arXiv subjects

Vanessa Li Zhang

Publications and source records attributed to Vanessa Li Zhang.

11 recordsLinked to original sources

arXiv2026

Spin-canting-induced Giant Nonlinear Optical Magnetochirality in a 2D Ferrotoroid

Achieving magnetically switchable chiral light emission is an important goal for 2D opto-spintronics. However, conventional strategies face a fundamental trade-off between dynamic tunability and polarization contrast. Nonlinear optics, particularly the emerging mechanism of chiral second-harmonic generation (SHG), offers a distinct strategy to bypass this restriction, yet its experimental realization remains elusive due to stringent symmetry requirements. Here, we report giant nonlinear optical magnetochirality in a centrosymmetric 2D ferrotoroid, bilayer (2L) CrSBr. We reveal that a field-induced spin-canting state breaks the parity-time (PT) symmetry of the unperturbed antiferromagnetic (AFM) ground state, activating a spin-chirality-driven i-type susceptibility. The coherent interference between this emergent i-type and intrinsic c-type SHG susceptibilities generates a macroscopic circularly polarized SHG signal whose helicity is magnetically switchable. Leveraging this sensitive mechanism, we uncover remanent magnetic states after field saturation that evade conventional linear probes. By exploiting the non-volatility of these states, we demonstrate magneto-optical memory and logic operations. Our work establishes a general symmetry-driven strategy for tailoring nonlinear magnetochirality, while providing a sensitive optical probe for subtle spin textures in the 2D limit.

physics.optics↗

arXiv2025

Spin light-emitting devices in a 2D magnet

Emerging two-dimensional (2D) magnetic semiconductors represent transformative platforms to explore magneto-optics and opto-spintronic applications. Though 2D opto-spintronics has attracted tremendous research efforts in spin-dependent photodetectors and non-volatile memory components, the realization of one core application - spin-modulated light-emitting device (spin-LED) - remains elusive so far. Here we successfully realize prototype spin-LED integrated with a 2D semiconducting magnet CrSBr, demonstrating considerable electroluminescence (EL) down to bilayers. Intriguingly, the EL of the spin-LED is discovered to be directly manipulated by spin-flip and spin-canting transitions. Notably, spin-flip transitions enable unprecedented hysteretic behaviors of EL characteristics, while spin-canting transitions induce EL continuous modulation with robust anisotropy. This versatile manipulation is originated from the synergy of magnetic-order mediated excitonic transitions and spintronic transport. The prototype demonstration of spin-LED establishes an indispensable scheme of opto-spintronic devices leveraging 2D spin transitions and strong excitonic effects, presenting a critical step towards integrated 2D opto-spintronics.

physics.app-ph↗

arXiv2025

Spontaneous Enhancement of Dzyaloshinskii-Moriya Interaction via Field-Cooling-Induced Interface Engineering in 2D van der Waals Ferromagnetic ternary Tellurides

The emergence of two-dimensional (2D) van der Waals (vdW) ferromagnets has opened new avenues for exploring topological spin textures and their applications in next-generation spintronics. Among these materials, Fe3GaTe2 (FGaT) emerges as a model system due to its room-temperature skyrmion phases, which are stabilized by strong Dzyaloshinskii-Moriya interaction (DMI). However, the atomistic origins of DMI in centrosymmetric vdW lattices remain elusive. Here, we report a spontaneous DMI enhancement mechanism driven by FC in FGaT and its analog Fe3GeTe2 (FGeT). Combining Raman spectroscopy and scanning transmission electron microscopy (STEM), we have observed the irreversible precipitation of FeTe2 in annealed FGaT. The resulting FeTe2/FGaT heterostructure is considered to break the symmetry and significantly enhance the DMI. Furthermore, similar phenomenon has been observed in the family ferromagnetic material FGeT as well. Additionally, the precipitation of FeTe2 varies significantly with different thicknesses of FGaT, aligning closely with the reported behavior of skyrmions. This discovery provides new insights into the mechanisms behind the origin of the DMI in ternary tellurides, paving the way for advanced spintronic applications.

