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Valeri N. Kotov

Publications and source records attributed to Valeri N. Kotov.

At least 37 records · Page 2Linked to original sources

Valley Order and Loop Currents in Graphene on Hexagonal Boron Nitride

In this letter, we examine the role of Coulomb interactions in the emergence of macroscopically ordered states in graphene supported on hexagonal boron nitride substrates. Due to incommensuration effects with the substrate, graphene can develop gapped low energy modes that spatially conform into a triangular superlattice of quantum rings. In the presence of these modes, we show that Coulomb interactions lead to spontaneous formation of chiral loop currents in bulk and to macroscopic spin-valley order at zero temperature. We show that this exotic state breaks time reversal symmetry and can be detected with interferometry and polar Kerr measurements.

cond-mat.str-el↗

Van der Waals forces and electron-electron interactions in two strained graphene layers

We evaluate the van der Waals (vdW) interaction energy at zero temperature between two undoped strained graphene layers separated by a finite distance. We consider the following three models for the anisotropic case: (a) where one of the two layers is uniaxially strained, (b) the two layers are strained in the same direction, and (c) one of the layers is strained in the perpendicular direction with respect to the other. We find that for all three models and given value of the electron-electron interaction coupling, the vdW interaction energy increases with increasing anisotropy. The effect is most striking for the case when both layers are strained in the same direction where we observe up to an order of magnitude increase in the strained relative to the unstrained case. We also investigate the effect of electron electron interaction renormalization in the region of large separation between the strained graphene layers. We find that the many-body renormalization contributions to the correlation energy are non negligible and the vdW interaction energy decreases as a function of increasing distance between the layers due to renormalization of the Fermi velocity, the anisotropy, and the effective interaction. Our analysis can be useful in designing novel graphene-based vdW heterostructures which, in recent times, has seen an upsurge in research activity.

cond-mat.mtrl-sci↗

Effect of Uniaxial Strain on Ferromagnetic Instability and Formation of Localized Magnetic States on Adatoms in Graphene

We investigate the effect of an applied uniaxial strain on the ferromagnetic instability due to long- range Coulomb interaction between Dirac fermions in graphene. In case of undeformed graphene the ferromagnetic exchange instability occurs at sufficiently strong interaction within the Hartree- Fock approximation. In this work we show that using the same theoretical framework but with an additional applied uniaxial strain, the transition can occur for much weaker interaction, within the range in suspended graphene. We also study the consequence of strain on the formation of localized magnetic states on adatoms in graphene. We systematically analyze the interplay between the anisotropic (strain- induced) nature of the Dirac fermions in graphene, on- site Hubbard interaction at the impurity and the hybridization between the graphene and impurity electrons. The polarization of the electrons in the localized orbital is numerically calculated within the mean- field self- consistent scheme. We obtain complete phase diagram containing non- magnetic as well as magnetic regions and our results can find prospective application in the field of carbon- based spintronics.

cond-mat.str-el↗

Interacting Anisotropic Dirac Fermions in Strained Graphene and Related Systems

We study the role of long-range electron-electron interactions in a system of two-dimensional anisotropic Dirac fermions, which naturally appear in uniaxially strained graphene, graphene in external potentials, some strongly anisotropic topological insulators, and engineered anisotropic graphene structures. We find that while for small interactions and anisotropy the system restores the conventional isotropic Dirac liquid behavior, strong enough anisotropy can lead to the formation of a quasi-one dimensional electronic phase with dominant charge order (anisotropic excitonic insulator).

cond-mat.str-el↗

Electron-Electron Interactions in Graphene: Current Status and Perspectives

We review the problem of electron-electron interactions in graphene. Starting from the screening of long range interactions in these systems, we discuss the existence of an emerging Dirac liquid of Lorentz invariant quasi-particles in the weak coupling regime, and strongly correlated electronic states in the strong coupling regime. We also analyze the analogy and connections between the many-body problem and the Coulomb impurity problem. The problem of the magnetic instability and Kondo effect of impurities and/or adatoms in graphene is also discussed in analogy with classical models of many-body effects in ordinary metals. We show that Lorentz invariance plays a fundamental role and leads to effects that span the whole spectrum, from the ultraviolet to the infrared. The effect of an emerging Lorentz invariance is also discussed in the context of finite size and edge effects as well as mesoscopic physics. We also briefly discuss the effects of strong magnetic fields in single layers and review some of the main aspects of the many-body problem in graphene bilayers. In addition to reviewing the fully understood aspects of the many-body problem in graphene, we show that a plethora of interesting issues remain open, both theoretically and experimentally, and that the field of graphene research is still exciting and vibrant.

