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V. Walther

Publications and source records attributed to V. Walther.

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Plasma effects on lifetimes and screening of Rydberg excitons

We simulate the effects of a neutral electron--hole plasma on Rydberg excitons in cuprous oxide (Cu$_2$O), focusing on the validity of Debye screening and the role of plasma-induced thermalization. Unlike atomic Rydberg states, excitons in Cu$_2$O consist of quasiparticles with comparable effective masses whose orbital frequencies can exceed the plasma frequency, invalidating the assumption of a stationary screened charge. Using two complementary approaches, a classical orbit model and a harmonic-oscillator representation evolved via the truncated Wigner approximation, we study exciton lifetimes and interaction screening under realistic plasma conditions. We find numerically that plasma-induced scattering induces finite exciton lifetimes with specific scaling relations with plasma density, principal quantum number $n$ and temperature, possibly providing an explanation for experimentally observed deviations from the $n^3$ scaling at high principal quantum numbers. By explicitly computing time-averaged electric fields, we show that Debye screening overestimates the screening of the exciton's internal field, especially for high angular momentum states. Furthermore, we demonstrate that exciton-exciton interactions are not Debye screened at separations comparable to the Debye length for Rydberg excitons that are well resolvable in absorption measurements.

quant-ph

The rise and fall of patterns in driven-dissipative Rydberg polaritons

Spatial structures commonly emerge in interacting nonlinear systems. In this study, we focus on the out-of-equilibrium dynamics of the recently-established platform of Rydberg exciton-polaritons, fueled by their characteristic long-range non-local interactions, in the presence of an external drive and dissipation. Our work elucidates how modulational instability sets off spontaneous density pattern formations in a Rydberg polariton system with characteristic scales in the micron range. Under conditions of an unstable flattop state, we track the evolution of the polariton ensemble, showing the emergence of meta-stable patterns and their collapse in the long-time limit. We trace this phenomenon back to the destructive interference between the polariton state and the pump in a driven ensemble. Finally, we map out conditions that allow stable patterns to form under incoherent pumping. These findings provide new opportunities for exploring the emerging field of long-range interacting gases through Rydberg exciton-polaritons.

cond-mat.quant-gas