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Valentina Brosco

Publications and source records attributed to Valentina Brosco.

At least 37 records · Page 2Linked to original sources

Quantum interference assisted spin filtering in graphene nanoflakes

We demonstrate that hexagonal graphene nanoflakes with zigzag edges display quantum interference (QI) patterns analogous to benzene molecular junctions. In contrast with graphene sheets, these nanoflakes also host magnetism. The cooperative effect of QI and magnetism enables spin-dependent quantum interference effects that result in a nearly complete spin polarization of the current, and holds a huge potential for spintronic applications. We understand the origin of QI in terms of symmetry arguments, which show the robustness and generality of the effect. This also allows us to devise a concrete protocol for the electrostatic control of the spin polarization of the current by breaking the sublattice symmetry of graphene, by deposition on hexagonal boron nitride, paving the way to switchable spin-filters. Such a system benefits of all the extraordinary conduction properties of graphene, and at the same time, it does not require any external magnetic field to select the spin polarization, as magnetism emerges spontaneously at the edges of the nanoflake.

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Pauli metallic ground-state in Hubbard clusters with Rashba spin-orbit coupling

We study the "phase diagram" of a Hubbard plaquette with Rashba spin-orbit coupling. We show that the peculiar way in which Rashba coupling breaks the spin-rotational symmetry of the Hubbard model allows a mixing of singlet and triplet components in the ground-state that slows down and it changes the nature of the Mott transition and of the Mott insulating phases.

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Two-dimensional Rashba metals: unconventional low-temperature transport properties

Rashba spin-orbit coupling emerges in materials lacking of structural inversion symmetry, such as heterostructures, quantum wells, surface alloys and polar materials, just to mention few examples. It yields a coupling between the spin and momentum of electrons formally identical to that arising from the weakly-relativistic limit of the Dirac equation. The purpose of the present work is to give an overview of the unconventional dc transport properties of two-dimensional metals with strong Rashba spin-orbit coupling, discussing in addition the effects of thermal broadening.

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Anisotropy of transport in bulk Rashba metals

The recent experimental discovery of three-dimensional (3D) materials hosting a strong Rashba spin-orbit coupling calls for the theoretical investigation of their transport properties. Here we study the zero temperature dc conductivity of a 3D Rashba metal in the presence of static diluted impurities. We show that, at variance with the two-dimensional case, in 3D systems spin-orbit coupling affects dc charge transport in all density regimes. We find in particular that the effect of spin-orbit interaction strongly depends on the direction of the current, and we show that this yields strongly anisotropic transport characteristics. In the dominant spin-orbit coupling regime where only the lowest band is occupied, the SO-induced conductivity anisotropy is governed entirely by the anomalous component of the renormalized current. We propose that measurements of the conductivity anisotropy in bulk Rashba metals may give a direct experimental assessment of the spin-orbit strength.

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Strong parameter renormalization from optimum lattice model orbitals

We revisit the old problem of which is the best single particle basis to express a Hubbard-like lattice model. A rigorous variational solution of this problem leads to equations in which the answer depends in a self-consistent manner on the solution of the lattice model itself. Contrary to naive expectations, for arbitrary small interactions, the optimized orbitals differ from the non-interacting ones, leading also to substantial changes in the model parameters as shown analytically and in an explicit numerical solution for a simple double-well one-dimensional case. At strong coupling, we obtain the direct exchange interaction with a very large renormalization with important consequences for the explanation of ferromagnetism with model hamiltonians. Moreover, in the case of two atoms and two fermions we show that the optimization equations are closely related to reduced density matrix functional theory thus establishing an unsuspected correspondence between continuum and lattice approaches.

