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V. V. Moshchalkov

Publications and source records attributed to V. V. Moshchalkov.

At least 37 records · Page 2Linked to original sources

Dynamic response of exchange bias in graphene nanoribbons

The dynamics of magnetic hysteresis, including the training effect and the field sweep rate dependence of the exchange bias, is experimentally investigated in exchange-coupled potassium split graphene nanoribbons (GNRs). We find that, at low field sweep rate, the pronounced absolute training effect is present over a large number of cycles. This is reflected in a gradual decrease of the exchange bias with the sequential field cycling. However, at high field sweep rate above 0.5 T/min, the training effect is not prominent. With the increase in field sweep rate, the average value of exchange bias field grows and is found to follow power law behavior. The response of the exchange bias field to the field sweep rate variation is linked to the difference in the time it takes to perform a hysteresis loop measurement compared with the relaxation time of the anti-ferromagnetically aligned spins. The present results may broaden our current understanding of magnetism of GNRs and would be helpful in establishing the GNRs based spintronic devices.

cond-mat.mes-hall↗

Magnetocaloric effect and nature of magnetic transition in nanoscale Pr0.5Ca0.5MnO3

Systematic measurements pertinent to the magnetocaloric effect and nature of magnetic transition around the transition temperature are performed in the 10 nm Pr0.5Ca0.5MnO3 nanoparticles (PCMO10) . Maxwell relation is employed to estimate the change in magnetic entropy. At Curie temperature TC, 83.5 K, the change in magnetic entropy discloses a typical variation with a value 0.57 J/kg K, and is found to be magnetic field dependent. From the area under the curve Delta S vs T, the refrigeration capacity is calculated at TC, 83.5 K and it is found to be 7.01 J/kg. Arrott plots infer that due to the competition between the ferromagnetic and anti ferromagnetic interactions, the magnetic phase transition in PCMO10 is broadly spread over both in temperature as well as in magnetic field coordinates. Upon tuning the particle size, size distribution, morphology, and relative fraction of magnetic phases, it may be possible to enhance the magnetocalorific effect further in PCMO10.

cond-mat.mes-hall↗

Negative-μ regime in the ac magnetic response of superconductor nanoshells

The time-dependent Ginzburg-Landau formalism is applied to analyze the vortex states and vortex dynamics in superconducting spherical nanoshells, subjected to mutually perpendicular strong dc and weak ac magnetic fields. We demonstrate that nonuniformity of the shell thickness can dramatically affect the ac magnetic response of a 3D array of superconducting nanoshells. Remarkably, this response is strongly influenced not only by the relevant geometric and material parameters and the ac-field frequency but also by the magnitude of the applied dc field: by changing this field the real part of the effective ac magnetic permeability can be tuned from positive values significantly larger than one down to negative values.

cond-mat.supr-con↗

Local mapping of dissipative vortex motion

We explore, with unprecedented single vortex resolution, the dissipation and motion of vortices in a superconducting ribbon under the influence of an external alternating magnetic field. This is achieved by combing the phase sensitive character of ac-susceptibility, allowing to distinguish between the inductive-and dissipative response, with the local power of scanning Hall probe microscopy. Whereas the induced reversible screening currents contribute only inductively, the vortices do leave a fingerprint in the out-of-phase component. The observed large phase-lag demonstrates the dissipation of vortices at timescales comparable to the period of the driving force (i.e. 13 ms). These results indicate the presence of slow microscopic loss mechanisms mediated by thermally activated hopping transport of vortices between metastable states.

cond-mat.supr-con↗

Localization of superconductivity in superconductor-electromagnet hybrids

We investigate the nucleation of superconductivity in a superconducting Al strip under the influence of the magnetic field generated by a current-carrying Nb wire, perpendicularly oriented and located underneath the strip. The inhomogeneous magnetic field, induced by the Nb wire, produces a spatial modulation of the critical temperature T_c, leading to a controllable localization of the superconducting order parameter (OP) wave function. We demonstrate that close to the phase boundary T_c(B_ext) the localized OP solution can be displaced reversibly by either applying an external perpendicular magnetic field B_ext or by changing the amplitude of the inhomogeneous field.