cond-mat.str-el↗

Thermodynamics of a gas of deconfined bosonic spinons in two dimensions

We consider the quantum phase transition between a Neel antiferromagnet and a valence-bond solid (VBS) in a two-dimensional system of S=1/2 spins. Assuming that the excitations of the critical ground state are linearly dispersing deconfined spinons obeying Bose statistics, we derive expressions for the specific heat and the magnetic susceptibility at low temperature T. Comparing with quantum Monte Carlo results for the J-Q model, which is a candidate for a deconfined Neel-VBS transition, we find excellent agreement, including a previously noted logarithmic correction in the susceptibility. In our treatment, this is a direct consequence of a confinement length scale Lambda which is proportional to the correlation length xi raised to a non-trivial power; Lambda ~ xi^(1+a) ~1/T^(1+a), with a>0 (with a approximately 0.2 in the model).

cond-mat.str-el↗

Quantum Phase Transition in the Four-Spin Exchange Antiferromagnet

We study the S=1/2 Heisenberg antiferromagnet on a square lattice with nearest-neighbor and plaquette four-spin exchanges (introduced by A.W. Sandvik, Phys. Rev. Lett. {\bf 98}, 227202 (2007).) This model undergoes a quantum phase transition from a spontaneously dimerized phase to Néel order at a critical coupling. We show that as the critical point is approached from the dimerized side, the system exhibits strong fluctuations in the dimer background, reflected in the presence of a low-energy singlet mode, with a simultaneous rise in the triplet quasiparticle density. We find that both singlet and triplet modes of high density condense at the transition, signaling restoration of lattice symmetry. In our approach, which goes beyond mean-field theory in terms of the triplet excitations, the transition appears sharp; however since our method breaks down near the critical point, we argue that we cannot make a definite conclusion regarding the order of the transition.

cond-mat.str-el↗

1/N Expansion in Correlated Graphene

We examine the 1/N expansion, where N is the number of two-component Dirac fermions, for Coulomb interactions in graphene with a gap of magnitude $Δ= 2 m$. We find that for $Nα\gg1$, where $α$ is graphene's "fine structure constant", there is a crossover as a function of distance $r$ from the usual 3D Coulomb law, $V(r) \sim 1/r$, to a 2D Coulomb interaction, $V(r) \sim \ln(Nα/mr)$, for $m^{-1} \ll r \ll m^{-1} N α/6$. This effect reflects the weak "confinement" of the electric field in the graphene plane. The crossover also leads to unusual renormalization of the quasiparticle velocity and gap at low momenta. We also discuss the differences between the interaction potential in gapped graphene and usual QED for different coupling regimes.

cond-mat.mes-hall↗

Adatoms in Graphene

We review the problem of adatoms in graphene under two complementary points of view, scattering theory and strong correlations. We show that in both cases impurity atoms on the graphene surface present effects that are absent in the physics of impurities in ordinary metals. We discuss how to observe these unusual effects with standard experimental probes such as scanning tunneling microscopes, and spin susceptibility.

cond-mat.mtrl-sci↗

Weak Antiferromagnetic Order in Anisotropic Quantum Pyrochlores

We study the ground state properties of an anisotropic, quasi-2D version of the quantum (S=1/2) pyrochlore antiferromagnet. In the presence of Dzyaloshinsky-Moriya interactions, in addition to the Heisenberg exchanges, it is shown that two types of ordered magnetic states are generally possible: non coplanar "chiral," and coplanar antiferromagnetic order. The magnetic moments in all cases are determined by the Dzyaloshinsky-Moriya interactions and in this sense the antiferromagnetic order is "weak."

