arXiv subjects

V. V. Dobrovitski

Publications and source records attributed to V. V. Dobrovitski.

At least 55 records · Page 3Linked to original sources

arXiv2008

Excited-state spectroscopy using single-spin manipulation in diamond

We use single-spin resonant spectroscopy to study the spin structure in the orbital excited-state of a diamond nitrogen-vacancy center at room temperature. We find that the excited state spin levels have a zero-field splitting that is approximately half of the value of the ground state levels, a g-factor similar to the ground state value, and a hyperfine splitting ~20x larger than in the ground state. In addition, the width of the resonances reflects the electronic lifetime in the excited state. We also show that the spin-splitting can significantly differ between NV centers, likely due to the effects of local strain, which provides a pathway to control over the spin Hamiltonian and may be useful for quantum information processing.

quant-ph↗

arXiv2008

Geometric Control Over the Motion of Magnetic Domain Walls

We propose a method, which enables precise control of magnetic patterns, relying only on the fundamental properties of the wire and the choice of the path in the controlled parameter space but not on the rate of motion along this path. Possible experimental realizations of this mechanism are discussed. In particular, we show that the domain walls in magnetic nanowires can be translated by rotation of the magnetic easy axis, or by applying pulses of magnetic field directed transverse to the magnetic easy axis.

cond-mat.mtrl-sci↗

arXiv2008

Correlation effects in the electronic structure of Mn$_4$ molecular magnet

We present joint theoretical-experimental study of the correlation effects in the electronic structure of (pyH)$_3$[Mn$_4$O$_3$Cl$_7$(OAc)$_3$]$\cdot$2MeCN molecular magnet (Mn$_4$). Describing the many-body effects by cluster dynamical mean-field theory, we find that Mn$_4$ is predominantly Hubbard insulator with strong electron correlations. The calculated electron gap (1.8 eV) agrees well with the results of optical conductivity measurements, while other methods, which neglect many-body effects or treat them in a simplified manner, do not provide such an agreement. Strong electron correlations in Mn$_4$ may have important implications for possible future applications.

cond-mat.mtrl-sci↗

arXiv2008

Magnetic field of Josephson vortices outside superconductors

We consider the structure of Josephson vortices approaching the junction boundary with vacuum in large area Josephson junctions with the Josephson length $λ_J$ large relative to the London penetration depth $λ_L$. Using the stability argument for one-dimentional solitons with respect to 2D perturbations, it is shown that on the scale $λ_J$ the Josephson vortices do not spread near the boundary in the direction of the junction. %, which is in a striking difference with behavior of Abrikosov vortices exiting superconductors. The field distribution in vacuum due to the Josephson vortex is evaluated, the information needed for the Scanning SQUID Microscopy.

cond-mat.supr-con↗

arXiv2008

Long-time electron spin storage via dynamical suppression of hyperfine-induced decoherence in a quantum dot

The coherence time of an electron spin decohered by the nuclear spin environment in a quantum dot can be substantially increased by subjecting the electron to suitable dynamical decoupling sequences. We analyze the performance of high-level decoupling protocols by using a combination of analytical and exact numerical methods, and by paying special attention to the regimes of large inter-pulse delays and long-time dynamics, which are outside the reach of standard average Hamiltonian theory descriptions. We demonstrate that dynamical decoupling can remain efficient far beyond its formal domain of applicability, and find that a protocol exploiting concatenated design provides best performance for this system in the relevant parameter range. In situations where the initial electron state is known, protocols able to completely freeze decoherence at long times are constructed and characterized. The impact of system and control non-idealities is also assessed, including the effect of intra-bath dipolar interaction, magnetic field bias and bath polarization, as well as systematic pulse imperfections. While small bias field and small bath polarization degrade the decoupling fidelity, enhanced performance and temporal modulation result from strong applied fields and high polarizations. Overall, we find that if the relative errors of the control parameters do not exceed 5%, decoupling protocols can still prolong the coherence time by up to two orders of magnitude.