cond-mat.mtrl-sci↗

arXiv2025

Strain Induced Robust Skyrmion lattice at Room Temperature in van der Waals Ferromagnet

Manipulating topological magnetic orders of two-dimensional (2D) magnets by strain, once achieved, offers enormous potential for future low-power flexible spintronic applications. In this work, by placing Fe3GaTe2 (FGaT), a room-temperature 2D ferromagnet, on flexible substrate, we demonstrate a field-free and robust formation of skyrmion lattice induced by strain. By applying a minimal strain of ~0.80% to pre-annealed FGaT flakes, the Magnetic Force Microscopy (MFM) tip directly triggers the transition from maze-like domains to an ordered skyrmion lattice while scanning the sample surface. The skyrmion lattice is rather stable against extensive cyclic mechanical testing (stretching, bending, and twisting over 2000 cycles each). It also exhibited stability across a wide range of magnetic fields (~2.9 kOe) and temperatures (~ 323 K), as well as long-term retention stability, highlighting its robustness and field free stabilization. The strain effect reduces the lattice symmetry and enhances the Dzyaloshinskii-Moriya interaction (DMI) of FGaT, thus stabilizing the skyrmion lattice. Our findings highlight the potential of FGaT for integrating magnetic skyrmions into future low-power-consumption flexible spintronics devices.

cond-mat.mtrl-sci↗

arXiv2024

On the relationship between orbital moment anisotropy, magnetocrystalline anisotropy, and Dzyaloshinskii-Moriya interaction in W/Co/Pt trilayers

We have studied the Co layer thickness dependences of magnetocrystalline anisotropy (MCA), Dzyaloshinskii-Moriya interaction (DMI), and orbital moment anisotropy (OMA) in W/Co/Pt trilayers, in order to clarify their correlations with each other. We find that the MCA favors magnetization along the film normal and monotonically increases with decreasing effective magnetic layer thickness ($t_\mathrm{eff}$). The magnitude of the Dzyaloshinskii-Moriya exchange constant ($|D|$) increases with decreasing $t_\mathrm{eff}$ until $t_\mathrm{eff} \sim$1 nm, below which $|D|$ decreases. The MCA and $|D|$ scale with $1/t_\mathrm{eff}$ for $t_\mathrm{eff}$ larger than $\sim$1 nm, indicating an interfacial origin. The increase of MCA with decreasing $t_\mathrm{eff}$ continues below $t_\mathrm{eff}$ $\sim$ 1 nm, but with a slower rate. To clarify the cause of the $t_\mathrm{eff}$ dependences of MCA and DMI, the OMA of Co in W/Co/Pt trilayers is studied using x-ray magnetic circular dichroism (XMCD). We find non-zero OMA when $t_\mathrm{eff}$ is smaller than $\sim$0.8 nm. The OMA increases with decreasing $t_\mathrm{eff}$ more rapidly than what is expected from the MCA, indicating that factors other than OMA contribute to the MCA at small $t_\mathrm{eff}$. The $t_\mathrm{eff}$ dependence of the OMA also suggests that $|D|$ at $t_\mathrm{eff}$ smaller than $\sim$1 nm is not related to the OMA at the interface. We propose that the growth of Co on W results in a strain and/or texture that reduces the interfacial DMI, and, to some extent, MCA at small $t_\mathrm{eff}$.

cond-mat.mtrl-sci↗

arXiv2017

Eigenmodes of Neel skyrmions in ultrathin magnetic films

The static and dynamic states of Néel skyrmions in ultrathin ferromagnetic films with interfacial Dzyaloshinskii-Moriya interaction (DMI) have been micromagnetically simulated as functions of the interfacial DMI strength and applied static magnetic field. Findings reveal that while the breathing, counterclockwise (CCW) and clockwise (CW) rotational eigenmodes exist in the skyrmion lattice (SkL) phase, only the first two modes are present in the isolated skyrmion (ISk) phase. Additionally, the eigenfrequency of the CCW mode is insensitive to the magnetic-field driven SkL-ISk phase transition, and the inter-skyrmion interaction is largely responsible for exciting the CW mode in the SkL phase. The findings provide physical insight into the dynamics of the phase transition and would be of use to potential skyrmion-based microwave applications.

