arXiv subjects

V. Zapf

Publications and source records attributed to V. Zapf.

7 recordsLinked to original sources

arXiv2018

Spin dynamics and field-induced magnetic phase transition in the honeycomb Kitaev magnet ${\alpha}$-Li$_2$IrO$_3$

The layered honeycomb iridate $\alpha$-Li$_2$IrO$_3$ displays an incommensurate magnetic structure with counterrotating moments on nearest-neighbor sites, proposed to be stabilized by strongly-frustrated anisotropic Kitaev interactions between spin-orbit entangled Ir$^{4+}$ magnetic moments. Here we report powder inelastic neutron scattering measurements that observe sharply dispersive low-energy magnetic excitations centered at the magnetic ordering wavevector, attributed to Goldstone excitations of the incommensurate order, as well as an additional intense mode above a gap $\Delta\simeq2.3$ meV. Zero-field muon-spin relaxation measurements show clear oscillations in the muon polarization below the N\'{e}el temperature $T_{\rm N}\simeq15$ K with a time-dependent profile consistent with bulk incommensurate long-range magnetism. Pulsed field magnetization measurements observe that only about half the saturation magnetization value is reached at the maximum field of 64 T. A clear anomaly near 25 T indicates a transition to a phase with reduced susceptibility. The transition field has a Zeeman energy comparable to the zero-field gapped mode, suggesting gap suppression as a possible mechanism for the field-induced transition.

cond-mat.str-el↗

arXiv2018

Quantum oscillations in flux-grown SmB6 with embedded aluminum

SmB6 is a candidate topological Kondo insulator that displays surface conduction at low temperatures. Here, we perform torque magnetization measurements as a means to detect de Haas-van Alphen (dHvA) oscillations in SmB6 crystals grown by aluminum flux. We find that dHvA oscillations occur in single crystals containing embedded aluminum, originating from the flux used to synthesize SmB6. Measurements on a sample with multiple, unconnected aluminum inclusions show that aluminum crystallizes in a preferred orientation within the SmB6 cubic lattice. The presence of aluminum is confirmed through bulk susceptibility measurements, but does not show a signature in transport measurements.

cond-mat.str-el↗

arXiv2015

The monoclinic crystal structure of $α$-RuCl$_3$ and the zigzag antiferromagnetic ground state

The layered honeycomb magnet alpha-RuCl3 has been proposed as a candidate to realize a Kitaev spin model with strongly frustrated, bond-dependent, anisotropic interactions between spin-orbit entangled jeff=1/2 Ru4+ magnetic moments. Here we report a detailed study of the three-dimensional crystal structure using x-ray diffraction on untwinned crystals combined with structural relaxation calculations. We consider several models for the stacking of honeycomb layers and find evidence for a crystal structure with a monoclinic unit cell corresponding to a stacking of layers with a unidirectional in-plane offset, with occasional in-plane sliding stacking faults, in contrast with the currently-assumed trigonal 3-layer stacking periodicity. We report electronic band structure calculations for the monoclinic structure, which find support for the applicability of the jeff=1/2 picture once spin orbit coupling and electron correlations are included. We propose that differences in the magnitude of anisotropic exchange along symmetry inequivalent bonds in the monoclinic cell could provide a natural mechanism to explain the spin gap observed in powder inelastic neutron scattering, in contrast to spin models based on the three-fold symmetric trigonal structure, which predict a gapless spectrum within linear spin wave theory. Our susceptibility measurements on both powders and stacked crystals, as well as neutron powder diffraction show a single magnetic transition at TN ~ 13K. The analysis of the neutron data provides evidence for zigzag magnetic order in the honeycomb layers with an antiferromagnetic stacking between layers. Magnetization measurements on stacked single crystals in pulsed field up to 60T show a single transition around 8T for in-plane fields followed by a gradual, asymptotic approach to magnetization saturation, as characteristic of strongly anisotropic exchange interactions.

cond-mat.str-el↗

arXiv2013

Criticality in a disordered quantum antiferromagnet by neutron diffraction

Field-induced magnetic ordering in the structurally disordered quantum magnets Ni(Cl$_{1-x}$Br$_x$)$_2$$\cdot$4SC(NH$_2$)$_2$, $x=8$% and 13%, is studied by means of neutron diffraction. The order parameter critical exponent is found to be very close to its value $β=0.5$ expected for magnetic Bose-Einstein condensation in the absence of disorder. This result applies to temperatures down to 40 mK, and a 1 T range in magnetic field. The crossover exponent is found to be $ϕ\sim 0.4$, for temperature ranges as small as 300 mK. Possible reasons for a discrepancy with recent numerical simulations and bulk measurements are discussed.

cond-mat.str-el↗

arXiv2008

Field-Controlled Magnetic Order in the Quantum Spin-Ladder System (Hpip)2CuBr4

Neutron diffraction is used to investigate the field-induced, antiferromagnetically ordered state in the two-leg spin-ladder material (Hpip)2CuBr4. This "classical" phase, a consequence of weak interladder coupling, is nevertheless highly unconventional: its properties are influenced strongly by the spin Luttinger-liquid state of the ladder subunits. We determine directly the order parameter (transverse magnetization), the ordering temperature, the spin structure, and the critical exponents around the transition. We introduce a minimal, microscopic model for the interladder coupling and calculate the quantum fluctuation corrections to the mean-field interaction.

cond-mat.str-el↗

arXiv2008

Thermodynamics of the Spin Luttinger-Liquid in a Model Ladder Material

The phase diagram in temperature and magnetic field of the metal-organic, two-leg, spin-ladder compound (C5H12N)2CuBr4 is studied by measurements of the specific heat and the magnetocaloric effect. We demonstrate the presence of an extended spin Luttinger-liquid phase between two field-induced quantum critical points and over a broad range of temperature. Based on an ideal spin-ladder Hamiltonian, comprehensive numerical modelling of the ladder specific heat yields excellent quantitative agreement with the experimental data across the complete phase diagram.

cond-mat.str-el↗

arXiv2005

Field-Dependent Hall Effect in Single Crystal Heavy Fermion YbAgGe below 1K

We report the results of a low temperature (T >= 50 mK) and high field (H <= 180 kOe) study of the Hall resistivity in single crystals of YbAgGe, a heavy fermion compound that demonstrates field-induced non-Fermi-liquid behavior near its field-induced quantum critical point. Distinct features in the anisotropic, field-dependent Hall resistivity sharpen on cooling down and at the base temperature are close to the respective critical fields for the field-induced quantum critical point. The field range of the non-Fermi-liquid region decreases on cooling but remains finite at the base temperature with no indication of its conversion to a point for T -> 0. At the base temperature, the functional form of the field-dependent Hall coefficient is field direction dependent and complex beyond existing simple models thus reflecting the multi-component Fermi surface of the material and its non-trivial modification at the quantum critical point.

cond-mat.str-el↗