cond-mat.str-el↗

Polarization Charge Distribution in Gapped Graphene

We study the distribution of vacuum polarization charge induced by a Coulomb impurity in massive graphene. By analytically computing the polarization function, we show that the charge density is distributed in space in a non-trivial fashion, and on a characteristic length-scale set by the effective Compton wavelength. The density crosses over from a logarithmic behavior below this scale, to a power law variation above it. Our results in the continuum limit are confirmed by explicit diagonalization of the corresponding tight-binding model on a finite-size lattice. Electron-electron interaction effects are also discussed.

cond-mat.mes-hall↗

Localized Magnetic States in Graphene

We examine the conditions necessary for the presence of localized magnetic moments on adatoms with inner shell electrons in graphene. We show that the low density of states at the Dirac point, and the anomalous broadening of the adatom electronic level,lead to the formation of magnetic moments for arbitrarily small local charging energy. As a result, we obtain an anomalous scaling of the boundary separating magnetic and non-magnetic states. We show that, unlike any other material, the formation of magnetic moments can be controlled by an electric field effect.

cond-mat.str-el↗

Supercritical Coulomb Impurities in Gapped Graphene

We study the problem of Coulomb field-induced charging of the ground state in a system of 2D massive Dirac particles (gapped graphene). As in its 3D QED counterpart, the critical Coulomb coupling is renormalized to higher values, compared to the massless case. We find that in gapped graphene a novel supercritical regime is possible, where the screening charge is comparable to the impurity charge, thus leading to suppression of the Coulomb field at nanometer scales. We corroborate this with numerical solution of the tight-binding problem in the honeycomb lattice.

cond-mat.mes-hall↗

Electron-Electron Interactions in the Vacuum Polarization of Graphene

We discuss the effect of electron-electron interactions on the static polarization properties of graphene beyond RPA. Divergent self-energy corrections are naturally absorbed into the renormalized coupling constant $α$. We find that the lowest order vertex correction, which is the first non-trivial correlation contribution, is finite, and about 30% of the RPA result at strong coupling $α\sim 1$. The vertex correction leads to further reduction of the effective charge. Finite contributions to dielectric screening are expected in all orders of perturbation theory.

cond-mat.str-el↗

Negative Hopping Magnetoresistance and Dimensional Crossover in Lightly Doped Cuprate Superconductors

We show that, due to the weak ferromagnetism of La$_{2-x}$Sr$_x$CuO$_4$, an external magnetic field leads to a dimensional crossover 2D $\to$ 3D for the in-plane transport. The crossover results in an increase of the hole's localization length and hence in a dramatic negative magnetoresistance in the variable range hopping regime. This mechanism quantitatively explains puzzling experimental data on the negative magnetoresistance in the Néel phase of La$_{2-x}$Sr$_x$CuO$_4$.

cond-mat.str-el↗

Screening of Coulomb Impurities in Graphene

We calculate exactly the vacuum polarization charge density in the field of a subcritical Coulomb impurity, $Z|e|/r$, in graphene. Our analysis is based on the exact electron Green's function, obtained by using the operator method, and leads to results that are exact in the parameter $Zα$, where $α$ is the "fine structure constant" of graphene. Taking into account also electron-electron interactions in the Hartree approximation, we solve the problem self-consistently in the subcritical regime, where the impurity has an effective charge $Z_{eff}$, determined by the localized induced charge. We find that an impurity with bare charge Z=1 remains subcritical, $Z_{eff} α< 1/2$, for any $α$, while impurities with $Z=2,3$ and higher can become supercritical at certain values of $α$.

cond-mat.mes-hall↗

AC Hopping Magnetotransport Across the Spin Flop Transition in Lightly Doped La_2CuO_4

The weak ferromagnetism present in insulating La_{2}CuO_4 at low doping leads to a spin flop transition, and to transverse (interplane) hopping of holes in a strong external magnetic field. This results in a dimensional crossover 2D $\to$ 3D for the in-plane transport, which in turn leads to an increase of the hole's localization length and increased conduction. We demonstrate theoretically that as a consequence of this mechanism, a frequency-dependent jump of the in-plane ac hopping conductivity occurs at the spin flop transition. We predict the value and the frequency dependence of the jump. Experimental studies of this effect would provide important confirmation of the emerging understanding of lightly doped insulating La_{2-x}Sr_xCuO_4.

cond-mat.str-el↗