cond-mat.supr-con↗

Ferromagnetism in graphene nanoribbons: split versus oxidative unzipped ribbons

Two types of graphene nanoribbons: (a) potassium-split graphene nanoribbons (GNRs), and (b) oxidative unzipped and chemically converted graphene nanoribbons (CCGNRs) were investigated for their magnetic properties using the combination of static magnetization and electron spin resonance measurements. The two types of ribbons possess remarkably different magnetic properties. While the low temperature ferromagnet-like feature is observed in both types of ribbons, such room temperature feature persists only in potassium-split ribbons. The GNRs show negative exchange bias, but the CCGNRs exhibit a 'positive exchange bias'. Electron spin resonance measurements infer that the carbon related defects may responsible for the observed magnetic behaviour in both types of ribbons. Furthermore, proton hyperfine coupling strength has been obtained from hyperfine sublevel correlation experiments performed on the GNRs. Electron spin resonance provides no indications for the presence of potassium (cluster) related signals, emphasizing the intrinsic magnetic nature of the ribbons. Our combined experimental results may infer the coexistence of ferromagnetic clusters with anti-ferromagnetic regions leading to disordered magnetic phase. We discuss the origin of the observed contrast in the magnetic behaviours of these two types of ribbons.

cond-mat.mes-hall↗

Oscillatory exchange bias and training effects in nanocrystalline Pr0.5Ca0.5MnO3

We report on exchange bias effects in 10 nm particles of Pr0.5Ca0.5MnO3 which appear as a result of competing interactions between the ferromagnetic (FM)/anti-ferromagnetic (AFM) phases. The fascinating new observation is the demonstration of the temperature dependence of oscillatory exchange bias (OEB) and is tunable as a function of cooling field strength below the SG phase, may be attributable to the presence of charge/spin density wave (CDW/SDW) in the AFM core of PCMO10. The pronounced training effect is noticed at 5 K from the variation of the EB field as a function of number of field cycles (n) upon the field cooling (FC) process. For n > 1, power-law behavior describes the experimental data well; however, the breakdown of spin configuration model is noticed at n \geq 1.

cond-mat.mes-hall↗

Martensite-like transition and spin-glass behavior in nanocrystalline Pr0.5Ca0.5MnO3

We report on isothermal pulsed (20 ms) field magnetization, temperature dependent AC - susceptibility, and the static low magnetic field measurements carried out on 10 nm sized Pr0.5Ca0.5MnO3 nanoparticles (PCMO10). The saturation field for the magnetization of PCMO10 (~ 250 kOe) is found to be reduced in comparison with that of bulk PCMO (~300 kOe). With increasing temperature, the critical magnetic field required to 'melt' the residual charge-ordered phase decays exponentially while the field transition range broadens, which is indicative of a Martensite-like transition. The AC - susceptibility data indicate the presence of a frequency-dependent freezing temperature, satisfying the conventional Vogel-Fulcher and power laws, pointing to the existence of a spin-glass-like disordered magnetic phase. The present results lead to a better understanding of manganite physics and might prove helpful for practical applications.

cond-mat.mtrl-sci↗

Exchange bias and training effects in antiferromagnetically coupled La0.7Sr0.3MnO3 / SrRuO3 superlattices