cond-mat.mes-hall↗

arXiv2015

In-plane angular dependence of the spin-wave nonreciprocity of an ultrathin film with Dzyaloshinskii-Moriya interaction

The nonreciprocal propagation of spin waves in an ultrathin Pt/Co/Ni film has been measured by Brillouin light scattering. The frequency nonreciprocity, due to the interfacial Dzyaloshinskii-Moriya interaction (DMI), has a sinusoidal dependence on the in-plane angle between the magnon wavevector and the applied magnetic field. The results, which are in good agreement with analytical predictions reported earlier, yield a value of the DMI constant which is the same as that obtained previously from a study of the magnon dispersion relations. We have demonstrated that our magnon-dynamics based method can experimentally ascertain the DMI constant of multilayer thin films.

cond-mat.mtrl-sci↗

arXiv2015

Asymmetric spin-wave dispersion due to Dzyaloshinskii-Moriya interaction in an ultrathin Pt/CoFeB film

Employing Brillouin spectroscopy, strong interfacial Dzyaloshinskii-Moriya interactions have been observed in an ultrathin Pt/CoFeB film. Our micromagnetic simulations show that spin-wave nonreciprocity due to asymmetric surface pinning is insignificant for the 0.8nmthick CoFeB film studied. The observed high asymmetry of the monotonic spin wave dispersion relation is thus ascribed to strong Dzyaloshinskii-Moriya interactions present at the Pt/CoFeB interface. Our findings should further enhance the significance of CoFeB as an important material for magnonic, spintronic and skyrmionic applications.

cond-mat.mes-hall↗

arXiv2015

Direct observation of the Dzyaloshinskii-Moriya interaction in a Pt/Co/Ni film

The interfacial Dzyaloshinskii-Moriya interaction (DMI) in an in-plane anisotropic Pt(4nm)/Co(1.6nm)/Ni(1.6nm) film has been directly observed by Brillouin spectroscopy. It is manifested in the asymmetry of the measured magnon dispersion relation, from which the DMI constant has been evaluated. Linewidth measurements reveal that the lifetime of the magnons is asymmetric with respect to their counter-propagating directions. The lifetime asymmetry is dependent on the magnon frequency, being more pronounced the higher the frequency. Analytical calculations of the magnon dispersion relation and linewidth agree well with experiments.

cond-mat.mtrl-sci↗

arXiv2014

Band structure of magnonic crystals with defects: Brillouin spectroscopy and micromagnetic simulations

Using Brillouin spectroscopy, the first observation has been made of the band structures of nanostructured defect magnonic crystals. The samples are otherwise one-dimensional periodic arrays of equal-width Ni80Fe20 and cobalt nanostripes, where the defects are stripes of a different width. A dispersionless defect branch emerges within the bandgap with a frequency tunable by varying the defect stripe width, while the other branches observed are similar to those of a defect-free crystal. Micromagnetic and finite-element simulations performed unveil additional tiny bandgaps and the frequency-dependent localization of the defect mode in the vicinity of the defects.

cond-mat.mes-hall↗

arXiv2013

Spin-wave nonreciprocity based on interband magnonic transitions

We theoretically demonstrate linear spin-wave nonreciprocity in a Ni80Fe20 nanostripe waveguide, based on interband magnonic transitions induced by a time-reversal and spatialinversion symmetry breaking magnetic field. An analytical coupled-mode theory of spin waves, developed to describe the transitions which are accompanied by simultaneous frequency and wavevector shifts of the coupled spin waves, is well corroborated by numerical simulations. Our findings could pave the way for the realization of spin-wave isolation and the dynamic control of spin-wave propagation in nanoscale magnonic integrated circuits via an applied magnetic field.

cond-mat.mes-hall↗