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Vadim Vorobyov

Publications and source records attributed to Vadim Vorobyov.

At least 19 recordsLinked to original sources

Electrically Reconfigurable Silicon Carbide Nanophotonic Cavities on Thin-Film Lithium Niobate

Interfacing integrated photonics with solid-state spin defects holds great promise for future quantum networks, but the scaling of spin-photon architectures is hindered by frequency mismatches arising from fabrication-induced variations in photonic cavity resonances and the inhomogeneous optical transition frequencies of individual spins. These challenges call for a photonic platform with deterministic and wide-range tunability. Here, we demonstrate a hybrid nanophotonic platform based on direct bonding of silicon carbide photonic crystal nanocavity arrays onto thin-film lithium niobate on insulator, enabling deterministic electrical tuning of multiple SiC nanocavities into mutual spectral resonance. By exploiting the strong electro-optic response of lithium niobate, we achieve continuous and wide-range cavity tuning of 380 GHz ($\sim$1.1 nm), sufficient to compensate both cavity disorder and spin inhomogeneity. The nanocavities balance strong optical confinement with electrical tunability, exhibiting a theoretical Purcell factor of approximately 400. This hybrid platform enables electrically reconfigurable spin-photon interfaces for large-scale integrated quantum photonics.

physics.optics

Color-Center-Compatible Freestanding Diamond Directional Couplers for Quantum Photonics

Freestanding all-diamond color-center photonics is a promising platform for optical integration of spin-based quantum defects. Within this geometry, we realize a key building block for quantum-network interconnects: a directional coupler that acts as an on-chip beam splitter. We design and simulate directional couplers with triangular cross sections using eigenmode and finite-difference time-domain simulations and target near-50:50 splitting at visible wavelengths. We fabricate the devices directly from bulk single-crystal diamond by angled oxygen reactive-ion-beam etching followed by a dry post-release hard-mask removal process. Room-temperature measurements at $λ_0\approx 637 \mathrm{nm}$ yield a mean coupling ratio of $C^\mathrm{meas}=46(16) \%$. Finally, we integrate SnV$^{-}$ centers into the nanophotonic structures and observe near-lifetime-limited optical linewidths and coherent optical Rabi oscillations without post-fabrication annealing, identifying the platform as a viable route towards integrated diamond quantum photonics.

physics.optics

RF-free driving of nuclear spins with color centers in silicon carbide

Color centers that enable nuclear-spin control without RF fields offer a powerful route towards simplified and scalable quantum devices. Such capabilities are especially valuable for quantum sensing and computing platforms that already find applications in biology, materials science, and geophysics. A key challenge is the coherent manipulation of nearby nuclear spins, which serve as quantum memories and auxiliary qubits but conventionally require additional high-power RF fields which increase the experimental complexity and overall power consumption. Finding systems where both electron and nuclear spins can be controlled using a single MW source is therefore highly desirable. Here, using a modified divacancy center in silicon carbide, we show that coherent control of a coupled nuclear spin is possible without any RF fields. Instead, MW pulses driving the electron spin also manipulate the nuclear spin through hyperfineenhanced effects, activated by a precisely tilted external magnetic field. We demonstrate high-fidelity nuclear-spin control, achieving 89% two-qubit tomography fidelity and nearly T1-limited nuclear coherence times. This approach offers a simplified and scalable route for future quantum applications.

quant-ph

Localization and coherent control of 25 nuclear spins in Silicon Carbide

Optically addressable spin defects are excellent candidate platform for quantum sensing and quantum network. Nuclear spins coupled to color centers naturally enable long lived quantum memories and local qubits registers. To fully leverage this potential precise characterization of the surrounding nuclear-spin environment augmented with refined DFT models is required. In this work, we report angstrom-level 3D localization of 25 nuclear spins around a single V2 center in 4H Silicon Carbide. Utilizing specially placed robust nuclear memory as a highly efficient readout ancilla for readout, we apply correlation based spectroscopy and by selecting multi-spin chains up to length four, we access and characterize extended nuclear spin cluster. Using the coupling map we reconstruct their couplings to the central electron spin and neighboring nuclei. This work paves the way towards advanced quantum register applications on Silicon Carbide platform.

