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Val Zwiller

Publications and source records attributed to Val Zwiller.

At least 73 records · Page 4Linked to original sources

On-demand generation of background--free single photons from a solid-state source

True on--demand high--repetition--rate single--photon sources are highly sought after for quantum information processing applications. However, any coherently driven two-level quantum system suffers from a finite re-excitation probability under pulsed excitation, causing undesirable multi--photon emission. Here, we present a solid--state source of on--demand single photons yielding a raw second--order coherence of $g^{(2)}(0)=(7.5\pm1.6)\times10^{-5}$ without any background subtraction nor data processing. To this date, this is the lowest value of $g^{(2)}(0)$ reported for any single--photon source even compared to the previously best background subtracted values. We achieve this result on GaAs/AlGaAs quantum dots embedded in a low--Q planar cavity by employing (i) a two--photon excitation process and (ii) a filtering and detection setup featuring two superconducting single--photon detectors with ultralow dark-count rates of $(0.0056\pm0.0007) s^{-1}$ and $(0.017\pm0.001) s^{-1}$, respectively. Re--excitation processes are dramatically suppressed by (i), while (ii) removes false coincidences resulting in a negligibly low noise floor.

cond-mat.mes-hall↗

Electromagnetically Induced Transparency of On-demand Single Photons in a Hybrid Quantum Network

Long range quantum communication and quantum information processing require the development of light-matter interfaces for distributed quantum networks. Even though photons are ideal candidates for network links to transfer quantum information, the system of choice for the realization of quantum nodes has not been identified yet. Ideally, one strives for a hybrid network architecture, which will consist of different quantum systems, combining the strengths of each system. However, interfacing different quantum systems via photonic channels remains a major challenge because a detailed understanding of the underlying light-matter interaction is missing. Here, we show the coherent manipulation of single photons generated on-demand from a semiconductor quantum dot using a rubidium vapor quantum memory, forming a hybrid quantum network. We demonstrate the engineering of the photons' temporal wave function using four-level atoms and the creation of a new type of electromagnetic induced transparency for quantum dot photons on resonance with rubidium transitions. Given the short lifetime of our quantum dot transition the observed dynamics cannot be explained in the established steady-state picture. Our results play a pivotal role in understanding quantum light-matter interactions at short time scales. These findings demonstrate a fundamental active node to construct future large-scale hybrid quantum networks.

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In-field entanglement distribution over a 96 km-long submarine optical fibre

Techniques for the distribution of quantum-secured cryptographic keys have reached a level of maturity allowing them to be implemented in all kinds of environments, away from any form of laboratory infrastructure. Here, we detail the distribution of entanglement between Malta and Sicily over a 96 km-long submarine telecommunications optical fibre cable. We used this standard telecommunications fibre as a quantum channel to distribute polarisation-entangled photons and were able to observe around 257 photon pairs per second, with a polarisation visibility above 90%. Our experiment demonstrates the feasibility of using deployed submarine telecommunications optical fibres as long-distance quantum channels for polarisation-entangled photons. This opens up a plethora of possibilities for future experiments and technological applications using existing infrastructure.

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A single-photon detector with high efficiency and sub-10ps time resolution

The observation of fast physical dynamics using optical techniques currently relies on indirect methods, such as pump-probe measurements. One reason for this is the lack of an efficient detector with high time resolution. Single-photon detectors with high efficiency and ultra-high time resolution serve as the best candidates for replacing such indirect methods. We engineer the nano-structure of Superconducting Nanowire Single-Photon Detectors (SNSPDs) to achieve a time resolution better than 10ps and at the same time a high efficiency (>86%). Furthermore, at the limit of multiphoton excitation, using an improved readout technique, we reach an unprecedented time resolution of <3ps. These findings set a new upper limit for the intrinsic time resolution of SNSPDs and open up new possibilities for direct observation of fast phenomena in different fields of science.

physics.ins-det↗

A stable wavelength-tunable triggered source of single photons and cascaded photon pairs at the telecom C-band

The implementation of fiber-based long-range quantum communication requires tunable sources of single photons at the telecom C-band. Stable and easy-to-implement wavelength- tunability of individual sources is crucial to (i) bring remote sources into resonance, to (ii) define a wavelength standard and to (iii) ensure scalability to operate a quantum repeater. So far, the most promising sources for true, telecom single photons are semiconductor quantum dots, due to their ability to deterministically and reliably emit single and entangled photons. However, the required wavelength-tunability is hard to attain. Here, we show a stable wavelength-tunable quantum light source by integrating strain-released InAs quantum dots on piezoelectric substrates. We present triggered single-photon emission at 1.55 μm with a multiphoton emission probability as low as 0.097, as well as photon pair emission from the radiative biexciton-exciton cascade. We achieve a tuning range of 0.25 nm which will allow to spectrally overlap remote quantum dots or tuning distant quantum dots into resonance with quantum memories. This opens up realistic avenues for the implementation of photonic quantum information processing applications at telecom wavelengths.