Exchange bias (EB) and the training effects (TE) in an antiferromagnetically coupled La0.7Sr0.3MnO3 / SrRuO3 superlattices were studied in the temperature range 1.8 - 150 K. Strong antiferromagnetic (AFM) interlayer coupling is evidenced from AC - susceptibility measurements. Below 100 K, vertical magnetization shifts are present due to the two remanent states corresponding to the two ferromagnetic (FM) layers at FM and AFM coupling condition. After field cooling (FC), significant decrease in the exchange bias field (HEB) is observed when cycling the system through several consecutive hysteresis loops. Quantitative analysis for the variation of HEB vs. number of field cycles (n) indicates an excellent agreement between the theory, based on triggered relaxation phenomena, and our experimental observations. Nevertheless, the crucial fitting parameter K indicates smooth training effect upon repeated field cycling, in accordance with our observation.

cond-mat.mtrl-sci↗

Sign reversal of the Hall resistance in the mixed-state of La$_{1.89}$ Ce$_{0.11}$CuO$_{4}$ and La$_{1.89}$Ce$_{0.11}$(Cu$_{0.99}$Co$_{0.01}$)O$_{4} $ thin films

The transport properties of La$_{1.89}$Ce$_{0.11}$CuO$_{4}$(LCCO) and La$_{1.89}$Ce$_{0.11}$(Cu$_{0.99}$Co$_{0.01}$)O$_{4}$ (LCCO:Co) superconducting thin films are investigated. When the external field $\bf H$ is applied along the crystallographic c-axis, a double sign reversal of the Hall voltage in the mixed state of LCCO:Co thin films is observed whereas a single sign reversal is detected in LCCO. A double sign reversal of the Hall signal in LCCO can be recovered if the magnetic field is tilted away from the plane of the film. We find that the transition from one to two of the Hall sign reversal coincides with the change in the pinning from strong to weak. This temperature/field induced transition is caused either by the magnetic impurities in LCCO:Co or by the coupling between the pancake vortices and the in-plane Josephson vortices in LCCO. These results are in agreement with early theoretical and numerical predictions.

cond-mat.supr-con↗

Crossover between different regimes of inhomogeneous superconductivity in planar superconductor-ferromagnet hybrids

We studied experimentally the effect of a stripe-like domain structure in a ferromagnetic BaFe_{12}O_{19} substrate on the magnetoresistance of a superconducting Pb microbridge. The system was designed in such a way that the bridge is oriented perpendicular to the domain walls. It is demonstrated that depending on the ratio between the amplitude of the nonuniform magnetic field B_0, induced by the ferromagnet, and the upper critical field H_{c2} of the superconducting material, the regions of the reverse-domain superconductivity in the H-T plane can be isolated or can overlap (H is the external magnetic field, T is temperature). The latter case corresponds to the condition B_0/H_{c2}<1 and results in the formation of superconductivity above the magnetic domains of both polarities. We discovered the regime of edge-assisted reverse-domain superconductivity, corresponding to localized superconductivity near the edges of the bridge above the compensated magnetic domains. Direct verification of the formation of inhomogeneous superconducting states and external-field-controlled switching between normal state and inhomogeneous superconductivity were obtained by low-temperature scanning laser microscopy.

cond-mat.supr-con↗

Anomalous flux avalanche morphology in a a-MoGe superconducting film with a square antidot lattice - experiment and simulation

We have employed magneto-optical imaging to visualize the occurrence of flux avalanches in a superconducting film of a-MoGe. The specimen was decorated with square antidots arranged in a square lattice. We observed avalanches with the anomalous habit of forming trees where the trunk is perpendicular to the main axis of the square lattice, whereas the branches form angles of 45 degrees. The overall features of the avalanches, and in particular the 45 degree direction of the branches, were confirmed by numerical simulations.

cond-mat.supr-con↗

Domain-wall and reverse-domain superconducting states of a Pb thin-film bridge on a ferromagnetic BaFe_{12}O_{19} single crystal

We report on imaging of the nonuniform superconducting states in a Pb thin film bridge on top of a ferromagnetic BaFe_{12}O_{19} single crystal with a single straight domain wall along the center of the bridge by low-temperature scanning laser microscopy. We have visualized domain wall superconductivity (DWS) close to the critical temperature of Pb, when the Pb film above the domain wall acts as a superconducting path for the current. The evolution of the DWS signal with temperature and the external-field-driven transition from DWS to reverse domain superconductivity was visualized.