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Unconventional dc transport in Rashba electron gases

We discuss the transport properties of a disordered two-dimensional electron gas with strong Rashba spin-orbit coupling. We show that in the high-density regime where the Fermi energy overcomes the energy associated with spin-orbit coupling, dc transport is accurately described by a standard Drude's law, due to a non-trivial compensation between the suppression of back-scattering and the relativistic correction to the quasi-particle velocity. On the contrary, when the system enters the opposite dominant spin-orbit regime, Drude's paradigm breaks down and the dc conductivity becomes strongly sensitive to the spin-orbit coupling strength, providing a suitable tool to test the entanglement between spin and charge degrees of freedom in these

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No-go theorem for the description of Mott phenomena with conventional Density Functional Theory methods

Density functional theory provides the most widespread framework for the realistic description of the electronic structure of solids, but the description of strongly-correlated systems has remained so far elusive. Here we consider a particular limit of electrons in a periodic ionic potential in which a one-band description becomes exact all the way from the weakly-correlated metallic regime to the strongly-correlated Mott-Hubbard regime. We provide a necessary condition a density functional should fulfill to describe Mott-Hubbard behavior and show that it is not satisfied by standard and widely used local, semilocal and hybrid functionals. We illustrate the condition in the case of a few-atom system and provide an analytic approximation to the exact exchange-correlation potential based on a variational wave function which shows explicitly the correct behavior providing a robust scheme to combine lattice and continuum methods.

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Solving lattice density functionals close to the Mott regime

We study a lattice version of the local density approximation (LDA) based on Behte ansatz (BALDA). Contrary to what happens in Density Functional Theory (DFT) in the continuum and despite its name, BALDA displays some very non-local features and it has a discontinuous functional derivative. The same features prevent the convergence of the self-consistent Kohn-Sham cycle thus hindering the study of BALDA solutions close to a Mott phase or in the Coulomb blockade regime. Here we propose a numerical approach which, differently from previous works, does not introduce ad hoc parameters to smear out the singularity. Our results are relevant for all lattice models where BALDA is applied ranging from Kondo systems to harmonically trapped Hubbard fermions. As an example we apply the method to the study of a one-dimensional lattice model with Hubbard interaction and a staggered potential which can be driven from an ionic to a Mott insulating state. In the Mott regime the presence of a "vacuum" allows us to calculate the different contribution to the gap and to highlight an ultranonlocality of BALDA.

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Exact exchange-correlation potential of a ionic Hubbard model with a free surface

We use Lanczos exact diagonalization to compute the exact exchange-correlation (xc) potential of a Hubbard chain with large binding energy ("the bulk") followed by a chain with zero binding energy ("the vacuum"). Several results of density functional theory in the continuum (sometimes controversial) are verified in the lattice. In particular we show explicitly that the fundamental gap is given by the gap in the Kohn-Sham spectrum plus a contribution due to the jump of the xc-potential when a particle is added. The presence of a staggered potential and a nearest-neighbor interaction V allows to simulate a ionic solid. We show that in the ionic regime in the small hopping amplitude limit the xc-contribution to the gap equals V, while in the Mott regime it is determined by the Hubbard U interaction. In addition we show that correlations generates a new potential barrier at the surface.

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Floquet theory of Cooper pair pumping

In this work we derive a general formula for the charge pumped in a superconducting nanocircuit. Our expression generalizes previous results in several ways, it is applicable both in the adiabatic and in the non-adiabatic regimes and it takes into account also the effect of an external environment. More specifically, by applying Floquet theory to Cooper pair pumping, we show that under a cyclic evolution the total charge transferred through the circuit is proportional to the derivative of the associated Floquet quasi-energy with respect to the superconducting phase difference. In the presence of an external environment the expression for the transferred charge acquires a transparent form in the Floquet representation. It is given by the weighted sum of the charge transferred in each Floquet state, the weights being the diagonal components of the stationary density matrix of the system expressed in the Floquet basis. In order to test the power of this formulation we apply it to the study of pumping in a Cooper pair sluice. We reproduce the known results in the adiabatic regime and we show new data in the non-adiabatic case.

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Single-qubit lasing in the strong-coupling regime

Motivated by recent ``circuit QED'' experiments we study the lasing transition and spectral properties of single-qubit lasers. In the strong coupling, low-temperature regime quantum fluctuations dominate over thermal noise and strongly influence the linewidth of the laser. When the qubit and the resonator are detuned, amplitude and phase fluctuations of the radiation field are coupled, and the phase diffusion model, commonly used to describe conventional lasers, fails. We predict pronounced effects near the lasing transition, with an enhanced linewidth and non-exponential decay of the correlation functions. We cover a wide range of parameters by using two complementary approaches, one based on the Liouville equation in a Fock state basis, covering arbitrarily strong coupling but limited to low photon numbers, the other based on the coherent-state representation, covering large photon numbers but restricted to weak or intermediate coupling.