cond-mat.mes-hall↗

arXiv2008

Suppression of electron spin decoherence in a quantum dot

The dominant source of decoherence for an electron spin in a quantum dot is the hyperfine interaction with the surrounding bath of nuclear spins. The decoherence process may be slowed down by subjecting the electron spin to suitable sequences of external control pulses. We investigate the performance of a variety of dynamical decoupling protocols using exact numerical simulation. Emphasis is given to realistic pulse delays and the long-time limit, beyond the domain where available analytical approaches are guaranteed to work. Our results show that both deterministic and randomized protocols are capable to significantly prolong the electron coherence time, even when using control pulse separations substantially larger than what expected from the {\em upper cutoff} frequency of the coupling spectrum between the electron and the nuclear spins. In a realistic parameter range, the {\em total width} of such a coupling spectrum appears to be the physically relevant frequency scale affecting the overall quality of the decoupling.

cond-mat.mes-hall↗

arXiv2007

Dynamical control of electron spin coherence in a quantum dot

We investigate the performance of dynamical decoupling methods at suppressing electron spin decoherence from a low-temperature nuclear spin reservoir in a quantum dot. The controlled dynamics is studied through exact numerical simulation, with emphasis on realistic pulse delays and long-time limit. Our results show that optimal performance for this system is attained by a periodic protocol exploiting concatenated design, with control rates substantially slower than expected from the upper spectral cutoff of the bath. For a known initial electron spin state, coherence can saturate at long times, signaling the creation of a stable ``spin-locked'' decoherence-free subspace. Analytical insight on saturation is obtained for a simple echo protocol, in good agreement with numerical results.

cond-mat.mes-hall↗

arXiv2006

Hyperfine interaction induced decoherence of electron spins in quantum dots

We investigate in detail, using both analytical and numerical tools, the decoherence of electron spins in quantum dots (QDs) coupled to a bath of nuclear spins in magnetic fields or with various initial bath polarizations, focusing on the longitudinal relaxation in low and moderate field/polarization regimes. An increase of the initial polarization of nuclear spin bath has the same effect on the decoherence process as an increase of the external magnetic field, namely, the decoherence dynamics changes from smooth decay to damped oscillations. This change can be observed experimentally for a single QD and for a double-QD setup. Our results indicate that substantial increase of the decoherence time requires very large bath polarizations, and the use of other methods (dynamical decoupling or control of the nuclear spins distribution) may be more practical for suppressing decoherence of QD-based qubits.

cond-mat.mes-hall↗

arXiv2006

Long-lived memory for electronic spin in a quantum dot: Numerical analysis

Techniques for coherent control of electron spin-nuclear spin interactions in quantum dots can be directly applied in spintronics and in quantum information processing. In this work we study numerically the interaction of electron and nuclear spins in the context of storing the spin-state of an electron in a collective state of nuclear spins. We take into account the errors inherent in a realistic system: the incomplete polarization of the bath of nuclear spins and the different hyperfine interactions between the electron and individual nuclei in the quantum dot. Although these imperfections deteriorate the fidelity of the quantum information retrieval, we find reasonable fidelities are achievable for modest bath polarizations.

cond-mat.mes-hall↗

arXiv2005

Numerical modeling of the central spin problem using the spin coherent states P-representation

In this work, we consider decoherence of a central spin by a spin bath. In order to study the non-perturbative decoherence regimes, we develop an efficient mean-field-based method for modeling the spin-bath decoherence, based on the P-representation of the central spin density matrix. The method can be applied to longitudinal and transversal relaxation at different external fields. In particular, by modeling large-size quantum systems (up to 16000 bath spins), we make controlled predictions for the slow long-time decoherence of the central spin.

cond-mat.mes-hall↗

arXiv2005

Parity Effects in Spin Decoherence

We demonstrate that decoherence of many-spin systems can drastically differ from decoherence of single-spin systems. The difference originates at the most basic level, being determined by parity of the central system, i.e. by whether the system comprises even or odd number of spin-1/2 entities. Therefore, it is very likely that similar distinction between the central spin systems of even and odd parity is important in many other situations. Our consideration clarifies the physical origin of the unusual two-step decoherence found previously in the two-spin systems.

