangle otherwise competing effects in the ground-state properties of atomic nuclei, the emergence of collectivity, and the role of proton-neutron interactions.

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The CeBrA demonstrator for particle-$γ$ coincidence experiments at the FSU Super-Enge Split-Pole Spectrograph

We report on a highly selective experimental setup for particle-$γ$ coincidence experiments at the Super-Enge Split-Pole Spectrograph (SE-SPS) of the John D. Fox Superconducting Linear Accelerator Laboratory at Florida State University (FSU) using fast CeBr$_3$ scintillators for $γ$-ray detection. Specifically, we report on the results of characterization tests for the first five CeBr$_3$ scintillation detectors of the CeBr$_3$ Array (CeBrA) with respect to energy resolution and timing characteristics. We also present results from the first particle-$γ$ coincidence experiments successfully performed with the CeBrA demonstrator and the FSU SE-SPS. We show that with the new setup, $γ$-decay branching ratios and particle-$γ$ angular correlations can be measured very selectively using narrow excitation energy gates, which are possible thanks to the excellent particle energy resolution of the SE-SPS. In addition, we highlight that nuclear level lifetimes in the nanoseconds regime can be determined by measuring the time difference between particle detection with the SE-SPS focal-plane scintillator and $γ$-ray detection with the fast CeBrA detectors. Selective excitation energy gates with the SE-SPS exclude any feeding contributions to these lifetimes.

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