arXiv subjects

V. Zlatić

Publications and source records attributed to V. Zlatić.

6 recordsLinked to original sources

arXiv2020

Dependence of transport coefficients of Yb(Rh$_{1-x}$Co$_x$)$_2$Si$_2$ intermetallics on temperature and cobalt concentration

Dependence of transport coefficients of the Yb(Rh$_{1-x}$Co$_x$)$_2$Si$_2$ series of alloys on temperature and cobalt concentration is explained by an asymmetric Anderson model which takes into account the exchange scattering of conduction electrons on ytterbium ions and the splitting of 4$f$-states by the crystalline electric field (CEF). The substitution of rhodium by cobalt is described as an increase of chemical pressure which reduces the exchange coupling and the CEF splitting. The scaling analysis and numerical NCA solution of the model show that the effective degeneracy of the 4$f$-state at a given temperature depends on the relative magnitude of the Kondo scale and the CEF splitting. Thus, we find that dependence of the thermopower, $S(T)$, on temperature and cobalt concentration can be understood as an interplay of quantum fluctuations, driven by the Kondo effect, and thermal fluctuations, which favor a uniform occupation of the CEF states. The theoretical model captures all the qualitative features of the experimental data and it explains the evolution of the shape of $S(T)$ with the increase of cobalt concentration.

cond-mat.str-el↗

arXiv2018

Thermopower evolution in Yb(Rh$_{1-x}$Co$_x$)$_2$Si$_2$

We present thermopower measurements on Yb(Rh$_{1-x}$Co$_x$)$_2$Si$_2$. Upon Co substitution the Kondo temperature is decreasing and the single large thermopower minimum observed for YbRh$_2$Si$_2$ splits into two minima. Simultaneously, the absolute thermopower values are strongly reduced due to a weaker exchange coupling between the $4f$ and the conduction electron states with increasing $x$. Pure YbCo$_2$Si$_2$ is considered a stable, trivalent system. Nevertheless, we still observe two minima in the thermopower indicative of weak residual Kondo scattering. This is in line with results from photo emission spectroscopy revealing a tiny contribution from Yb$^{2+}$. The value at the high-$T$ minimum in $S(T)$ is found to be proportional to the Sommerfeld coefficient for the whole series. This unexpected finding is discussed in relation to recent measurements of the valence and Fermi surface evolution with temperature.

cond-mat.str-el↗

arXiv2017

Resonant enhancement of thermoelectric properties by correlated hopping for the Falicov-Kimball model on Bethe lattice

The effect of correlated hopping on the charge and heat transport of strongly correlated particles is studied for the Falicov-Kimball model on the Bethe lattice. Exact solutions for the one particle density of states (DOS) and two particle transport function (the "quasiparticle" scattering time) are derived using dynamical mean field theory. For a wide range of the correlated hopping, the transport function exhibits singularities due to the resonant two-particle contribution, whereas the one particle DOS does not show any anomalous features. By tuning the number of itinerant electrons, so as to bring the Fermi level close to the resonant frequency, we get a large increase of the electrical and thermal conductivities, and the thermoelectric power. When the hopping amplitude between the occupied sites is reduced sufficiently, the itinerant electrons localize in the clusters of sites occupied by $f$ electrons. This gives rise to an additional narrow band in the DOS between the lower and upper Hubbard bands, but has only a minor effect on the thermoelectric properties.

cond-mat.str-el↗

arXiv2013

Charge Kondo Effect in Thermoelectric Properties of Lead Telluride doped with Thallium Impurities

We investigate the thermoelectric properties of PbTe doped with a small concentration $x$ of Tl impurities acting as acceptors and described by Anderson impurities with negative on-site (effective) interaction. The resulting charge Kondo effect naturally accounts for a number of the low temperature anomalies in this system, including the unusual doping dependence of the carrier concentration, the Fermi level pinning and the self-compensation effect. The Kondo anomalies in the low temperature resistivity at temperatures $T\leq 10\, {\rm K}$ and the $x$-dependence of the residual resistivity are also in good agreement with experiment. Our model also captures the qualitative aspects of the thermopower at higher temperatures $T>300\, {\rm K}$ for high dopings ($x>0.6%$) where transport is expected to be largely dominated by carriers in the heavy hole band of PbTe.

cond-mat.str-el↗

arXiv2012

Strongly enhanced thermal transport in a lightly doped Mott insulator at low temperature

We show how a lightly doped Mott insulator has hugely enhanced electronic thermal transport at low temperature. It displays universal behavior independent of the interaction strength when the carriers can be treated as nondegenerate fermions and a nonuniversal "crossover" region where the Lorenz number grows to large values, while still maintaining a large thermoelectric figure-of-merit. The electron dynamics are described by the Falicov-Kimball model which is solved for arbitrary large on-site correlation with a dynamical mean-field theory algorithm on a Bethe lattice. We show how these results are generic for lightly doped Mott insulators as long as the renormalized Fermi liquid scale is pushed to very low temperature and the system is not magnetically ordered.

cond-mat.str-el↗

arXiv2008

Enhancement of thermal transport in the degenerate periodic Anderson model

The low-temperature transport coefficients of the degenerate periodic SU(N) Anderson model are calculated in the limit of infinite correlation between {\it f} electrons, within the framework of dynamical mean-field theory. We establish the Fermi liquid (FL) laws in the clean limit, taking into account the quasiparticle damping. The latter yields a reduced value of the Lorenz number in the Wiedemann-Franz law. Our results indicate that the renormalization of the thermal conductivity and of the Seebeck coefficient can lead to a substantial enhancement of the electronic thermoelectric figure-of-merit at low temperature. Using the FL laws we discuss the low-temperature anomalies that show up in the electrical resistance of the intermetallic compounds with Cerium and Ytterbium ions, when studied as a function of pressure. Our calculations explain the sharp maximum of the coefficient of the $T^2$-term of the electrical resistance and the rapid variation of residual resistance found in a number of Ce and Yb intermetallics at some critical pressure.

cond-mat.str-el↗