quant-ph↗

arXiv2004

Decoherence by a chaotic many-spin bath

We numerically investigate decoherence of a two-spin system (central system) by a bath of many spins 1/2. By carefully adjusting parameters, the dynamical regime of the bath has been varied from quantum chaos to regular, while all other dynamical characteristics have been kept practically intact. We explicitly demonstrate that for a many-body quantum bath, the onset of quantum chaos leads to significantly faster and stronger decoherence compared to an equivalent non-chaotic bath. Moreover, the non-diagonal elements of the system's density matrix decay differently for chaotic and non-chaotic baths. Therefore, knowledge of the basic parameters of the bath (strength of the system-bath interaction, bath's spectral density of states) is not always sufficient, and much finer details of the bath's dynamics can strongly affect the decoherence process.

quant-ph↗

arXiv2003

Decoherence in quantum spin systems

Computer simulations of decoherence in quantum spin systems require the solution of the time-dependent Schrodinger equation for interacting quantum spin systems over extended periods of time. We use exact diagonalization, Chebyshev polynomial technique, four Suzuki-formula algorithms, and the short-iterative-Lanczos method to solve a simple model for decoherence of a quantum spin system by an environment consisting of quantum spins, and compare advantages and limitations of different algorithms.

quant-ph↗

arXiv2003

An efficient scheme for numerical simulations of the spin-bath decoherence

We demonstrate that the Chebyshev expansion method is a very efficient numerical tool for studying spin-bath decoherence of quantum systems. We consider two typical problems arising in studying decoherence of quantum systems consisting of few coupled spins: (i) determining the pointer states of the system, and (ii) determining the temporal decay of quantum oscillations. As our results demonstrate, for determining the pointer states, the Chebyshev-based scheme is at least a factor of 8 faster than existing algorithms based on the Suzuki-Trotter decomposition. For the problems of second type, the Chebyshev-based approach has been 3--4 times faster than the Suzuki-Trotter-based schemes. This conclusion holds qualitatively for a wide spectrum of systems, with different spin baths and different Hamiltonians.

quant-ph↗

arXiv2002

Electronic structure of magnetic molecules V15: LDA+U calculations, X-ray emission and photoelectron spectra

Electronic structure of V$_{15}$ magnetic molecules (K$_6$ [V$_{15}$ As$_6$ O$_{42}$ (H$_2$O)] \cdot 8H$_2$O)$ has been studied using LSDA+U band structure calculations, and measurements of X-ray photoelectron (valence band, core levels) and X-ray fluorescence spectra (vanadium K$β_5$ and L$_{2,3}$, and oxygen K$α$). Experiments confirm that vanadium ions are tetravalent in V$_{15}$, and their local atomic structure is close to that of CaV$_3$O$_7$. Comparison of experimental data with the results of electronic structure calculations show that the LSDA+U method provides a description of the electronic structure of V$_{15}$ which agrees well with experiments.

cond-mat.mtrl-sci↗

arXiv2002

Destruction of the Kondo effect by a local measurement

We show that the local spin measurement which decoheres the localized spin in a Kondo system, suppresses the Abrikosov-Suhl resonance and destroys the Kondo effect. This happens due to elimination of the entanglement between the localized spin and the conduction electrons, and differs essentially from smearing of the resonance by dissipation. Considering decoherence by a spin bath, we predict that the Kondo effect disappears when the Kondo temperature becomes smaller than the coupling with a bath. This effect can be detected in experiments on ``quantum corrals'' or quantum dots doped by impurities with internal degrees of freedom.

cond-mat.mes-hall↗

arXiv2002

Many-spin effects and tunneling splittings in Mn12 magnetic molecules

We calculate the tunneling splittings in a Mn$_{12}$ magnetic molecule taking into account its internal many-spin structure. We discuss the precision and reliability of these calculations and show that restricting the basis (limiting the number of excitations taken into account) may lead to significant error (orders of magnitude) in the resulting tunneling splittings for the lowest energy levels, so that an intuitive picture of different decoupled energy scales does not hold in this case. Possible routes for further development of the many-spin model of Mn$_{12}$ are discussed.

cond-mat.mes-hall↗

arXiv2001

Quantum oscillations without quantum coherence

We study numerically the damping of quantum oscillations and the increase of entropy with time in model spin systems decohered by a spin bath. In some experimentally relevant cases, the oscillations of considerable amplitude can persist long after the entropy has saturated near its maximum, i.e. when the system has been decohered almost completely. Therefore, the pointer states of the system demonstrate non-trivial dynamics. The oscillations exhibit slow power-law decay, rather than exponential or Gaussian, and may be observable in experiments.

quant-ph↗