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Single-photon detectors combining ultra-high efficiency, detection-rates, and timing resolution

Single-photon detection with high efficiency, high timing resolution, low dark counts and high photon detection-rates is crucial for a wide range of optical measurements. Although efficient detectors have been reported before, combining all performance parameters in a single device remains a challenge. Here, we show a broadband NbTiN superconducting nanowire detector with an efficiency exceeding 92%, over 150MHz photon detection-rate, a dark count-rate below 130Hz, operated in a Gifford-McMahon cryostat. Furthermore, with careful optimization of the detector design and readout electronics, we reach an ultra-low system timing jitter of 14.80ps (13.95ps decoupled) while maintaining high detection efficiencies.

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Two-photon interference from two blinking quantum emitters

We investigate the effect of blinking on the two-photon interference measurement from two independent quantum emitters. We find that blinking significantly alters the statistics in the second-order intensity correlation function g$^{(2)}(τ)$ and the outcome of two-photon interference measurements performed with independent quantum emitters. We theoretically demonstrate that the presence of blinking can be experimentally recognized by a deviation from the g$^{(2)}_{D}(0)=0.5$ value when distinguishable photons impinge on a beam splitter. Our results show that blinking imposes a mandatory cross-check measurement to correctly estimate the degree of indistinguishablility of photons emitted by independent quantum emitters.

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Bright nanoscale source of deterministic entangled photon pairs violating Bell's inequality

Global, secure quantum channels will require efficient distribution of entangled photons. Long distance, low-loss interconnects can only be realized using photons as quantum information carriers. However, a quantum light source combining both high qubit fidelity and on-demand bright emission has proven elusive. Here, we show a bright photonic nanostructure generating polarization-entangled photon-pairs that strongly violates Bell's inequality. A highly symmetric InAsP quantum dot generating entangled photons is encapsulated in a tapered nanowire waveguide to ensure directional emission and efficient light extraction. We collect $\sim$200 kHz entangled photon-pairs at the first lens under 80\,MHz pulsed excitation, which is a 20 times enhancement as compared to a bare quantum dot without a photonic nanostructure. The performed Bell test using the Clauser-Horne-Shimony-Holt inequality reveals a clear violation ($S_{\text{CHSH}}>2$) by up to 9.3 standard deviations. By using a novel quasi-resonant excitation scheme at the wurtzite InP nanowire resonance to reduce multi-photon emission, the entanglement fidelity ($F=0.817\,\pm\,0.002$) is further enhanced without temporal post-selection, allowing for the violation of Bell's inequality in the rectilinear-circular basis by 25 standard deviations. Our results on nanowire-based quantum light sources highlight their potential application in secure data communication utilizing measurement-device-independent quantum key distribution and quantum repeater protocols.

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Phonon-assisted two-photon interference from remote quantum emitters

Photonic quantum technologies are on the verge of finding applications in everyday life with quantum cryptography and the quantum internet on the horizon. Extensive research has been carried out to determine suitable quantum emitters and single epitaxial quantum dots are emerging as near-optimal sources of bright, on-demand, highly indistinguishable single photons and entangled photon pairs. In order to build up quantum networks, it is now essential to interface remote quantum emitters. However, this is still an outstanding challenge, as the quantum states of dissimilar 'artificial atoms' have to be prepared on-demand with high fidelity, and the generated photons have to be made indistinguishable in all possible degrees of freedom. Here, we overcome this major obstacle and show an unprecedented two-photon interference (visibility of 51+/-5%) from remote strain-tunable GaAs quantum dots, emitting on-demand photon-pairs. We achieve this result by exploiting for the first time the full potential of the novel phonon-assisted two-photon excitation scheme, which allows for the generation of highly indistinguishable (visibility of 71+/-9%) entangled photon-pairs (fidelity of 90+/-2%), it enables push-to button biexciton state preparation (fidelity of 80+/-2%) and it outperforms conventional resonant two-photon excitation schemes in terms of robustness against environmental decoherence. Our results mark an important milestone for the practical realization of quantum repeaters and complex multi-photon entanglement experiments involving dissimilar artificial atoms.