quant-ph

Waveguide-integrated colour centres in silicon carbide with broadband photonic crystal reflectors for efficient readout

Spin-active colour centres in 4H silicon carbide are promising candidates as building blocks for quantum information applications. To increase the photon count rate of the emitters at low temperatures, the colour centres must be integrated into nanophotonic structures and characterised under cryogenic conditions. Here, we design and fabricate waveguide structures attached with an efficient Dinosaur photonic crystal reflector at one side. The devices show broadband reflection over a range of 60 THz with a peak reflectance above 80 %. Additionally, colour centres were integrated into these structures and characterised at cryogenic conditions. The emission was collected by a tapered-waveguide-tapered-fibre interface. Although the spectral stability of the emitters must be further improved for high excitation powers, the saturation intensity in standard PLE measurements is about 104 kcps. The count rate can be further improved to about 125 kcps with a charge-resonance check measurement scheme. To highlight the relevance of our devices, we theoretically show that these count rates enable optical single-shot readout with a fidelity exceeding 98 %.

quant-ph

Converting coherence into work with a fully quantum engine

Heat engines convert thermal energy into mechanical work. We here report the experimental realization of a fully quantum engine that converts quantum coherence into work. A single solid-state spin in diamond is fueled by a coherent bath and cyclically stores energy in a spin quantum battery. We establish quantum-enhanced performance by showing that almost 200$\%$ more work is produced after a few cycle compared to the corresponding classical engine. We obtain concrete criteria for successful coherence-to-work conversion, and highlight the importance of a coherent motor-battery interaction. This device harnesses nonclassical features during all stages of its cycle, and demonstrates the functionality of a nanomachine whose parts are all quantum coherent.

quant-ph

Readout of a solid state spin ensemble at the projection noise limit

Spin ensembles are central to quantum science, from frequency standards and fundamental physics searches to magnetic resonance spectroscopy and quantum sensing. Their performance is ultimately constrained by spin projection noise, yet solid-state implementations have so far been limited by much larger photon shot noise. Here we demonstrate a direct, quantum non-demolition readout of a mesoscopic ensemble of nitrogen-vacancy (NV) centers in diamond that surpasses the photon shot-noise limit and approaches the intrinsic spin projection noise. By stabilizing the $^{14}$N nuclear spin bath at high magnetic fields and employing repetitive nuclear-assisted spin readout, we achieve a noise reduction of 3.8 dB below the thermal projection noise level. This enables direct access to the intrinsic fluctuations of the spin ensemble, allowing us to directly observe the signatures of correlated spin states. Our results establish projection noise-limited readout as a practical tool for solid-state quantum sensors, opening pathways to quantum-enhanced metrology, direct detection of many-body correlations, and the implementation of spin squeezing in mesoscopic solid-state ensembles.

quant-ph

Efficient Detection of Statistical RF Fields at High Magnetic Field with a Quantum Sensor

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform due to an unprecedented sensitivity down to the single spin level. At the nanoscale, high nuclear spin polarization through spin fluctuations (statistical polarization) far outweighs thermal polarization. However, until now efficient NMR detection using coherent averaging techniques could not be applied to the detection of statistical polarization, leading to long measurement times. Here we present two protocols to enable coherent averaging of statistical oscillating signals through rectification. We demonstrate these protocols on an artificial radiofrequency signal detected with a single NV center at 2.7 T. Through this, the signal-to-noise scaling with number of measurements $N$ is improved from $N^{0.5}$ to $N^1$, improving the measurement time significantly. The relevance of rectification for the detection of statistical polarization using NV ensembles is outlined, paving the way for efficient nanoscale NMR spectroscopy.

quant-ph

Optical levitation of fluorescent silicon carbide nanoparticles in vacuum

Levitated optomechanics is an emerging field in quantum science that explores the quantum motion of mesoscopic particles levitated in a vacuum. Expanding this approach to particles with intrinsic quantum defects opens new opportunities for quantum sensing and nontrivial quantum state generation. Here, we explore silicon carbide (SiC) nanoparticles as a promising platform that offers a range of controllable quantum defects and material tunability. We demonstrate stable optical levitation of 3C-polytype SiC nanoparticles containing single photon emitters in a vacuum. We observe stable fluorescence from the levitated particle, confirming the preservation of the emitters in the levitated state. We also investigate particle loss at low pressure and explore thermal annealing as a potential method to improve trapping stability. Our results establish SiC as a viable platform for levitated optomechanics, providing additional quantum degrees of freedom and material engineering capabilities.