cond-mat.supr-con↗

Vortex core deformation and stepper motor behavior in a superconducting ratchet

We investigated experimentally the frequency dependence of a superconducting vortex ratchet effect by means of electrical transport measurements and modeled it theoretically using the time dependent Ginzburg-Landau formalism. We demonstrate that the high frequency vortex behavior can be described as a discrete motion of a particle in a periodic potential, i.e. the so called stepper motor behavior. Strikingly, in the more conventional low frequency response a transition takes place from an Abrikosov vortex rectifier to a phase slip line rectifier. This transition is characterized by a strong increase in the rectified voltage and the appearance of a pronounced hysteretic behavior.

cond-mat.supr-con↗

Hall effect in the vicinity of quantum critical point in Tm1-xYbxB12

The angular, temperature and magnetic field dependences of Hall resistance roH for the rare-earth dodecaboride solid solutions Tm1-xYbxB12 have been studied in a wide vicinity of the quantum critical point (QCP) xC~0.3. The measurements performed in the temperature range 1.9-300 K on high quality single crystals allowed to find out for the first time in these fcc compounds both an appearance of the second harmonic contribution in ro2H at QCP and its enhancement under the Tm to ytterbium substitution and/or with increase of external magnetic field. When the Yb concentration x increases a negative maximum of a significant amplitude was shown to appear on the temperature dependences of Hall coefficient RH(T) for the Tm1-xYbxB12 compounds. Moreover, a complicated activation type behavior of the Hall coefficient is observed at intermediate temperatures for x>0.5 with activation energies Eg~200K and Ea~55-75K in combination with the sign inversion of RH(T) at low temperatures in the coherent regime. The density of states renormalization effects are analyzed within the variation of Yb concentration and the features of the charge transport in various regimes (charge gap formation, intra-gap manybody resonance and coherent regime) are discussed in detail in Tm1-xYbxB12 solid solutions.

cond-mat.str-el↗

Mesoscopic cross-film cryotrons: Vortex trapping and dc-Josephson-like oscillations of the critical current

We investigate theoretically and experimentally the transport properties of a plain Al superconducting strip in the presence of a single straight current-carrying wire, oriented perpendicular to the superconducting strip. It is well known that the critical current of the superconducting strip, Ic, in such cryotron--like system can be tuned by changing the current in the control wire, Iw. We demonstrated that the discrete change in the number of the pinned vortices/antivortices inside the narrow and long strip nearby the current-carrying wire results in a peculiar oscillatory dependence of Ic on Iw.

cond-mat.supr-con↗

Reverse-domain superconductivity in superconductor-ferromagnet hybrids: effect of a vortex-free channel on the symmetry of I-V characteristics

We demonstrate experimentally that the presence of a single domain wall in an underlying ferromagnetic BaFe_{12}O_{19} substrate can induce a considerable asymmetry in the current (I) - voltage (V) characteristics of a superconducting Al bridge. The observed diode-like effect, i.e. polarity-dependent critical current, is associated with the formation of a vortex-free channel inside the superconducting area which increases the total current flowing through the superconducting bridge without dissipation. The vortex-free region appears only for a certain sign of the injected current and for a limited range of the external magnetic field.

cond-mat.supr-con↗

Giant vortices, vortex rings and reentrant behavior in type-1.5 superconductors

We predict that in a bulk type-1.5 superconductor the competing magnetic responses of the two components of the order parameter can result in a vortex interaction that generates group-stabilized giant vortices and unusual vortex rings in the absence of any extrinsic pinning or confinement mechanism. We also find within the Ginzburg-Landau theory a rich phase diagram with successions of behaviors like type-1 -> type-1.5 -> type-2 -> type-1.5 as temperature decreases.

cond-mat.supr-con↗