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Resonant all-electric spin pumping with spin-orbit coupling

All-electric devices for the generation and filtering of spin currents are of crucial importance for spintronics experiments and applications. Here we consider a quantum dot between two metallic leads in the presence of spin-orbit coupling, and we analyze in the frame of a scattering matrix approach the conditions for generating spin currents in an adiabatically driven two-terminal device. We then focus on a dot with two resonant orbitals and show by specific examples that both spin filtering and pure spin current generation can be achieved. Finally, we discuss the effect of the Coulomb interaction.

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Few-Qubit lasing in circuit QED

Motivated by recent experiments, which demonstrated lasing and cooling of the electromagnetic modes in a resonator coupled to a superconducting qubit, we describe the specific mechanisms creating the population inversion, and we study the spectral properties of these systems in the lasing state. Different levels of the theoretical description, i.e., the semi-classical and the semi-quantum approximation, as well as an analysis based on the full Liouville equation are compared. We extend the usual quantum optics description to account for strong qubit-resonator coupling and include the effects of low-frequency noise. Beyond the lasing transition we find for a single- or few-qubit system the phase diffusion strength to grow with the coupling strength, which in turn deteriorates the lasing state.

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Phase diffusion and locking in single-qubit lasers

Motivated by recent experiments, which demonstrated lasing and cooling of the electromagnetic field in an electrical resonator coupled to a superconducting qubit, we study the phase coherence and diffusion of the system in the lasing state. We also discuss phase locking and synchronization induced by an additional {\sl ac} driving of the resonator. We extend earlier work to account for the strong qubit-resonator coupling and to include the effects of low-frequency qubit's noise. We show that the strong coupling may lead to a double peak structure of the spectrum, while the shape and width are determined to the low-frequency noise.

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Dissipation in circuit quantum electrodynamics: lasing and cooling of a low-frequency oscillator

Superconducting qubits coupled to electric or nanomechanical resonators display effects previously studied in quantum electrodynamics (QED) and extensions thereof. Here we study a driven qubit coupled to a low-frequency tank circuit with particular emphasis on the role of dissipation. When the qubit is driven to perform Rabi oscillations, with Rabi frequency in resonance with the oscillator, the latter can be driven far from equilibrium. Blue detuned driving leads to a population inversion in the qubit and lasing behavior of the oscillator ("single-atom laser"). For red detuning the qubit cools the oscillator. This behavior persists at the symmetry point where the qubit-oscillator coupling is quadratic and decoherence effects are minimized. Here the system realizes a "single-atom-two-photon laser".

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Geometric effects of noise on Cooper pair pumping

Several works investigated the connection between Cooper pair pumping and the geometric and topological properties of the pumping cycle in the parameters space. Recently the predicted connection between Berry's phase and pumped charge was observed experimentally. In the present work we analyze the effects of noise on Cooper pair pumping. We show that dissipation induces a new geometric contribution in the transferred charge and we propose an experiment where the theory can be probed.

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Non-abelian superconducting pumps

Cooper pair pumping is a coherent process. We derive a general expression for the adiabatic pumped charge in superconducting nanocircuits in the presence of level degeneracy and relate it to non-Abelian holonomies of Wilczek and Zee. We discuss an experimental system where the non-Abelian structure of the adiabatic evolution manifests in the pumped charge.

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Qubits as devices to detect the third moment of current fluctuations

Under appropriate conditions controllable two-level systems can be used to detect the third moment of current fluctuations. We derive a Master Equation for a quantum system coupled to a bath valid to the third order in the coupling between the system and the environment. In this approximation the reduced dynamics of the quantum system depends on the frequency dependent third moment. Specializing to the case of a controllable two-level system (a qubit) and in the limit in which the splitting between the levels is much smaller than the characteristic frequency of the third moment, it is possible to show that the decay of the qubit has additional oscillations whose amplitude is directly proportional to the value of the third moment. We discuss an experimental setup where this effect can be seen.

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