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On-Chip Single-Photon Sifter

Quantum states of light play a pivotal role in modern science[1] and future photonic applications[2]. While impressive progress has been made in their generation and manipulation with high fidelities, the common table-top approach is reaching its limits for practical quantum applications. Since the advent of integrated quantum nanophotonics[3] different material platforms based on III-V nanostructures-, color centers-, and nonlinear waveguides[4-8] as on-chip light sources have been investigated. Each platform has unique advantages and limitations in terms of source properties, optical circuit complexity, and scaling potentials. However, all implementations face major challenges with efficient and tunable filtering of individual quantum states[4], scalable integration and deterministic multiplexing of on-demand selected quantum emitters[9], and on-chip excitation-suppression[10]. Here we overcome all of these challenges with a novel hybrid and scalable nanofabrication approach to generate quantum light on-chip, where selected single III-V quantum emitters are positioned and deterministically integrated in a CMOS compatible circuit[11] with controlled on-chip filtering and excitation-suppression.Furthermore, we demonstrate novel on-chip quantum wavelength division multiplexing, showing tunable routing of single-photons. Our reconfigurable quantum photonic circuits with a foot print one million times smaller than similar table-top approaches, offering outstanding excitation suppression of more than 95 dB and efficient routing of single photons over a bandwidth of 40 nm, are essential to unleash integrated quantum optical technologies full potential.

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Design of polarization-insensitive superconducting single photon detectors with high-index dielectrics

In this paper, the design of superconducting-nanowire single-photon detectors which are insensitive to the polarization of the incident light is investigated. By using high-refractive-index dielectrics, the index mismatch between the nanowire and the surrounding media is reduced. This enhances the absorption of light with electric field vector perpendicular to the nanowire segments, which is generally hindered in this kind of detectors. Building on this principle and focusing on NbTiN nanowire devices, we present several easy-to-realize cavity architectures which allow high absorption efficiency (in excess of 90%) and polarization insensitivity simultaneously. Designs based on ultranarrow nanowires, for which the polarization sensitivity is much more marked, are also presented. Finally, we briefly discuss the specific advantages of this approach in the case of WSi or MoSi nanowires.

physics.ins-det↗

Initialization of a spin qubit in a site-controlled nanowire quantum dot

A fault-tolerant quantum repeater or quantum computer using solid-state spin-based quantum bits will likely require a physical implementation with many spins arranged in a grid. Self-assembled quantum dots (QDs) have been established as attractive candidates for building spin-based quantum information processing devices, but such QDs are randomly positioned, which makes them unsuitable for constructing large-scale processors. Recent efforts have shown that quantum dots embedded in nanowires can be deterministically positioned in regular arrays, can store single charges, and have excellent optical properties, but so far there have been no demonstrations of spin qubit operations using nanowire quantum dots. Here we demonstrate optical pumping of individual spins trapped in site-controlled nanowire quantum dots, resulting in high-fidelity spin-qubit initialization. This represents the next step towards establishing spins in nanowire quantum dots as quantum memories suitable for use in a large-scale, fault-tolerant quantum computer or repeater based on all-optical control of the spin qubits.

cond-mat.mes-hall↗

Design of broadband high-efficiency superconducting-nanowire single photon detectors

In this paper several designs to maximize the absorption efficiency of superconducting-nanowire single-photon detectors are investigated. Using a simple optical cavity consisting of a gold mirror and a SiO2 layer, the absorption efficiency can be boosted to over 97%: this result is confirmed experimentally by the realization of an NbTiN-based detector having an overall system detection efficiency of 85% at 1.31 micrometers. Calculations show that by sandwiching the nanowire between two dielectric Bragg reflectors, unity absorption (> 99.9%) could be reached at the peak wavelength for optimized structures. To achieve broadband high efficiency, a different approach is considered: a waveguide-coupled detector. The calculations performed in this work show that, by correctly dimensioning the waveguide and the nanowire, polarization-insensitive detectors absorbing more than 95% of the injected photons over a wavelength range of several hundred nm can be designed. We propose a detector design making use of GaN/AlN waveguides, since these materials allow lattice-matched epitaxial deposition of Nb(Ti)N films and are transparent on a very wide wavelength range.

physics.ins-det↗

Single pairs of time-bin entangled photons

Time-bin entangled photons are ideal for long-distance quantum communication via optical fibers. Here we present a source where, even at high creation rates, each excitation pulse generates at most one time-bin entangled pair. This is important for the accuracy and security of quantum communication. Our site-controlled quantum dot generates single polarization-entangled photon pairs, which are then converted, without loss of entanglement strength, into single time-bin entangled photon pairs.