physics.optics

Two-Photon Interference of Photons from Remote Tin-Vacancy Centers in Diamond

Scalable quantum networks rely on optical connections between long-lived qubits to distribute entanglement. Tin vacancies in diamond have emerged as promising long-lived qubits, offering extended spin coherence times at liquid helium temperatures and spin-dependent, highly coherent optical transitions for effective photon-based communication. Connecting remote nodes requires quantum interference of indistinguishable photons, which is challenging in an inhomogeneous solid-state environment. Here, we demonstrate a two-node experiment with tin vacancies in diamond, which exhibit a resonant frequency distribution spanning approximately 8 GHz. To overcome the frequency mismatch, we tune the resonant frequencies of one node using the Stark effect. We achieve tunability up to 4 GHz while maintaining optical coherence. As a demonstration, we achieve detuning-dependent remote two-photon interference between separate nodes, obtaining 80(6)% interference visibility without postprocessing when the defects' optical transitions are tuned into resonance, and 63(8)% with detuning up to 20 times their natural linewidths. These results highlight the potential of tin-vacancy centres in diamond for establishing robust optical links between remote quantum registers.

quant-ph

Readout of strongly coupled NV center-pair spin states with deep neural networks

Optically addressable electron spin clusters are of interest for quantum computation, simulation and sensing. However, with interaction length scales of a few tens of nanometers in the strong coupling regime, they are unresolved in conventional confocal microscopy, making individual readout problematic. Here we show that when using a single shot readout technique, collective states of the combined register space become accessible. By using spin to charge conversion of the defects we draw the connection between the intricate photon count statistics with spin state tomography using deep neural networks. This approach is particularly versatile with further scaling the number of constituent spins in a cluster due to complexity of the analytical treatment. We perform a proof of concept measurement of the correlated classical signal, paving the way for using our technique in realistic applications.

quant-ph

Modeling Quantum Volume Using Randomized Benchmarking of Room-Temperature NV Center Quantum Registers

Accurately estimating the performance of quantum hardware is crucial for comparing different platforms and predicting the performance and feasibility of quantum algorithms and applications. In this paper, we tackle the problem of benchmarking a quantum register based on the NV center in diamond operating at room temperature. We define the connectivity map as well as single qubit performance. Thanks to an all-to-all connectivity the 2 and 3 qubit gates performance is promising and competitive among other platforms. We experimentally calibrate the error model for the register and use it to estimate the quantum volume, a metric used for quantifying the quantum computational capabilities of the register, of 8. Our results pave the way towards the unification of different architectures of quantum hardware and evaluation of the joint metrics.

quant-ph

Single V2 defect in 4H Silicon Carbide Schottky diode at low temperature

Nanoelectrical and photonic integration of quantum optical components is crucial for scalable solid-state quantum technologies. Silicon carbide stands out as a material with mature quantum defects and a wide variety of applications in semiconductor industry. Here, we study the behaviour of single silicon vacancy (V2) colour centres in a metal-semiconductor (Au/Ti/4H-SiC) epitaxial wafer device, operating in a Schottky diode configuration. We explore the depletion of free carriers in the vicinity of the defect, as well as electrical tuning of the defect optical transition lines. By detecting single charge traps, we investigate their impact on V2 optical line width. Additionally, we investigate the charge-photon-dynamics of the V2 centre and find its dominating photon-ionisation processes characteristic rate and wavelength dependence. Finally, we probe the spin coherence properties of the V2 system in the junction and demonstrate several key protocols for quantum network applications. Our work shows the first demonstration of low temperature integration of a Schottky device with optical microstructures for quantum applications and paves the way towards fundamentally scalable and reproducible optical spin defect centres in solids.

quant-ph

Efficient nuclear spin - photon entanglement with optical routing

Quantum networks and distributed quantum computers rely on entanglement generation between photons and long-lived quantum memories. For large-scale architectures, one of the most crucial parameters is the efficiency at which entanglement can be created and detected. Here, we maximize the efficiency for the detection of hybrid entanglement between a nuclear spin qubit in diamond with a photonic time-bin qubit. Our approach relies on an optimal implementation of the photonic qubit analyzer, for which we use a high-speed electro-optic deflector to direct photons deterministically along the optimal interferometer paths. This way, we completely eliminate all cases in which photons are randomly lost due to the propagation in the wrong interferometer path. In this first demonstration experiment, we use nitrogen-vacancy center in diamond, for which we immediately demonstrate the presence of the entanglement. An extension to other spin-photon entanglement systems is straightforward. Further, our scheme can be used in the framework of quantum repeater networks, including spectral and temporal multiplexing strategies. Our results thus pave the way for the future high-performance quantum networks.

quant-ph

High fidelity optical readout of a nuclear spin qubit in Silicon Carbide

Quantum state readout is a key requirement for a successful qubit platform. In this work we demonstrate a high fidelity quantum state readout of a V2 center nuclear spin based on a repetitive readout technique. We demonstrate up to 99.5$\,\%$ readout fidelity and 99$\,\%$ for state preparation. Using this efficient readout we initialise the nuclear spin by measurement and demonstrate its Rabi and Ramsey nutation. Finally, we use the nuclear spin as a long lived memory for quantum sensing application of weakly coupled diatomic nuclear spin bath.

quant-ph

Blueprint for efficient nuclear spin characterization with color center

Nuclear spins in solids offer a promising avenue for developing scalable quantum hardware. Leveraging nearby single-color centers, these spins can be efficiently addressed at the single-site level through spin resonance. However, characterising individual nuclear spins is quite cumbersome since the characterisation protocols may differ depending on the strength of the hyperfine coupling, necessitating tailored approaches and experimental conditions. While modified electron spin Hahn echoes like CPMG and XY8 pulse sequences are commonly employed, they encounter significant limitations in scenarios involving spin-1/2 systems, strongly coupled spins, or nuclear spin baths comprising distinct isotopes. Here, we present a more straightforward approach for determining the hyperfine interactions among each nuclear and the electron spin. This method holds promise across diverse platforms, especially for emerging S=1/2 group IV defects in diamond (e.g., SiV, GeV, SnV, PbV) or silicon (T-centre, P-donors). We provide a theoretical framework and adapt it for color-centers exhibiting various spins. Through simulations conducted on nuclear spin clusters, we evaluate different protocols and compare their performance using the Fisher information matrix and Cramer Rao bounds.

quant-ph

Measuring nuclear spin qubits by qudit-enhanced spectroscopy in Silicon Carbide

Nuclear spins with hyperfine coupling to single electron spins are highly valuable quantum bits. In this work we probe and characterise the particularly rich nuclear spin environment around single silicon vacancy color-centers (V2) in 4H-SiC. By using the electron spin-3/2 qudit as a 4 level sensor, we identify several groups of $^{29}$Si and $^{13}$C nuclear spins through their hyperfine interaction. We extract the major components of their hyperfine coupling via optical detected nuclear resonance, and assign them to shell groups in the crystal via the DFT simulations. We utilise the ground state level anti-crossing of the electron spin for dynamic nuclear polarization and achieve a nuclear spin polarization of up to $98\pm6\,\%$. We show that this scheme can be used to detect the nuclear magnetic resonance signal of individual spins and demonstrate their coherent control. Our work provides a detailed set of parameters for future use of SiC as a multi-qubit memory and quantum computing platform.

quant-ph

The Transition from Quantum to Classical in weak measurements and reconstruction of Quantum Correlation

The ability to follow the dynamics of a quantum system in a quantitative manner is of key importance for quantum technology. Despite its central role, justifiable deduction of the quantum dynamics of a single quantum system in terms of a macroscopical observable remains a challenge. Here we show that the relation between the readout signal of a single electron spin and the quantum dynamics of the single nuclear spin is given by a parameter related to the measurement strength. We determine this measurement strength in independent experiments and use this value to compare our analysis of the quantum dynamics with experimental results. We prove the validity of our approach by measuring violations of the Leggett-Garg inequality.

quant-ph