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On-chip quantum interference between silicon photon-pair sources

Large-scale integrated quantum photonic technologies will require the on-chip integration of identical photon sources with reconfigurable waveguide circuits. Relatively complex quantum circuits have already been demonstrated, but few studies acknowledge the pressing need to integrate photon sources and waveguide circuits together on-chip. A key step towards such large-scale quantum technologies is the integration of just two individual photon sources within a waveguide circuit, and the demonstration of high-visibility quantum interference between them. Here, we report a silicon-on-insulator device combining two four-wave mixing sources, in an interferometer with a reconfigurable phase shifter. We configure the device to create and manipulate two-colour (non-degenerate) or same-colour (degenerate), path-entangled or path-unentangled photon pairs. We observe up to 100.0+/-0.4% visibility quantum interference on-chip, and up to 95+/-4% off-chip. Our device removes the need for external photon sources, provides a path to increasing the complexity of quantum photonic circuits, and is a first step towards fully-integrated quantum technologies.

quant-ph↗

Observation of strongly entangled photon pairs from a nanowire quantum dot

A bright photon source that combines high-fidelity entanglement, on-demand generation, high extraction efficiency, directional and coherent emission, as well as position control at the nanoscale is required for implementing ambitious schemes in quantum information processing, such as that of a quantum repeater. Still, all of these properties have not yet been achieved in a single device. Semiconductor quantum dots embedded in nanowire waveguides potentially satisfy all of these requirements; however, although theoretically predicted, entanglement has not yet been demonstrated for a nanowire quantum dot. Here, we demonstrate a bright and coherent source of strongly entangled photon pairs from a position controlled nanowire quantum dot with a fidelity as high as 0.859 +/- 0.006 and concurrence of 0.80 +/- 0.02. The two-photon quantum state is modified via the nanowire shape. Our new nanoscale entangled photon source can be integrated at desired positions in a quantum photonic circuit, single electron devices and light emitting diodes.

cond-mat.mes-hall↗

Overcoming power broadening of the quantum dot emission in a pure wurtzite nanowire

One of the key challenges in developing quantum networks is to generate single photons with high brightness, purity, and long temporal coherence. Semiconductor quantum dots potentially satisfy these requirements; however, due to imperfections in the surrounding material, the coherence generally degrades with increasing excitation power yielding a broader emission spectrum. Here we overcome this power broadening regime and demonstrate the longest coherence at exciton saturation where the detection count rates are highest. We detect single-photon count rates of 460,000 counts per second under pulsed laser excitation while maintaining a single-photon purity of greater than 99%. Importantly, the enhanced coherence is attained with quantum dots in ultraclean wurtzite InP nanowires, where the surrounding charge traps are filled by exciting above the wurtzite InP nanowire bandgap. By raising the excitation intensity, the number of possible charge configurations in the quantum dot environment is reduced, resulting in a narrower emission spectrum. Via Monte Carlo simulations we explain the observed narrowing of the emission spectrum with increasing power. Cooling down the sample to 300 mK, we further enhance the single-photon coherence two-fold as compared to operation at 4.5 K, resulting in a homogeneous coherence time, T2, of 1.2 ns.

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Gallium Arsenide (GaAs) Quantum Photonic Waveguide Circuits

Integrated quantum photonics is a promising approach for future practical and large-scale quantum information processing technologies, with the prospect of on-chip generation, manipulation and measurement of complex quantum states of light. The gallium arsenide (GaAs) material system is a promising technology platform, and has already successfully demonstrated key components including waveguide integrated single-photon sources and integrated single-photon detectors. However, quantum circuits capable of manipulating quantum states of light have so far not been investigated in this material system. Here, we report GaAs photonic circuits for the manipulation of single-photon and two-photon states. Two-photon quantum interference with a visibility of 94.9 +/- 1.3% was observed in GaAs directional couplers. Classical and quantum interference fringes with visibilities of 98.6 +/- 1.3% and 84.4 +/- 1.5% respectively were demonstrated in Mach-Zehnder interferometers exploiting the electro-optic Pockels effect. This work paves the way for a fully integrated quantum technology platform based on the GaAs material system.

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